Featured
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Letter |
Evolution and control of oxygen order in a cuprate superconductor
The arrangement of defects in solid-state phases has an enormous influence on material properties. It is here shown that powerful X-rays can be used to change the properties of an oxide superconductor, thus effectively writing superconducting regions within an insulating matrix. The results open the way to the manipulation of superconductors and potentially other phases.
- Nicola Poccia
- , Michela Fratini
- & Antonio Bianconi
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Article |
Interface-induced room-temperature multiferroicity in BaTiO3
With only a few known useful room-temperature multiferroics, other ways of achieving materials showing magnetism as well as electrical polarization are sought. The discovery that the ferroelectric BaTiO3 also shows magnetism at room temperature at the interface with iron or cobalt marks a new approach to achieving multiferroic properties.
- S. Valencia
- , A. Crassous
- & M. Bibes
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Article |
Probing bulk electronic structure with hard X-ray angle-resolved photoemission
Angle-resolved photoemission spectroscopy is possibly the most widely used technique to probe the electronic structure of crystals. Unfortunately the technique is usually too sensitive to surface properties. It is now demonstrated that by using hard X-rays as the incident radiation it is possible to probe the electronic structure in the bulk.
- A. X. Gray
- , C. Papp
- & C. S. Fadley
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Letter |
Magnetic manipulation of self-assembled colloidal asters
A suspension of magnetic colloidal particles confined at a liquid–liquid interface and energized by an external periodic magnetic field self-assembles into star-shaped structures that can be magnetically manipulated to capture and transport smaller non-magnetic particles.
- Alexey Snezhko
- & Igor S. Aranson
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Letter |
Tailoring hot-exciton emission and lifetimes in semiconducting nanowires via whispering-gallery nanocavity plasmons
Typically, the light-emission of semiconductors always occurs from thermalized electrons, as electrons excited above the bandgap energy relax quickly. In contrast, non-thermalized excitonic light emission has now been observed in nanowires using resonant plasmonic nanocavities. The much higher radiative light-emission rates of the hot excitons suggest their use for ultrafast nanophotonic devices.
- Chang-Hee Cho
- , Carlos O. Aspetti
- & Ritesh Agarwal
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Article |
Nanoscale surfaces for the long-term maintenance of mesenchymal stem cell phenotype and multipotency
On standard tissue culture platforms, mesenchymal stem cells tend to spontaneously differentiate with the loss of multi-lineage potential. Now, a robust and reproducible nanotopographical platform has been shown to maintain stem cell phenotype and promote stem cell growth over several months whilst implicating mechanisms for the observed stem cell behaviour
- Rebecca J. McMurray
- , Nikolaj Gadegaard
- & Matthew J. Dalby
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Article |
A fast, high-endurance and scalable non-volatile memory device made from asymmetric Ta2O5−x/TaO2−x bilayer structures
Resistive switching is a promising technology to replace current non-volatile memory technologies such as flash. The demonstration of a fast, stable and highly scalable resistive-switching memory device represents a significant advance towards the practical implementation of this technology.
- Myoung-Jae Lee
- , Chang Bum Lee
- & Kinam Kim
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Letter |
Controlled enhancement of spin-current emission by three-magnon splitting
Spin current, that is, the flow of angular momentum without charge transfer, may be used in efficient spintronics devices. One problem is that spin current tends to decrease, owing to spin–orbit interaction. It is now shown that through interaction with spin waves it is possible to reverse this effect and enhance the spin current back.
- Hidekazu Kurebayashi
- , Oleksandr Dzyapko
- & Sergej O. Demokritov
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Letter |
Electrically tunable spin injector free from the impedance mismatch problem
Spin injection from a magnetic electrode into the non-magnetic active element of a spintronics device is seriously hampered by the impedance mismatch between the two materials. One common solution is to use high-quality tunnel barriers. An alternative strategy is now demonstrated through spin pumping based on dynamical spin exchange.
- K. Ando
- , S. Takahashi
- & E. Saitoh
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News & Views |
Filtering spins with molecules
Conventional magnetoresistive devices are composed of magnetic and non-magnetic films. It is now shown that, at low temperature, a carbon nanotube decorated with single-molecule magnets can function as an all-organic spin valve.
- Stefano Sanvito
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Article |
Giant Rashba-type spin splitting in bulk BiTeI
A very large Rashba-type spin splitting, which is a consequence of spin–orbit interaction, has been observed in the heavy-element semiconductor BiTeI. The results show the possibility, in principle, of using the material in spintronics devices in which the electron spin is controlled by electric currents.
