Featured
-
-
Article |
Phagocytosis-inspired behaviour in synthetic protocell communities of compartmentalized colloidal objects
Droplets with magnetite membranes are designed to engulf in a phagocytosis-inspired manner smaller colloidal objects, demonstrating a route for sequential cargo delivery and release followed by internalized reactions.
- Laura Rodríguez-Arco
- , Mei Li
- & Stephen Mann
-
Article |
Molecular engineering of chiral colloidal liquid crystals using DNA origami
DNA origami allows the design of rod-shaped particles with specific geometrical features. This is exploited to examine how particle-level characteristics affect properties of the bulk phase and the superstructures such colloids assemble into.
- Mahsa Siavashpouri
- , Christian H. Wachauf
- & Zvonimir Dogic
-
Article |
Tuning crystallization pathways through sequence engineering of biomimetic polymers
AFM measurements of peptoids assembling into sheets and networks show that the crystallization mechanism is determined by the molecular structure, where the addition of a hydrophobic segment alters the crystal formation process into a two-step pathway.
- Xiang Ma
- , Shuai Zhang
- & James J. De Yoreo
-
Article |
Two-dimensional assemblies from crystallizable homopolymers with charged termini
Uniform, hierarchical 2D nanostructures with controlled shapes can be prepared from homopolymers with charged end-groups using a crystallization-driven assembly process.
- Xiaoming He
- , Ming-Siao Hsiao
- & Ian Manners
-
-
News & Views |
Controlled collective motions
Self-propelled Janus particles with externally regulated anisotropic interactions can be made to swarm, cluster and form slithering chains.
- Roberto Di Leonardo
-
Article |
Porous microwells for geometry-selective, large-scale microparticle arrays
A porous microwell platform that generates large-scale arrays of microparticles with varying shape, size and modulus with high specificity shows applicability in anti-counterfeiting and cell-screening applications.
- Jae Jung Kim
- , Ki Wan Bong
- & Patrick S. Doyle
-
Letter |
In situ study of the formation mechanism of two-dimensional superlattices from PbSe nanocrystals
A real-time study of the growth of two-dimensional nanocrystal superlattices with square periodicity shows the formation mechanism leading to the oriented attachment of the nanocrystals.
- Jaco J. Geuchies
- , Carlo van Overbeek
- & Daniel Vanmaekelbergh
-
Letter |
Reconfiguring active particles by electrostatic imbalance
Metal–dielectric Janus colloids subjected to perpendicular a.c. electric fields can self-organize into swarms, chains, clusters and isotropic gases, depending on the frequency of the field.
- Jing Yan
- , Ming Han
- & Steve Granick
-
News & Views |
Frustrated shapes
Geometric frustration governs shape selection in fibrous materials.
- Eran Sharon
- & Hillel Aharoni
-
News & Views |
Hand-twisting light
Macroscopic deformation can induce chirality in initially achiral nanoparticle composites, and reversibly modulate their chiroptical properties.
- Daeyeon Lee
- & Sang Eon Han
-
Letter |
Morphology selection via geometric frustration in chiral filament bundles
Geometric frustration selects the equilibrium morphology of cohesive bundles of chiral filaments by controlling the relative costs of filament bending and the straining of the cohesive bonds.
- Douglas M. Hall
- , Isaac R. Bruss
- & Gregory M. Grason
-
Article |
Lattice engineering through nanoparticle–DNA frameworks
Designed DNA-based polyhedral frames, whose vertices are connected to nanoparticles, facilitate their self-assembly into predetermined crystalline and open three-dimensional lattices.
- Ye Tian
- , Yugang Zhang
- & Oleg Gang
-
Article |
Programming curvature using origami tessellations
Elementary geometric constructions and constrained optimization algorithms can be used to fit origami tessellations to any curved surface.
- Levi H. Dudte
- , Etienne Vouga
- & L. Mahadevan
-
-
-
-
Letter |
Mechanics of fire ant aggregations
Aggregations of fire ants are viscoelastic with identical elastic and viscous moduli, and exhibit shear-thinning behaviour when deformed beyond the linear regime.
- Michael Tennenbaum
- , Zhongyang Liu
- & Alberto Fernandez-Nieves
-
Article |
Topological defects in liquid crystals as templates for molecular self-assembly
Nanoscale environments created by topological defects in liquid crystals can template the self-assembly of molecular amphiphiles within the defects.
- Xiaoguang Wang
- , Daniel S. Miller
- & Nicholas L. Abbott
-
Article |
Microtubules self-repair in response to mechanical stress
Experiments show that the progressive softening of microtubules under mechanical stress results from the enlargement of pre-existing structural defects, and that the incorporation of tubulin dimers can restore the microtubule’s initial stiffness.
- Laura Schaedel
- , Karin John
- & Manuel Théry
-
Article |
Phage-mediated counting by the naked eye of miRNA molecules at attomolar concentrations in a Petri dish
An ultrasensitive method that uses a genetically engineered bacteriophage to bind miRNA in a one-to-one manner allows the counting, by the naked eye, of miRNA molecules at attomolar concentrations on Petri dishes.
- Xin Zhou
- , Peng Cao
- & Chuanbin Mao
-
Article |
Fast and long-range triplet exciton diffusion in metal–organic frameworks for photon upconversion at ultralow excitation power
Controlled overlap of molecular orbitals in metal–organic frameworks enhances triplet exciton diffusion in these structures, which are now used in solid-state photon upconverters operating under excitation power comparable to solar irradiance.
- Prasenjit Mahato
- , Angelo Monguzzi
- & Nobuo Kimizuka
-
Article |
Fluctuation-driven mechanotransduction regulates mitochondrial-network structure and function
Vascular smooth muscle cells can harness fluctuations in external cyclic stretching by altering their cytoskeletal organization and the associated mitochondrial network.
