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| Open AccessStrong structuring arising from weak cooperative O-H···π and C-H···O hydrogen bonding in benzene-methanol solution
Understanding liquid behavior is a challenge due to their disorder nature and rapid molecular rearrangements. Here, the authors show how weak interactions between OH groups and aromatic rings can participate in cooperative mechanisms that give rise to highly structured molecular arrangements in the liquid state.
- Camilla Di Mino
- , Andrew G. Seel
- & Neal T. Skipper
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Article
| Open AccessIntrinsic 1\({T}^{{\prime} }\) phase induced in atomically thin 2H-MoTe2 by a single terahertz pulse
A single field-enhanced terahertz pulse was used to create 1\({T}^{{\prime} }\)-MoTe2 out of few-layer H-MoTe2 crystals, providing insights into the ultrafast polymorphic transition dynamics and resolving a long-standing debate over the realization of this transition by high-energy photon irradiation.
- Jiaojian Shi
- , Ya-Qing Bie
- & Keith A. Nelson
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Article
| Open AccessAnomalous spin current anisotropy in a noncollinear antiferromagnet
Symmetry is an essential ingredient that governs numerous physical phenomena, including spin transport. Following this principle, spin current sources with a highly symmetric cubic structure are not expected to support anisotropic spin currents. Here, the authors demonstrate an anomalous spin current anisotropy in a cubic noncollinear antiferromagnet Mn3Pt by exploiting the combination of conventional and magnetic spin-hall effects.
- Cuimei Cao
- , Shiwei Chen
- & Qingfeng Zhan
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Article
| Open AccessKapitza-resistance-like exciton dynamics in atomically flat MoSe2-WSe2 lateral heterojunction
Here, the authors use tip-enhanced photoluminescence spectroscopy to show a discontinuity of the exciton density distribution on each side of the interface of a MoSe2/WSe2 lateral heterostructure. They introduce the concept of ‘exciton Kapitza resistance’ by analogy with the interfacial thermal resistance known as ‘Kapitza resistance’.
- Hassan Lamsaadi
- , Dorian Beret
- & Jean-Marie Poumirol
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Article
| Open AccessObservation of suppressed viscosity in the normal state of 3He due to superfluid fluctuations
Early theoretical work predicted that fluctuations above the superfluid transition in liquid 3He should be observable in viscosity. Baten et al. document the reduction of the viscosity due to fluctuations, by monitoring the quality factor of a resonator immersed in 3He as a function of pressure and temperature.
- Rakin N. Baten
- , Yefan Tian
- & Jeevak M. Parpia
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Article
| Open AccessMicrorollers flow uphill as granular media
Kinetic energy put into a granular medium as a collective is typically dissipated as friction. The situation is different when forces are applied to the individual particles. An experiment now shows that when torques are applied to particles in a dense bed of microrollers, the grains roll uphill.
- Samuel R. Wilson-Whitford
- , Jinghui Gao
- & James F. Gilchrist
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Article
| Open AccessOrganic radical ferroelectric crystals with martensitic phase transition
Organic martensitic compounds are emerging smart materials with intriguing physical properties. Here authors show that upon H/F substitution a series of 1,4,5,8-naphthalenediimide derivatives exhibit reversible ferroelectric and martensitic transitions with a large thermal hysteresis.
- Nan Zhang
- , Wencong Sun
- & Han-Yue Zhang
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Article
| Open AccessReviving product states in the disordered Heisenberg chain
Many-body localized systems are believed to reach a stationary state without thermalizing. By using analytical and numerical calculations, the authors construct simple initial states for a typical MBL model, which neither equilibrate nor thermalize, similar to non-ergodic behavior in many-body scarred systems.
- Henrik Wilming
- , Tobias J. Osborne
- & Christoph Karrasch
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Article
| Open AccessA molecular pyroelectric enabling broadband photo-pyroelectric effect towards self-driven wide spectral photodetection
Broadband spectral photoresponse has potential for optoelectronic devices, but obtaining high photoactivity beyond the material bandgap is challenging. Here, the authors report the development of a molecular pyroelectric material with broadband photopyroelectric effects.
- Xi Zeng
- , Yi Liu
- & Zhihua Sun
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Article
| Open AccessWeyl nodal ring states and Landau quantization with very large magnetoresistance in square-net magnet EuGa4
The tunability of electronic properties is a central goal of research into topological semimetals. Here, the authors report Weyl nodal ring states in the magnetic semimetal EuGa4 and link the nodal ring state to the observed large non-saturating magnetoresistance.