- K. Ishizaka
- , M. S. Bahramy
- & Y. Tokura
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Letter |
Supramolecular spin valves
In macroscopic spin valves, the current between two magnetic electrodes can be tuned by external magnetic fields. Here, a molecular-scale spin valve is demonstrated in which a single-molecule magnet, through its localized magnetic moment, modulates the conductance of a single-walled carbon nanotube quantum dot with magnetoresistance ratios reaching 300%.
- M. Urdampilleta
- , S. Klyatskaya
- & W. Wernsdorfer
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Article |
Atomic layer-deposited tunnel oxide stabilizes silicon photoanodes for water oxidation
Electrochemical energy can be produced by using solar energy to oxidize water, providing an abundant source of electrons, which are needed in fuel synthesis. The operation of an efficient and stable semiconductor nanocomposite anode, made of a protective TiO2 layer that protects a silicon substrate during photoelectrochemical water oxidation in both dark and light conditions, is now reported.
- Yi Wei Chen
- , Jonathan D. Prange
- & Paul C. McIntyre
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Article |
Giant enhancement of spin accumulation and long-distance spin precession in metallic lateral spin valves
Pure spin current—the flow of spin angular momentum involving no charge movement—could lead to highly efficient spintronic devices. It is now shown that through low-resistivity magnetic tunnelling junctions it is possible to induce spin accumulation in solid-state devices one hundred times higher than previously obtained. This is the main requirement for generation of large spin currents.
- Yasuhiro Fukuma
- , Le Wang
- & YoshiChika Otani
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Article |
Tailoring organic heterojunction interfaces in bilayer polymer photovoltaic devices
The energy-level alignment at the heterojunction critically influences the performance of organic photovoltaic devices. It is now shown that the surface dipole moments of individual organic semiconductor films can be tuned with surface-segregated monolayers before forming bilayer solar cells by a simple film-transfer method.
- Akira Tada
- , Yanfang Geng
- & Keisuke Tajima
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Letter |
Bioinspired molecular co-catalysts bonded to a silicon photocathode for solar hydrogen evolution
The production of fuels from sunlight is crucial to the development of a sustainable energy system. Although noble metals are efficient catalysts for photoelectrochemical hydrogen evolution, earth-abundant alternatives are needed for large-scale use. Bioinspired molecular clusters based on molybdenum and sulphur are now shown to produce hydrogen at rates comparable to platinum.
- Yidong Hou
- , Billie L. Abrams
- & Ib Chorkendorff
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News & Views |
An alternating alternative
The experimental demonstration of antiferromagnetic tunnelling anisotropic magnetoresistance paves the way for spintronic devices based on antiferromagnets, rather than ferromagnets.
- Rembert Duine
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News & Views |
Let's do the twist
Local rotations in crystals change our view at the inner structure of crystals and may be the key for a whole range of hidden symmetries and novel physical effects in condensed-matter systems.
- Manfred Fiebig
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Article |
Low-temperature fabrication of high-performance metal oxide thin-film electronics via combustion processing
Solution-deposited metal oxides show great potential for large-area electronics, but they generally require high annealing temperatures, which are incompatible with flexible polymeric substrates. Combustion processing is now reported as a new low-temperature route for the deposition of diverse metal oxide films, and high-performance transistors are demonstrated using this method.
- Myung-Gil Kim
- , Mercouri G. Kanatzidis
- & Tobin J. Marks
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Article |
Rotation-reversal symmetries in crystals and handed structures
The symmetries of crystals are an important factor in the understanding of their properties. The discovery of a new symmetry type, rotation-reversal symmetry, may lead to the discovery of new rotation-based phenomena, for example in multiferroic materials.
- Venkatraman Gopalan
- & Daniel B. Litvin
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Letter |
Bottom-gated epitaxial graphene
Bottom gates in epitaxial graphene structures can now be fabricated through a technique based on nitrogen implantation. This is an important achievement to increase both the versatility of the material for fundamental studies and the potential for its use in devices.
- Daniel Waldmann
- , Johannes Jobst
- & Heiko B. Weber
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Editorial |
The super century
One hundred years after its discovery, superconductivity is still one of the most fascinating and challenging topics in condensed-matter physics.
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Interview |
SQUIDs for everything
John Clarke told Nature Materials about his work on superconducting quantum interference devices — SQUIDs — and his fascination with their applicability to many fields, from medicine to geophysics to quantum information and cosmology.
- Fabio Pulizzi
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News & Views |
Coupling of three lattice instabilities
The interaction between ferroelectric distortion and two rotational modes in some transition-metal oxides promises a strategy for strong magnetoelectronic coupling, possibly at room temperature.
- Philippe Ghosez
- & Jean-Marc Triscone
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Commentary |
To use or not to use cool superconductors?
