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| Open AccessRemote near-field spectroscopy of vibrational strong coupling between organic molecules and phononic nanoresonators
Vibrational strong coupling (VSC) promises ultrasensitive IR spectroscopy and modification of material properties. Here, nanoscale mapping of VSC between organic molecules and individual IR nanoresonators is achieved by remote near-field spectroscopy.
- Irene Dolado
- , Carlos Maciel-Escudero
- & Rainer Hillenbrand
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Article
| Open AccessOptical cavity-mediated exciton dynamics in photosynthetic light harvesting 2 complexes
Light-matter interaction can induce changes to the properties of the system by creating hybrid collective states of light and molecular excitations, the so called polaritons. Here the authors use femtosecond pump-probe spectroscopy to explore exciton-polariton dynamics in a photosynthetic protein, light harvesting 2 complexes, and find evidence for rapid energy transfer to dark polariton states.
- Fan Wu
- , Daniel Finkelstein-Shapiro
- & Tönu Pullerits
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Article
| Open AccessHelicity dependent photoresistance measurement vs. beam-shift thermal gradient
Many recent studies have explored the response of magnetic systems to circularly polarised light. To achieve this, typically experiments use a birefringent crystal. Here, Yang et al show that any small error in the alignment of the crystal can result in a beam shift, and this shift can lead to spurious signals similar yet unrelated to the electron spin.
- Haozhe Yang
- , Eva Schmoranzerová
- & Ioan-Mihai Miron
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Article
| Open AccessTwo-dimensional Thouless pumping of light in photonic moiré lattices
Extending the control over topological system will open the doors to both fundamental studies and applications. Here the authors demonstrate thouless topological transport of light in a bulk tunable moiré lattice.
- Peng Wang
- , Qidong Fu
- & Fangwei Ye
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Article
| Open AccessDemonstration of intracellular real-time molecular quantification via FRET-enhanced optical microcavity
The authors introduce an active-mode optical microcavity sensor with enhanced sensitivity via Förster resonant energy transfer. Changes in lasing wavelengths of both donor and acceptor enable quantitative molecular analysis and real-time monitoring of intracellular molecules.
- Yaping Wang
- , Marion C. Lang
- & Pu Wang
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Article
| Open AccessStokes meta-hologram toward optical cryptography
Achieving optical cryptography scheme with both high capacity and security is highly desirable. Here, authors report a Stokes meta-hologram with a hierarchical encryption strategy that allows vector encryptions to produce depth-masked ciphertexts.
- Xuyue Guo
- , Peng Li
- & Jianlin Zhao
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Article
| Open AccessUltrasensitive probing of plasmonic hot electron occupancies
Experimental evidence is given that upon the optical excitation of surface plasmon polaritons, a nonthermal electron population appears in the topmost domain of the plasmonic film directly coupled to the local fields.
- Judit Budai
- , Zsuzsanna Pápa
- & Péter Dombi
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Article
| Open AccessQuantum capacities of transducers
A unified metric to assess the performances of quantum transducers, i.e., converters of quantum information between different physical systems - is still lacking. Here the authors propose quantum capacity as such metric, and use it to investigate the optimal designs of generic quantum transduction schemes.
- Chiao-Hsuan Wang
- , Fangxin Li
- & Liang Jiang
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Article
| Open AccessSuper-resolution microscopy enabled by high-efficiency surface-migration emission depletion
The authors report high-efficiency emission depletion through a surface migration emission depletion mechanism, which takes advantage of the effects of surface quenching and energy migration in nanocrystals. They demonstrate super-resolution microscopy with very low depletion saturation intensities.
- Rui Pu
- , Qiuqiang Zhan
- & Xiaogang Liu
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Article
| Open AccessHyperbolic material enhanced scattering nanoscopy for label-free super-resolution imaging
The authors demonstrate a label-free superresolution imaging method by using a hyperbolic material as a substrate for tailored light-matter interactions. The hyperbolic material enhanced scattering, combined with dark-field detection, result in 5.5-fold resolution improvement beyond the diffraction limit.
