Optical spectroscopy articles within Nature Communications

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  • Article
    | Open Access

    Chiral recognition of amino acids with luminescence, despite its advantages, is usually slow and lacks generality. Here, the authors demonstrate that L-phenylalanine derived benzamide can manifest the structural difference between the natural, left-handed amino acid and its right-handed counterpart via the difference in room-temperature phosphorescence, irrespective of the specific chemical structure.

    • Xiaoyu Chen
    • , Renlong Zhu
    •  & Guoqing Zhang

  • Article
    | Open Access

    Here the authors induce asymmetric transmission in planar Fabry–Pérot microcavities by embedding organic thin films exhibiting apparent circular dichroism (ACD), an optical phenomenon based on 2D chirality.

    • Tzu-Ling Chen
    • , Andrew Salij
    •  & Randall H. Goldsmith

  • Article
    | Open Access

    Authors present a centimeter-scale miniaturized Raman spectrometer using cheap nonstabilized laser diodes, densely packed optics, and non-cooled small sensors while the performance is comparable with expensive bulky research-grade Raman systems.

    • Oleksii Ilchenko
    • , Yurii Pilhun
    •  & Anja Boisen

  • Article
    | Open Access

    Li et al. report large circular dichroism in 2D chiral perovskite single crystals, arises from the inorganic sublattice, instead of chiral ligands, driven by electron-hole exchange interactions. This is evidenced by both reflective circular dichroism spectroscopy and ab initio theory.

    • Shunran Li
    • , Xian Xu
    •  & Peijun Guo

  • Article
    | Open Access

    Bioimaging with photocontrol and multiplexing capability is vital for studying cellular interactions and dynamics, but multiplexed stimulated Raman scattering (SRS) imaging with reversible photocontrol is elusive. Here, the authors report SRS microscopy with Carbow-switch enabling multiplexed SRS imaging and tracking in live cells with reversible photocontrol and high spatiotemporal selectivity.

    • Yueli Yang
    • , Xueyang Bai
    •  & Fanghao Hu

  • Article
    | Open Access

    The performance of Y6-containing donor-acceptor active layers in organic solar cells is highly related to the charge-transfer nature in Y6 aggregates. Here, authors study charge-transfer characteristics of excitations of isolated and aggregated Y6 molecules through electroabsorption spectroscopy.

    • Sudhi Mahadevan
    • , Taili Liu
    •  & Sai-Wing Tsang

  • Article
    | Open Access

    Polaritons, light-matter hybridized quasiparticles, are the fundamental excitation of strong coupling systems and are widely applicable in information technologies. Here the authors applied the concept of time-of-flight measurement in terahertz induced second harmonic generation experiments in various systems to comprehensively study the dispersion relation of phonon-polaritons and reveal potential spin-lattice couplings.

    • Tianchuang Luo
    • , Batyr Ilyas
    •  & Nuh Gedik

  • Article
    | Open Access

    The nature of the molecule-metal interface is crucial for many technological applications. Here, the authors show that the photostability of the material can be sensitive to room light when coated with a single molecular layer, with implications for devices and processes.

    • Chenyang Guo
    • , Philip Benzie
    •  & Jeremy J. Baumberg

  • Article
    | Open Access

    Using gas cells for spectroscopic studies opens possibility for miniaturized platforms that can be integrated with other optical components. Here the authors demonstrate molecular rovibrational spectroscopy by confining molecules in a cell of subwavelength thickness.

    • Guadalupe Garcia Arellano
    • , Joao Carlos de Aquino Carvalho
    •  & Athanasios Laliotis

  • Article
    | Open Access

    The miniaturization of spectrometers to a submillimeter-scale footprint opens opportunities for applications in hyperspectral imaging and lab-on-a-chip systems. Here, the authors report a high-performance single-pixel photodetector spectrometer based on the III-V semiconductor p-graded-n junction, featuring a voltage-tunable optical response.

    • Jingyi Wang
    • , Beibei Pan
    •  & Baile Chen

  • Article
    | Open Access

    Studying the fluctuations of biological membranes with high resolution is challenging. Here, the authors combine metal- and graphene-induced energy transfer (MIET/GIET) with fluorescence correlation spectroscopy (FCS) to monitor such fluctuations with nanometer and microsecond resolution.

    • Tao Chen
    • , Narain Karedla
    •  & Jörg Enderlein

  • Article
    | Open Access

    Graphene oxide is in demand for various applications - however, this is complicated by changing physicochemical properties over time. Here, the authors show the intrinsic, metastable, and transient states of graphene oxide colloids upon ripening.

