Featured
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Research Briefing |
Drift-free iontronic sensing enabled by a creep-free polyelectrolyte elastomer
Soft pressure sensors drift under prolonged high stress because of the creep of soft materials, which causes inaccurate measurements. Now, through molecular-level design, a leakage-free and creep-free polyelectrolyte elastomer is synthesized, and an iontronic sensor using the polyelectrolyte elastomer shows very low signal drift under a high static pressure.
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Article |
Creep-free polyelectrolyte elastomer for drift-free iontronic sensing
Conventional iontronic pressure sensors suffer from signal drift and inaccuracy owing to creep of soft materials and ion leakage. Here the authors report a leakage-free and creep-free polyelectrolyte-elastomer-based iontronic sensor that achieves a drift rate two to three orders of magnitude lower than those of conventional iontronic sensors.
- Yunfeng He
- , Yu Cheng
- & Chuan Fei Guo
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Feature |
Lifting the fog in ferroelectric thin-film synthesis
Frustrated by reproducibility in electrical measurements on ferroelectric films, Lane Martin, Jon-Paul Maria and Darrell Schlom discuss tactics to reliably synthesize ‘good’ ferroelectric samples, especially in the search for superior materials and device heterostructures.
- Lane W. Martin
- , Jon-Paul Maria
- & Darrell G. Schlom
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Article |
Frictionless multiphasic interface for near-ideal aero-elastic pressure sensing
Solid-state pressure sensors have performance limitations in liquid environments. Here, the authors design a pressure sensor using solid–liquid–liquid–gas multiphasic interfaces where a trapped air layer modulates capacitance changes with pressure to achieve near-friction-free contact line motions for near-ideal pressure sensing.
- Wen Cheng
- , Xinyu Wang
- & Benjamin C. K. Tee
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News & Views |
Compound semiconductor devices for the skin
Nanomembranes of GaN grown by remote epitaxy form the basis of surface acoustic wave sensors in wireless electronic skins for health monitoring.
- Jong Uk Kim
- , Seung Gi Seo
- & John A. Rogers
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Article
| Open AccessRobust cholesteric liquid crystal elastomer fibres for mechanochromic textiles
Robust cholesteric liquid crystal elastomer fibres with rapid and reversible mechanochromic responses are woven and sewn into garments to create smart clothing.
- Yong Geng
- , Rijeesh Kizhakidathazhath
- & Jan P. F. Lagerwall
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News & Views |
Dynamic soft materials as tough as glass
Slow, tunable dissociation of non-covalent host–guest complexes confers supramolecular polymer networks with excellent compressive strength and self-recovery.
- Matthew J. Webber
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Article |
Mechano-tunable chiral metasurfaces via colloidal assembly
Stacked elastomeric arrays containing plasmonic nanoparticles show efficient chiral responses that can be fully controlled by mechanical compression and stack rotation. These simple layered materials may be useful modulators for photonic applications.
- Patrick T. Probst
- , Martin Mayer
- & Andreas Fery
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Article |
Hydrogen-doped viscoplastic liquid metal microparticles for stretchable printed metal lines
Hydrogen doping and polymer adsorption at the oxide surface of liquid metal microparticles increase the conductivity and viscoplastic behaviour of the oxide, leading to liquid-metal-based printed circuits with stable resistance up to 500% strain.
- Selvaraj Veerapandian
- , Woosun Jang
- & Unyong Jeong
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News & Views |
Learning with brain chemistry
Organic neuromorphic devices are now able to take direct input from cellular neurotransmitter release.
- Tobias Cramer
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Letter |
A biohybrid synapse with neurotransmitter-mediated plasticity
A cell culture interfacing an organic neuromorphic device in a microfluidic system reversibly modifies the device synaptic weight through chemical reactions mediated by the release of dopamine, a neurotransmitter used in biological synapses.
- Scott T. Keene
- , Claudia Lubrano
- & Francesca Santoro
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News & Views |
Lowering the threshold for bioelectronics
A high-speed, high-gain enhancement-mode ion-gated transistor shows promise for low-power chronically implanted bioelectronic systems.
