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| Open AccessLow-k nano-dielectrics facilitate electric-field induced phase transition in high-k ferroelectric polymers for sustainable electrocaloric refrigeration
Low-k nanodiamonds are discovered to possess the ability to concurrently enhance the electrocaloric effect, thermal conductivity, and electrical stability of polymeric nanocomposites, providing support for electrocaloric refrigeration.
- Qiang Li
- , Luqi Wei
- & Xiaoshi Qian
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Article
| Open AccessTowards near-term quantum simulation of materials
The use of NISQ devices for useful quantum simulations of materials and chemistry is still mainly limited by the necessary circuit depth. Here, the authors propose to combine classically-generated effective Hamiltonians, hybrid fermion-to-qubit mapping and circuit optimisations to bring this requirement closer to experimental feasibility.
- Laura Clinton
- , Toby Cubitt
- & Evan Sheridan
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Article
| Open AccessMagnon thermal Hall effect via emergent SU(3) flux on the antiferromagnetic skyrmion lattice
Strongly correlated and topological phases of matter can be often described using the tools of quantum field theory. Here the authors report the thermal Hall effect in the antiferromagnetic skyrmion lattice of MnSc2S4, revealing transport features that can be attributed to an emergent SU(3) gauge field.
- Hikaru Takeda
- , Masataka Kawano
- & Chisa Hotta
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Article
| Open AccessInvestigating the role of undercoordinated Pt sites at the surface of layered PtTe2 for methanol decomposition
Methanol on under-coordinated Pt sites at surface Te vacancies on layered PtTe2 decomposes at a probability >90 % which ultimately produces gaseous molecular hydrogen, methane, water and formaldehyde.
- Jing-Wen Hsueh
- , Lai-Hsiang Kuo
- & Meng-Fan Luo
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Article
| Open AccessUnraveling the crucial role of trace oxygen in organic semiconductors
Conventional deoxygenation methods typically result in inevitable trace oxygen residue in organic semiconductors. Here, Huang et al. reports a non-destructive soft-plasma treatment for deoxygenation and that removal of trace oxygen can be used to modulate p-type characteristics.
- Yinan Huang
- , Kunjie Wu
- & Wenping Hu
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Article
| Open AccessMicrowave quantum diode
Quantum devices exhibiting non-reciprocal behaviour have been attracting attention for fundamental studies and applications. Here the authors report a microwave quantum diode based on a superconducting flux qubit coupled to two resonators, which has the advantage of compactness and scalability.
- Rishabh Upadhyay
- , Dmitry S. Golubev
- & Jukka P. Pekola
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Article
| Open AccessDirect bandgap emission from strain-doped germanium
The authors proposed a Silicon technology-compatible approach to convert Germanium from an indirect bandgap to a direct bandgap via doping. This is done to expand the lattice to produce tunable effective tensile strain, aiming towards the on-chip light sources.
- Lin-Ding Yuan
- , Shu-Shen Li
- & Jun-Wei Luo
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Article
| Open AccessMicroscopic mechanisms of pressure-induced amorphous-amorphous transitions and crystallisation in silicon
The mechanism of amorphous-amorphous transitions is highly debated. Here, the authors use molecular dynamics simulations to reveal transitions via nucleation-growth or spinodal decomposition, resembling a thermodynamic phase transition but influenced by mechanics.
- Zhao Fan
- & Hajime Tanaka
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Article
| Open AccessSpin-resolved topology and partial axion angles in three-dimensional insulators
3D higher-order topological insulators (HOTIs) exhibit 1D hinge states depending on extrinsic sample details, while intrinsic features of HOTIs remain unknown. Here, K.S. Lin et al. introduce the framework of spin-resolved topology to show that helical HOTIs can realize a doubled axion insulator phase with nontrivial partial axion angles.
- Kuan-Sen Lin
- , Giandomenico Palumbo
- & Barry Bradlyn
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Article
| Open AccessA ferroelectric fin diode for robust non-volatile memory
Designing efficient high-density crossbar arrays are nowadays highly demanded for many artificial intelligence applications. Here, the authors propose a two-terminal ferroelectric fin diode non-volatile memory in which a ferroelectric capacitor and a fin-like semiconductor channel are combined to share both top and bottom electrodes with high performance and easy fabrication process
- Guangdi Feng
- , Qiuxiang Zhu
- & Chungang Duan
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Article
| Open AccessField control of quasiparticle decay in a quantum antiferromagnet
Quasiparticles’ have formed an extremely effective explanation for the charge, spin and lattice excitations of materials, allowing for the otherwise complex response to be explained in terms of a single (quasi)particle with an effective Hamiltonian. Here, Hasegawa et al demonstrate the tuning of magnon quasiparticle decay in the quantum antiferromagnet, RbFeCl3.’