- Shiming Lei
- , Kevin Allen
- & Emilia Morosan
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Article
| Open AccessStrong electron-phonon coupling driven pseudogap modulation and density-wave fluctuations in a correlated polar metal
Electronic bandwidth modulation by static pressure has been explored in several material families. Wang et al. use temperature-dependent Raman spectroscopy and density functional theory to reveal phonon-driven modulation of electronic pseudogap and density wave fluctuations in a ruthenate Ca3Ru2O7.
- Huaiyu (Hugo) Wang
- , Yihuang Xiong
- & Venkatraman Gopalan
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Article
| Open AccessInterlayer donor-acceptor pair excitons in MoSe2/WSe2 moiré heterobilayer
The nature of localized interlayer excitons (LIXs) in moiré superlattices is still elusive Here, the authors propose a donor-acceptor pair mechanism for LIXs in MoSe2/WSe2 heterobilayers.
- Hongbing Cai
- , Abdullah Rasmita
- & Weibo Gao
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Article
| Open AccessMicrocavity phonoritons – a coherent optical-to-microwave interface
Photonic, electronic and lattice resonances in patterned semiconductor microcavities are tailored to demonstrate coherent bidirectional microwave-to-optical conversion via phonon-exciton-photon quasi-particles in the strong-coupling regime.
- Alexander Sergeevich Kuznetsov
- , Klaus Biermann
- & Paulo Ventura Santos
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Article
| Open AccessDislocation interactions during plastic relaxation of epitaxial colloidal crystals
Mechanical properties of materials are governed by dislocations, yet it remains a challenge to resolve their evolution on the atomic scale. Svetlizky et al. use colloidal crystals to investigate, in three dimensions, how dislocations enable plastic relaxation and the formation of networks.
- Ilya Svetlizky
- , Seongsoo Kim
- & Frans Spaepen
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Article
| Open AccessCharge density wave surface reconstruction in a van der Waals layered material
Recent work has reported puzzling results on the surface of 1T-TaS2. Based on first-principles calculations, the authors show that charge density wave order undergoes surface reconstruction, leading to modifications in the surface electronic structure, which can explain recent experiments.
- Sung-Hoon Lee
- & Doohee Cho
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Article
| Open AccessBroad-high operating temperature range and enhanced energy storage performances in lead-free ferroelectrics
One of the key challenges in dielectric ceramics for energy storage lies in the comprehensive optimization of their properties. Here, the authors establish an equitable system considering performance and structure evolution in a lead-free ceramic capacitor, achieving a broad-high temperature performance.
- Weichen Zhao
- , Diming Xu
- & Di Zhou
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Article
| Open AccessUnraveling bilayer interfacial features and their effects in polar polymer nanocomposites
The nanoparticle-polymer interface plays a key role in nanoparticle-polymer composites but understanding the structures and properties of the interfacial region remains challenging. Here, the authors directly observe the presence of two interfacial polymer layers around a nanoparticle in polar polymers with different polar molecular conformations from the bulk polymer leading to an enhancement in polarity-related properties of polymer nanocomposites
- Xinhui Li
- , Shan He
- & Ce-Wen Nan
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Article
| Open AccessPhotoluminescence upconversion in monolayer WSe2 activated by plasmonic cavities through resonant excitation of dark excitons
Here, the authors perform statistical measurements on hundreds of plasmonic nano-cavities embedding WSe2 monolayers, and show the activation of anti-Stokes photoluminescence in WSe2 through resonant excitation of a dark exciton at room temperature.
- Niclas S. Mueller
- , Rakesh Arul
- & Jeremy J. Baumberg
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Article
| Open AccessReal-space observation of ergodicity transitions in artificial spin ice
Artificial spin ice systems have been used to simulate a variety of phenomena including phase transitions. Here, the authors expand the scope of applications to encompass non-ergodic dynamics, by reporting real-space imaging of ergodicity transitions in a vortex-frustrated artificial spin ice.
- Michael Saccone
- , Francesco Caravelli
- & Alan Farhan
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| Open AccessInterplay of valley polarized dark trion and dark exciton-polaron in monolayer WSe2
Here, the authors observe that valley-polarized dark excitons in monolayer WSe2 show a distinct doping dependence when the carriers reach a critical density. This is indicative of the onset of strongly modified Fermi sea interactions.
