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Featured
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Article |
Light-induced electronic polarization in antiferromagnetic Cr2O3
A light-induced polar electronic state is generated in Cr2O3; the symmetry reduction occurs on an ultrafast timescale, ruling out contributions from the lattice or spins.
- Xinshu Zhang
- , Tyler Carbin
- & Anshul Kogar
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Article |
Phase patterning of liquid crystal elastomers by laser-induced dynamic crosslinking
Lack of local phase patterning in liquid crystal elastomers has hindered their broad implementation. The authors report a laser-induced dynamic crosslinking approach with allyl sulfide groups to achieve reconfigurable high-resolution patterning of multiple liquid crystalline phases in a single film.
- Seok Hwan Choi
- , Ju Hee Kim
- & Seung Hwan Ko
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Article
| Open AccessSuppression of Dexter transfer by covalent encapsulation for efficient matrix-free narrowband deep blue hyperfluorescent OLEDs
Suppressed Dexter transfer is needed to achieve efficient and stable hyperfluorescence, but complex matrices must be involved. A molecular design strategy has been proposed where Dexter transfer can be substantially reduced by an encapsulated terminal emitter, leading to ‘matrix-free’ hyperfluorescence.
- Hwan-Hee Cho
- , Daniel G. Congrave
- & Hugo Bronstein
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Article |
High-quality nanocavities through multimodal confinement of hyperbolic polaritons in hexagonal boron nitride
Exploiting optical multimodal confinement, the deep-subwavelength confinement of hyperbolic phonon polaritons is demonstrated in isotopically pure hexagonal boron nitride, enabling nanoscale polariton manipulation.
- Hanan Herzig Sheinfux
- , Lorenzo Orsini
- & Frank H. L. Koppens
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Article |
General room-temperature Suzuki–Miyaura polymerization for organic electronics
A general process for a room-temperature, homogeneous Suzuki–Miyaura-type polymerization is reported, demonstrating a route for the scalable production of device-quality conjugated polymers.
- Haigen Xiong
- , Qijie Lin
- & Hui Huang
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Article
| Open AccessReal-time single-proton counting with transmissive perovskite nanocrystal scintillators
Current organic proton detectors have poor detection sensitivities due to low light yields and limited radiation toleration. Here the authors report a perovskite nanocrystal-based transmissive thin scintillator that can detect seven protons per second, enabled by radiative emission from biexcitons.
- Zhaohong Mi
- , Hongyu Bian
- & Xiaogang Liu
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Article
| Open AccessUltrafast vibrational control of organohalide perovskite optoelectronic devices using vibrationally promoted electronic resonance
Optically stimulated vibrational control for materials has the potential to improve the performance of optoelectronic devices. The vibrational control of FAPbBr3 perovskite solar cells has been demonstrated, where the fast dynamics of coupling between cations and inorganic sublattice may suppress non-radiative recombinations in perovskites, leading to reduced voltage losses.
- Nathaniel. P. Gallop
- , Dmitry R. Maslennikov
- & Artem A. Bakulin
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News & Views |
Magnetic proximity boosts chiral quantum emission
Chiral single-photon emitters are desirable, versatile tools for quantum information processing. Exploiting proximity to a strain-induced local magnetic field in the van der Waals antiferromagnet NiPS3 enables the emission of high-purity chiral single photons from monolayer WSe2 at zero external magnetic field.
- Jing Tang
- & Xi Ling
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Letter |
Proximity-induced chiral quantum light generation in strain-engineered WSe2/NiPS3 heterostructures
Proximity-induced chiral quantum emission is generated by applying nanoindentation on monolayer WSe2 on an antiferromagnetic van der Waals material (NiPS3) at zero external magnetic fields, reporting a degree of circular polarization of 0.89 and a single-photon purity of 95%.
- Xiangzhi Li
- , Andrew C. Jones
- & Han Htoon
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Research Briefing |
A strategy for obtaining AlN heteroepitaxial films with high crystalline quality
High-quality aluminium nitride (AlN) heteroepitaxial films are obtained by the controlled discretization and coalescence of columns using nanopatterned AlN/sapphire templates with regular hexagonal holes. The density of dislocation etch pits in the AlN heteroepitaxial films is reduced to approximately 104 cm–2, approaching the value of that in AlN bulk single crystals.
