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High-quality nanocavities through multimodal confinement of hyperbolic polaritons in hexagonal boron nitride
Exploiting optical multimodal confinement, the deep-subwavelength confinement of hyperbolic phonon polaritons is demonstrated in isotopically pure hexagonal boron nitride, enabling nanoscale polariton manipulation.
- Hanan Herzig Sheinfux
- , Lorenzo Orsini
- & Frank H. L. Koppens
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Article |
Compensating losses in polariton propagation with synthesized complex frequency excitation
Propagation losses have limited the practical use of polaritons in photonic applications. Here the authors demonstrate a substantial enhancement in the propagation distance of phonon polaritons, employing synthetic optical excitation of complex frequency with virtual gain synthesized by combining multiple real frequency measurements.
- Fuxin Guan
- , Xiangdong Guo
- & Shuang Zhang
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Article |
Imaging moiré excited states with photocurrent tunnelling microscopy
The authors combine laser excitation and scanning tunnelling spectroscopy to visualize the electron and hole distributions in photoexcited moiré excitons in twisted bilayer WS2. This photocurrent tunnelling microscopy approach enables the study of photoexcited non-equilibrium moiré phenomena at atomic scales.
- Hongyuan Li
- , Ziyu Xiang
- & Feng Wang
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Research Briefing |
A spin-optical monolayer laser based on a photonic spin lattice
Inspired by valley pseudospins in two-dimensional materials, high-quality-factor (high-Q) spin–valley states were created through the photonic Rashba-type spin splitting of a bound state in the continuum. This approach enabled the construction of a coherent and controllable spin-optical laser using monolayer-integrated spin–valley microcavities without requiring magnetic fields or cryogenic temperatures.
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Article |
Broadband mid-infrared non-reciprocal absorption using magnetized gradient epsilon-near-zero thin films
Using doped InAs multilayers under moderate external magnetic fields with gradient epsilon-near-zero frequencies, broadband non-reciprocal absorption that can be tailored within the mid-infrared spectral region has been demonstrated.
- Mengqi Liu
- , Shuang Xia
- & Cheng-Wei Qiu
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Article |
Spin-valley Rashba monolayer laser
The authors introduce a spin-optical laser based on a monolayer transition metal dichalcogenide coupled to a heterostructure microcavity supporting high-Q spin-valley resonances originating from photonic Rashba-type spin splitting of a bound state in the continuum.
- Kexiu Rong
- , Xiaoyang Duan
- & Erez Hasman
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News & Views |
A twist for nanolight
Controlling the twist angles between three α-phase molybdenum trioxide single layers enables the programmable and reconfigurable canalization of phonon polaritons along multiple in-plane directions.
- Siyuan Dai
- & Qiong Ma
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Article
| Open AccessIntrinsic strong light-matter coupling with self-hybridized bound states in the continuum in van der Waals metasurfaces
The authors demonstrate strong coupling in bound state in the continuum metasurfaces on nanostructured bulk WS2 and exhibiting sharp resonances with tailored linewidths and controllable light-matter coupling strength.
- Thomas Weber
- , Lucca Kühner
- & Andreas Tittl
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Article |
Multiple and spectrally robust photonic magic angles in reconfigurable α-MoO3 trilayers
The direction of polariton canalization—its diffractionless propagation—in twisted bilayers at the magic angle is hindered by the lack of multiple magic angles. By controlling the twist angles between three α-MoO3 layers, reconfigurable and spectrally robust polariton canalization along any in-plane direction is demonstrated.
- J. Duan
- , G. Álvarez-Pérez
- & P. Alonso-González
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News & Views |
Writing above the bandgap
Above-bandgap, nanosecond laser pulses enable the localized in situ writing of spin defects in prefabricated nanophotonic cavities. The approach preserves defect and cavity mode properties, key requirements towards cavity–emitter coupling in quantum networks.
- Sridhar Majety
- & Marina Radulaski
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Article |
Strongly enhanced light–matter coupling of monolayer WS2 from a bound state in the continuum
Combining a tungsten disulfide monolayer and a topologically protected bound state in the continuum formed by a one-dimensional photonic crystal, strong light–matter interaction enhancement and large exciton–polariton nonlinearities at room temperature are demonstrated.