- Yeon Ui Lee
- , Shilong Li
- & Zhaowei Liu
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Article
| Open AccessGate-tunable quantum pathways of high harmonic generation in graphene
Under strong laser fields, materials exhibit extreme non-linear optical response, such as high harmonic generation. These higher harmonics provide insights into electron behaviour in materials in sub-laser cycle timescale. Here, Cha et al study higher harmonic generation resulting from the laser driven motion of massless Dirac fermions in graphene.
- Soonyoung Cha
- , Minjeong Kim
- & Jonghwan Kim
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Article
| Open AccessPhotonic quadrupole topological insulator using orbital-induced synthetic flux
Here the authors experimentally demonstrate a photonic quadrupole topological insulator in a photonic lattice, in which required synthetic π flux is induced by different symmetry representations of the orbitals in a mixed-orbital lattice.
- Julian Schulz
- , Jiho Noh
- & Georg von Freymann
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Article
| Open AccessNanoscale heterogeneity of ultrafast many-body carrier dynamics in triple cation perovskites
The optoelectronic performance of lead halide perovskite in highfluence applications are hindered by heterogeneous multi-polaron interactions in the nanoscale. Here, Nishda et al. spatially resolve sub-ns relaxation dynamics on the nanometer scale by ultrafast infrared pumpprobe nanoimaging.
- Jun Nishida
- , Peter T. S. Chang
- & Markus B. Raschke
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Article
| Open AccessTowards highly efficient NIR II response up-conversion phosphor enabled by long lifetimes of Er3+
Development of efficient upconversion (UC) phosphors that emit under irradiation in the NIR II region is challenging - most UC materials rely on the presence of sensitizers absorbing at shorter wavelengths. Here, authors synthesize Er3+ doped ternary sulfides phosphors with visible UC efficiency up to 2.6% and long emission lifetimes under 1532 nm irradiation, via an excited state absorption mechanism.
- Xiumei Yin
- , Wen Xu
- & Bin Dong
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Article
| Open AccessHigh-speed, scanned laser structuring of multi-layered eco/bioresorbable materials for advanced electronic systems
Designing and manufacturing eco/bioresorbable electronic systems remains a challenge. The authors introduce a picosecond-pulsed laser-based scheme that exploits controlled patterning, thinning, and/or cutting to manipulate multilayers of eco/bioresorbable materials for a wide range of advanced electronic systems.
- Quansan Yang
- , Ziying Hu
- & John A. Rogers
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Article
| Open AccessTopological polarization singular lasing with highly efficient radiation channel
Here the authors develop topological polarization singular lasers that feature paired radiation channels carrying distinct topological properties which leads to single mode lasing with high external quantum efficiency.
- Yun-Gang Sang
- , Jing-Yu Lu
- & Ren-Min Ma
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Article
| Open AccessA warm-white light-emitting diode based on single-component emitter aromatic carbon nitride
Designing single-component materials with white-light electroluminescence is highly demanded for artificial lighting applications. Here, the authors fabricate a single-component white-light electroluminescence device based on an aromatic carbon nitride material with high maximum luminance and external quantum efficiency.
- Yunhu Wang
- , Kunpeng Wang
- & Jun Xing
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Article
| Open AccessSensitivity and spectral control of network lasers
Nanophotonic light sources with programmable emission spectrum are important building blocks for integrated photonics, sensing and optical computing. Here the authors tune the complex laser spectrum of a network laser achieving selective lasing of a single, two or more modes.
- Dhruv Saxena
- , Alexis Arnaudon
- & Riccardo Sapienza
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Article
| Open AccessFlexible hyperspectral surface plasmon resonance microscopy
The authors developed a pristine hyperspectral SPR microscopy that enables monochromatic and polychromatic SPR imaging with flexible field-of-view option, single-pixel spectral SPR sensing and 2D quantification of thin films with resonant wavelength images.
- Ziwei Liu
- , Jingning Wu
- & Zhi-mei Qi
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Article
| Open AccessNon-classical correlations over 1250 modes between telecom photons and 979-nm photons stored in 171Yb3+:Y2SiO5
Multimode operation would greatly improve the performances of quantum repeaters. Here, the authors demonstrate a fixed-delay atomic frequency comb quantum memory, based on a Y2SiO5 crystal doped with Ytterbium ions, with a time-domain mode capacity of 1250 modes and a bandwidth of 100 MHz.