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News & Views |
A twist for nanolight
Controlling the twist angles between three α-phase molybdenum trioxide single layers enables the programmable and reconfigurable canalization of phonon polaritons along multiple in-plane directions.
- Siyuan Dai
- & Qiong Ma
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Article |
Group-III nitride heteroepitaxial films approaching bulk-class quality
High-quality AlN heteroepitaxial films are obtained by controllable discretization and coalescence of columns on nano-patterned AlN/sapphire templates with hexagonal holes, where the density of dislocation etch pits is greatly reduced to ~10 × 104 cm−2.
- Jiaming Wang
- , Nan Xie
- & Bo Shen
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Article
| Open AccessIntrinsic strong light-matter coupling with self-hybridized bound states in the continuum in van der Waals metasurfaces
The authors demonstrate strong coupling in bound state in the continuum metasurfaces on nanostructured bulk WS2 and exhibiting sharp resonances with tailored linewidths and controllable light-matter coupling strength.
- Thomas Weber
- , Lucca Kühner
- & Andreas Tittl
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Article |
Real-space observation of ultraconfined in-plane anisotropic acoustic terahertz plasmon polaritons
Employing terahertz nanoscopy, we image highly confined, in-plane anisotropic acoustic terahertz plasmon polaritons in monoclinic Ag2Te platelets placed above a Au layer, verifying a linear dispersion and elliptical isofrequency contour in momentum space.
- S. Chen
- , P. L. Leng
- & R. Hillenbrand
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Letter |
Laser writing of spin defects in nanophotonic cavities
Using direct laser writing with a nanosecond pulsed laser operating at above-bandgap photon energies, we demonstrate the selective formation of spin defects in photonic crystal cavities in 4H-silicon carbide and their in situ characterization.
- Aaron M. Day
- , Jonathan R. Dietz
- & Evelyn L. Hu
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Letter |
Compact spin-valley-locked perovskite emission
We report compact spin-valley-locked perovskite emitting metasurfaces where spin-dependent geometric phases are imparted into bound states in the continuum via Brillouin zone folding, simultaneously enabling chiral purity, directionality and large emission angles.
- Yang Chen
- , Jiangang Feng
- & Cheng-Wei Qiu
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Article |
High-efficiency stretchable light-emitting polymers from thermally activated delayed fluorescence
We synthesized stretchable electroluminescent polymers capable of reaching a near-unity theoretical quantum yield through thermally activated delayed fluorescence. Their polymers show 125% stretchability with 10% external quantum efficiency and demonstrate a fully stretchable organic light-emitting diode.
- Wei Liu
- , Cheng Zhang
- & Sihong Wang
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Letter |
Observation of a massive phason in a charge-density-wave insulator
We report the observation of narrowband terahertz emission from a quasi-one-dimensional charge-density-wave insulator, (TaSe4)2I. The origin of the emitted radiation is interpreted as a phason that obtains mass due to the long-range Coulomb interaction.
- Soyeun Kim
- , Yinchuan Lv
- & Fahad Mahmood
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News & Views |
Ultrafast plasmonics shapes electron beams
By exploiting optical phase-modulation at complex surface plasmon polariton patterns, as well as energy-filtered imaging, femtosecond electron pulses are dynamically shaped in phase and amplitude.
- Armin Feist
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Article |
From enhanced diffusion to ultrafast ballistic motion of hybrid light–matter excitations
The authors study ultrafast spatiotemporal dynamics of polaritons formed by mixing surface-bound optical waves with excitons observing a mobility transition from diffusive to ballistic transport flow at two-thirds the speed of light.
- Mukundakumar Balasubrahmaniyam
- , Arie Simkhovich
- & Tal Schwartz
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Article |
Topological steering of light by nematic vortices and analogy to cosmic strings
Liquid crystal (LC) applications typically rely on defining the non-topological spatial patterns of the optical axis. Here, the authors demonstrate the topological steering of light by LC nematic vortices, futher establishing an analogy between topological light steering by LC vortices and cosmic strings.
- Cuiling Meng
- , Jin-Sheng Wu
- & Ivan I. Smalyukh
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News & Views |
The colour of stress
Periodic nanostructures create brilliant colours, termed structural colouration, through light scattering and refraction. Now, using a simple and scalable method, stress- and strain-induced dynamic colour shifts are realized in stretchable polymers.
