Featured
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Three-dimensional imaging of cavity vacuum with single atoms localized by a nanohole array
An optical cavity can be used to measure fluctuations in the vacuum due to creation and annihilation of virtual particles. Using a nanohole array to control the position of probe atoms, Lee et al.map the vacuum field in two directions and combine this with spontaneous emission spectra to obtain a 3D profile.
- Moonjoo Lee
- , Junki Kim
- & Kyungwon An
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Laser printing of silicon nanoparticles with resonant optical electric and magnetic responses
Silicon nanoparticles are of interest for their optical properties, for example, in light scattering. Here, Zywietz et al. achieve the laser printing of silicon nanoparticles on a substrate at predefined positions, and with control over their crystalline phase.
- Urs Zywietz
- , Andrey B. Evlyukhin
- & Boris N. Chichkov
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Two-photon polarization-selective etching of emergent nano-structures on diamond surfaces
Using light to manipulate matter on scales smaller than its wavelength presents a major challenge. Here, the authors show that two-photon surface excitation of diamond surfaces etches a variety of nano-scale patterns, comprising evidence for carbon ejection via a highly localized photon interaction with the crystal bonds.
- A. Lehmann
- , C. Bradac
- & R. P. Mildren
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| Open AccessAdaptive real-time dual-comb spectroscopy
The precision of frequency combs makes them the ideal tool for applications in areas such as optical metrology. Here, Ideguchi et al. demonstrate real-time spectroscopy with frequency combs where laser instabilities are electronically compensated, and which is based on commercially available components.
- Takuro Ideguchi
- , Antonin Poisson
- & Theodor W. Hänsch
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A 1.7 nm resolution chemical analysis of carbon nanotubes by tip-enhanced Raman imaging in the ambient
Tip-enhanced Raman spectroscopy allows chemical imaging of materials with high spatial resolution. Here, using plasmonic effects from a gold tip and gold substrate, Chen et al.achieve the chemical imaging of a carbon nanotube down to 1.7 nm resolution at ambient conditions.
- Chi Chen
- , Norihiko Hayazawa
- & Satoshi Kawata
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| Open AccessAll-optical phase modulation in a cavity-polariton Mach–Zehnder interferometer
Quantum fluids such as cavity-polaritons show nonlinear optical properties of interest in applications such as quantum optics. Here, Sturm and colleagues demonstrate an optical control of the phase of a polariton flow, and make use of this to realize a compact exciton–polariton interferometer.
- C. Sturm
- , D. Tanese
- & J. Bloch
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Wavefront sensing reveals optical coherence
The coherence of light is vital for applications like imaging and sensing, but is hard to measure with normal photodetectors. Stoklasa et al.show that, when combined with methods from quantum information processing, wavefront sensors can measure the complete coherence properties of a signal in a single-shot.
- B. Stoklasa
- , L. Motka
- & L. L. Sánchez-Soto
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| Open AccessDeterministic and electrically tunable bright single-photon source
Bright and tunable single-photon sources are essential for future quantum technologies. Here, the authors deterministically couple a quantum dot to a pillar structure that enables application of electric fields to provide a tunable single-photon source with a demonstrated extraction efficiency of 53%.
- A. K. Nowak
- , S. L. Portalupi
- & P. Senellart
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Precision spectroscopy by photon-recoil signal amplification
Quantum logic spectroscopy gives precise measurements of atoms and molecules with long-lived states by transferring information to a second trapped ion via light pulses. By detecting photon recoil imparted to the trapped ion, Wan et al.extend this method to fast dipole-allowed transitions.
- Yong Wan
- , Florian Gebert
- & Piet O Schmidt
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| Open AccessQuantum metrology with parametric amplifier-based photon correlation interferometers
Interferometers play a key role in precision measurements and metrology. Here, the authors demonstrate a new type of interferometer that replaces the standard beam splitter elements with parametric amplifiers, which provides enhanced performance compared with a Mach–Zehnder interferometer.