The high critical temperature and magnetic field in cuprates and Fe-based superconductors are not enough to assure applications at higher temperatures. Making these superconductors useful involves complex and expensive technologies to address many conflicting physics and materials requirements.
- Alex Gurevich
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Commentary |
Still alluring and hard to predict at 100
Superconductivity has gone from a rare event to a ground state that pops up in materials once considered improbable, if not impossible. Although we cannot predict its occurrence yet, recent discoveries give us some clues about how to look for new — hopefully more useful — superconducting materials.
- Paul C. Canfield
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Article |
Support nanostructure boosts oxygen transfer to catalytically active platinum nanoparticles
Explaining why interactions of metal particles with oxide supports can improve their catalytic performance has proved challenging. The origin and nature of metal–oxide interactions on industrially important platinum–ceria catalysts are now clarified, together with the dependence of the catalytic activity on the structure of the support.
- Georgi N. Vayssilov
- , Yaroslava Lykhach
- & Jörg Libuda
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Letter |
A spin-valve-like magnetoresistance of an antiferromagnet-based tunnel junction
Spin-valve structures used in modern hard-drive read heads and magnetic random access memories comprise two ferromagnetic electrodes. It is now shown that antiferromagnets can be used as electrodes in spin valves. The results open a wide range of new possibilities for the choice of materials for spintronics devices.
- B. G. Park
- , J. Wunderlich
- & T. Jungwirth
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Letter |
Nodeless superconducting gap in AxFe2Se2 (A=K,Cs) revealed by angle-resolved photoemission spectroscopy
Knowledge of the symmetry of the superconducting order parameter is essential to understand the origin of superconductivity itself. Studies on the recently discovered heavily doped Fe2Se2 now show that in these compounds the order parameter has a relatively simple symmetry compared with most other Fe-based superconductors, questioning again the generality of the results obtained so far.
- Y. Zhang
- , L. X. Yang
- & D. L. Feng
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News & Views |
Interface takes charge over Si
The formation of a two-dimensional electron liquid at the interface between two insulating oxides, now extended to oxides on Si, joins a wealth of observations that reveal how electron transfer between layers is responsible for this unusual effect.
- Darrell G. Schlom
- & Jochen Mannhart
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Letter |
Observation of the intrinsic pinning of a magnetic domain wall in a ferromagnetic nanowire
Magnetic domain walls can be controlled through a spin torque, which is usually influenced by extrinsic factors, such as defects, that pin the domain walls to specific configurations. It is now shown that intrinsic pinning conditions can be achieved, which will facilitate the development of efficient information storage devices based on domain wall control.
- T. Koyama
- , D. Chiba
- & T. Ono
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Letter |
Scanning tunnelling microscopy and spectroscopy of ultra-flat graphene on hexagonal boron nitride
Using boron nitride as a substrate for graphene has been suggested as a promising way to reduce the disorder in graphene caused by space fluctuations. It is now shown by scanning tunnelling microscopy that graphene conforms perfectly to boron nitride and the charge fluctuations are minimal compared with the conventionally used substrate, silica. Boron nitride could really be the natural graphene substrate.
- Jiamin Xue
- , Javier Sanchez-Yamagishi
- & Brian J. LeRoy
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Article |
Mesophase behaviour of polyhedral particles
Monte Carlo simulations are performed to study the assembly of polyhedrons into various mesophases and crystalline states. The formation of new liquid-crystalline and plastic-crystalline phases is predicted at intermediate volume fractions and, by correlating these results with particle anisotropy and rotational symmetry, guidelines for predicting phase behaviour are proposed.
- Umang Agarwal
- & Fernando A. Escobedo
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Article |
Efficiency enhancement in organic solar cells with ferroelectric polymers
One of the key loss mechanisms in the operation of organic solar cells is the separation and extraction of the generated charge carriers from the active region. The use of a ferroelectric layer is now shown to create large internal electric fields, resulting in an enhanced carrier extraction and increased device efficiency.
- Yongbo Yuan
- , Timothy J. Reece
- & Jinsong Huang
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Letter |
Orbital reflectometry of oxide heterostructures
The occupation of electronic orbitals on the surface and interface of oxide thin films and heterostructures is a key influence over their properties, including magnetism and superconductivity. A new spectroscopy technique now provides the first quantitative, spatially resolved data of orbital occupation in oxide structures.
- Eva Benckiser
- , Maurits W. Haverkort
- & Bernhard Keimer
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Review Article |
Single dopants in semiconductors
Single dopants in semiconductors have an atom-like electron-energy spectrum whose discrete character gives them the potential for applications such as quantum information or transistors. This Review describes the marked advances in the past decade towards observing, controllably creating and manipulating single dopants, as well as their application in devices.
