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| Open AccessUltralow contact resistance in organic transistors via orbital hybridization
The limitation in metal-semiconductor contact has been a major challenge for high-performance organic field-effect transistors. Here, the authors fabricate the contact by transferring platinum electrode on solution-processed organic films, realizing ultralow total contact resistance down to 14 Ω ∙ cm.
- Junpeng Zeng
- , Daowei He
- & Xinran Wang
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Article
| Open AccessCleavage of non-polar C(sp2)‒C(sp2) bonds in cycloparaphenylenes via electric field-catalyzed electrophilic aromatic substitution
Novel methodologies for cleaving inherently inert C(sp2)‒ C(sp2) bonds are desirable. Here, the authors report the use of an oriented electric field to cleave C(sp2)‒ C(sp2) in cycloparaphenylenes via electrophilic aromatic substitution.
- Junfeng Lin
- , Yaxin Lv
- & Daoben Zhu
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Article
| Open AccessHigh-performance Kerr microresonator optical parametric oscillator on a silicon chip
Flexible and coherent light generation is of paramount importance to enable new functionalities in integrated silicon photonics. Here the authors, develop an optical parametric oscillator with high conversion efficiency and high output power, based on the third order nonlinearity in a silicon nitride microresonator
- Edgar F. Perez
- , Grégory Moille
- & Kartik Srinivasan
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Article
| Open AccessProgrammable frequency-bin quantum states in a nano-engineered silicon device
Frequency-bin qubits get the best of time-bin and dual-rail encodings, but require external modulators and pulse shapers to build arbitrary states. Here, instead, the authors work directly on-chip by controlling the interference of biphoton amplitudes generated in multiple, coherently-pumped ring resonators.
- Marco Clementi
- , Federico Andrea Sabattoli
- & Daniele Bajoni
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Article
| Open AccessOne-dimensional semimetal contacts to two-dimensional semiconductors
2D semiconductors are attracting increasing attention as potentially scalable channels for future transistors, but the scaling of their contact length remains challenging. Here, the authors report the realization of 1D semimetal-2D semiconductor contacts based on individual carbon nanotubes with contact length down to 2 nm.
- Xuanzhang Li
- , Yang Wei
- & Yuegang Zhang
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Article
| Open AccessHumanlike spontaneous motion coordination of robotic fingers through spatial multi-input spike signal multiplexing
With advances in robotic technology, the complexity of control of robot has been increasing owing to fundamental von Neumann bottlenecks. Here, we demonstrate coordinated movement by a fully parallel-processable synaptic array with reduced control complexity.
- Dong Gue Roe
- , Dong Hae Ho
- & Jeong Ho Cho
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Article
| Open AccessElectrical spectroscopy of defect states and their hybridization in monolayer MoS2
Deep level transient spectroscopy (DLTS) is an established characterization technique used to study electrically active defects in 3D semiconductors. Here, the authors show that DLTS can also be applied to monolayer semiconductors, enabling in-situ characterization of the energy states of different defects and their interactions.
- Yanfei Zhao
- , Mukesh Tripathi
- & Andras Kis
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Article
| Open AccessMulti-dimensional data transmission using inverse-designed silicon photonics and microcombs
The authors demonstrate a multi-dimensional communication scheme that combines wavelength- and mode- multiplexing on photonic integrated circuits using foundry-compatible photonic inverse design and spectrally flattened microcombs
- Ki Youl Yang
- , Chinmay Shirpurkar
- & Jelena Vučković
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Article
| Open AccessAn epitaxial graphene platform for zero-energy edge state nanoelectronics
Here, the authors show robust edge state transport in patterned nanoribbon networks produced on epigraphene—graphene that is epitaxially grown on non-polar faces of SiC wafers. The edge state forms a zero-energy, one-dimensional ballistic network with dissipationless nodes at ribbon–ribbon junctions.
- Vladimir S. Prudkovskiy
- , Yiran Hu
- & Walt A. de Heer
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Article
| Open AccessUltrasensitive rapid cytokine sensors based on asymmetric geometry two-dimensional MoS2 diodes
Detection of cytokine biomarkers has the potential to aid in diagnosis and treatment of different diseases. Here, the authors report on the creation of an asymmetric geometry MoS2 diode-based biosensor for the detection of TNF-α as a model biomarker in a proof of concept study.
