Nanoscience and technology articles within Nature Communications

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  • Article
    | Open Access

    Crystallization of noble metal atoms usually leads to the thermodynamically stable face-centred cubic phase. Sunet al. show that internal strain in silver nanoparticles leads to lattice distortion and a stable body-centred tetragonal phase.

    • Yugang Sun
    • , Yang Ren
    •  & Dean J. Miller

  • Article
    | Open Access

    Downsizing antennas to the nanoscale is a promising way to manipulate light emission from fluorescent sources. Bussonet al. used a short DNA strand to position a lone fluorescent molecule between two gold particles with nanometre resolution, achieving enhanced decay rates and single photon emission.

    • Mickaël P. Busson
    • , Brice Rolly
    •  & Sébastien Bidault

  • Article |

    Controlling the behaviour of single molecules on electrode interfaces is crucial for the development of molecular spintronics. This study reports spin-polarized scanning tunnelling microscopy data of the spin-split molecular orbitals of a single-molecule magnet adsorbed on a cobalt surface.

    • Jörg Schwöbel
    • , Yingshuang Fu
    •  & Roland Wiesendanger

  • Article |

    Molecular systems with rigid macrocyclic backbones self-assemble into synthetic nanopores that mimic the mass-transport characteristics of biological channels. Zhouet al. produce self-assembling hydrophobic nanopores that mediate highly selective transmembrane ion transport and highly efficient transmembrane water permeability.

    • Xibin Zhou
    • , Guande Liu
    •  & Bing Gong

  • Article |

    Single electron pumps have been proposed as potential candidates for redefining the ampere. This study reports measurements of the quantized current flowing through a semiconductor electron pump with a precision that makes a substantial step towards establishing a direct metric for electrical currents.

    • S.P. Giblin
    • , M. Kataoka
    •  & D.A. Ritchie

  • Article
    | Open Access

    Switches made up of single molecules form the basis for the concept of molecular electronics. Miyamachiet al.demonstrate that an iron-based spin crossover molecule can be switched between different spin states, provided it is decoupled from a metallic substrate by a thin insulating layer.

    • Toshio Miyamachi
    • , Manuel Gruber
    •  & Wulf Wulfhekel

  • Article |

    Scanning probe microscopy and related techniques rely on the availability of very sharp tips. Here, a sharpening technique based on field-directed sputtering is demonstrated, resulting in ultrasharp metallic tips for use in scanning tunnelling microscopy as well as atomic-scale lithographic experiments.

    • S.W. Schmucker
    • , N. Kumar
    •  & J.W. Lyding

  • Article |

    Stretchable electronics based on conducting polymers offer new opportunities for designing flexible technologies. Parket al. build three-dimensional nanostructures from elastomers soaked with liquid metal to produce stretchable conductors with greatly improved strain properties over solid films.

    • Junyong Park
    • , Shuodao Wang
    •  & Seokwoo Jeon

  • Article
    | Open Access

    Nanocrystal quantum dots can exhibit photoluminescence blinking, where the intensity of the emitted light fluctuates due to random charging and discharging. Gallandet al.study thick shell nanocrystals and find that the photoluminescence lifetime can also undergo blinking, without intensity changes.

    • Christophe Galland
    • , Yagnaseni Ghosh
    •  & Victor I. Klimov

  • Article
    | Open Access

    Ultrasmall clusters of atoms form the building blocks of many nanoscale materials. Using a combination of aberration-corrected transmission electron microscopy and numerical simulations, this study uncovers the geometry of these clusters in three dimensions.

    • S. Bals
    • , S. Van Aert
    •  & G. Van Tendeloo

  • Article |

    Ink-jet printing methods are an attractive approach to nanofabrication, where electrohydrodynamic control allows for flexible and cheap fabrication. Here, a new approach is presented using electrostatic nanodroplet autofocussing to produce high aspect ratio nanoscale structures like plasmonic nanoantennas.

    • P. Galliker
    • , J. Schneider
    •  & D. Poulikakos

  • Article |

    Devices made up of nanowires offer promise for a range of electronic, photonic and energy applications. Liuet al. fabricate a miniature capacitor by employing a thin layer of Cu2O as a separator between layers of carbon and copper.

    • Zheng Liu
    • , Yongjie Zhan
    •  & Pulickel M. Ajayan

  • Article |

    Three-dimensional optical metamaterials provide a range of exciting features, such as broadband circular dichroism, yet their fabrication is challenging. Here, a broadband optical circular polarizer is presented based on twisted stacks of metasurfaces, avoiding the issues of three-dimensional fabrication.

    • Y. Zhao
    • , M.A. Belkin
    •  & A. Alù

  • Article |

    Strain engineering has been proposed as a promising strategy for manipulating the electronic properties of graphene. This scanning tunnelling microscopy study demonstrates the feasibility of controlling strain patterns in graphene down to the nanoscale.