- F. Hudelist
- , Jia Kong
- & Weiping Zhang
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Highly stretchable and transparent nanomesh electrodes made by grain boundary lithography
One of the key components in stretchable electronics is the electrical conductors, which need to show a low electrical resistance even when strained. Here, by using sacrificial grain boundaries as a fabrication template, Guo and colleagues fabricate highly transparent gold nanomesh electrodes with exceptionally high stretchability.
- Chuan Fei Guo
- , Tianyi Sun
- & Zhifeng Ren
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| Open AccessSingle-shot tomographic movies of evolving light-velocity objects
Tomography enables the reconstruction of objects, and its application to moving objects uncovers otherwise hidden phenomena, particularly at light velocity. Li et al.present a tomographic method that can visualize evolving laser-induced structures in a single shot.
- Zhengyan Li
- , Rafal Zgadzaj
- & Michael C. Downer
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Optical measurements of long-range protein vibrations
Many biological processes rely on fluctuations in protein structure, but the characterization of extended structural motions is challenging. Here the authors use orientation-sensitive terahertz near-field microscopy to report the optical observation of long-range protein vibrational modes.
- Gheorghe Acbas
- , Katherine A. Niessen
- & A.G. Markelz
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| Open AccessMonolithic focused reference beam X-ray holography
There is a trade-off between image contrast and spatial resolution in Fourier transform holography, which limits its application in single-shot X-ray imaging. Here Geilhufe et al. use a Fresnel zone plate to decouple these two factors, which improves the efficiency of high-resolution holography imaging.
- J. Geilhufe
- , B. Pfau
- & S. Eisebitt
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| Open AccessChiral plasmonic DNA nanostructures with switchable circular dichroism
Plasmonic resonances in nanoparticle helices arranged by the DNA origami method can give rise to strong circular dichroism at visible wavelengths. Schreiber et al. show that aligning and then toggling the orientation of such nanoparticle helices enables reversible switching of the dichroic response.
- Robert Schreiber
- , Ngoc Luong
- & Tim Liedl
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An angular fluidic channel for prism-free surface-plasmon-assisted fluorescence capturing
Fluorescence enhancement utilizing surface plasmon excitation is widely used for biomolecular recognition. Here the authors employ a V-shaped trench, incorporating some typical functionalities of a detection system—prism, sensing plate and flow channel—into a single feature.
- Ken-ichi Nomura
- , Subash C.B. Gopinath
- & Makoto Fujimaki
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| Open AccessFocused plasmonic trapping of metallic particles
Focused light beams can be used as optical tweezers for manipulating small dielectric particles, but they normally repel metallic ones. By exploiting surface plasmons excited by a radially polarized beam, Min et al.show that it is possible to trap metallic particles with diameters up to 2.2 μm.
- Changjun Min
- , Zhe Shen
- & Xiaocong Yuan
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| Open AccessStructural analysis and mapping of individual protein complexes by infrared nanospectroscopy
Mid-infrared spectroscopy offers important chemical and structural information about biological samples but diffraction prevents nanoscale studies. Amenabar et al.demonstrate Fourier transform infrared nanospectroscopy for analysing the secondary structure of protein complexes with 30 nm spatial resolution.
- Iban Amenabar
- , Simon Poly
- & Rainer Hillenbrand
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| Open AccessAll-optical control and visualization of ultrafast two-dimensional atomic motions in a single crystal of bismuth
Controlling the motion of atoms in solids with light allows for a deeper understanding of their fundamental properties, yet most studies only deal with one spatial dimension. Katsuki et al.extend this approach to two-dimensional control and use it to visualize atomic motion in bismuth.
- H. Katsuki
- , J.C. Delagnes
- & K. Ohmori
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| Open AccessThree-dimensional optical holography using a plasmonic metasurface
Holographic techniques allow for the construction of 3D images by controlling the wave front of light beams. Huang et al.develop ultrathin plasmonic metasurfaces to provide 3D optical holographic image reconstruction in the visible and near-infrared regions for circularly polarized light.