- Thushani De Silva
- , Mirette Fawzy
- & Michael M. Adachi
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Article
| Open AccessSpin-decoupling of vertical cavity surface-emitting lasers with complete phase modulation using on-chip integrated Jones matrix metasurfaces
Here the authors harness the on-chip integration of Jones matrix metasurfaces to demonstrate an ultra-compact approach to access and manipulate the optical spin states of vertical cavity surface-emitting lasers (VCSELs) with previously unattainable phase controllability.
- Pei-Nan Ni
- , Pan Fu
- & Patrice Genevet
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Article
| Open AccessSiGe quantum wells with oscillating Ge concentrations for quantum dot qubits
Quantum-dot spin qubits in Si/SiGe quantum wells require a large and uniform valley splitting for robust operation and scalability. Here the authors introduce and characterize a new heterostructure with periodic oscillations of Ge atoms in the quantum well, which could enhance the valley splitting.
- Thomas McJunkin
- , Benjamin Harpt
- & M. A. Eriksson
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Article
| Open AccessRoom-temperature valley transistors for low-power neuromorphic computing
Valleytronic devices employ the electronic valley degree of freedom to realize potential low-power electronic applications. Here, the authors utilize a topological semiconductor to engineer valley polarization transistors with long lifetimes and demonstrate low-power neuromorphic functionality at room temperature.
- Jiewei Chen
- , Yue Zhou
- & Yang Chai
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Article
| Open AccessBa+2 ion trapping using organic submonolayer for ultra-low background neutrinoless double beta detector
One of the possible events signaling a neutrinoless double beta decay is a Xe atom decaying into a Ba ion and two electrons. Aiming at the realisation of a detector for such a process, the authors show that Ba ions can be efficiently trapped (chelated) in vacuum by an organic molecule layer on a surface.
- P. Herrero-Gómez
- , J. P. Calupitan
- & J. T. White
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Article
| Open AccessUltra-low loss quantum photonic circuits integrated with single quantum emitters
Applications of ultra-low-loss photonic circuitry in quantum photonics, in particular including triggered single photon sources, are rare. Here, the authors show how InAs quantum dot single photon sources can be integrated onto wafer-scale, CMOS compatible ultra-low loss silicon nitride photonic circuits.
- Ashish Chanana
- , Hugo Larocque
- & Marcelo Davanco
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Article
| Open AccessA one-dimensional conductive metal-organic framework with extended π-d conjugated nanoribbon layers
2D and 3D conductive MOFs have performed well in the fields of energy and catalysis. Here, authors synthesise a 1D conductive MOF in which DDA ligands are connected by double Cu ions, forming nanoribbon layers with π-d conjugated nanoribbon planes and out-of-plane π-π stacking, which facilitates charge transport along two dimensions.
- Shengcong Shang
- , Changsheng Du
- & Jianyi Chen
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Article
| Open AccessObservation of full-parameter Jones matrix in bilayer metasurface
The realization of Jones matrix with full eight free parameters is particularly challenging. Here, the authors construct spatially varying Jones matrix with eight free parameters by cascading two-layer metasurfaces and use it for new optical functionalities.
- Yanjun Bao
- , Fan Nan
- & Baojun Li
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Article
| Open AccessDirect retrieval of Zernike-based pupil functions using integrated diffractive deep neural networks
Retrieving the pupil phase of a optical beam path is a central problem for imaging systems across scales. The authors use Diffractive Neural Networks to directly extract pupil phase information with a single, compact optoelectronic device.
- Elena Goi
- , Steffen Schoenhardt
- & Min Gu
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| Open AccessSpin-defect qubits in two-dimensional transition metal dichalcogenides operating at telecom wavelengths
Defect centers in two-dimensional materials has shown promise for applications in quantum information and sensing. Lee et al. computationally discover a class of substitutional defect centers in monolayer transition metal dichalcogenides with promising qubit characteristics operating at telecom wavelengths.