    • Jiong Lu
    • , A.H. Castro Neto
    •  & Kian Ping Loh

  • Article
    | Open Access

    Micromechanical oscillators present a route to miniaturisation of devices and may be used as frequency references or sensitive sensors, but their small size means that they often behave nonlinearly. Antonioet al. demonstrate frequency stabilisation of nonlinear resonators by coupling two vibrational modes.

    • Dario Antonio
    • , Damián H. Zanette
    •  & Daniel López

  • Article |

    The singular properties of topological insulators are defined by the topological nature of their metallic surface states. This study shows that by doping Bi2Se3nanoribbons with antimony, the transport properties of these surface states are measurable and can be distinguished from the contributions due to the bulk of the samples.

    • Seung Sae Hong
    • , Judy J. Cha
    •  & Yi Cui

  • Article |

    The spin-dependent thermal and electrical transport properties of nanostructures are central for future applications of spintronic devices. Here, Linet al. report an enhanced spin-dependent thermoelectric effect in an Al2O3-based magnetic tunnel junction.

    • Weiwei Lin
    • , Michel Hehn
    •  & Stéphane Mangin

  • Article
    | Open Access

    Single-photon sources are important for quantum optical technologies, although achieving efficient light extraction from them with waveguides is limited in top-down approaches. Reimeret al. show a high extraction efficiency using a bottom-up method to grow quantum dots on the axis of nanowire waveguides.

    • Michael E. Reimer
    • , Gabriele Bulgarini
    •  & Val Zwiller

  • Article |

    Resistive switching devices are promising candidates for non-volatile memories. Usingin-situ and ex-situ transmission electron microscopy, Yang et al. present an extensive study of the dynamics of filaments forming across the electrodes of resisting switching devices known as electrochemical metallization memories.

    • Yuchao Yang
    • , Peng Gao
    •  & Wei Lu

  • Article
    | Open Access

    Advances in nanoelectromechanical systems have brought improvements in the quality factor of nanomechanical resonators, yet few low-loss transduction schemes exist at high temperature. Using non-dissipative dielectric coupling to a microwave cavity, Faustet al. present an integrated nanomechanical transducer.

    • T. Faust
    • , P. Krenn
    •  & E.M. Weig

  • Article |

    Imaging and tracking the motion of single molecules on cell plasma membranes requires high spatial resolution in three dimensions. Honget al. develop a plasmonic ruler based on the fluorescence enhancement of carbon nanotubes on a gold plasmonic substrate, allowing the observation of nanotube endocytosis in three dimensions.

    • Guosong Hong
    • , Justin Z. Wu
    •  & Hongjie Dai

  • Article
    | Open Access

    Multicompartment micelles can be assembled from block copolymers but it is difficult to manipulate their hierarchical superstructures using straightforward concepts. Here, methods are developed that involve the pre-assembly of subunits for the structurally controlled production of micelles.

    • André H. Gröschel
    • , Felix H. Schacher
    •  & Axel H.E. Müller

  • Article
    | Open Access

    Minimising reflection from the interface between materials is an important goal for optical devices such as solar cells or photodetectors. Spinelliet al. show almost total loss of reflection over a broad spectral range from a silicon surface using periodic arrays of sub-wavelength silicon nanocylinders.

    • P. Spinelli
    • , M.A. Verschuuren
    •  & A. Polman

  • Article
    | Open Access

    Graphene's broad bandwidth makes it promising as a photodetector, but common electronics cannot analyse the currents at high frequencies. Here, using photocurrent measurements, laser-induced carrier generation effects in freely suspended graphene and at graphene–metal interfaces are clarified up to 1 THz.

    • Leonhard Prechtel
    • , Li Song
    •  & Alexander W. Holleitner

  • Article |

    A dual-contrast agent has been developed for combined ultrasound and photoacoustic imaging. This agent uses vaporization for ultrasound contrast enhancement and photoacoustic signal generation, providing significantly higher signals than thermal expansion, the most commonly used photoacoustic mechanism.

    • Katheryne Wilson
    • , Kimberly Homan
    •  & Stanislav Emelianov

  • Article
    | Open Access

    Fluctuations of the electrical current in nanoscale devices reveal important details of the physical processes occurring inside them. Using a quantum point contact placed in its vicinity, Ubbelohde et al. measure the electrical fluctuations in a single-electron transistor, and determine the dynamical features of the transport.

    • Niels Ubbelohde
    • , Christian Fricke
    •  & Rolf J. Haug

  • Article
    | Open Access

    Studying carrier multiplication in materials is important to understand their transport properties and interaction with light. Hiroriet al. show that intense terahertz pulses can generate electron-hole pairs in GaAs quantum wells that then emit infrared light, contrary to the effect with a DC field.