- Xin Cong
- , Parisa Ali Mohammadi
- & Xiao-Xiao Zhang
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Article
| Open AccessVoltage control of magnetism in Fe3-xGeTe2/In2Se3 van der Waals ferromagnetic/ferroelectric heterostructures
The control of magnetism by electric field is an important goal for future development of low-power spintronics. Here, the authors demonstrate voltage control of magnetism in van der Waals ferromagnetic/ferroelectric heterostructure devices via the strain-mediated magnetoelectric effect.
- Jaeun Eom
- , In Hak Lee
- & Jun Woo Choi
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Article
| Open AccessPossible intermediate quantum spin liquid phase in α-RuCl3 under high magnetic fields up to 100 T
Recent theoretical work predicted an intermediate quantum spin liquid state in α-RuCl3 in out-of-plane magnetic field. Zhou et al. present experimental evidence for this state between two magnetic transitions identified by high-field magnetization measurements.
- Xu-Guang Zhou
- , Han Li
- & Hidekazu Tanaka
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Article
| Open AccessDirected exciton transport highways in organic semiconductors
Optical properties of organic semiconductors enable various optoelectronic applications. Müller et al. report a large exciton bandwidth in a crystalline organic material and attribute it to the strong Coulomb interaction in directed exciton pathways induced by the donor–acceptor type molecular structure.
- Kai Müller
- , Karl S. Schellhammer
- & Frank Ortmann
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Article
| Open AccessUnexpected doping effects on phonon transport in quasi-one-dimensional van der Waals crystal TiS3 nanoribbons
Doping generally hinders phonon transport. Here, authors significantly increase the thermal conductivity of TiS3 nanoribbons through doping, originating from the intensified bonding strength along the molecular chain direction without distorting the one-dimensional structure induced by doped atoms.
- Chenhan Liu
- , Chao Wu
- & Yunfei Chen
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Article
| Open AccessEnhanced thermally-activated skyrmion diffusion with tunable effective gyrotropic force
Skyrmions are topological spin textures, which have been proposed as useful for a diverse array of applications. One such proposal is to make use of a skyrmion’s thermally activated Brownian-like diffusive motion for unconventional computing and true random number generation. Here, Dohi et al show how, in a synthetic antiferromagnet, this diffusive motion can be significantly enhanced.
- Takaaki Dohi
- , Markus Weißenhofer
- & Mathias Kläui
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Article
| Open AccessQuantized resistance revealed at the criticality of the quantum anomalous Hall phase transitions
Magnetization reversal in magnetic topological insulators drives quantum phase transitions between quantum anomalous Hall, axion insulator, and normal insulator states. Using novel analysis protocol, the authors investigate critical behaviours of these transitions and establish their electronic origin.
- Peng Deng
- , Peng Zhang
- & Kang L. Wang
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Article
| Open AccessAn anisotropic van der Waals dielectric for symmetry engineering in functionalized heterointerfaces
Here, the authors demonstrate that a layered anisotropic dielectric material, SiP2, can break the rotational symmetry of 2D MoS2, leading to linearly polarized photoluminescence emission and conductance anisotropy ratios up to 1000 in gated SiP2/MoS2 heterostructures.
- Zeya Li
- , Junwei Huang
- & Hongtao Yuan
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Article
| Open AccessSynergistic correlated states and nontrivial topology in coupled graphene-insulator heterostructures
Here, the authors theoretically predict the formation of synergistic correlated and topological states in Coulomb-coupled and gate-tunable graphene/insulator heterostructures, proposing a number of promising substrate candidates and a possible explanation for recent experimental observations in graphene/CrOCl heterostructures.
- Xin Lu
- , Shihao Zhang
- & Jianpeng Liu
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Article
| Open AccessSequential order dependent dark-exciton modulation in bi-layered TMD heterostructure
Here, the authors report the emergence of dark-excitons in transition-metal-dichalcogenide heterostructures that strongly rely on the stacking sequence, i.e., momentum-dark K-Q excitons located exclusively at the top layer of the heterostructure.
- Riya Sebait
- , Roberto Rosati
- & Young Hee Lee
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Article
| Open AccessNanoscale ductile fracture and associated atomistic mechanisms in a body-centered cubic refractory metal
Understanding the competing modes of brittle versus ductile fracture is critical for preventing material failure. Here, the authors reveal the atomic-scale processes of crack growth in Mo crystals, providing mechanistic insights into the ductile to brittle transition in BCC refractory metals.