- M. Businger
- , L. Nicolas
- & Mikael Afzelius
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| Open AccessSynthesized spatiotemporal mode-locking and photonic flywheel in multimode mesoresonators
Here the authors demonstrate spatiotemporal mode-locked dissipative Kerr soliton and enhanced photonic flywheel performances in both the fundamental comb linewidth and DKS timing jitter.
- Mingming Nie
- , Kunpeng Jia
- & Shu-Wei Huang
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Article
| Open AccessStrongly enhanced THz generation enabled by a graphene hot-carrier fast lane
THz imaging and spectroscopy always request even more efficient components. Here the authors, thanks to a modified photoconductive switch that includes a graphene layer, demonstrate a high-speed photoconductive switch without sacrificing the generated power.
- Dehui Zhang
- , Zhen Xu
- & Zhaohui Zhong
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| Open AccessMonolithically integrated, broadband, high-efficiency silicon nitride-on-silicon waveguide photodetectors in a visible-light integrated photonics platform
Efficient and broadband visible-light photodetectors will bring great advantages in applications such as biosensing and quantum information. Here the authors develop a photodetector with high quantum efficiency across broad wavelength range suitable for monolithic integration in photonics circuits.
- Yiding Lin
- , Zheng Yong
- & Joyce K. S. Poon
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Article
| Open AccessHighly nonlinear dipolar exciton-polaritons in bilayer MoS2
Dipolar excitons enable large nonlinear interaction but are usually hampered by their weak oscillator strength. Here, the authors demonstrate the strong light-matter coupling of interlayer dipolar excitons having unusually large oscillator strength in bilayer MoS2 resulting in highly nonlinear dipolar polaritons.
- Biswajit Datta
- , Mandeep Khatoniar
- & Vinod M. Menon
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Article
| Open AccessMirror-induced reflection in the frequency domain
We show frequency domain mirrors that provide reflections of optical mode propagation in the frequency domain. We theoretically investigated the mirror properties and experimentally demonstrate it using polarization and coupled-resonator-based coupling on thin film Lithium Niobate.
- Yaowen Hu
- , Mengjie Yu
- & Marko Lončar
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| Open AccessNanometer-scale photon confinement in topology-optimized dielectric cavities
Here, the authors integrate measured fabrication constraints in topology optimization to design a highly optimized dielectric nanocavity. The theoretically predicted confinement of light below the diffraction limit is confirmed by near- and far-field spectroscopy.
- Marcus Albrechtsen
- , Babak Vosoughi Lahijani
- & Søren Stobbe
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Article
| Open AccessSynthetic five-wave mixing in an integrated microcavity for visible-telecom entanglement generation
High-order optical nonlinearities are a key tool in photonics and quantum optics, but their use is hindered by materials’ small intrinsic high-order susceptibility. Here, the authors show how to realize high-order nonlinear processes by combining intrinsic low-order ones in a microcavity.
- Jia-Qi Wang
- , Yuan-Hao Yang
- & C.-L. Zou
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Article
| Open AccessSlow light in a 2D semiconductor plasmonic structure
Slow light effects are interesting for telecommunications and quantum photonics applications. Here, the authors use coupled exciton-surface plasmon polaritons (SPPs) in a hybrid monolayer WSe2-metallic waveguide structure to demonstrate a 1300-fold reduction of the SPP group velocity.
- Matthew Klein
- , Rolf Binder
- & John R. Schaibley
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Article
| Open AccessMolecular doping of nucleic acids into light emitting crystals driven by multisite-intermolecular interaction
DNAs exhibit a unique molecular doping structure, unseen in conventional hybrid assemblies, when doped into light-emitting organic materials. Here authors unveil doping mechanism of DNAs into organic semiconducting crystals and tailor their photoluminescence and optical waveguide phenomena.
