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| Open AccessReal-time single-proton counting with transmissive perovskite nanocrystal scintillators
Current organic proton detectors have poor detection sensitivities due to low light yields and limited radiation toleration. Here the authors report a perovskite nanocrystal-based transmissive thin scintillator that can detect seven protons per second, enabled by radiative emission from biexcitons.
- Zhaohong Mi
- , Hongyu Bian
- & Xiaogang Liu
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Letter |
Proximity-induced chiral quantum light generation in strain-engineered WSe2/NiPS3 heterostructures
Proximity-induced chiral quantum emission is generated by applying nanoindentation on monolayer WSe2 on an antiferromagnetic van der Waals material (NiPS3) at zero external magnetic fields, reporting a degree of circular polarization of 0.89 and a single-photon purity of 95%.
- Xiangzhi Li
- , Andrew C. Jones
- & Han Htoon
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News & Views |
Locking exciton fine-structure splitting
Ensemble-level experimental evidence of exciton fine-structure splitting in perovskite quantum dots has been demonstrated, correlated to the intrinsic symmetry of these nanocrystals.
- Gabriele Rainò
- & Maksym V. Kovalenko
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Article |
Lattice distortion inducing exciton splitting and coherent quantum beating in CsPbI3 perovskite quantum dots
Halide perovskites feature highly dynamic lattices, but their impact on exciton fine structure remains unexplored. Here, the authors show that these lattices lead to a bright-exciton fine structure gap, enabling observation of quantum beats in a non-uniform ensemble.
- Yaoyao Han
- , Wenfei Liang
- & Kaifeng Wu
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Article |
Nuclear spin polarization and control in hexagonal boron nitride
Unlike electron spins, nuclear spins in van der Waals materials remain a largely untapped quantum resource. Here we report the fast coherent control of nuclear spins and strong electron-mediated nuclear–nuclear spin coupling in hexagonal boron nitride.
- Xingyu Gao
- , Sumukh Vaidya
- & Tongcang Li
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Comment |
Engineering quantum materials with chiral optical cavities
Strong light–matter coupling in quantum cavities provides a pathway to break fundamental materials symmetries, like time-reversal symmetry in chiral cavities. This Comment discusses the potential to realize non-equilibrium states of matter that have so far been only accessible in ultrafast and ultrastrong laser-driven materials.
- Hannes Hübener
- , Umberto De Giovannini
- & Angel Rubio
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Article |
Identifying carbon as the source of visible single-photon emission from hexagonal boron nitride
Comparison of hexagonal boron nitride samples grown with different techniques and with varying carbon-doping content provides evidence that the defects emitting single photons in the visible range are carbon related.
- Noah Mendelson
- , Dipankar Chugh
- & Igor Aharonovich
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News & Views |
Quantum registers hit the right wavelength
Controlling nuclear spins coupled to an electron spin in silicon carbide has enabled development of a ‘quantum register’ interfaced with telecom photons, leading to the possibility of distant transport of quantum information.
- Siddharth Dhomkar
- & John J. L. Morton
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Letter |
An integrated optical modulator operating at cryogenic temperatures
The integration of barium titanate thin films with silicon-based waveguides enables the operation of efficient electro-optic switches and modulators at temperatures as low as 4 K, with potential applications in quantum computing and cryogenic computing technologies.
- Felix Eltes
- , Gerardo E. Villarreal-Garcia
- & Stefan Abel
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Article |
Dipolar interactions between localized interlayer excitons in van der Waals heterostructures
Repulsive dipole–dipole interactions between localized interlayer excitons are shown to modify the optical response of van der Waals heterobilayers, forming the basis to obtain strong optical nonlinearity and excitonic many-body states in two-dimensional materials.
- Weijie Li
- , Xin Lu
- & Ajit Srivastava
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Article |
Scalable in operando strain tuning in nanophotonic waveguides enabling three-quantum-dot superradiance
Local tuning of quantum dots embedded in a photonic waveguide can be achieved through the strain produced by laser heating of a thin layer of HfO2 deposited around the waveguide. The method is exploited to tune three quantum dots in resonance.
- Joel Q. Grim
- , Allan S. Bracker
- & Daniel Gammon
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News & Views |
Shedding light on dark excitons
A magnetic-field-dependent spectroscopy study on single perovskite nanocrystals reveals the spectral signatures of an exciton dark state below the bright triplet states.
- Andries Meijerink
- & Freddy T. Rabouw
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Letter |
Simultaneous coherence enhancement of optical and microwave transitions in solid-state electronic spins
Long coherence times in a subset of states that allows for transitions in both microwave and optical range have been reported using an isotopically purified 171Yb3+:Y2SiO5 crystal, rendering the system suitable for quantum information applications.
- Antonio Ortu
- , Alexey Tiranov
- & Mikael Afzelius
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Letter |
Solid-state electron spin lifetime limited by phononic vacuum modes
A systematic investigation of the spin relaxation in nitrogen vacancy centres in diamonds, induced by phononic vacuum modes at low temperature, reveals an upper limit of eight hours.
- T. Astner
- , J. Gugler
- & J. Majer
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Article |
Nonlinear interactions in an organic polariton condensate
Cavity polaritons have been extensively studied in inorganic materials. An organic polariton condensate is now demonstrated to occur in the strongly interacting regime, at room temperature, in a cavity containing an organic polymer.
- K. S. Daskalakis
- , S. A. Maier
- & S. Kéna-Cohen
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Letter |
A silicon carbide room-temperature single-photon source
The generation and manipulation of single photons is important for quantum information and metrology. Highly bright and stable single-photon sources are now identified in silicon carbide, a wide-bandgap semiconductor widely used for photonic and electronic devices.
- S. Castelletto
- , B. C. Johnson
- & T. Ohshima
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Article |
Self-assembled quantum dots in a nanowire system for quantum photonics
Current strategies for fabricating quantum dots embedded within nanowires suffer from a number of shortcomings. Now, a versatile self-assembly approach is demonstrated for fabricating core–shell GaAs–AlGaAs nanowires with appealing optical properties.
- M. Heiss
- , Y. Fontana
- & A. Fontcuberta i Morral
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News & Views |
Two dimensions are brighter
The synthesis of a family of plate-like semiconductor nanocrystals yields solutions of small quantum wells with excellent optical properties.
- Gregory D. Scholes