- Eugenio Maggiolini
- , Laura Polimeno
- & Dario Ballarini
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Letter
| Open AccessPicophotonic localization metrology beyond thermal fluctuations
The authors report subatomic precision in measuring the displacement of a nanowire. Such precision is achieved by employing deep-learning enabled analysis of single-shot scattering of topologically structured superoscillatory illumination.
- Tongjun Liu
- , Cheng-Hung Chi
- & Nikolay I. Zheludev
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Article |
Real-space observation of ultraconfined in-plane anisotropic acoustic terahertz plasmon polaritons
Employing terahertz nanoscopy, we image highly confined, in-plane anisotropic acoustic terahertz plasmon polaritons in monoclinic Ag2Te platelets placed above a Au layer, verifying a linear dispersion and elliptical isofrequency contour in momentum space.
- S. Chen
- , P. L. Leng
- & R. Hillenbrand
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Letter |
Laser writing of spin defects in nanophotonic cavities
Using direct laser writing with a nanosecond pulsed laser operating at above-bandgap photon energies, we demonstrate the selective formation of spin defects in photonic crystal cavities in 4H-silicon carbide and their in situ characterization.
- Aaron M. Day
- , Jonathan R. Dietz
- & Evelyn L. Hu
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Letter |
Compact spin-valley-locked perovskite emission
We report compact spin-valley-locked perovskite emitting metasurfaces where spin-dependent geometric phases are imparted into bound states in the continuum via Brillouin zone folding, simultaneously enabling chiral purity, directionality and large emission angles.
- Yang Chen
- , Jiangang Feng
- & Cheng-Wei Qiu
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Letter |
Ambipolar charge-transfer graphene plasmonic cavities
Employing an oxidation-activated charge transfer strategy to oxidize transition-metal dichalcogenides into transition-metal oxides, the authors imprint plasmonic cavities with laterally abrupt doping profiles and nanoscale precision demonstrating plasmonic whispering-gallery resonators.
- Brian S. Y. Kim
- , Aaron J. Sternbach
- & D. N. Basov
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Article |
Scalable manufacturing of high-index atomic layer–polymer hybrid metasurfaces for metaphotonics in the visible
The authors propose a method for the scalable manufacturing of metalenses using deep-ultraviolet argon fluoride immersion lithography and wafer-scale nanoimprint lithography, opening a route towards their low-cost, high-throughput mass production.
- Joohoon Kim
- , Junhwa Seong
- & Junsuk Rho
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Article |
Tip-induced excitonic luminescence nanoscopy of an atomically resolved van der Waals heterostructure
Tip-induced excitonic luminescence nanoscopy of an atomically resolved van der Waals heterostructure.
- Luis E. Parra López
- , Anna Rosławska
- & Guillaume Schull
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News & Views |
Ultrafast plasmonics shapes electron beams
By exploiting optical phase-modulation at complex surface plasmon polariton patterns, as well as energy-filtered imaging, femtosecond electron pulses are dynamically shaped in phase and amplitude.
- Armin Feist
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Article |
Tunable photon-induced spatial modulation of free electrons
On-demand electron wavefront shaping is desirable for applications from nanolithography to imaging. Here, the authors present tunable photon-induced spatial modulation of electrons through their interaction with externally controlled surface plasmon polaritons.
- Shai Tsesses
- , Raphael Dahan
- & Ido Kaminer
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Article |
From enhanced diffusion to ultrafast ballistic motion of hybrid light–matter excitations
The authors study ultrafast spatiotemporal dynamics of polaritons formed by mixing surface-bound optical waves with excitons observing a mobility transition from diffusive to ballistic transport flow at two-thirds the speed of light.
- Mukundakumar Balasubrahmaniyam
- , Arie Simkhovich
- & Tal Schwartz
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News & Views |
The colour of stress
Periodic nanostructures create brilliant colours, termed structural colouration, through light scattering and refraction. Now, using a simple and scalable method, stress- and strain-induced dynamic colour shifts are realized in stretchable polymers.
- Daeyeon Won
- & Seung Hwan Ko
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News & Views |
On-demand emission from Tamm plasmons
Tamm plasmon thermal emitters can provide efficient infrared emission, but are limited by design complexity. Now, the inverse design of Tamm modes facilitated by CdO films on aperiodic dielectric reflectors enables emission with an on-demand spectrum.