- Lingling Huang
- , Xianzhong Chen
- & Shuang Zhang
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Metasurface holograms for visible light
Holographic techniques provide phase and amplitude information for images of objects, but normally the hologram thickness is comparable to the light wavelength used. Ni et al.present ultra-thin plasmonic holograms that control amplitude and phase in the visible region and are just 30 nm thick.
- Xingjie Ni
- , Alexander V. Kildishev
- & Vladimir M. Shalaev
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| Open AccessSubnanoradian X-ray phase-contrast imaging using a far-field interferometer of nanometric phase gratings
Phase-contrast imaging has become popular for medical diagnostic purposes because of the ability to see transparent structures at relatively small radiation energy dosed to samples. Wenet al.further develop this technique using nanometric phase gratings to achieve subnanoradian sensitivity.
- Han Wen
- , Andrew A. Gomella
- & Douglas E. Wolfe
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| Open AccessA search for varying fundamental constants using hertz-level frequency measurements of cold CH molecules
Some theories predict that fundamental constants may depend on time, position or the local density of matter. Truppe et al.compare new precise frequency measurements of microwave transitions in cold CH with Milky Way data, placing a new limit on variation in the fine structure constant.
- S. Truppe
- , R.J. Hendricks
- & M.R. Tarbutt
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Tip-enhanced nano-Raman analytical imaging of locally induced strain distribution in carbon nanotubes
Tip-enhanced Raman scattering microscopy gives high-resolution information on nanostructures, yet measurements on more intrinsic properties have been elusive. Yano et al. develop a tip-enhanced method to induce strain in carbon nanotubes and image its distribution along the tube length.
- Taka-aki Yano
- , Taro Ichimura
- & Satoshi Kawata
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Demonstration of a novel focusing small-angle neutron scattering instrument equipped with axisymmetric mirrors
Small-angle neutron scattering is an important technique for a number of fields, but most instruments are inefficient in terms of neutron flux. Using a design based on axisymmetric focussing mirrors, Liu et al. build a compact small-angle neutron-scattering setup that could overcome the present limitations.
- Dazhi Liu
- , Boris Khaykovich
- & David E. Moncton
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Direct measurement of the absolute absorption spectrum of individual semiconducting single-wall carbon nanotubes
A detailed knowledge of the properties of carbon nanotubes is required for their utilization in practical devices. Here the measurement of the absorption spectra of individual carbon nanotubes by Blancon et al.provides an important feedback to the modelling of their intrinsic properties.
- Jean-Christophe Blancon
- , Matthieu Paillet
- & Fabrice Vallée
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An entanglement-enhanced microscope
In microscopy, the standard quantum limit represents the best achievable signal-to-noise ratio for a given light intensity. Here, the authors build an optical microscope that uses entanglement between photon pairs to overcome this barrier.
- Takafumi Ono
- , Ryo Okamoto
- & Shigeki Takeuchi
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Atomic layer lithography of wafer-scale nanogap arrays for extreme confinement of electromagnetic waves
Electromagnetic waves passing through nanogaps can be strongly enhanced, leading to novel physical phenomena. Chen et al. present a new method of atomic layer lithography for patterning uniform arrays of subnanometre gaps in metal films using adhesive tape and show unprecedented field enhancements.
- Xiaoshu Chen
- , Hyeong-Ryeol Park
- & Sang-Hyun Oh
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Complete tomography of a high-fidelity solid-state entangled spin–photon qubit pair
Future quantum communication technologies require entanglement between stationary and flying qubits, in systems that are inherently scalable. To this end, De Greveet al.present full state tomography of a qubit pair formed by entangling a quantum dot spin and a photon, with a fidelity of over 90%.
- Kristiaan De Greve
- , Peter L. McMahon
- & Yoshihisa Yamamoto
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A hybrid high-speed atomic force–optical microscope for visualizing single membrane proteins on eukaryotic cells
Scanning probe microscopy techniques are hard to apply to live cell membrane imaging at high resolution as the temporal and force sensitivity are insufficient to monitor the fast processes. Colom et al.present a solution to this problem by combining high-speed atomic force microscopy with optical microscopy.
