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| Open AccessFlexible calorimetric flow sensor with unprecedented sensitivity and directional resolution for multiple flight parameter detection
Accurate perception of flight parameters is critical for flight control of micro air vehicles. Here, authors present a flexible calorimetric flow sensor with vanadium oxide thermistor arrays for flight parameters estimation, such as angle of attack and sideslip, flight velocity, and wing vibration.
- Zheng Gong
- , Weicheng Di
- & Huawei Chen
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Article
| Open AccessMultilevel design and construction in nanomembrane rolling for three-dimensional angle-sensitive photodetection
Zhang et al. report a quasistatic multilevel finite element model to predict the 3D structures assembled by 2D nanomembranes, validated by large-scale, high-yield, and configurable fabrication. 3D Si/Cr photodetectors assisted by neural network are employed to resolve the incident light angle.
- Ziyu Zhang
- , Binmin Wu
- & Yongfeng Mei
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Article
| Open AccessAggregation induced emission dynamic chiral europium(III) complexes with excellent circularly polarized luminescence and smart sensors
Chiral luminescent materials are of increasing interest in various applications, but achieving a desirable balance of properties can be challenging. Here, the authors report the development of Eu-based complexes with chiral luminescence and aggregation induced emission.
- Yun-Lan Li
- , Hai-Ling Wang
- & Hua-Hong Zou
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Article
| Open AccessMonolithic thin-film lithium niobate broadband spectrometer with one nanometre resolution
A framework to break the inherent trade-off barrier between spectral resolution and operational bandwidth of integrated optical spectrometers is developed and demonstrated on thin-film lithium niobate without sacrificing the compact footprint.
- Giovanni Finco
- , Gaoyuan Li
- & Rachel Grange
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Article
| Open AccessAn integrated self-optimizing programmable chemical synthesis and reaction engine
A limitation of robotic platforms in chemistry is the lack of feedback loops to adjust the conditions in-operando. Here the authors present a dynamically programmable robotic system that uses sensors for real-time adaptation, achieving yield improvements in syntheses and discovering new molecules.
- Artem I. Leonov
- , Alexander J. S. Hammer
- & Leroy Cronin
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Article
| Open AccessMolecular imprinting-based indirect fluorescence detection strategy implemented on paper chip for non-fluorescent microcystin
Fluorescence analysis is a fast and sensitive method for the trace detection of environmental toxins, but it remains challenging to develop a fluorescence method for detecting nonfluorescent toxins. Here, the authors report an indirect fluorescent sensing strategy for the rapid, selective and sensitive detection of the non-fluorescent microcystin as a model target.
- Bowei Li
- , Ji Qi
- & Lingxin Chen
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Article
| Open AccessDual-modal piezotronic transistor for highly sensitive vertical force sensing and lateral strain sensing
Developing mechanical sensors with two working modes for detecting vertical force and lateral strain is challenging. Here, Ge et al. report a piezotronic transistor with protrusions that enable dual-modal functionality and improve sensing performance.
- Rui Ge
- , Qiuhong Yu
- & Yong Qin
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Article
| Open AccessMultimaterial fiber as a physical simulator of a capillary instability
Capillary breakup in multimaterial fibers is explored for the self-assembly of optoelectronic systems. However, its insights primarily stem from numerical simulations, qualitative at best. The authors formulate an analytical model of such breakup, obtaining a window in the governing parameters where the generally chaotic breakup becomes predictable and thus engineerable.
- Camila Faccini de Lima
- , Fan Wang
- & Alexander Gumennik
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Article
| Open AccessCell-inspired design of cascade catalysis system by 3D spatially separated active sites
Cells contain isolated compartments that spatially confine different enzymes, enabling high-efficiency enzymatic cascade reactions. Herein, the authors report a cell-inspired design of biomimetic cascade catalysis system by immobilizing Fe single atoms and Au nanoparticles on the inner and outer layers of three-dimensional nanocapsules, respectively, to enable highly selective colorimetric glucose detection.
- Qiuping Wang
- , Kui Chen
- & Yuen Wu
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Article
| Open AccessLong-wave infrared photothermoelectric detectors with ultrahigh polarization sensitivity
Infrared polarization-sensitive photodetectors are attractive owing to their widespread applications. Here, the authors report a long-wave infrared photodetector with an ultrahigh polarization sensitivity by leveraging the 1D geometry of Tellurium nanoribbon and the finite-size effect of a perfect plasmonic absorber.