- Juerg Leuthold
- & Alexander Dorodnyy
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Article |
Deterministic inverse design of Tamm plasmon thermal emitters with multi-resonant control
Tamm plasmon thermal emitters can provide low-cost, efficient mid to long infrared emission, but have been limited by a challenging design. Here the authors apply an inverse design protocol to demonstrate tailorable multi-band emission on CdO films.
- Mingze He
- , J. Ryan Nolen
- & Joshua D. Caldwell
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Article |
Mechano-tunable chiral metasurfaces via colloidal assembly
Stacked elastomeric arrays containing plasmonic nanoparticles show efficient chiral responses that can be fully controlled by mechanical compression and stack rotation. These simple layered materials may be useful modulators for photonic applications.
- Patrick T. Probst
- , Martin Mayer
- & Andreas Fery
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News & Views |
Hot plasmons make graphene shine
Bright hot plasmon emission is observed in graphene due to the ultrafast relaxation of hot carriers that were excited by femtosecond laser pulses of visible light.
- Frank H. L. Koppens
- & Klaas-Jan Tielrooij
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Article |
Mid-infrared radiative emission from bright hot plasmons in graphene
The optical emission of graphene under pumping with femtosecond laser pulses contains a strong component linked to plasmon emission from the hot electrons in the system.
- Laura Kim
- , Seyoon Kim
- & Harry A. Atwater
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Article |
Identifying carbon as the source of visible single-photon emission from hexagonal boron nitride
Comparison of hexagonal boron nitride samples grown with different techniques and with varying carbon-doping content provides evidence that the defects emitting single photons in the visible range are carbon related.
- Noah Mendelson
- , Dipankar Chugh
- & Igor Aharonovich
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Article |
Direct observation of highly confined phonon polaritons in suspended monolayer hexagonal boron nitride
Monochromatic electron energy-loss spectroscopy enables the observation of highly confined and ultraslow hyperbolic phonon polaritons in suspended monolayer hexagonal boron nitride, expanding the potential of van der Waals materials for nanophotonic applications.
- Ning Li
- , Xiangdong Guo
- & Peng Gao
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Article |
Ultrafast hot-hole injection modifies hot-electron dynamics in Au/p-GaN heterostructures
Photo-excited gold nanoparticles are shown to provide ultrafast and efficient hot-hole injection to the valence band of p-type GaN, substantially altering hot-electron dynamics in the nanoparticles and forming a basis to design hot-hole-based optoelectronics.
- Giulia Tagliabue
- , Joseph S. DuChene
- & Harry A. Atwater
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Article |
Configurable phonon polaritons in twisted α-MoO3
Infrared nanoimaging of phonon polaritons in twisted α-phase molybdenum trioxide bilayers reveals tunable wavefront geometries and topological transitions over a broad range of twist angles, offering a configurable platform for nanophotonic applications.
- Mingyuan Chen
- , Xiao Lin
- & Siyuan Dai
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Letter |
An integrated optical modulator operating at cryogenic temperatures
The integration of barium titanate thin films with silicon-based waveguides enables the operation of efficient electro-optic switches and modulators at temperatures as low as 4 K, with potential applications in quantum computing and cryogenic computing technologies.
- Felix Eltes
- , Gerardo E. Villarreal-Garcia
- & Stefan Abel
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Letter |
Broad spectral tuning of ultra-low-loss polaritons in a van der Waals crystal by intercalation
The spectral range of long-lived and confined phonon polaritons in a polar van der Waals crystal is shown to be tunable by intercalation of Na atoms, expanding their potential for nanophotonic applications in the mid-infrared domain.
- Javier Taboada-Gutiérrez
- , Gonzalo Álvarez-Pérez
- & Pablo Alonso-González
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Article |
Realizing spin Hamiltonians in nanoscale active photonic lattices
Vectorial electromagnetic modes in coupled metallic nanolasers are used to emulate the behaviour of complex magnetic materials, providing an integrated nanophotonic platform to study spin exchange interactions and map large-scale optimization problems.
- Midya Parto
- , William Hayenga
- & Mercedeh Khajavikhan
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Article |
Revealing multiple classes of stable quantum emitters in hexagonal boron nitride with correlated optical and electron microscopy
Defects in hexagonal boron nitride exhibit room-temperature quantum emission, but their unknown structural origin challenges their technological utility. A combination of optical and electron microscopy helps to distinguish at least four classes of defects and correlate them with local strain.