    • H. Hirori
    • , K. Shinokita
    •  & K. Tanaka

  • Article |

    Ferroelectric materials are characterized by a spontaneous polarization, which in practical applications is manipulated by an electric field. This study examines how defects affect the switching with atomic resolution, by usingin situaberration-corrected transmission electron microscopy.

    • Peng Gao
    • , Christopher T. Nelson
    •  & Xiaoqing Pan

  • Article |

    The unique band structure of topological insulators gives rise to insulating bulk and unusual metallic surface properties. By tuning the content of Sb in the ternary compound (Bi1–xSbx)2Te3, Wang and collaborators show it is possible to control the precise features of the band structure in a continuous fashion.

    • Jinsong Zhang
    • , Cui-Zu Chang
    •  & Yayu Wang

  • Article
    | Open Access

    Quantum objects are subject to decoherence effects due to the surrounding environment. This study demonstrates experimentally a counterintuitive example of anomalous decoherence, in which electron spins residing at nitrogen vacancy centres in diamond display longer coherence times under stronger noises.

    • Pu Huang
    • , Xi Kong
    •  & Jiangfeng Du

  • Article
    | Open Access

    Chiral liquid crystals of two-dimensional colloids have not been extensively investigated. Xu and Gao show that graphene oxide can form chiral liquid crystals, and demonstrate that they can be spun into macroscopic fibres, and that subsequent chemical reduction provides graphene fibres with high conductivity.

    • Zhen Xu
    •  & Chao Gao

  • Article |

    Among the wide range of potential applications of graphene, photodetection is believed to be among the most promising. By combining graphene with plasmonic nanostructures, Duan and colleagues observe dramatic improvements in the efficiency and spectral sensitivity of graphene-based photodetectors.

    • Yuan Liu
    • , Rui Cheng
    •  & Xiangfeng Duan

  • Article
    | Open Access

    Topological insulators are a unique class of materials characterized by exotic metallic states at their surface, while remaining insulated in the bulk. Sacépéet al. show how to manipulate normal and superconducting electronic transport at the surface of the topological insulator Bi2Se3, by tuning a gate-voltage to vary the electronic density.

    • Benjamin Sacépé
    • , Jeroen B. Oostinga
    •  & Alberto F. Morpurgo

  • Article |

    X-ray ptychography has been used to extend the field of view in high-resolution quantitative imaging. Godardet al. develop Bragg-mode ptychography to reconstruct, in three dimensions, a crystalline specimen that is too large to be studied as a single object with a coherence-limited X-ray beam.

    • P. Godard
    • , G. Carbone
    •  & V. Chamard

  • Article
    | Open Access

    The propagation of magnetic domain walls in nanowires offers promise as the basis of future memory storage technologies. Muñoz and Prieto show that the random pinning of domain walls to structural defects in the nanowires can be suppressed at low fields, thus improving the reliability of the transmission of the domain walls substantially.

    • Manuel Muñoz
    •  & José L. Prieto

  • Article |

    The controllable modification of graphene by chemical functionalization can modulate its optical and electronic properties. Sunet al. devise a functionalisation-based method to pattern graphane/graphene superlattices within a single sheet of graphene.

    • Zhengzong Sun
    • , Cary L. Pint
    •  & James M. Tour

  • Article |

    Charge density waves in the structure and electron density of layered materials are closely linked to superconductivity. Using scanning tunnelling techniques, Rahnejatet al. demonstrate the occurrence of such waves in the doped graphene sheets of the superconductor CaC6.

    • K.C. Rahnejat
    • , C.A. Howard
    •  & M. Ellerby

  • Article
    | Open Access

    Tunnelling transitions triggered by microwave irradiation between coupled quantum dots have generally been assumed to be spin-conserving. This study shows that this condition is violated in the presence of spin–orbit coupling, thus opening new possibilities for manipulating a two–spin qubit system by microwave irradiation.

    • L.R. Schreiber
    • , F.R. Braakman
    •  & L.M.K. Vandersypen

  • Article
    | Open Access

    External electric fields have been used to control the motion of small objects through electrostatic repulsion. Here, electric fields are used to polarize conducting objects, triggering their movement by spatially separated electrochemical reactions leading to directionally controlled bubble evolution.

    • Gabriel Loget
    •  & Alexander Kuhn

  • Article |

    DNA nanotubes could be used to transport nano-cargo and incorporated into nano-devices. In this study, rolling circle amplification is used to generate DNA subunits, and their thermodynamic growth results in the formation of nanotubes with a controlled diameter.

    • Ofer I. Wilner
    • , Ron Orbach
    •  & Itamar Willner

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