- Daeyeon Won
- & Seung Hwan Ko
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News & Views |
Metasurfaces provide the extra bling
Structuring surfaces coated with nanoparticles in the subwavelength range allows almost complete control over the optical appearance of an object.
- Frank Scheffold
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Article |
Nuclear spin polarization and control in hexagonal boron nitride
Unlike electron spins, nuclear spins in van der Waals materials remain a largely untapped quantum resource. Here we report the fast coherent control of nuclear spins and strong electron-mediated nuclear–nuclear spin coupling in hexagonal boron nitride.
- Xingyu Gao
- , Sumukh Vaidya
- & Tongcang Li
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Letter |
Scalable optical manufacture of dynamic structural colour in stretchable materials
Desired for optical sensing or visual communications, structural colour-changing materials are hindered by the lack of scalable manufacturing. Here, by adapting Lippmann photography, large-area manufacturing of colour patterns in photosensitive elastomers is realized.
- Benjamin Harvey Miller
- , Helen Liu
- & Mathias Kolle
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News & Views |
A tale of two dimensionalities
Excitonic states with hybrid dimensionality in layered silicon diphosphide exhibit interesting features such as linearly dichroic photoluminescence and unusually strong exciton–phonon coupling.
- Matthieu Fortin-Deschênes
- & Fengnian Xia
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Article |
Halide perovskites enable polaritonic XY spin Hamiltonian at room temperature
The realization of large-scale exciton–polariton platforms operating at room temperature and exhibiting long-lived, strongly interacting excitons has been elusive. Here, the authors demonstrate a room-temperature perovskite-based polaritonic platform with a polariton lattice size of up to 10 × 10.
- Renjie Tao
- , Kai Peng
- & Wei Bao
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News & Views |
More nodes bring more Floquet modes
A temporal modulation protocol enriches topological Floquet physics by enabling the realization of bimorphic Floquet systems where Chern and anomalous Floquet phases coexist in a single platform of laser-written waveguides.
- Alexander B. Khanikaev
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Article |
The visual appearances of disordered optical metasurfaces
A multiscale modelling platform combining nanoscale resonant scattering, mesoscale multiple scattering and macroscale light transport effectively predicts the macroscopic visual effects created by optical metamaterials with disordered nanostructures.
- Kevin Vynck
- , Romain Pacanowski
- & Philippe Lalanne
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Article |
Topological Wannier cycles induced by sub-unit-cell artificial gauge flux in a sonic crystal
Gauge fields are essential for detecting and controlling quantum dynamical systems, but their potential has yet to be fully exploited. Here, the authors insert a single-unit-cell synthetic gauge flux into a sonic crystal with the gauge phase ranging from 0 to 2π, leading to topological Wannier cycles.
- Zhi-Kang Lin
- , Ying Wu
- & Jian-Hua Jiang
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Article |
Organic long-persistent luminescence stimulated by visible light in p-type systems based on organic photoredox catalyst dopants
Organic blends based on cationic photoredox catalyst dopants in neutral donor hosts show p-type charge transport behaviour. This favours reduced reactivity to oxygen in organic long-persistent luminescence materials responsive to visible light.
- Kazuya Jinnai
- , Ryota Kabe
- & Chihaya Adachi
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Article |
Thermally activated delayed fluorescence (TADF) organic molecules for efficient X-ray scintillation and imaging
Triplet exciton harvesting through thermally activated delayed fluorescence is shown to be effective also under X-ray excitation, increasing the efficiency and imaging quality of X-ray detectors based on organic scintillation.
- Wenbo Ma
- , Yirong Su
- & Yang Michael Yang
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Article |
Photocurrent-driven transient symmetry breaking in the Weyl semimetal TaAs
The authors demonstrate ultrafast symmetry breaking by optically driven photocurrents.
- N. Sirica
- , P. P. Orth
- & R. P. Prasankumar
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Article |
Confining isolated chromophores for highly efficient blue phosphorescence
A strategy to confine phosphorescent organic chromophores within ionic crystals proves effective in suppressing non-radiative recombination channels and increasing the phosphorescence efficiency of blue-emitting heavy-atom-free emitters.
- Wenpeng Ye
- , Huili Ma
- & Wei Huang
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Perspective |
Perovskite semiconductors for room-temperature exciton-polaritonics
An outlook on the potential of lead-halide perovskites as a playground for exciton-polariton studies and for the development of polaritonic devices operating at room temperature is provided.