- Adai Colom
- , Ignacio Casuso
- & Simon Scheuring
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| Open AccessIntegrated Mach–Zehnder interferometer for Bose–Einstein condensates
Atom interferometers exploit wave-particle duality and can be used as sensitive measurement devices. Berrada et al.present a Mach–Zehnder interferometer for Bose–Einstein condensates trapped on an atom chip and demonstrate enhanced performance using non-classical states.
- T. Berrada
- , S. van Frank
- & J Schmiedmayer
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| Open AccessThree-dimensional deep sub-diffraction optical beam lithography with 9 nm feature size
The fabrication of three-dimensional nanoscale structures is important to nanophotonic applications where light is guided and controlled. The optical beam lithography scheme developed by Gan and colleagues enables the fabrication of three-dimensional structures with feature sizes down to 9 nm.
- Zongsong Gan
- , Yaoyu Cao
- & Min Gu
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| Open AccessA nanometre-scale resolution interference-based probe of interfacial phenomena between microscopic objects and surfaces
Interferometric techniques can provide valuable contact and profile information of microscopic objects on surfaces. This work uses reflection interference contrast microscopy to directly observe contact phenomena and presents novel analytical methods offering high-accuracy nanoscale resolution.
- Jose C. Contreras-Naranjo
- & Victor M. Ugaz
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Large-scale organic nanowire lithography and electronics
The high-speed, large-area printing of aligned semiconducting nanowires is vital for practical device applications. Here, the authors use a high-speed printing technique to print semiconducting nanowire arrays onto device substrates with precise nanowire control, and high field-effect mobilities are observed.
- Sung-Yong Min
- , Tae-Sik Kim
- & Tae-Woo Lee
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Single-shot pulse duration monitor for extreme ultraviolet and X-ray free-electron lasers
Free-electron lasers offer exciting new possibilities for X-ray studies on ultrafast timescales, but their shot-to-shot variability requires new diagnostic tools. Using a plasma switch cross-correlator, Riedel et al. present a single-shot online diagnostic to retrieve the duration of extreme ultraviolet pulses.
- R. Riedel
- , A. Al-Shemmary
- & F. Tavella
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Soft X-ray spectromicroscopy using ptychography with randomly phased illumination
Ptychographic methods can retrieve the complex sample transmittance from diffraction patterns that may have a large dynamic range. For soft X-ray spectromicroscopy, Maiden et al. use a diffuser to randomize the probe phase, reducing the dynamic range of the diffraction data by an order of magnitude.
- A.M. Maiden
- , G.R. Morrison
- & J.M. Rodenburg
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Two-dimensional structure from random multiparticle X-ray scattering images using cross-correlations
A model-independent protocol is developed for reconstructing a two-dimensional particle from multiparticle diffraction images. The method is verified experimentally with gold nanostructures, paving the way towards single-molecule imaging using high-intensity X-ray free-electron laser pulses.
- B. Pedrini
- , A. Menzel
- & R. Abela
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High-resolution correlation spectroscopy of 13C spins near a nitrogen-vacancy centre in diamond
The spin states associated with nitrogen vacancies in diamond could be useful in the development of solid-state quantum information processing. Laraoui et al. resolve the temporal dynamics of spins associated with C-13 atoms near such vacancies to better understand and perhaps better exploit their behaviour.
- Abdelghani Laraoui
- , Florian Dolde
- & Carlos A. Meriles
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Narrowband photodetection in the near-infrared with a plasmon-induced hot electron device
Plasmons excited in gratings create strong resonant absorptions that depend on the nanostructure period. By patterning a gold grating on a silicon substrate, Sobhani et al. exploit plasmon-induced hot electron photocurrent generation to create a narrowband infrared photodetector with greatly enhanced absorption efficiency.