- Shunsuke Hasegawa
- , Hodaka Kikuchi
- & Takatsugu Masuda
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Article
| Open AccessTracking a spin-polarized superconducting bound state across a quantum phase transition
The Yu-Shiba-Rusinov state, arising from exchange coupling between a magnetic impurity and a superconductor, undergoes a quantum phase transition at a critical coupling. In a scanning tunnelling microscopy experiment, Karan et al. reveal distinct tunnelling spectra on each side of the transition in a magnetic field, which allows them to distinguish the free spin regime from the screened spin regime.
- Sujoy Karan
- , Haonan Huang
- & Christian R. Ast
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Article
| Open AccessLow-temperature grapho-epitaxial La-substituted BiFeO3 on metallic perovskite
In the field of multiferroic thin films, attaining low-temperature epitaxy has been a long-standing problem. In this work, authors propose a pathway to significantly reduce the BiFeO3 thin film growth temperature using the BaBiPbO3 template.
- Sajid Husain
- , Isaac Harris
- & Ramamoorthy Ramesh
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Article
| Open AccessTemperature and quantum anharmonic lattice effects on stability and superconductivity in lutetium trihydride
Superconductivity was recently reported experimentally in nitrogen-doped lutetium hydride with Tc = 294 K at 1 GPa. Here, via theoretical calculations taking into account temperature and quantum anharmonic lattice effects, the authors find that room-temperature superconductivity in the suggested parent phase of LuH3 cannot be explained by a conventional electron-phonon mediated pairing mechanism.
- Roman Lucrezi
- , Pedro P. Ferreira
- & Christoph Heil
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Article
| Open AccessField-induced bound-state condensation and spin-nematic phase in SrCu2(BO3)2 revealed by neutron scattering up to 25.9 T
SrCu2(BO3)2 realizes the Shastry-Sutherland model (SSM), a 2D frustrated dimer model. Here, via high-magnetic-field inelastic neutron scattering measurements and matrix-product-state calculations, Fogh et al. find evidence for Bose-Einstein condensation of S = 2 two-triplon bound states, which is a spin-nematic phase.
- Ellen Fogh
- , Mithilesh Nayak
- & Henrik M. Rønnow
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Article
| Open AccessMotion and teleportation of polar bubbles in low-dimensional ferroelectrics
Nanoscale ferroelectric domains called electric bubbles are shown to behave as dynamical particles. Using atomistic simulations and experiments, the authors reveal a bubble liquid phase and demonstrate teleportation-like displacements of single bubbles.
- S. Prokhorenko
- , Y. Nahas
- & L. Bellaiche
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Article
| Open AccessDirect observation of strong surface reconstruction in partially reduced nickelate films
Surface polarity affects the electronic and structural properties of oxide thin films through electrostatic effects, which is challenging to control. Here, the authors probe the tunable surface polarity at the atomic scale.
- Chao Yang
- , Rebecca Pons
- & Peter A. van Aken
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Article
| Open AccessSwitchable tribology of ferroelectrics
The interaction of flexoelectric polarization arising from strain gradients with ferroelectricity impacts tribological properties and facilitates fine physical lithography without masks or chemicals, with potential applications in various fields.
- Seongwoo Cho
- , Iaroslav Gaponenko
- & Seungbum Hong
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Article
| Open AccessTunable and parabolic piezoelectricity in hafnia under epitaxial strain
The sign of longitudinal piezoelectric coefficients is typically positive. Here, the authors tune the sign of the linear piezoelectric coefficient of HfO2 from positive to negative via epitaxial strain, finding nonlinear and parabolic piezoelectric behaviors at tensile epitaxial strain.
- Hao Cheng
- , Peijie Jiao
- & Yurong Yang
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Article
| Open AccessElectrically and mechanically driven rotation of polar spirals in a relaxor ferroelectric polymer
Polar spirals induced in a relaxor ferroelectric can be quasi-continuously rotated by applying electric/mechanical fields, due to an asymmetric Coulomb interaction. The rotations are non-volatile with robust retention, and can be optically read out.