- Scott Keene
- & Yoeri van de Burgt
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Article |
Synthesis of orthogonally assembled 3D cross-stacked metal oxide semiconducting nanowires
Orthogonal self-assembly of amphiphilic diblock copolymers and polyoxometallates followed by calcination allows the formation of cross-stacked multilayer 3D arrays of tungsten oxide nanowires.
- Yuan Ren
- , Yidong Zou
- & Yonghui Deng
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Article |
Metal–polymer hybrid nanomaterials for plasmonic ultrafast hydrogen detection
Sensing hydrogen by the change in plasmonic response upon metal hydride formation is safe, but trace gas poisoning and low sensitivity can occur. Here, a PdAu alloy/polymer sensor is poison resistant and can sense 3 ppm H2 with a response time of 1 s.
- Ferry A. A. Nugroho
- , Iwan Darmadi
- & Christoph Langhammer
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Editorial |
Multiferroics march on
Much academic and industrial effort has been devoted to the study of multiferroics, but if related technologies are to have real-world impact, market awareness and reproducibility are also key.
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Q&A |
Multiferroics and the path to the market
Nian Sun, a professor at Northeastern University (Electrical and Computer Engineering Department), talks to Nature Materials about the potential applications of multiferroic materials, and issues associated with commercializing these technologies.
- Stephen Shevlin
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Article |
Three-dimensional printing of piezoelectric materials with designed anisotropy and directional response
Piezoelectrics convert force into electrical charge, and vice versa, but the coefficients that determine piezoelectric behaviour are constrained by crystal structure. Here, metamaterials are 3D printed that show arbitrary piezoelectric coefficients.
- Huachen Cui
- , Ryan Hensleigh
- & Xiaoyu (Rayne) Zheng
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News & Views |
How slow can you go?
Use of graphene in a transistor configuration offers an alternative to metal electrodes for the recording of ultraslow neural potentials that occur in neurologic diseases.
- Jed A. Hartings
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Article |
Highly mechanosensitive ion channels from graphene-embedded crown ethers
Tuning ionic permeation across nanoscale pores is important for areas ranging from nanofluidic computing to drug delivery. Complex formation between crown ethers and dissolved metal ions is used to demonstrate graphene-based ion channels with high mechanosensitivity.
- A. Fang
- , K. Kroenlein
- & A. Smolyanitsky
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News & Views |
High piezoelectricity via enhanced disorder
Ultrahigh piezoelectricity in relaxor-ferroelectric ceramics is engineered by chemical and structural heterogeneities at the nanoscale.
- Barbara Malic
- & Tadej Rojac
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Article |
Ultrahigh piezoelectricity in ferroelectric ceramics by design
Simulations were used to investigate the effects of local structural heterogeneity on piezoelectricity in ceramics. From this, a Sm-doped PMN–PT composition was designed with an extremely high piezoelectric coefficient for polycrystalline systems.
- Fei Li
- , Dabin Lin
- & Shujun Zhang
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Article |
Nanostructured organic semiconductor films for molecular detection with surface-enhanced Raman spectroscopy
Highly nanostructured purely organic films are shown to enhance the Raman signal of methylene blue molecules by three orders of magnitude, due to the unique molecular geometry, morphology and electronic properties of the films.
- Mehmet Yilmaz
- , Esra Babur
- & Gokhan Demirel
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Article |
Dopant compensation in alloyed CH3NH3PbBr3−xClx perovskite single crystals for gamma-ray spectroscopy
Hybrid organic–inorganic perovskite single crystals with optimized combination of Cl and Br ions are used to fabricate γ-ray detectors operating at room temperature and competing with the performance of sodium iodide scintillators.
- Haotong Wei
- , Dylan DeSantis
- & Jinsong Huang
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Article |
Nitroaromatic detection and infrared communication from wild-type plants using plant nanobionics
Plants can be engineered to serve as self-powered pre-concentrators and autosamplers of analytes in ambient groundwater and as infrared communication platforms that can send information to a smartphone.
