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| Open AccessAdiabatic elimination-based coupling control in densely packed subwavelength waveguides
Optical communications and quantum operations require active coupling control in closely packed integrated photonic circuits. Here, Mrejen et al.exploit adiabatic elimination to demonstrate active coupling control between two closely packed waveguides by tuning the mode index of an in-between decoupled waveguide.
- Michael Mrejen
- , Haim Suchowski
- & Xiang Zhang
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Article
| Open AccessLead iodide perovskite light-emitting field-effect transistor
Hybrid organic–inorganic perovskites have shown great potential for use in optoelectronic applications. Here, the authors create solution-processed lead iodide perovskite light-emitting field-effect transistors and demonstrate both ambipolar behaviour and gate-assisted electroluminescence.
- Xin Yu Chin
- , Daniele Cortecchia
- & Cesare Soci
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Aging mechanisms in amorphous phase-change materials
Phase-change materials are a route to high-density data storage, but changes in their properties in time are a limiting factor. Here, the authors combine numerical simulations, photothermal deflection spectroscopy and impedance spectroscopy experiments to investigate the aging process in germanium telluride.
- Jean Yves Raty
- , Wei Zhang
- & Matthias Wuttig
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Article
| Open AccessIonic transport in hybrid lead iodide perovskite solar cells
Understanding the mechanism of ionic transport in organic–inorganic halide perovskites is crucial for the design of future solar cells. Here, Eames et al.undertake a combined experimental and computational study to elucidate the ion conducting species and help rationalize the unusual behaviour observed in these perovskite-based devices.
- Christopher Eames
- , Jarvist M. Frost
- & M. Saiful Islam
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Temporal tweezing of light through the trapping and manipulation of temporal cavity solitons
Optical tweezing typically refers to the trapping and manipulation of particles using lasers. Here, Jang et al. demonstrate analogous manipulation of ultrashort cavity soliton-pulses in the time domain, trapped by the phase modulation of a continuous wave laser beam, and moved by modifying the phase profile.
- Jae K. Jang
- , Miro Erkintalo
- & Stuart G. Murdoch
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| Open AccessHigh-quality sandwiched black phosphorus heterostructure and its quantum oscillations
Black phosphorus is an atomically thin material that exhibits excellent properties for electronics applications, but these degrade in atmospheric conditions. Here, the authors demonstrate the fabrication of stable, ultra-clean and high-mobility black phosphorus sandwiched between the layers of boron nitride.
- Xiaolong Chen
- , Yingying Wu
- & Ning Wang
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Article
| Open AccessHigh-performance flexible perovskite solar cells exploiting Zn2SnO4 prepared in solution below 100 °C
There has been impressive progress in the development of perovskite solar cells in recent years, but the best performing systems tend to be fabricated on glass surfaces. Here, the authors present a cell built on a polymer substrate, allowing flexibility whilst maintaining high efficiency.
- Seong Sik Shin
- , Woon Seok Yang
- & Sang Il Seok
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Article
| Open AccessOptoelectronic crystal of artificial atoms in strain-textured molybdenum disulphide
Periodically strained monolayer molybdenum disulphide funnels photogenerated electron-hole pairs across an electric field induced by a spatially graded band gap, mimicking a crystal of artificial atoms. Here, the authors experimentally demonstrate the artificial crystal in strain-textured molybdenum disulphide.
- Hong Li
- , Alex W. Contryman
- & Xiaolin Zheng
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Article
| Open AccessEnabling unassisted solar water splitting by iron oxide and silicon
Water splitting using earth-abundant materials promises a low cost solution to the problem of large scale energy storage. Here, the authors fabricate a haematite and silicon-based high-efficiency water splitting device, which operates without the need for an externally applied bias.
- Ji-Wook Jang
- , Chun Du
- & Dunwei Wang
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Article
| Open AccessThe optoelectronic role of chlorine in CH3NH3PbI3(Cl)-based perovskite solar cells
Chlorine incorporation into CH3NH3PbI3improves solar cell performance, but its optoelectronic role is still unclear. Here the authors present a strategy that decouples the morphological impact, to reveal that chlorine incorporation affects carrier transport across the heterojunction interface rather than within the perovskite crystal.