- Mengfan Guo
- , Erxiang Xu
- & Yang Shen
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Article
| Open AccessPhase transitions in 2D multistable mechanical metamaterials via collisions of soliton-like pulses
In high-dimensional multistable mechanical metamaterials, phase transitions can be remotely nucleated and controlled via collisions of nonlinear pulses, potentially bringing new insights for the design of reconfigurable structures.
- Weijian Jiao
- , Hang Shu
- & Jordan R. Raney
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Article
| Open AccessControllable strain-driven topological phase transition and dominant surface-state transport in HfTe5
Manipulating the topological phases of quantum materials is necessary to fully leverage their potential for future electronics. Here, the authors experimentally demonstrate the controllable transition from a weak to a strong topological insulator phase through the in-situ application of high strain.
- Jinyu Liu
- , Yinong Zhou
- & Luis A. Jauregui
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Article
| Open AccessMultiresistance states in ferro- and antiferroelectric trilayer boron nitride
Here, the authors use three-layer boron nitride to construct interfacial ferro- and antiferroelectric tunnel junctions and find that the polarization is flipped in a layer-by-layer way, resulting in multiresistance states.
- Ming Lv
- , Jiulong Wang
- & Jiamin Xue
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Article
| Open AccessResolving electron and hole transport properties in semiconductor materials by constant light-induced magneto transport
Here, the authors introduce a constant light-induced magneto-transport method which seamlessly integrates light, current, and a magnetic field to characterize electron and hole properties across an expansive array of materials.
- Artem Musiienko
- , Fengjiu Yang
- & Antonio Abate
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Article
| Open AccessSpin relaxation of electron and hole polarons in ambipolar conjugated polymers
Spin and charge dynamics are inevitably linked, the study of the one often illuminating the other. Here, the authors study spin relaxation in ambipolar polymers and, backed by simulations, show how charge dynamics and wavefunction localization together set relaxation times up to room temperature.
- Remington L. Carey
- , Samuele Giannini
- & Henning Sirringhaus
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Article
| Open AccessThermal Hall effects due to topological spin fluctuations in YMnO3
The thermal Hall effect has been reported in several materials, but it is not expected in triangular lattice systems due to chirality cancellation. Kim et al. report the thermal Hall effect attributed to topological spin fluctuations in the supposedly paramagnetic phase of YMnO3 with a trimerized triangular lattice.
- Ha-Leem Kim
- , Takuma Saito
- & Je-Geun Park
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Article
| Open AccessNonlinear transport and radio frequency rectification in BiTeBr at room temperature
The second order nonlinear Hall effect leads to a direct voltage generated from the rectification effect. While this rectification property is appeal for use in devices, most materials exhibiting a second order nonlinear hall effect are constrained to low temperatures. Here, Lu et al demonstrate a second order nonlinear transport behaviour that persists above room temperature in BiTeBr, and construct a prototype rectifier based on this effect.
- Xiu Fang Lu
- , Cheng-Ping Zhang
- & Kian Ping Loh
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Article
| Open AccessQuasi-2D Fermi surface in the anomalous superconductor UTe2
A. G. Eaton et al. directly probe the Fermi surface of the candidate triplet superconductor UTe2 by measuring magnetic quantum oscillations in ultra-pure crystals. By comparison with model calculations, the data are found to be consistent with a Fermi surface that consists of two cylindrical sections of electron and hole-type respectively.
- A. G. Eaton
- , T. I. Weinberger
- & M. Vališka
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Article
| Open AccessOrbital-flop transition of superfluid 3He in anisotropic silica aerogel
When imbibed in an anisotropic silica aerogel, superfluid 3He undergoes a temperature-driven “orbital flop" transition, where the orbital quantization axis rotates by 90 degrees. Here, by simulating planar and nematic aerogel, M. D. Nguyen et al. show that the orbital flop transition is driven by the distinct large- and small-scale structures of the aerogel.
- M. D. Nguyen
- , Joshua Simon
- & W. P. Halperin
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Article
| Open AccessFrequency-hopping wave engineering with metasurfaces
Metasurfaces show variable scattering with frequency sequence. This frequency-hopping response breaks a conventional linear frequency concept and markedly expands available frequency channels from a linear number to its factorial number.