- Min Hao Wong
- , Juan P. Giraldo
- & Michael S. Strano
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Letter |
Instrumented cardiac microphysiological devices via multimaterial three-dimensional printing
Heart-on-a-chip devices with integrated strain gauges for direct readout of tissue contractile strength allow for multiplexed drug-dose experiments and studies of functional maturation of cardiac tissue.
- Johan U. Lind
- , Travis A. Busbee
- & Kevin K. Parker
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Editorial |
Restoring touch
Medical professionals and robotics engineers count on materials scientists for the development of electronic skins with lifelike tactile sensing capabilities.
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Commentary |
Robots with a sense of touch
Tactile sensors provide robots with the ability to interact with humans and the environment with great accuracy, yet technical challenges remain for electronic-skin systems to reach human-level performance.
- Chiara Bartolozzi
- , Lorenzo Natale
- & Giorgio Metta
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News & Views |
A sensor web for neurons
An implantable, flexible mesh with embedded electrodes for sensing neural activity in vivo improves brain-sampling efficiency and reduces the amount of cortical tissue injured.
- Tarun Saxena
- & Ravi V. Bellamkonda
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News & Views |
Skin health monitoring
Ultrathin and conformal piezoelectric transducers enable high-resolution mapping of the mechanical properties of human skin.
- Stéphanie P. Lacour
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Article |
Conformal piezoelectric systems for clinical and experimental characterization of soft tissue biomechanics
Piezoelectric sensors and actuators are embedded in pliable devices that conform to human skin and organ surfaces. These devices enable rapid characterization of the mechanical properties of soft tissues under various clinical conditions.
- Canan Dagdeviren
- , Yan Shi
- & John A. Rogers
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Article |
Ultrathin conformal devices for precise and continuous thermal characterization of human skin
A strategy for assessing blood microcirculation and tissue hydration relies on monitoring the temperature and thermal conductivity of skin, respectively. It is now shown that arrays of micrometre-sized sensors and heaters can be integrated on stretchable substrates that conformably adhere to the skin; these devices allow spatially resolved heating and real-time temperature mapping in patients without limiting their motion.
- R. Chad Webb
- , Andrew P. Bonifas
- & John A. Rogers
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Letter |
User-interactive electronic skin for instantaneous pressure visualization
Flexible devices mimicking the sensitivity of human skin typically turn pressure stimuli into electronic signals, which must be further processed to be interpreted by the user. By integrating an active matrix of organic light-emitting diodes in these foldable sensors, pressure can now control the brightness of each coloured pixel, enabling the direct visualization and quantification of the applied stimulus.
- Chuan Wang
- , David Hwang
- & Ali Javey
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Article |
A transparent organic transistor structure for bidirectional stimulation and recording of primary neurons
A transparent organic field-effect transistor allows the stimulation and recording of the bioelectrical activity of primary neural cells. The cells grow, differentiate and function on the device, which then provides the electrical stimulation, and enables the recording of extracellular current and optical imaging of the modulation of neuronal membrane potential.
- Valentina Benfenati
- , Stefano Toffanin
- & Michele Muccini
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Article |
MRI-detectable pH nanosensors incorporated into hydrogels for in vivo sensing of transplanted-cell viability
The monitoring of cell survival and functionality following their in vivo transplantation remains a challenge in clinical cell therapy. Now, using magnetic resonance imaging techniques and microcapsules with pH-sensitive components, in vivo cell death and cell viability patterns can be assessed with high anatomical accuracy.
- Kannie W. Y. Chan
- , Guanshu Liu
- & Michael T. McMahon
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News & Views |
Sustainable sensors from silk
A biocompatible method for fabricating three-dimensional photonic crystals opens up unique opportunities for structurally coloured biodegradable materials, but also for implantable biosensing and targeted therapeutics on the microscale.