- Yan Lu
- , Yongchao Chen
- & Xiaodong Han
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Article
| Open AccessMagnetic quasi-atomic electrons driven reversible structural and magnetic transitions between electride and its hydrides
Interstitial quasi-atomic electrons (IQE) have shown promising magnetic elements. Here authors present the reversible hydrogenation and dehydrogenation of ferromagnetic [Gd2C]2+ 2e− electride to canted antiferromagnet by reducing and restoring IQEs.
- Seung Yong Lee
- , Dong Cheol Lim
- & Sung Wng Kim
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Article
| Open AccessAn electronic origin of charge order in infinite-layer nickelates
Recent experiments reported charge order with a stripe pattern in parent compounds of infinite-layer nickelate superconductors. Chen et al. use first principles and effective model calculations to propose an electronic, charge-transfer-driven mechanism of the charge order.
- Hanghui Chen
- , Yi-feng Yang
- & Hongquan Liu
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Article
| Open AccessField-free spin-orbit switching of perpendicular magnetization enabled by dislocation-induced in-plane symmetry breaking
Switching the magnetization of a ferromagnetic layer with a current induced spin-orbit torques requires the breaking symmetry, either via an in-plane magnetic field, or in the case of field-free switching via a device asymmetry. Here, Liang et al carefully control the Burgers vector of crystal dislocations to break the in-plane symmetry and allow for field-free switching of magnetization in a Pt/Co heterostructure.
- Yuhan Liang
- , Di Yi
- & Yuan-Hua Lin
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Article
| Open AccessSimulating Chern insulators on a superconducting quantum processor
Quantum simulations of topological matter with superconducting qubits have been attracting attention recently. Xiang et al. realize 2D and bilayer Chern insulators with synthetic dimensions on a programmable 30-qubit-ladder superconducting processor, showing bulk-boundary correspondence.
- Zhong-Cheng Xiang
- , Kaixuan Huang
- & Heng Fan
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Article
| Open AccessTopological magneto-optical effect from skyrmion lattice
In the magneto-optical Kerr effect, light incident on a magnetic material is reflected with a shifted polarization, the size of the shift characterized by the Kerr angle. Here, Kato et al introduce a topological magneto-optical Kerr effect, where the presence of skyrmions, a type of topological spin texture, leads to a significant enhancement of the Kerr signal.
- Yoshihiro D. Kato
- , Yoshihiro Okamura
- & Youtarou Takahashi
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Article
| Open AccessEntanglement in the quantum phases of an unfrustrated Rydberg atom array
Rydberg atom arrays are a promising platform for simulating many-body systems. The authors introduce a tensor-network method to compute phase diagrams of infinite arrays with long-range interactions and experimental-scale finite arrays, unveiling a new entangled phase and offering a guide for experiments.
- Matthew J. O’Rourke
- & Garnet Kin-Lic Chan
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Article
| Open AccessLong-lived spin waves in a metallic antiferromagnet
Magnons (spin-waves) in magnetic materials offer the potential for fast and efficient information processing. To avoid excessive damping due to free electrons, one is typically limited to magnetic insulators as host materials. Here, Poelchen et al demonstrate long lived spin-waves, at terahertz frequencies in the metallic antiferromaget CeCo2P2, opening up the possibility of using metallic aniferromagnets for spinwave information processing.
- G. Poelchen
- , J. Hellwig
- & K. Kummer
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Article
| Open AccessSearch for ambient superconductivity in the Lu-N-H system
Superconductivity was recently reported experimentally in nitrogen-doped lutetium hydride with Tc = 294 K at a pressure of 1 GPa. Here, via theoretical calculations, the authors find no structures capable of supporting conventional superconductivity in the Lu-N-H system at ambient pressure.
- Pedro P. Ferreira
- , Lewis J. Conway
- & Lilia Boeri
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Article
| Open AccessLarge and tunable magnetoresistance in van der Waals ferromagnet/semiconductor junctions
Van der Waals materials are composed of layers held weakly by van der Waals forces. This feature allows different materials to be combined into heterostructures, with fewer restrictions on growth and lattice matching. Here, Zhu et al make use of this feature to create a van der Waals magnetic tunnel junction with a semiconducting spacer, allowing for improved tunability and reduced device thickness.
- Wenkai Zhu
- , Yingmei Zhu
- & Kaiyou Wang
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Article
| Open AccessFrom Stoner to local moment magnetism in atomically thin Cr2Te3
Over the last few years, several van der Waals materials have been found that retain magnetic ordering down to monolayer thickness. These materials provide a simple platform for studying the magnetism in reduced dimensions. Here, Zhong et al study the thickness dependence of magnetic ordering in Cr2Te3, and find a crossover from Stoner to Heisenberg-type magnetism as thicknesses are reduced.