- Ali Sobhani
- , Mark W. Knight
- & Naomi J. Halas
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Bright solid-state sources of indistinguishable single photons
For quantum technologies to become widespread and scalable, bright sources of indistinguishable single photons are essential. Through deterministic positioning of quantum dots in pillar cavities, Gazzano et al.present a solid-state single-photon source with brightness as large as 0.65 photons per pulse.
- O. Gazzano
- , S. Michaelis de Vasconcellos
- & P. Senellart
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| Open AccessUnraveling quantum pathways using optical 3D Fourier-transform spectroscopy
Knowledge of the Hamiltonian of a quantum system is essential for predicting and controlling its behaviour. Li et al.use optical three-dimensional Fourier-transform spectroscopy to separate and study each pathway, gaining quantitative insight into the quantum pathways of an atomic vapour Hamiltonian.
- Hebin Li
- , Alan D. Bristow
- & Steven T. Cundiff
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Review Article |
Hyperlenses and metalenses for far-field super-resolution imaging
The diffraction limit of light constrains the achievable resolution of conventional optical systems, but metamaterials provide numerous avenues to beat it. Lu and Liu review recent advances in super-resolution imaging with hyperlenses and metalenses, and discuss future directions and hurdles for the field.
- Dylan Lu
- & Zhaowei Liu
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Single-shot ultrafast tomographic imaging by spectral multiplexing
Computed tomography relies on scanning to measure an object from many angles, which fails for shot-to-shot changes and ultrafast phenomena. Matliset al. demonstrate an approach based on spectral multiplexing for single-shot tomographic imaging and use it to measure femtosecond plasma filaments.
- N.H. Matlis
- , A. Axley
- & W.P. Leemans
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| Open AccessExploiting multimode waveguides for pure fibre-based imaging
Fibre-based technologies provide miniaturization, flexibility and the capability to access hard to reach areas. Čižmár and Dholakia exploit disorder in multimode fibres to enable a variety of imaging modalities, including bright- and dark-field microscopy and fluorescent imaging, using a single waveguide.
- Tomáš Čižmár
- & Kishan Dholakia
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Article
| Open AccessOptical detection of a single rare-earth ion in a crystal
The optical transitions that occur in rare-earth-doped crystals offer promise for quantum information storage and processing. Kolesovet al.report the optical detection of a single praseodymium ion residing in a crystal host by using an excited-state absorption process to enhance its fluorescence yield.
- R. Kolesov
- , K. Xia
- & J. Wrachtrup
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Optical separation of mechanical strain from charge doping in graphene
The spectral position of Raman peaks is a useful diagnostic for determining the degree of strain and excess electronic charges present in graphene. This study demonstrates that these two contributions can be separated from each other and therefore be obtained at the same time.
- Ji Eun Lee
- , Gwanghyun Ahn
- & Sunmin Ryu
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| Open AccessImaging high-dimensional spatial entanglement with a camera
Measuring the entanglement between down-converted photons is central to many quantum optical experiments, and is normally performed by scanning detectors stepwise across a plane. Edgaret al. use a CCD camera to measure the entire entangled light field, finding strong correlations in position and momentum.
- M.P. Edgar
- , D.S. Tasca
- & M.J. Padgett
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High-resolution three-dimensional partially coherent diffraction imaging
Coherent diffractive imaging exploits coherent X-ray sources to image objects from their diffraction patterns, but fails for decreasing coherence. Using partially coherent diffraction patterns, Clarket al. obtain three dimensional reconstructions of nanocrystals and determine the wavefield coherence.
- J.N. Clark
- , X. Huang
- & I.K. Robinson
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| Open AccessLight-induced spiral mass transport in azo-polymer films under vortex-beam illumination
Non-uniform light beams can create patterns in azo-polymer films by inducing mass transport, yet the process is not well understood. Using optical vortex beams, Ambrosioet al. observe the formation of spiral patterns that are surprisingly sensitive to the optical phase, which they explain with a new model.
- Antonio Ambrosio
- , Lorenzo Marrucci
- & Pasqualino Maddalena