- Mingjin Dai
- , Chongwu Wang
- & Qi Jie Wang
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Article
| Open AccessSemiconducting MOFs on ultraviolet laser-induced graphene with a hierarchical pore architecture for NO2 monitoring
NO2 monitoring is important in urban areas where pollutant levels are typically higher. Here authors present a hybrid structure of laser-induced graphene and Cu3HHTP2, a 2D semiconducting MOF, for highly sensitive and rapid detection of NO2 at the parts-per-billion level.
- Hyeongtae Lim
- , Hyeokjin Kwon
- & Hyuk-Jun Kwon
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Article
| Open AccessHigh-resolution discrimination of homologous and isomeric proteinogenic amino acids in nanopore sensors with ultrashort single-walled carbon nanotubes
Ultrashort single-walled carbon nanotubes inserted in lipid bilayers can be used as nanopore sensors. Here, the authors demonstrate the high-resolution discrimination of homologous and isomeric proteinogenic amino acids with such carbon-based nanopores.
- Weichao Peng
- , Shuaihu Yan
- & Yuliang Zhao
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Article
| Open AccessSwitchable biomimetic nanochannels for on-demand SO2 detection by light-controlled photochromism
Conventional nanochannel sensors are passively responsive and may be slowly damaged by analytes present in the environment before detection. Here, authors developed a light-controlled inert/active-switchable biomimetic nanochannel sensor to achieve SO2 on-demand detection and long-term preservation.
- Dan Zhang
- , Yongjie Sun
- & Xuanjun Zhang
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Article
| Open AccessTwo-photon fluorescence imaging and specifically biosensing of norepinephrine on a 100-ms timescale
Norepinephrine (NE) is a key neurotransmitter in the central nervous system of organisms however specifically tracking the transient NE dynamics with high spatiotemporal resolution in living systems remains a great challenge. Herein, the authors developed a small molecular fluorescent probe that can precisely anchor on neuronal cytomembranes and specifically respond to NE on a 100-ms timescale.
- Leiwen Mao
- , Yujie Han
- & Yang Tian
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Article
| Open AccessTunable metasurfaces via the humidity responsive swelling of single-step imprinted polyvinyl alcohol nanostructures
PVA is a hydrogel that has attractive swelling properties for use in tunable photonic applications. Here, the authors exploit PVA with nanoimprint lithography to realize multiplexed optical encryption metasurfaces to display, hide, and destroy encrypted information.
- Byoungsu Ko
- , Trevon Badloe
- & Junsuk Rho
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Article
| Open AccessContinuous biomarker monitoring with single molecule resolution by measuring free particle motion
Various applications would benefit from the ability to continuously measure biomolecules. Here the authors describe a biosensing technology based on the free diffusion of biofunctionalized particles hovering over a sensor surface, which enables monitoring of analytes (pM-µM) over long timespans.
- Alissa D. Buskermolen
- , Yu-Ting Lin
- & Menno W. J. Prins
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Article
| Open AccessMetasurface-driven full-space structured light for three-dimensional imaging
3D depth sensing with structured light enables simultaneous imaging of multiple objects, but has limited field of view and low efficiency. Here, the authors demonstrate 3D imaging with scattered light from a metasurface composed of periodic supercells, covering a 180° field of view with a high-density dot array.
- Gyeongtae Kim
- , Yeseul Kim
- & Junsuk Rho
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Article
| Open AccessChiral molecular imprinting-based SERS detection strategy for absolute enantiomeric discrimination
Absolute chiral discrimination in chiral imprinted systems is complicated by the nonspecific binding of enantiomers. Here, the authors report a SERS “inspector” recognition mechanism to distinguish between specifically and nonspecifically bound enantiomers, even in seawater and urine.
- Maryam Arabi
- , Abbas Ostovan
- & Lingxin Chen
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Article
| Open AccessHumidity-sensitive chemoelectric flexible sensors based on metal-air redox reaction for health management
Self-powered sensors are of interest in wearable technology and other applications. Here, the authors report on the creation of a metal-air redox reaction humidity sensor where the conductance and charge generated is influenced by the amount of absorbed water and demonstrate application in respiration monitoring.