- Woo Hyuk Jung
- , Jin Hyuk Park
- & Dong June Ahn
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Article
| Open AccessControlled filamentation instability as a scalable fabrication approach to flexible metamaterials
The simple and scalable fabrication of high aspect ratio encapsulated flexible nanowire arrays with controlled size and periodicity is demonstrated and modelled, enabling nanophotonics applications requiring long-range order over several meters.
- William Esposito
- , Louis Martin-Monier
- & Fabien Sorin
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Article
| Open AccessObservation and control of Casimir effects in a sphere-plate-sphere system
Experimental studies of the Casimir effect have involved only interactions between two bodies so far. Here, the authors observe a micrometer-thick cantilever under the Casimir force exerted by microspheres from two sides simultaneously.
- Zhujing Xu
- , Peng Ju
- & Tongcang Li
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Article
| Open AccessContinuous entanglement distribution over a transnational 248 km fiber link
Fibre-based entanglement distribution represents a key primitive for quantum applications such as QKD. Here, the authors demonstrate it across 248 km of deployed fiber, observing stable detected pair rates of 9 Hz for 110 h.
- Sebastian Philipp Neumann
- , Alexander Buchner
- & Rupert Ursin
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Article
| Open AccessAn ultra-high gain single-photon transistor in the microwave regime
Successfully controlling an optical signal by a single gate photon would have great applicability for quantum networks and all-optical computing. Here, the authors realise a single-photon transistor in the microwave regime based on superconducting quantum circuits.
- Zhiling Wang
- , Zenghui Bao
- & Luming Duan
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Article
| Open AccessSpray-coated perovskite hemispherical photodetector featuring narrow-band and wide-angle imaging
Hemispherical photodetectors allow wide sight angle without the complex optical paths of fisheye lenses. Here, Wei et al, report a spray-coated quasi-two-dimensional perovskite hemispherical photodetector with wavelength selective response from the visible to the near-infrared.
- Xiaopeng Feng
- , Yuhong He
- & Haotong Wei
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Article
| Open AccessNonlinear germanium-silicon photodiode for activation and monitoring in photonic neuromorphic networks
Large-scale silicon-based integrated artificial neural networks lack of silicon-integrated optical neurons. Here, Yu et al, report a self-monitored all-optical neural network enabled by nonlinear germanium-silicon photodiodes, making the photonic neural network more versatile and compact.
- Yang Shi
- , Junyu Ren
- & Xinliang Zhang
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Article
| Open AccessReal-time holographic lensless micro-endoscopy through flexible fibers via fiber bundle distal holography
Fiber-based micro-endoscopes are minimally invasive, but 3D imaging is limited by the need for bulky optical elements or rigid fibers. Here, the authors demonstrate holographic imaging through flexible and dynamically bent multi-core fibers by adding partially reflecting mirror to the distal fiber-tip.
- Noam Badt
- & Ori Katz
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Article
| Open AccessDiffraction-engineered holography: Beyond the depth representation limit of holographic displays
Improving the image depth perception of holograms while maintaining high image quality is a current challenge. Here the authors propose an efficient solution relying on a multi-plane hologram technique that reconstruct different blurred images and sharply focused images depending on a propagation distance.
- Daeho Yang
- , Wontaek Seo
- & Hong-Seok Lee
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Article
| Open AccessQuantized topological pumping of solitons in nonlinear photonics and ultracold atomic mixtures
Synthetic lattice systems are powerful platforms for studying the influence of intrinsic nonlinearities on topological phenomena. Here the authors elucidate the topological transport of solitons in terms of Wannier functions displacement and they introduce a nonlinearity-induced topological transport effect that could be observed in ultracold quantum mixtures.
- Nader Mostaan
- , Fabian Grusdt
- & Nathan Goldman
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Article
| Open AccessMetasurface-driven full-space structured light for three-dimensional imaging
3D depth sensing with structured light enables simultaneous imaging of multiple objects, but has limited field of view and low efficiency. Here, the authors demonstrate 3D imaging with scattered light from a metasurface composed of periodic supercells, covering a 180° field of view with a high-density dot array.