- Yeonghun Lee
- , Yaoqiao Hu
- & Kyeongjae Cho
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| Open AccessReconfigurable neuromorphic memristor network for ultralow-power smart textile electronics
Neuromorphic computing memristors are attractive to construct low-power- consumption electronic textiles. Here, authors report an ultralow-power textile memristor network of Ag/MoS2/HfAlOx/carbon nanotube with reconfigurable characteristics and firing energy consumption of 1.9 fJ/spike.
- Tianyu Wang
- , Jialin Meng
- & Lin Chen
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Article
| Open AccessLamellar carbon nitride membrane for enhanced ion sieving and water desalination
Traditional carbon nitride membranes are generally presented with random stacking behavior leading to undesired separation performance. Here, authors create lamellar membranes via polycation pillaring to afford adaptive subnanochannels, overcoming the selectivity-permeability trade-off in forward osmosis.
- Yang Wang
- , Tingting Lian
- & Markus Antonietti
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Article
| Open AccessA soft and ultrasensitive force sensing diaphragm for probing cardiac organoids instantaneously and wirelessly
It is challenging to directly characterize mechanical properties of soft 3D cardiac organoids with current sensors. Here the authors report an electronic skin-based all-soft organoid-sensing system which can wirelessly monitor minute force profiles of cardiac organoids in real-time in-situ.
- Quanxia Lyu
- , Shu Gong
- & Wenlong Cheng
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Article
| Open AccessElectro-active metaobjective from metalenses-on-demand
Future optical devices, e.g., for AR and VR, will require sophisticated flat metaoptics with unique optical functionalities. The authors demonstrate a metaobjective based on electrically switchable metallic polymer metalenses, whose optical states and focal length is adjustable via CMOS compatible voltages.
- Julian Karst
- , Yohan Lee
- & Harald Giessen
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Article
| Open AccessThree-to-one analog signal modulation with a single back-bias-controlled reconfigurable transistor
Designing efficient reconfigurable field effect transistors remains a challenge. Here, the authors develop a transistor with three distinct operation modes, realized directly on an industrial 22nm FDSOI platform, demonstrating a reconfigurable analog circuit element with signal follower, phase shifter, and frequency doubler operation.
- Maik Simon
- , Halid Mulaosmanovic
- & Jens Trommer
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Article
| Open AccessCritical role of hydrogen sorption kinetics in electrocatalytic CO2 reduction revealed by on-chip in situ transport investigations
Electrochemical hydrogen-participating processes are commonly relevant in multiple clean energy technologies. Here, authors achieve in situ quantification of H sorption kinetics during Pd-catalyzed CO2 reduction, unravelling its key role within the interfacial network of local pH, proton donors and CO2 molecules.
- Zhangyan Mu
- , Na Han
- & Mengning Ding
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Article
| Open AccessUnimon qubit
While transmon is the most widely used superconducting qubit, the search for alternative qubit designs with improved characteristic is ongoing. Hyyppä et al. demonstrate a novel superconducting qubit, the unimon, that combines high anharmonicity and protection against low-frequency charge noise and flux noise.
- Eric Hyyppä
- , Suman Kundu
- & Mikko Möttönen
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Article
| Open AccessRemote near-field spectroscopy of vibrational strong coupling between organic molecules and phononic nanoresonators
Vibrational strong coupling (VSC) promises ultrasensitive IR spectroscopy and modification of material properties. Here, nanoscale mapping of VSC between organic molecules and individual IR nanoresonators is achieved by remote near-field spectroscopy.
- Irene Dolado
- , Carlos Maciel-Escudero
- & Rainer Hillenbrand
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Article
| Open AccessA biomimetic ocular prosthesis system: emulating autonomic pupil and corneal reflections
The adoption of photonic synapses with biosimilarity to realize analog signal transmission is of significance in realizing artificial illuminance modulation responses. Here, the authors report a biomimetic ocular prosthesis system based on quantum dots embedded photonic synapses with improved depression properties through mid-gap trap.
- Seongchan Kim
- , Yoon Young Choi
- & Jeong Ho Cho
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Article
| Open AccessCarbon nanotube-based flexible high-speed circuits with sub-nanosecond stage delays
High-speed flexible circuits are essential in flexible systems for real-time information analysis and wireless communication. Here, flexible circuits are reported with a 281 ps stage delay based on scaled carbon nanotube thin film transistors.