- Shuo Li
- , Yong Zhang
- & Yingying Zhang
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Matters Arising
| Open AccessPitfalls in the location of guest molecules in metal-organic frameworks
- Tomasz Poręba
- , Piero Macchi
- & Michelle Ernst
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Article
| Open AccessIn-sensor image memorization and encoding via optical neurons for bio-stimulus domain reduction toward visual cognitive processing
Designing in-sensor computing systems remains a challenge. Here, the authors demonstrate artificial optical neurons based on the in-sensor computing architecture that fuses sensory and computing nodes into a single platform capable of reducing data transfer time and energy for encoding and classification.
- Doeon Lee
- , Minseong Park
- & Kyusang Lee
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Article
| Open AccessControllable synthesis of conjugated microporous polymer films for ultrasensitive detection of chemical warfare agents
The high toxicity of nerve agents makes the development of fluorescence sensors with suitable limit of detection challenging. Here, the authors propose a sensor design based on a conjugated microporous polymer film for the detection of diethyl chlorophosphate, a substitute of Sarin, with low detection limit of 2.5 ppt.
- Wanqi Mo
- , Zihao Zhu
- & Bin Li
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Article
| Open AccessIntegrated biosensor platform based on graphene transistor arrays for real-time high-accuracy ion sensing
The potential of 2D materials for biosensing applications is often limited by large device-to-device variation. Here, the authors report a calibration method and a machine learning approach leveraging the redundancy of a sensing platform based on 256 integrated graphene transistors to enhance the system accuracy in real-time ion classification.
- Mantian Xue
- , Charles Mackin
- & Tomás Palacios
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Article
| Open AccessElectrically tunable two-dimensional heterojunctions for miniaturized near-infrared spectrometers
Miniaturized infrared spectrometers are required for imaging and remote sensing applications, but they are usually characterized by a cm-scale footprint. Here, the authors report the realization of near-infrared spectrometers based on Au-atom-intercalated ReS2/WSe2 heterostructures with an active footprint < 10 μm and electrically tunable photoresponse.
- Wenjie Deng
- , Zilong Zheng
- & Yongzhe Zhang
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Article
| Open AccessOn-chip mid-infrared photothermoelectric detectors for full-Stokes detection
Mid-infrared polarization-sensitive photodetectors are desired for several applications, such as chemical analysis and biomedical diagnosis. Here, the authors report on-chip polarimeters based on the combination of plasmonic chiral metamaterials and 2D thermoelectric materials, showing tunable full-Stokes detection of linearly and circularly polarized light at room temperature.
- Mingjin Dai
- , Chongwu Wang
- & Qi Jie Wang
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Article
| Open AccessHost-guest liquid gating mechanism with specific recognition interface behavior for universal quantitative chemical detection
In field, visual, chemical detection is of use for a wide range of possible applications. Here, the authors report on the creation of a host-guest liquid gating mechanism where detection of the target host triggers gate opening allowing for gas through the liquid gate, which can be used for visual detection.
- Huimeng Wang
- , Yi Fan
- & Xu Hou
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Article
| Open AccessFast custom wavelet analysis technique for single molecule detection and identification
The authors introduce an accurate, fast and efficient technique to analyze sensory data. They use a continuous wavelet transform concept to look for certain patterns in noisy raw data. The superiority of this approach is demonstrated with fluorescence signals from a chip-based, optofluidic single particle sensor.
- Vahid Ganjalizadeh
- , Gopikrishnan G. Meena
- & Holger Schmidt
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Article
| Open AccessHighly sensitive strain sensors based on piezotronic tunneling junction
Strain-induced piezoelectric polarization can be used to modulate the interface electrical transport. Here, the authors achieved a piezotronic tunneling strain sensor at device scale with optimized performance based on the structure of Ag/HfO2/n-ZnO.
- Qiuhong Yu
- , Rui Ge
- & Yong Qin
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Article
| Open AccessIntegrated near-infrared spectral sensing
What are the minimal hardware requirements for a given class of sensing problems? Here, authors investigate this while proposing a miniaturized near-infrared spectral sensor, based on an array of resonant-cavity enhanced photodetectors, and capable of operating without the need for spectral reconstruction.
- Kaylee D. Hakkel
- , Maurangelo Petruzzella
- & Andrea Fiore
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Article
| Open AccessOptical deciphering of multinary chiral compound mixtures through organic reaction based chemometric chirality sensing
The stereoselective analysis of mixtures of chiral compounds typically requires time-consuming chromatography. Here, the authors combine reaction based chiroptical sensing and chemometric tools to directly determine the absolute configuration, enantiomeric composition and concentration of convoluted samples without physical separation.