- Hiroki Takeshita
- , Ashif Aminulloh Fathnan
- & Hiroki Wakatsuchi
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Article
| Open AccessField-induced compensation of magnetic exchange as the possible origin of reentrant superconductivity in UTe2
The superconductor UTe2 exhibits a reentrant superconducting phase at magnetic fields above 40 T for particular field angles. Here, from high-field Hall-effect measurements, T. Helm et al. find evidence for a partial compensation between the applied field and an exchange field, pointing to the Jaccarino-Peter effect as a possible mechanism for the reentrant superconductivity.
- Toni Helm
- , Motoi Kimata
- & Jean-Pascal Brison
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Article
| Open AccessFractional quantum ferroelectricity
A concept of fractional quantum ferroelectricity is proposed, where the direction of ferroelectric polarization difference no longer subjects to the symmetry restrictions of Neumann’s principle. It indicates that ferroelectricity can exist in nonpolar systems, which may lead to discovery of many overlooked ferroelectrics.
- Junyi Ji
- , Guoliang Yu
- & H. J. Xiang
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Article
| Open AccessParity-conserving Cooper-pair transport and ideal superconducting diode in planar germanium
M. Valentini et al. study superconducting quantum interference devices (SQUIDs) where the weak link of the Josephson junctions is a germanium 2D hole gas. They report signatures of the tunneling of pairs of Cooper pairs. For a particular microwave drive power, they observe a 100% efficient superconducting diode effect.
- Marco Valentini
- , Oliver Sagi
- & Georgios Katsaros
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Article
| Open AccessExact inversion of partially coherent dynamical electron scattering for picometric structure retrieval
By combining real and diffraction space data recorded in electron microscopes, ptychography retrieves specimen details with super-resolution. Here, the inverse problem is solved in the presence of thermal diffuse scattering and applied to measure ferroelectric displacements with picometer precision.
- Benedikt Diederichs
- , Ziria Herdegen
- & Knut Müller-Caspary
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Article
| Open AccessUnderstanding the light induced hydrophilicity of metal-oxide thin films
Light-induced hydrophilicity of TiO2 and ZnO surfaces rely on the same physics and involve excitation of electron-hole pairs. Here, the authors propose and test a model for the photowetting of TiO2 and ZnO thin films. The results suggest design rules for materials exhibiting photocatalytic wetting.
- Rucha Anil Deshpande
- , Jesper Navne
- & Rafael Taboryski
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Article
| Open AccessHow spin relaxes and dephases in bulk halide perovskites
Halide perovskites exhibit largely tunable spin-orbit interactions, and long carrier lifetimes, making this class of materials promising for spintronic applications. Here, Xu et al present first principles calculations to determine the spin lifetimes, and identify the dominant spin-relaxation and dephasing processes.
- Junqing Xu
- , Kejun Li
- & Yuan Ping
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Article
| Open AccessTransition to the Haldane phase driven by electron-electron correlations
At the microscopic level, the localized spins arise due to the electron-electron interactions. Here, the authors show how a topological phase of the Haldane spin chain emerges in a two-orbital Hubbard model with increasing interaction strength.
- A. Jażdżewska
- , M. Mierzejewski
- & J. Herbrych
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Article
| Open AccessLarge exchange bias enhancement and control of ferromagnetic energy landscape by solid-state hydrogen gating
“Exchange bias” occurs in heterostructures of antiferromagnets and ferromagnetic materials, which biases the magnetization of the ferromagnet so that it exhibits a preferred direction. This phenomenon has proven critical for the development of a variety of spintronic devices. Here, Hasan et al demonstrate reversible control of exchange bias via solid-state hydrogen gating.
- M. Usama Hasan
- , Alexander E. Kossak
- & Geoffrey S. D. Beach
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Article
| Open AccessMagnetic order in 2D antiferromagnets revealed by spontaneous anisotropic magnetostriction
Van der Waals antiferromagnets offer a unique platform for studying magnetism in reduced dimensions, however, the low dimensionality, combined with lack of net magnetization, renders investigation challenging with conventional experimental probes. Here, Houmes et al show how van der Waals antiferromagnets can be investigated via the resonances of a vibrating rectangular membranes of this material.
- Maurits J. A. Houmes
- , Gabriele Baglioni
- & Herre S. J. van der Zant
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Article
| Open AccessA broad-spectrum gas sensor based on correlated two-dimensional electron gas
Gas sensors typically detect only few specific gases; the authors show a broad-spectrum sensor based on correlated 2-dimensional electron gas (C-2DEG), which detects various gases quantitatively and measures partial pressures, through a purely physical mechanism.