- Paul M. Koenraad
- & Michael E. Flatté
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Letter |
A heteroepitaxial perovskite metal-base transistor
Electronic devices based on complex oxides offer the possibility to connect electrical devices with phenomena such as magnetism and superconductivity. However, existing oxide field-effect transistors have drawbacks such as high operation voltage. The demonstration of a metal-base transistor whose geometry makes use of the strong internal electric fields in oxide heterojunctions may now offer a new platform for oxide electronics.
- Takeaki Yajima
- , Yasuyuki Hikita
- & Harold Y. Hwang
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Article |
Ultralow-voltage field-ionization discharge on whiskered silicon nanowires for gas-sensing applications
Devices that can field-ionize gas molecules at low bias voltages are promising for selective gas-sensing applications and for ion-mobility spectrometry. Field ionization is now observed at very low voltage on semiconducting whiskered silicon nanowires.
- Ramin Banan Sadeghian
- & M. Saif Islam
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Article |
Disorder-induced localization in crystalline phase-change materials
Phase-change materials are used in computer memories for their switching between amorphous and crystalline phases. However, even the crystalline state shows disorder, with extremely small electron mean free paths. The discovery that, depending on annealing temperature, this disorder leads to a metal–insulator transition in the crystalline phase provides a completely new look at the transport properties of these compounds.
- T. Siegrist
- , P. Jost
- & M. Wuttig
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Letter |
Suppression of electronic friction on Nb films in the superconducting state
Is friction dominated by electrons or by lattice vibrations? A nano-contact experiment shows that on a Nb surface friction drops by a factor of three when crossing the superconductivity transition, showing that it has essentially an electronic nature in the metallic state, whereas the phononic contribution dominates in the superconducting state.
- Marcin Kisiel
- , Enrico Gnecco
- & Ernst Meyer
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Article |
From local structure to nanosecond recrystallization dynamics in AgInSbTe phase-change materials
Phase-change materials are key components in rewritable optical disks and are promising for non-volatile electronic memories. The very different structure and ultrafast recrystallization dynamics of another class of phase-change materials, Sb–Te-based alloys, now suggests their use in future memory applications.
- Toshiyuki Matsunaga
- , Jaakko Akola
- & Rie Kojima
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News & Views |
Interfaces are critical
A suitably chosen thin layer inserted between a ferromagnetic electrode and an organic semiconductor allows control over the polarization of the injected spins.
- Paul Ruden
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News & Views |
Transistors pick up steam
High annealing temperatures have limited the technological potential of solution-processed metal oxide semiconductors. It is now shown that high-quality films can be formed below 250 °C using precursors that are hydrolysed on-chip.
- Douglas Keszler
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Letter |
Low-temperature, high-performance solution-processed metal oxide thin-film transistors formed by a ‘sol–gel on chip’ process
A low-temperature, solution-based preparation of amorphous, metal oxide semiconducting thin-films is reported. This ‘sol–gel on chip’ hydrolysis approach yields thin-film transistors with high field-effect mobilities, reproducible and stable turn-on voltages and high operational stability.
- K. K. Banger
- , Y. Yamashita
- & H. Sirringhaus
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Letter |
Degradable polyester scaffolds with controlled surface chemistry combining minimal protein adsorption with specific bioactivation
A one-step preparation method of electrospun, synthetic scaffolds with controlled surface chemistry and functionality is reported. On addition of amphiphilic macromolecules, non-specific protein adsorption on the fibres’ surfaces is reduced, and by the further covalent attachment of certain peptide sequences to the fibres, specific bioactivation of the scaffold is achieved.
- Dirk Grafahrend
- , Karl-Heinz Heffels
- & Jürgen Groll
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Letter |
Organic electronic ratchets doing work
Ratchet systems can extract work from non-equilibrium processes. Yet present electronic ratchets only operate at cryogenic temperatures and generate low currents, which are clear limitations for their practical use. Now, organic electronic ratchets providing enough power to drive simple logic circuits at room temperature have been realized.
- Erik M. Roeling
- , Wijnand Chr. Germs
- & Martijn Kemerink
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Article |
A polycationic antimicrobial and biocompatible hydrogel with microbe membrane suctioning ability
A polymeric hydrogel coating shows impressive antimicrobial activity against both bacteria and fungi. The biocompatible and reusable coating, formed of a polycationic nanoporous hydrogel, is thought to act by drawing anionic sections of phospholipids on bacterial cell membranes into its pores, causing membrane disruption and cell death.
- Peng Li
- , Yin Fun Poon
- & Mary B. Chan-Park
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