- Yong Zhong
- , Cheng Peng
- & Zhi-Xun Shen
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Article
| Open AccessUnconventional specular optical rotation in the charge ordered state of Kagome metal CsV3Sb5
Kagome materials, such as CsV3Sb5, a rich array of correlated phase, including a time-reversal symmetry breaking phase, which could possibly be the result of loop currents. Attempts to verify this with magneto-optical measurements have yielded mixed results. Here, Farhang et al show that the magneto-optical signals are due to specular optical rotation. ‘
- Camron Farhang
- , Jingyuan Wang
- & Jing Xia
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Article
| Open AccessAnomalous isotope effect on mechanical properties of single atomic layer Boron Nitride
Two-dimensional materials could be good platforms to study the extremely subtle mechanical behaviors. Here, the authors measure an anomalous isotope effect on the mechanical properties of boron nitride monolayers, originated from ultrafine isotopic nuclear charge.
- Alexey Falin
- , Haifeng Lv
- & Lu Hua Li
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Article
| Open AccessIdentifying s-wave pairing symmetry in single-layer FeSe from topologically trivial edge states
The nature of the pairing symmetry in superconducting single-layer FeSe has been the subject of intense debate. Here, the authors use scanning tunneling microscopy/spectroscopy to show the absence of topological edge/corner modes, providing evidence for sign-preserving s-wave pairing.
- Zhongxu Wei
- , Shengshan Qin
- & Qi-Kun Xue
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Article
| Open AccessUncovering spin-orbit coupling-independent hidden spin polarization of energy bands in antiferromagnets
A hidden effect can occur in materials where locally a symmetry is broken, even though global symmetry is preserved. An example is hidden spin-polarization, arising from local inversion symmetry breaking in otherwise globally centro-symmetric materials. Here, Yuan et al uncover a hidden spin-polarization that can occur in antiferromagnets without spin-orbit coupling and identify the key material requirements for this to occur.
- Lin-Ding Yuan
- , Xiuwen Zhang
- & Alex Zunger
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Article
| Open AccessObservation of an Alice ring in a Bose–Einstein condensate
An Alice ring is related to the unusual topology of the monopole field and its decay. Here the authors demonstrate a topological monopole defect in the form of an Alice ring using gaseous Bose–Einstein condensates of 87Rb atoms.
- Alina Blinova
- , Roberto Zamora-Zamora
- & David S. Hall
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Article
| Open AccessRevealing intrinsic domains and fluctuations of moiré magnetism by a wide-field quantum microscope
By carefully inducing twists or lattice stacking offsets between two adjacent van der Waals crystals, a superlattice potential can be introduced. This Moire lattice offers an incredibly rich physics, ranging from superconductivity to exotic magnetism, depending on van der Waals materials in question. Here, Du et al. study the magnetic domains in twisted CrI3, and show that despite this domain structure, spin fluctuations are spatially homogenous.
- Mengqi Huang
- , Zeliang Sun
- & Chunhui Rita Du
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Article
| Open AccessControlling the propagation asymmetry of hyperbolic shear polaritons in beta-gallium oxide
Hyperbolic phonon polaritons occurring in anisotropic materials exhibit strong light confinement and propagation directionality. Matson et al. report real-space imaging and control of recently discovered hyperbolic shear phonon-polaritons in beta-Ga2O3, arising from symmetry breaking in the dielectric response.
- Joseph Matson
- , Sören Wasserroth
- & Joshua D. Caldwell
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Article
| Open AccessResonating holes vs molecular spin-orbit coupled states in group-5 lacunar spinels
Dressing is a concept used to describe moderately interacting electrons. Here authors present the notion of dressed spin-orbit 3/2 moments and how this picture breaks down with increasing electronic interactions across group-5 lacunar spinel magnets.
- Thorben Petersen
- , Pritam Bhattacharyya
- & Liviu Hozoi
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Article
| Open AccessDiscovery and construction of surface kagome electronic states induced by p-d electronic hybridization in Co3Sn2S2
Kagome materials host 2D planes which give rise to kagome physics, but these are typically embedded in the bulk. Huang et al. demonstrate a strategy for generating surface kagome electronic states by vertical p-d electronic hybridization between surface atoms and the buried Co kagome network in Co3Sn2S2.
- Li Huang
- , Xianghua Kong
- & Hong-Jun Gao
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