    • Hayato Otsuka
    • , Koki Urita
    •  & Katsumi Kaneko

  • Article
    | Open Access

    The authors showcase a video-rate hyperspectral imager based on a single-pixel photodetector that can achieve high-throughput hyperspectral video recording at a low bandwidth. Specifically, they propose a joint spatial-spectral encoding scheme which can encode the scene into highly compressed single-pixel measurements and obtain temporal correlation at the same time.

    • Yibo Xu
    • , Liyang Lu
    •  & Kevin F. Kelly

  • Article
    | Open Access

    Differential absorption of polarized light, called dichroism, does not exist in amorphous solids due to the disordered arrangements of atoms. Here, the authors demonstrate that dichroism is intrinsic to all solids and can be controlled using helical light beams carrying orbital angular momentum.

    • Ashish Jain
    • , Jean-Luc Bégin
    •  & Ravi Bhardwaj

  • Article
    | Open Access

    Using femtosecond time-resolved heterodyne-detected vibrational sum-frequency generation spectroscopy the authors determine the vibrational relaxation (T1) time of the O-H stretch at the air/water interface by observing the decay of excited-state OH signals, providing a comprehensive picture of the interfacial vibrational relaxation process of water.

    • Woongmo Sung
    • , Ken-ichi Inoue
    •  & Tahei Tahara

  • Article
    | Open Access

    Here, using single molecule FRET, the unfolding and folding of a discontinuous two-domain protein was studied. The authors find that a dynamic, intermediate population entropically limits the rate of folding while the order of domain folding is kept in a slow-folding mutant.

    • Ganesh Agam
    • , Anders Barth
    •  & Don C. Lamb

  • Article
    | Open Access

    The precise role of cochaperones and ATP hydrolysis in driving Hsp90’s chaperone cycle is largely unclear. Here, the authors use single-molecule FRET to show that several cochaperones are necessary to establish directionality in Hsp90’s conformational cycle.

    • Leonie Vollmar
    • , Julia Schimpf
    •  & Thorsten Hugel

  • Article
    | Open Access

    The authors propose and demonstrate a novel integrated spectrometer that measures any arbitrary spectrum with two-dimensional Fourier transform, breaking the scalability limit in chip-scale spectrometry.

    • Hongnan Xu
    • , Yue Qin
    •  & Hon Ki Tsang

  • Article
    | Open Access

    The requirement for sophisticated objective lenses hinders the miniaturisation of single molecule fluorescence spectroscopy for portable sensing applications. Here, the authors demonstrate a dual-wavelength metalens for real-time monitoring of individual fluorescent nanoparticles.

    • Aleksandr Barulin
    • , Yeseul Kim
    •  & Inki Kim

  • Article
    | Open Access

    Probing molecules in excited vibrational states requires precise methods to extract the spectroscopic parameters. Here the authors demonstrate optical-optical double-resonance spectroscopy of excited-bands of methane using single pass high power continuous wave pump and cavity-enhanced frequency comb probe.

    • Vinicius Silva de Oliveira
    • , Isak Silander
    •  & Aleksandra Foltynowicz

  • Comment
    | Open Access

    The enhanced Coulomb interaction in two dimensions leads to not only tightly bound excitons but also many-particle excitonic complexes: excitons interacting with other quasiparticles, which results in improved and even new exciton properties with better controls. Here, we summarize studies of excitonic complexes in monolayer transition metal dichalcogenides and their moiré heterojunctions, envisioning how to utilize them for exploring quantum many-body physics.

    • Xiaotong Chen
    • , Zhen Lian
    •  & Su-Fei Shi

  • Article
    | Open Access

    A fundamental challenge for molecular electronics is the change in photophysical properties of molecules upon direct electrical contact. Here, the authors observe hot luminescence emitted by single-molecule chromophores that are electrically and mechanically self-decoupled by a tripodal scaffold.

    • Vibhuti Rai
    • , Nico Balzer
    •  & Michal Valášek

  • Article
    | Open Access

    The researchers showcase all-crystalline and hybrid mid-infrared supermirrors with the lowest optical losses ever demonstrated in this wavelength range, representing an unprecedented improvement over any existing mirrors made with any production technology.

    • Gar-Wing Truong
    • , Lukas W. Perner
    •  & Garrett D. Cole

  • Article
    | Open Access

    Conventional spectroscopic techniques are not sufficiently selective to follow the dynamics of trapped carriers in working perovskite solar cells. Here, authors use infrared optical activation spectroscopy to observe real time evolution of trapped carriers and compare the behaviour of trapped holes.