- Guanhua Long
- , Wanlin Jin
- & Youfan Hu
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Article
| Open AccessGenerating intense electric fields in 2D materials by dual ionic gating
The application of electric fields >1 V/nm in solid state devices could provide access to unexplored phenomena, but it is currently difficult to implement. Here, the authors develop a double-sided ionic liquid gating technique to generate electric fields as large as 4 V/nm across few-layer WSe2, leading to field-induced semiconductor-to-metal transitions.
- Benjamin I. Weintrub
- , Yu-Ling Hsieh
- & Kirill I. Bolotin
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Article
| Open AccessUltra-low-noise microwave to optics conversion in gallium phosphide
Coherently interfacing microwave and optical radiation at the single photon level is an outstanding challenge in quantum technologies. Here, the authors show bi-directional on-chip conversion between MW and optical frequencies exploiting piezoelectric actuation of a gallium phosphide optomechanical resonator.
- Robert Stockill
- , Moritz Forsch
- & Simon Gröblacher
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Article
| Open AccessOptomechanical measurement of single nanodroplet evaporation with millisecond time-resolution
Understanding the behaviors of droplets at nanoscales is crucial to many applications, yet it remains experimentally challenging to track them in real time. Here, Sbarra et al. use a miniature optomechanical resonator to probe the evaporation dynamics of attoliter droplets with millisecond resolution.
- Samantha Sbarra
- , Louis Waquier
- & Ivan Favero
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Article
| Open AccessSliding nanomechanical resonators
The motion of a vibrating object is set by the way it is held. Here, the authors show a nanomechanical resonator reversibly slides on its supporting substrate as it vibrates and exploit this unconventional dynamics to quantify friction at the nanoscale.
- Yue Ying
- , Zhuo-Zhi Zhang
- & Guo-Ping Guo
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Article
| Open AccessAtomically precise control of rotational dynamics in charged rare-earth complexes on a metal surface
Rare-earth elements are vital to advanced technological applications ranging from spintronic devices to quantum information science. Here, the authors formed charged rare-earth complexes on a material surface and demonstrated atomically precise control on their rotational dynamics.
- Tolulope Michael Ajayi
- , Vijay Singh
- & Saw Wai Hla
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Article
| Open AccessMirror-induced reflection in the frequency domain
We show frequency domain mirrors that provide reflections of optical mode propagation in the frequency domain. We theoretically investigated the mirror properties and experimentally demonstrate it using polarization and coupled-resonator-based coupling on thin film Lithium Niobate.
- Yaowen Hu
- , Mengjie Yu
- & Marko Lončar
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Article
| Open AccessTunable metasurfaces via the humidity responsive swelling of single-step imprinted polyvinyl alcohol nanostructures
PVA is a hydrogel that has attractive swelling properties for use in tunable photonic applications. Here, the authors exploit PVA with nanoimprint lithography to realize multiplexed optical encryption metasurfaces to display, hide, and destroy encrypted information.
- Byoungsu Ko
- , Trevon Badloe
- & Junsuk Rho
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Article
| Open AccessExperimentally validated memristive memory augmented neural network with efficient hashing and similarity search
Memory augmented neural network for lifelong on-device learning is bottlenecked by limited bandwidth in conventional hardware. Here, the authors demonstrate its efficient in-memristor realization with a close-software accuracy, supported by hashing and similarity search in crossbars.
- Ruibin Mao
- , Bo Wen
- & Can Li
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Article
| Open AccessSlow light in a 2D semiconductor plasmonic structure
Slow light effects are interesting for telecommunications and quantum photonics applications. Here, the authors use coupled exciton-surface plasmon polaritons (SPPs) in a hybrid monolayer WSe2-metallic waveguide structure to demonstrate a 1300-fold reduction of the SPP group velocity.
- Matthew Klein
- , Rolf Binder
- & John R. Schaibley
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Article
| Open AccessZero energy states clustering in an elemental nanowire coupled to a superconductor
Topological superconductivity (TSC) is predicted to exist in nanowires with strong spin-orbit coupling (SOC) when they are in proximity to superconductors, with a key signature being zero-energy states in conductance measurements. Here, using weak-SOC carbon nanotubes as the nanowires, the authors show that similar looking zero-energy states can appear even in nanowires which cannot, in principle, host TSC.