- Fariah Hayee
- , Leo Yu
- & Jennifer A. Dionne
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Letter |
Ultrafast pyroelectric photodetection with on-chip spectral filters
The ultrafast response of a pyroelectric sensor with near-infrared responsivity is demonstrated by combining a pyroelectric thermal detector with wavelength-selective nanoparticle absorbers.
- Jon W. Stewart
- , Jarrett H. Vella
- & Maiken H. Mikkelsen
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Review Article |
Nanophotonic engineering of far-field thermal emitters
This Review covers the basic physics of thermal emission, ways to engineer the thermal field radiated by hot objects in the far field and applications, such as thermophotovoltaics, radiative cooling, camouflage and privacy.
- Denis G. Baranov
- , Yuzhe Xiao
- & Mikhail A. Kats
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Article |
Ultrafast generation and control of an electron vortex beam via chiral plasmonic near fields
By exciting chiral plasmons within a nanohole by means of circularly polarized light pulses, orbital angular momentum can be imparted onto charged matter waves (here, electrons) and controlled at terahertz speed (femtosecond intervals).
- G. M. Vanacore
- , G. Berruto
- & F. Carbone
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Article |
Impacts of surface depletion on the plasmonic properties of doped semiconductor nanocrystals
Degenerately doped semiconductor nanocrystals exhibit localized surface plasmon resonance in the infrared. Semiconducting properties such as band structure modification due to doping and surface states are now shown to strongly affect plasmonic modulation.
- Omid Zandi
- , Ankit Agrawal
- & Delia J. Milliron
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Perspective |
Carbon nanotubes as emerging quantum-light sources
This Perspective describes the recent advances in understanding and controlling the properties of single-wall carbon nanotubes as well as the progress towards the fabrication of new electrically driven single-photon sources.
- X. He
- , H. Htoon
- & C. Voisin
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Letter |
Ultralow-loss polaritons in isotopically pure boron nitride
Isotopic enrichment in hexagonal boron nitride is shown to enhance the propagation properties of phonon polaritons, achieving a threefold enhancement in their lifetime.
- Alexander J. Giles
- , Siyuan Dai
- & Joshua D. Caldwell
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Article |
Optical gain in colloidal quantum dots achieved with direct-current electrical pumping
Core/shell type-I semiconductor nanocrystals with compositionally graded shell and embedded in a current-focusing device architecture reach population inversion, a condition required for lasing, when excited with direct current.
- Jaehoon Lim
- , Young-Shin Park
- & Victor I. Klimov
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Article |
Electrotunable nanoplasmonic liquid mirror
Designing fully tunable metamaterials for applications ranging from sensors to superlenses remains a challenge. A reversible electrotuneable liquid mirror based on voltage-controlled self-assembly/disassembly plasmonic nanoparticles is now reported.
- Yunuen Montelongo
- , Debabrata Sikdar
- & Alexei A. Kornyshev
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News & Views |
Here comes the spaser
Plasmonic nanolasers embedded in living cells and animal tissues are shown to emit strongly, making them promising potential biocompatible probes.
- Catherine Alix-Panabières
- & Klaus Pantel
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Review Article |
Polaritons in layered two-dimensional materials
This Review discusses the properties of polariton modes (plasmon, phonon and exciton) in graphene, hexagonal boron nitride and transition metal dichalcogenides for applications across the terahertz to visible spectrum.
- Tony Low
- , Andrey Chaves
- & Frank Koppens
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Letter |
Thermoelectric detection and imaging of propagating graphene plasmons
A device is presented that can detect mid-infrared plasmons in graphene encapsulated by hexagonal boron nitride via the thermoelectric effect; the natural decay product of the plasmons (electronic heat) is converted into a measurable voltage signal.
- Mark B. Lundeberg
- , Yuanda Gao
- & Frank H. L. Koppens
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Letter |
A sub-femtojoule electrical spin-switch based on optically trapped polariton condensates
The spin-switching of optically induced polariton condensates can be externally controlled with an electric field, with switching energies below 0.5 fJ.
- Alexander Dreismann
- , Hamid Ohadi
- & Jeremy J. Baumberg
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News & Views |
To scatter or not to scatter
A rewritable platform for subwavelength optical components is demonstrated by combining surface phonon–polaritons, sustained in a polar dielectric layer, with the switching functionality provided by a phase-change material.
- Isabelle Staude
- & Carsten Rockstuhl