- Rui Su
- , Antonio Fieramosca
- & Qihua Xiong
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News & Views |
The sound of Weyl hinges
Clever 3D-printed acoustic materials allow probing a new higher-order semimetallic topological phase using audible sound.
- R. Fleury
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Article |
Bosonic condensation of exciton–polaritons in an atomically thin crystal
A coherent condensate of exciton–polaritons, extending spatially up to 4 µm and spin-polarizable with an external magnetic field, is observed at cryogenic temperatures in a MoSe2 monolayer embedded in a vertical microcavity.
- Carlos Anton-Solanas
- , Maximilian Waldherr
- & Christian Schneider
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Article |
Mechano-tunable chiral metasurfaces via colloidal assembly
Stacked elastomeric arrays containing plasmonic nanoparticles show efficient chiral responses that can be fully controlled by mechanical compression and stack rotation. These simple layered materials may be useful modulators for photonic applications.
- Patrick T. Probst
- , Martin Mayer
- & Andreas Fery
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Letter |
Observation of a phononic higher-order Weyl semimetal
Symmetry is utilized to realize a phononic higher-order Weyl semimetal.
- Li Luo
- , Hai-Xiao Wang
- & Jian-Hua Jiang
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Article |
Mid-infrared radiative emission from bright hot plasmons in graphene
The optical emission of graphene under pumping with femtosecond laser pulses contains a strong component linked to plasmon emission from the hot electrons in the system.
- Laura Kim
- , Seyoon Kim
- & Harry A. Atwater
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News & Views |
Shaking up topology with light
A light-induced topological phase transition is realized in the Dirac semimetal ZrTe5 by coherently driving symmetry-breaking phonons.
- N. S. Sirica
- & R. P. Prasankumar
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Article |
A light-induced phononic symmetry switch and giant dissipationless topological photocurrent in ZrTe5
Femtosecond optical pulses are used to generate coherent phonons that break inversion symmetry and drive anisotropic terahertz photocurrents in the topological material ZrTe5.
- Liang Luo
- , Di Cheng
- & Jigang Wang
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Article |
Dynamic multimodal holograms of conjugated organogels via dithering mask lithography
Periodic patterns with varying cross-linking densities are realized in conjugated polydiacetylene films, creating multiple holographic images—all dynamically responsive to exposure to various solvents—simultaneously in the same polymeric structures.
- Jongwon Oh
- , Dahye Baek
- & Jiseok Lee
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News & Views |
Immediately produced, immortally preserved
A complementary use of cutting-edge techniques reveals an ultrafast generation of topological magnetic textures.
- Taka-hisa Arima
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Article |
Identifying carbon as the source of visible single-photon emission from hexagonal boron nitride
Comparison of hexagonal boron nitride samples grown with different techniques and with varying carbon-doping content provides evidence that the defects emitting single photons in the visible range are carbon related.
- Noah Mendelson
- , Dipankar Chugh
- & Igor Aharonovich
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News & Views |
Quantum registers hit the right wavelength
Controlling nuclear spins coupled to an electron spin in silicon carbide has enabled development of a ‘quantum register’ interfaced with telecom photons, leading to the possibility of distant transport of quantum information.
- Siddharth Dhomkar
- & John J. L. Morton
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Letter |
Carbazole isomers induce ultralong organic phosphorescence
A carbazole isomer, typically present as an impurity in commercially produced carbazole batches, is shown to be responsible for the ultralong phosphorescence observed in these compounds and their derivatives.
- Chengjian Chen
- , Zhenguo Chi
- & Bin Liu
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Article |
Configurable phonon polaritons in twisted α-MoO3
Infrared nanoimaging of phonon polaritons in twisted α-phase molybdenum trioxide bilayers reveals tunable wavefront geometries and topological transitions over a broad range of twist angles, offering a configurable platform for nanophotonic applications.
- Mingyuan Chen
- , Xiao Lin
- & Siyuan Dai
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Letter |
An integrated optical modulator operating at cryogenic temperatures
The integration of barium titanate thin films with silicon-based waveguides enables the operation of efficient electro-optic switches and modulators at temperatures as low as 4 K, with potential applications in quantum computing and cryogenic computing technologies.
- Felix Eltes
- , Gerardo E. Villarreal-Garcia
- & Stefan Abel