- Lauriane C. Contamin
- , Lucas Jarjat
- & Matthieu R. Delbecq
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Article
| Open AccessObservation and control of Casimir effects in a sphere-plate-sphere system
Experimental studies of the Casimir effect have involved only interactions between two bodies so far. Here, the authors observe a micrometer-thick cantilever under the Casimir force exerted by microspheres from two sides simultaneously.
- Zhujing Xu
- , Peng Ju
- & Tongcang Li
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Article
| Open AccessA steep switching WSe2 impact ionization field-effect transistor
The potential energy efficiency of impact ionization field-effect transistors (I2FETs) is usually limited by stringent operational conditions. Here, the authors report I2FETs based on 2D WSe2, showing average subthreshold slopes down to 2.3 mV/dec and on/off ratios of ~106 at room temperature and bias voltages <1 V.
- Haeju Choi
- , Jinshu Li
- & Sungjoo Lee
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Article
| Open AccessMetasurface-driven full-space structured light for three-dimensional imaging
3D depth sensing with structured light enables simultaneous imaging of multiple objects, but has limited field of view and low efficiency. Here, the authors demonstrate 3D imaging with scattered light from a metasurface composed of periodic supercells, covering a 180° field of view with a high-density dot array.
- Gyeongtae Kim
- , Yeseul Kim
- & Junsuk Rho
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Article
| Open AccessTopological current divider in a Chern insulator junction
Topological materials hold great promise for dissipationless information transmission. Here, the authors create Chern insulator junctions between domains with different Chern numbers in MnBi2Te4 to realize the basic operation of a topological circuit.
- Dmitry Ovchinnikov
- , Jiaqi Cai
- & Xiaodong Xu
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Article
| Open AccessDual sensing signal decoupling based on tellurium anisotropy for VR interaction and neuro-reflex system application
The accumulation of single-function sensors can increase the complexity of virtual reality systems. Here, Shen et al. exploit the intrinsic anisotropy of tellurium nanowires to design a multi-function pressure and temperature sensor, which can be used as tactile experience in the virtual world.
- Linlin Li
- , Shufang Zhao
- & Guozhen Shen
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Article
| Open AccessSelective control of conductance modes in multi-terminal Josephson junctions
Multiterminal Josephson junctions may provide a novel way to realize topologically non-trivial band structures in an n-dimensional phase space. Here, the authors experimentally demonstrate the proposed necessary conditions to measure these states.
- Gino V. Graziano
- , Mohit Gupta
- & Vlad S. Pribiag
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Article
| Open AccessMode coupling bi-stability and spectral broadening in buckled carbon nanotube mechanical resonators
Computing, memories, and digital electronics are based on the operation principle of bi-stable systems. Here, Yaish et al. report the unusual non-linear behaviour of buckled up carbon nanotubes mechanical resonators, which allows high electrical frequency tunability and snap-through bi-stability.
- Sharon Rechnitz
- , Tal Tabachnik
- & Yuval E. Yaish
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Article
| Open AccessTopologically-imposed vacancies and mobile solid 3He on carbon nanotube
Probing fundamental quantum systems and their phase change is interesting. Here the authors demonstrate the existence of mobile quantum solid phase composed of dimerized 3He atoms and topology-induced vacancies using 3He adsorbed on carbon nanotube.
- I. Todoshchenko
- , M. Kamada
- & P. J. Hakonen
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Article
| Open AccessNano-electromechanical spatial light modulator enabled by asymmetric resonant dielectric metasurfaces
This work experimentally demonstrates nano-electromechanically tunable asymmetric dielectric metasurfaces. The metasurfaces enable large phase tuning, high reflection, a wavelength-scale pixel size, and electrical control of diffraction patterns.
- Hyounghan Kwon
- , Tianzhe Zheng
- & Andrei Faraon
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Article
| Open AccessUltrathin crystalline-silicon-based strain gauges with deep learning algorithms for silent speech interfaces
Designing an efficient platform that enables verbal communication without vocalization remains a challenge. Here, the authors propose a silent speech interface by utilizing a deep learning algorithm combined with strain sensors attached near the subject’s mouth, able to collect 100 words and classify at a high accuracy rate.
- Taemin Kim
- , Yejee Shin
- & Ki Jun Yu