- Diandra S. Hassan
- & Christian Wolf
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Article
| Open AccessReaching silicon-based NEMS performances with 3D printed nanomechanical resonators
NEMS devices, nano-electro-mechanical systems, by virtue of their minute size, offer ultra-high sensitivity, though at the expense of manufacturing complexity. Here, Stassi et al succeed in manufacturing high quality factor NEMS devices using high resolution 3D printing.
- Stefano Stassi
- , Ido Cooperstein
- & Carlo Ricciardi
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Article
| Open AccessGrain-boundary-rich polycrystalline monolayer WS2 film for attomolar-level Hg2+ sensors
Here, the authors report the controlled growth of polycrystalline WS2 films with high density of grain boundaries to realize surface plasmon Hg2+ ion sensors exhibiting attomolar sensitivity and enhanced selectivity.
- Lixuan Liu
- , Kun Ye
- & Yongjun Tian
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Article
| Open AccessRapid custom prototyping of soft poroelastic biosensor for simultaneous epicardial recording and imaging
Printed biosensors are important for health monitoring and research purposes. Here, the authors report on the development of a soft poroelastic silicone based sensor which can be easily printed and is resistant to mechanical strain hysteresis, allowing for more accurate electrophysiology readings and imaging.
- Bongjoong Kim
- , Arvin H. Soepriatna
- & Chi Hwan Lee
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Article
| Open AccessCritical angle reflection imaging for quantification of molecular interactions on glass surface
Here, the authors present a method for quantifying molecular interactions on a glass surface, based on measuring surface refractive index changes via the reflectivity near the critical angle. They demonstrate tunable sensitivity and dynamic range, deep vertical sensing range, also for intracellular signals.
- Guangzhong Ma
- , Runli Liang
- & Shaopeng Wang
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Article
| Open AccessTunneling current modulation in atomically precise graphene nanoribbon heterojunctions
Here, the authors characterize the spectroscopic and transport properties of heterojunctions composed of quasi-metallic and semiconducting graphene nanoribbons (GNRs) with different widths, showing a predominant quantum tunnelling mechanism. The GNR heterojunctions can also be used to realize adsorbate sensors with high sensitivity.
- Boris V. Senkovskiy
- , Alexey V. Nenashev
- & Alexander Grüneis
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Article
| Open AccessSub-second and ppm-level optical sensing of hydrogen using templated control of nano-hydride geometry and composition
Detecting hydrogen is important for development of renewable energy sources. Here, the authors present lightweight optical hydrogen sensors based on a metasurface of PdCo nano-patchy particle arrays, which achieve sensitive hydrogen detection in less than 1 s, and without risk of sparking.
- Hoang Mai Luong
- , Minh Thien Pham
- & Tho Duc Nguyen
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Article
| Open AccessGiant gauge factor of Van der Waals material based strain sensors
The Gauge factor (GF) enhancement in strain sensors remains a key challenge. Here the authors leverage the piezoelectric and photoelectric effects in a class of van der Waals materials to tune the GF, and obtain a record GF up to 3933 for a SnS2-based strain sensor.
- Wenjie Yan
- , Huei-Ru Fuh
- & Han-Chun Wu
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Article
| Open AccessRapid electrochemical detection of coronavirus SARS-CoV-2
Currently the most common method of COVID-19 diagnosis is by qRT-PCR which is slow and requires expensive instrumentation. Here the authors report an electrochemical biosensor based on isothermal rolling circle amplification for rapid detection of SARS-CoV-2 in clinical samples.
- Thanyarat Chaibun
- , Jiratchaya Puenpa
- & Benchaporn Lertanantawong
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Article
| Open AccessRobust all-optical single-shot readout of nitrogen-vacancy centers in diamond
The NV center in diamond has been used extensively in sensing; however single shot readout of its spin remains challenging, requiring complex optical setups. Here, Irber et al. demonstrate a more robust scheme that achieves single-shot readout even when using inefficient detection optics.