    • Jiaxin Pan
    • , Ziming Chen
    •  & Artem A. Bakulin

  • Article
    | Open Access

    Low-temperature spectroscopy of single fluorescent molecules can be of use to study dynamics in the nano-environment around them. Here, Smit et al. show that the fluorescence wavelength of molecules on the surface of hexagonal boron-nitride is particularly sensitive to how clean this surface is.

    • Robert Smit
    • , Arash Tebyani
    •  & Michel Orrit

  • Article
    | Open Access

    Recent experiments have shown the formation of ferroelectric domains in twisted van der Waals bilayers. Here, the authors report near-field infrared nano-imaging and nano-photocurrent measurements to investigate ferroelectricity in minimally twisted WSe2 by visualizing the plasmonic and photo-thermoelectric response of an adjacent graphene monolayer.

    • Shuai Zhang
    • , Yang Liu
    •  & D. N. Basov

  • Article
    | Open Access

    Nano-environmental probes and advance imaging microscopy provide deep insight into protein phase separation and the interaction of condensates with membranes, revealing that wetting by condensates can modulate membrane lipid packing and hydration.

    • Agustín Mangiarotti
    • , Macarena Siri
    •  & Rumiana Dimova

  • Article
    | Open Access

    Spectroscopic gas sensing with high sensitivity and selectivity finds an increasing number of applications. Here, the authors report an approach to ultrasensitive multiplexed gas sensing by integrating dual-comb spectroscopy with cavity optomechanics.

    • Xinyi Ren
    • , Jin Pan
    •  & Heping Zeng

  • Article
    | Open Access

    Multicolor imaging employing genetically-encodable fluorescent proteins permits spatiotemporal live cell imaging of multiple cues. Here, authors use multicolor lifetime imaging to visualize quadruple-labelled human immunodeficiency viruses within cellular contexts.

    • Tobias Starling
    • , Irene Carlon-Andres
    •  & Sergi Padilla-Parra

  • Article
    | Open Access

    Testing general relativity with optical clocks is important both as a fundamental test and for metrological applications. Here, a vertical linear array of 5 separate ensembles of strontium atoms trapped in a single optical lattice is used to perform a blinded lab-based test of the gravitational redshift at the mm to cm scale.

    • Xin Zheng
    • , Jonathan Dolde
    •  & Shimon Kolkowitz

  • Article
    | Open Access

    Nanoresonator is proven to be an excellent platform for molecular detection, yet a set of them is necessary to identify a molecule fingerprint. Here, the authors utilise low quality resonators with large radiative losses, despite its lower quality factor, to identify molecular absorption spectrum between 5 and 10 μm.

    • Laura Paggi
    • , Alice Fabas
    •  & Patrick Bouchon

  • Article
    | Open Access

    The authors observe the signatures of quadrupolar excitons in a WSe2-WS2-WSe2 trilayer moiré superlattice, originating from the hybridization of the WSe2 valence moiré flatbands. They further use electrostatic gating to reveal a hybridized interlayer Mott insulator state, with holes shared between the two WSe2 layers but laterally confined in moiré superlattices.

    • Zhen Lian
    • , Dongxue Chen
    •  & Su-Fei Shi

  • Article
    | Open Access

    The authors present μeV electron spectromicroscopy, a technique that combines free-space light and electron beams to achieve unmatched spatial and spectral resolution. This approach enables detailed investigation of photonic structures, promising advancements in microscopy and quantum optics.

    • Yves Auad
    • , Eduardo J. C. Dias
    •  & Mathieu Kociak

  • Article
    | Open Access

    Hyperbolic phonon polaritons (HPhPs) in anisotropic van der Waals materials hold promise for nanophotonic applications, but their far-field characterization remains challenging. Here, the authors demonstrate the application of Raman spectroscopy in a backscattering configuration to determine the dispersion of HPhPs in thin GaSe crystals.

    • Alaric Bergeron
    • , Clément Gradziel
    •  & Sébastien Francoeur

  • Article
    | Open Access

    The authors present a fast mid-infrared hyperspectral chemical imaging technique that uses chirped pulse upconversion of sub-cycle pulses at the image plane, with lateral resolution of 15 µm and an adjustable field of view and large spectral range. They demonstrate identification and mapping different components in a microfluidic device, plant cell, and mouse embryo.

    • Yue Zhao
    • , Shota Kusama
    •  & Takao Fuji

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