- Gyeongtae Kim
- , Yeseul Kim
- & Junsuk Rho
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Article
| Open AccessAll-optical control of spin in a 2D van der Waals magnet
The use of light in driving the magnetization of materials has great technological potential, as well as allowing for insights into the fast dynamics of magnetic systems. Here, the authors combine CrI3, a van der Waals magnet, with WSe2, and demonstrate all optical switching of the resulting heterostructure.
- Maciej Da̧browski
- , Shi Guo
- & Robert J. Hicken
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Article
| Open AccessMetamaterial-enabled asymmetric negative refraction of GHz mechanical waves
Known examples of negative refraction in metamaterials do not distinguish between positive and negative angles of incidence. Here, the authors show that it is possible to break this symmetry using an asymmetric unit cell, and demonstrate it using a mechanical metamaterial working at GHz frequencies.
- Simone Zanotto
- , Giorgio Biasiol
- & Alessandro Pitanti
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Article
| Open AccessSub-optical-cycle light-matter energy transfer in molecular vibrational spectroscopy
Energy transfer between the electromagnetic field and atoms or molecules is fundamentally interesting. Here the authors demonstrate stepwise energy transfer between broadband mid-infrared optical pulses and vibrating methylsulfonylmethane molecules in aqueous solution.
- Martin T. Peschel
- , Maximilian Högner
- & Ioachim Pupeza
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Article
| Open AccessHigh-quality microresonators in the longwave infrared based on native germanium
Developing longwave infrared technology hide intrinsic challenges but at the same time is important to develop sensing and imaging for detection, ranging, and monitoring systems. Here the authors demonstrate the fabrication of high-quality microresonators in the LWIR with the simple use of native germanium.
- Dingding Ren
- , Chao Dong
- & David Burghoff
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Article
| Open AccessNoise-injected analog Ising machines enable ultrafast statistical sampling and machine learning
Ising machines are accelerators for computing difficult optimization problems. In this work, Böhm et al. demonstrate a method that extends their use to perform statistical sampling and machine learning orders-of-magnitudes faster than digital computers.
- Fabian Böhm
- , Diego Alonso-Urquijo
- & Guy Van der Sande
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Article
| Open AccessNano-electromechanical spatial light modulator enabled by asymmetric resonant dielectric metasurfaces
This work experimentally demonstrates nano-electromechanically tunable asymmetric dielectric metasurfaces. The metasurfaces enable large phase tuning, high reflection, a wavelength-scale pixel size, and electrical control of diffraction patterns.
- Hyounghan Kwon
- , Tianzhe Zheng
- & Andrei Faraon
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Article
| Open AccessSub-wavelength patterned pulse laser lithography for efficient fabrication of large-area metasurfaces
Fabrication of metasurfaces with nanoscale structures is inefficient for large areas. Here, the authors introduce patterned pulse laser lithography for creating structured arrays with sub-wavelength feature on large-area thin films under ambient conditions.
- Lingyu Huang
- , Kang Xu
- & Shaolin Xu
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Article
| Open AccessFarey tree and devil’s staircase of frequency-locked breathers in ultrafast lasers
Fractal optical solitons were studied in theory while it is cumbersome their experimental realization in optics setups. Here, the authors find that breathing solitons in lasers constitute fractals―the devil’s staircases, which are around 3000 times more stable than classical ones.
- Xiuqi Wu
- , Ying Zhang
- & Heping Zeng
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Article
| Open AccessChip-scale high-peak-power semiconductor/solid-state vertically integrated laser
Here the authors demonstrate chip-scale high-peak-power lasers by vertical integration of semiconductor and solid state laser gain mediums to reach the same maturity level as existing semiconductor lasers, which are suitable for miniaturization and cost-effective mass production.
- Jianglin Yue
- , Kenji Tanaka
- & Masanao Kamata
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Article
| Open AccessTracking moving objects through scattering media via speckle correlations
Imaging though strongly scattering media is challenging and computationally intensive. Here, the authors show that tracking of moving objects can be achieved with minimal computational effort by combining cross-correlations of the measured speckle pattern at different times.
- Y. Jauregui-Sánchez
- , H. Penketh
- & J. Bertolotti