- Yuhao Hong
- , Long Wei
- & Zhaoliang Liao
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Article
| Open AccessOrbital perspective on high-harmonic generation from solids
Here the authors identify real-space contributions to the characteristics of high-harmonic generation in ReS2 and demonstrate the possibility of laser-controlled emission. They find that the spectrum is not just determined by the band structure, but also by the interference between HHG signals coming from different atoms within the unit cell.
- Álvaro Jiménez-Galán
- , Chandler Bossaer
- & Giulio Vampa
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Article
| Open AccessStrain-driven Kovacs-like memory effect in glasses
An abnormal stress memory effect is discovered in different types of glassy materials when they are subjected to a low strain after a high strain. This strategy can be used to depress the stress relaxation and increase the stability under loading.
- Yu Tong
- , Lijian Song
- & Jun-Qiang Wang
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Article
| Open AccessTetrahedral triple-Q magnetic ordering and large spontaneous Hall conductivity in the metallic triangular antiferromagnet Co1/3TaS2
Skyrmion crystals, where skyrmions are arranged close packed in a triangular lattice arise due to the superposition of three magnetic spin spirals, each with a distinct wave vector, Q. Such skrymion crystals have been found in a diverse array of materials. Here, Park et al find a short wavelength (or dense skyrmion) limit of this skyrmion crystal structure in Co1/3TaS2, a metallic triangular lattice antiferromagnet, in the form of a triple Q magnetic ordering, with four magnetic sublattices.’
- Pyeongjae Park
- , Woonghee Cho
- & Je-Geun Park
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Article
| Open AccessOn-chip phonon-magnon reservoir for neuromorphic computing
Developing efficient reservoir computing hardware that combines optically excited acoustic and spin waves with high spatial density remains a challenge. In this work, the authors propose a design capable of recognizing visual shapes drawn by a laser within remarkably confined spaces, down to 10 square microns.
- Dmytro D. Yaremkevich
- , Alexey V. Scherbakov
- & Manfred Bayer
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Article
| Open AccessHow frictional slip evolves
Conventionally, a continuous motion or “dynamic friction” is expected to take place after the initial rupture under friction. Here, the authors perform direct measurement of real contact and slip at the frictional interface and show that the secondary rupture takes place after each initial rupture.
- Songlin Shi
- , Meng Wang
- & Jay Fineberg
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Article
| Open AccessHyperbolic exciton polaritons in a van der Waals magnet
Hyperbolic exciton polaritons (HEPs) are anisotropic light-matter excitations with promising applications, but their steady-state observation is challenging. Here, the authors report experimental evidence of HEPs in a van der Waals magnet, CrSBr, via cryogenic infrared near-field microscopy.
- Francesco L. Ruta
- , Shuai Zhang
- & D. N. Basov
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Article
| Open AccessThermodynamic behavior of correlated electron-hole fluids in van der Waals heterostructures
Transition metal dichalcogenide bilayers offer a novel platform for studying correlated electron-hole fluids. Here the authors use optical spectroscopy to probe thermodynamic properties of coupled electron-hole states in MoSe2/hBN/WSe2 heterostructures, providing evidence for an excitonic insulator ground state.
- Ruishi Qi
- , Andrew Y. Joe
- & Feng Wang
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Article
| Open AccessPhase-dependent Andreev molecules and superconducting gap closing in coherently-coupled Josephson junctions
S. Matsuo et al. report tunneling spectroscopy measurements on a device consisting of two Josephson junctions (JJ) sharing a single superconducting electrode. In isolation, each JJ would host an Andreev bound state (ABS). In their coherently-coupled JJs, the authors report the formation of an Andreev molecule due to hybridization of the two ABSs.
- Sadashige Matsuo
- , Takaya Imoto
- & Seigo Tarucha
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Article
| Open AccessA coherent phonon-induced hidden quadrupolar ordered state in Ca2RuO4
Ultrafast laser excitation can generate metastable states in quantum materials, with no counterpart in equilibrium. Here the authors demonstrate a transient quadrupolar ordered state in Ca2RuO4 single crystals via excitation of a phonon mode coupled to the order parameter.
- Honglie Ning
- , Omar Mehio
- & David Hsieh
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