- Dominik M. Irber
- , Francesco Poggiali
- & Friedemann Reinhard
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Article
| Open AccessUltra-high dynamic range quantum measurement retaining its sensitivity
Usually, quantum sensing protocols impose a trade-off between sensitivity and maximum range. Here, the authors demonstrate a non-adaptive algorithm for quantum sensors to measure AC fields with a large range for which the loss in sensitivity is negligible.
- E. D. Herbschleb
- , H. Kato
- & N. Mizuochi
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Article
| Open AccessTwisted-Planar-Twisted expanded porphyrinoid dimer as a rudimentary reaction-based methanol indicator
Directly linked porphyrin dimers show intriguing electronic features but emphasis has been placed on planar monomeric units. Here, the authors report a Twisted-Planar-Twisted framework which can undergo a cis-trans transformation accompanied by a colour change in presence of methanol, making this framework applicable as a methanol sensor.
- Qizhao Li
- , Chengjie Li
- & Yongshu Xie
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Article
| Open AccessOptical imaging of single-protein size, charge, mobility, and binding
Protein identification at the single-molecule level is the ultimate goal for biological research and disease diagnosis. Here, the authors identify the size, charge, mobility, and binding of individual protein molecules by measuring the optical and electrical responses of each protein molecule tethered to a surface.
- Guangzhong Ma
- , Zijian Wan
- & Nongjian Tao
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Article
| Open AccessMagnetic field detection limits for ultraclean graphene Hall sensors
The development of high-performance magnetic field sensors is important for magnetic sensing and imaging. Here, the authors fabricate Hall sensors from graphene encapsulated in hBN and few-layer graphite, demonstrating high performance over a wide range of temperature and background magnetic field.
- Brian T. Schaefer
- , Lei Wang
- & Katja C. Nowack
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Article
| Open AccessDesigner patterned functional fibers via direct imprinting in thermal drawing
Creating micro/nanostructures on fibers is beneficial to many fiber-based devices, which remains a challenge in large-scale fabrication due to elongation and reflow. Here, the authors demonstrate a method for generating high-resolution, arbitrarily designed surface patterns on fiber during the thermal drawing process.
- Zhe Wang
- , Tingting Wu
- & Lei Wei
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Article
| Open AccessQuantum effect-based flexible and transparent pressure sensors with ultrahigh sensitivity and sensing density
Though flexible pressure sensors with high sensitivity are attractive for health monitoring applications, existing device sensing mechanisms limit their practical applicability. Here, the authors report quantum tunnelling-based pressure sensors with high sensitivity and fast signal readout.
- Lan Shi
- , Zhuo Li
- & Limin Wu
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Article
| Open AccessSelective ion sensing with high resolution large area graphene field effect transistor arrays
The authors demonstrate wafer-scale, graphene-based ion sensitive field effect transistors arrays for simultaneous concentration measurement of K+, Na+, NH4+, NO3−, SO42−, HPO42− and Cl−, and use their technology for real-time ion concentration measurements in an aquarium with lemnoideae lemna over a period of three weeks.
- Ibrahim Fakih
- , Oliver Durnan
- & Thomas Szkopek
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Article
| Open AccessShape adaptable and highly resilient 3D braided triboelectric nanogenerators as e-textiles for power and sensing
Low power output and poor sensing ability are bottlenecks for the practical application of fabric-based triboelectric nanogenerators (TENGs). The authors develop a shape adaptable and highly resilient 3D braided TENG, which is endowed with enhanced power output and improved pressure sensitivity.
- Kai Dong
- , Xiao Peng
- & Zhong Lin Wang
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Article
| Open AccessInsights into the mechanism of coreactant electrochemiluminescence facilitating enhanced bioanalytical performance
Electrochemiluminescence (ECL) is a leading technique in biosensing. Here the authors identify an ECL generation mechanism near the electrode surface, which they exploit in combination with the use of branched amine coreactants to improve the ECL signal beyond the state-of-the-art immunoassays.
- Alessandra Zanut
- , Andrea Fiorani
- & Francesco Paolucci
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Article
| Open AccessUltrathin 2 nm gold as impedance-matched absorber for infrared light
Long-term stability and broad spectral response are highly desired features of absorbers. Here, the authors report impedance matched absorbers based on 2 nm thick gold layer operating within the mid-infrared range from 2 to 20 μm, enabling stable long term absorptivity of 47(3) % which is mostly wavelength independent.
- Niklas Luhmann
- , Dennis Høj
- & Silvan Schmid