- Erzsébet Bartolák-Suki
- , Jasmin Imsirovic
- & Béla Suki
-
Editorial |
Mighty linkers
The versatility of DNA linkers as selective binders is accelerating the rational design of the assembly of nanoparticle crystals with unprecedented structural complexity.
-
News & Views |
Flip-flop lattices
The structure of crystals made of DNA-bridged nanoparticles can be selectively switched between various lattices by reprogramming the DNA-mediated interactions between the nanoparticles.
- Erika Eiser
-
News & Views |
Exploiting shape complementarity
Improved control over the shape of nanoparticles and the interactions between them allows the rational construction of intricate microscale assemblies.
- Jean-Philippe Sobczak
- & Hendrik Dietz
-
Commentary |
DNA-linked superlattices get into shape
Advances in the control of the shape, bonding direction and valency of DNA-coated nanoparticles allow the synthesis of nanoparticle crystallites of ever increasing complexity.
- Bert Nickel
- & Tim Liedl
-
Letter |
Liquid-crystalline ordering of antimicrobial peptide–DNA complexes controls TLR9 activation
Liquid-crystalline arrangements of complexes of DNA and antimicrobial peptides can lead to multivalent electrostatic interactions that drastically amplify TLR9-mediated immune responses.
- Nathan W. Schmidt
- , Fan Jin
- & Gerard C. L. Wong
-
-
Letter |
Memoryless self-reinforcing directionality in endosomal active transport within living cells
A general memoryless molecular mechanism explains the self-organization of Brownian-like steps into truncated Lévy walks in the classic system of intracellular trafficking.
- Kejia Chen
- , Bo Wang
- & Steve Granick
-
-
Editorial |
Assembling insight
Model colloidal systems are a testbed for understanding aspects of the organization of matter.
-
News & Views |
A switch for phase shifting
Temperature can switch the thermodynamic phase of colloid–polymer mixtures by tipping the balance between competing attractive interactions induced by polymer depletion or adsorption.
- Ah-Young Jee
- , Boyce Tsang
- & Steve Granick
-
News & Views |
Assembled with one component
Computer simulations of one-component three-dimensional icosahedral quasicrystals will help to understand the mechanisms that may stabilize them in experiments.
- Marc de Boissieu
-
News & Views |
Enantioselective photoactivation
Circularly polarized light actualizes the formation of chiral twisted ribbons from achiral semiconductor nanoparticles.
- Bart Kahr
- & Alexander G. Shtukenberg
-
News & Views |
Reversible actuation
Janus ellipsoids self-assemble into self-limiting fibres that can be reversibly actuated by applying an electric field.
- Eric M. Furst
-
News & Views |
Mediated by a liquid
The nucleation of a crystal within another can involve intermediate liquid nuclei.
- Eduardo Sanz
- & Chantal Valeriani
-
Commentary |
Order through entropy
Understanding entropic contributions to common ordering transitions is essential for the design of self-assembling systems with addressable complexity.
- Daan Frenkel
-
Commentary |
Programmable self-assembly
Two conceptual strategies for encoding information into self-assembling building blocks highlight opportunities and challenges in the realization of programmable colloidal nanostructures.
- Ludovico Cademartiri
- & Kyle J. M. Bishop
-
Article |
Computational self-assembly of a one-component icosahedral quasicrystal
A body-centred icosahedral quasicrystal has been assembled, by using molecular dynamics simulations, from a one-component fluid of particles interacting via a tunable, isotropic pair potential.
- Michael Engel
- , Pablo F. Damasceno
- & Sharon C. Glotzer
-
-
Article |
Actuation of shape-memory colloidal fibres of Janus ellipsoids
Experiments and computer simulations show that Janus ellipsoids can self-assemble into self-limiting fibres that have shape-memory properties and can be actuated by applying an external electric field.
- Aayush A. Shah
- , Benjamin Schultz
- & Michael J. Solomon
-
-
Article |
Gradated assembly of multiple proteins into supramolecular nanomaterials
Peptide-based nanofibres with bioactive proteins attached can now be made such that the protein ligands are introduced in a controlled manner. This tailoring of the nanofibre’s composition enables the ratio of multiple different proteins to be highly tuned within the assemblies. By changing the protein content of the nanofibres, it is possible to adjust the antibody responses in mice to the different nanofibres.
- Gregory A. Hudalla
- , Tao Sun
- & Joel H. Collier
-
-
Article |
Synthesis and patterning of tunable multiscale materials with engineered cells
Biofilms are multifunctional and environmentally responsive assemblies of living and non-living components. By using synthetic gene networks in engineered cells to regulate the production of extracellular amyloid fibrils, and by interfacing the fibrils with inorganic materials such as metal nanoparticles, stimuli-responsive synthetic biofilms with switchable functions and tunable composition and structure have now been produced.
- Allen Y. Chen
- , Zhengtao Deng
- & Timothy K. Lu
-
News & Views |
A loop of two rods
The spontaneous organization of semiconductor nanoparticles into uniform pairs of parallel nanorods bridged at their ends illustrates the potential of hierarchical self-assembly processes for the formation of inorganic superstructures with complexity comparable to that of small self-organized biological aggregates.
- Bongjun Yeom
- & Nicholas A. Kotov
-
News & Views |
DNA-bonded 'atoms'
DNA-capped nanoparticles crystallize into uniform microcrystals of Wulff polyhedra when cooled slowly through the melting temperature of the DNA linkers.
- Shogo Hamada
- , Shawn J. Tan
- & Dan Luo
-