- Jennifer MacLeod
- & Federico Rosei
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Letter |
Singular phase nano-optics in plasmonic metamaterials for label-free single-molecule detection
A suitably engineered plasmonic metamaterial featuring topologically protected sharp phase variations close to a zero-reflection point of incident lightwaves has now been demonstrated. Exploiting the high sensitivity of the abrupt phase changes, and by using reversible hydrogenation of graphene and binding of streptavidin–biotin, the detection of individual biomolecules and an areal mass sensitivity of the order of fg mm−2 is reported.
- V. G. Kravets
- , F. Schedin
- & A. N. Grigorenko
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Article |
Self-assembled nanoparticle arrays for multiphase trace analyte detection
Nanoplasmonic structures that can detect trace analytes via surface-enhanced Raman spectroscopy typically require sophisticated nanofabrication techniques. Self-assembly of gold nanoparticles into close-packed arrays at liquid/liquid and liquid/air interfaces is now used for the detection of multi-analytes from aqueous, organic or air phases.
- Michael P. Cecchini
- , Vladimir A. Turek
- & Joshua B. Edel
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News & Views |
Striped cation-trappers
Toxic metal cations in environmental samples can be detected with ultrahigh sensitivity through measurements of the tunnelling current across crosslinked films of nanoparticles decorated with striped monolayers of organic ligands.
- Knut Rurack
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Article |
Ultrasensitive detection of toxic cations through changes in the tunnelling current across films of striped nanoparticles
Solid-state sensors for the detection of heavy-metal cations require for the most part sophisticated chemistry and equipment. It is now shown that toxic cations in environmental samples can be detected with ultrahigh sensitivity and over a broad range of cation concentrations by measuring the tunnelling current across films of nanoparticles decorated with striped monolayers of organic ligands.
- Eun Seon Cho
- , Jiwon Kim
- & Bartosz A. Grzybowski
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Article |
A flexible and highly sensitive strain-gauge sensor using reversible interlocking of nanofibres
Flexible strain-gauge sensors, which could eventually be used in electronic skin, generally require complex device architectures. A simple and highly sensitive resistive sensor for the detection of pressure, shear and torsion with discernible strain-gauge factors has now been fabricated using two interlocked arrays of platinum-coated polymer nanofibres.
- Changhyun Pang
- , Gil-Yong Lee
- & Kahp-Yang Suh
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News & Views |
Inverse sensitivity
Enzyme-modified plasmonic nanoparticles that generate a signal that is larger when the concentration of the target molecule is lower can detect ultralow levels of the cancer biomarker prostate-specific antigen in whole serum.
- Mikael Käll
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Letter |
Plasmonic nanosensors with inverse sensitivity by means of enzyme-guided crystal growth
Conventional sensors generate a signal that is directly proportional to the concentration of the target molecule. Now, by means of an enzyme that controls the growth of silver nanocrystals on plasmonic transducers, a nanosensor with sensitivity that is inversely proportional to concentration and that can detect ultralow concentrations of the cancer biomarker prostate-specific antigen in whole serum is demonstrated.
- Laura Rodríguez-Lorenzo
- , Roberto de la Rica
- & Molly M. Stevens
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Article |
Exchange biasing of magnetoelectric composites
Magnetoelectric composite materials are of interest for sensitive magnetic-field sensors. The realization of a magnetoelectric composite that does not require an applied external magnetic field, but instead relies on internal bias via exchange coupling, promises sensitive sensors even for small magnetic fields.
- Enno Lage
- , Christine Kirchhof
- & Dirk Meyners
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Letter |
Gated three-terminal device architecture to eliminate persistent photoconductivity in oxide semiconductor photosensor arrays
The slow decay of photoconductivity in amorphous oxide semiconductors hampers their use in photosensor arrays with viable frame rates. A gated sensor architecture now provides direct control over the Fermi-level position in the semiconductor layer, and eliminates persistent photoconductivity by accelerating electron recombination with ionized oxygen vacancy sites.
- Sanghun Jeon
- , Seung-Eon Ahn
- & Kinam Kim