- Qi Chen
- , Huanping Zhou
- & Yang Yang
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Article
| Open AccessEfficient photosynthesis of carbon monoxide from CO2 using perovskite photovoltaics
Artificial photosynthesis is a means of harnessing solar energy to generate fuels but has traditionally been exploited for the generation of hydrogen. Here, Schreier et al. instead employ a perovskite photovoltaic device to effect the solar conversion of CO2to CO with high efficiency.
- Marcel Schreier
- , Laura Curvat
- & Michael Grätzel
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Article
| Open AccessHigh-performance ternary blend polymer solar cells involving both energy transfer and hole relay processes
Ternary blend solar cells offer the potential for high-power conversion efficiencies (PCEs); however their performances can be limited by design complexity. Here, the authors integrate multiple materials into a single junction device with 9.2% PCE and elucidate the mechanisms of enhancement at play.
- Luyao Lu
- , Wei Chen
- & Luping Yu
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High-density waveguide superlattices with low crosstalk
High-density integration will be vital for silicon photonics, but as we approach sub-wavelength distances between components, the crosstalk becomes intolerable. Here, Song et al. demonstrate waveguide integration at a half-wavelength pitch with low crosstalk using advanced superlattice design concepts.
- Weiwei Song
- , Robert Gatdula
- & Wei Jiang
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Article
| Open AccessPerovskite–fullerene hybrid materials suppress hysteresis in planar diodes
Metal halide perovskites are promising for solar energy harvesting, but currently prone to a large hysteresis and current instability. Here, Xu et al. show improvements in a hybrid material in which the fullerene is distributed at perovskite grain boundaries and thus passivates defects effectively.
- Jixian Xu
- , Andrei Buin
- & Edward H. Sargent
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Subwavelength-thick lenses with high numerical apertures and large efficiency based on high-contrast transmitarrays
Replacing conventional components with flat optic devices such as flat lenses is desirable for imaging and on-chip integration, but performance has hindered their use. Here, Arbabi et al. report a wavelength-thin, high-contrast transmitarray micro-lens with a 0.57 λfocal spot and 82% focusing efficiency.
- Amir Arbabi
- , Yu Horie
- & Andrei Faraon
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Article
| Open AccessWitnessing magnetic twist with high-resolution observation from the 1.6-m New Solar Telescope
Understanding the behaviour of magnetic flux ropes in the Sun is crucial for explaining solar phenomena such as flares and space weather. Exploiting the high resolution available in the 1.6 m New Solar Telescope, Wang et al.capture the evolution of a flaring twisted flux rope in the low solar corona.
- Haimin Wang
- , Wenda Cao
- & Haisheng Ji
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Article
| Open AccessImpact of charge transport on current–voltage characteristics and power-conversion efficiency of organic solar cells
Fitting current–voltage curves of organic solar cells with the Shockley equation often results in artificially high ideality factors. Here, the authors analyse inadequacy of the equation and propose an analytic model, which allows prediction of the efficiency potentials by explicit consideration of charge-carrier mobilities.
- Uli Würfel
- , Dieter Neher
- & Steve Albrecht
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Article
| Open AccessThree-terminal heterojunction bipolar transistor solar cell for high-efficiency photovoltaic conversion
Multiple junction solar cells offer the means to high-efficiency photovoltaics but suffer from complicated manufacturing and packing. Here Martí et al., propose a three-terminal heterojuntion bipolar transistor solar cell that simplifies the structure reducing the number of layers while maintaining the efficiency.
- A. Martí
- & A. Luque
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Article
| Open AccessActive control of all-fibre graphene devices with electrical gating
Active control of light in optical fibres is of great interest, to this end, electric control of all-fibre graphene devices is desirable but highly challenging. Here, Lee et al. demonstrate electric control of the optical properties of a graphene sheet deposited on a side-polished fibre mediated by an ion liquid.
- Eun Jung Lee
- , Sun Young Choi
- & Dong-Il Yeom
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Article
| Open AccessPatterning two-dimensional chalcogenide crystals of Bi2Se3 and In2Se3 and efficient photodetectors
Two-dimensional chalcogenides offer great potential in electronics, but accurate control of their growth is difficult. Here, the authors combine microintaglio printing and van der Waals epitaxy to pattern various large-area arrays of single-crystal chalcogenides with remarkable properties.
- Wenshan Zheng
- , Tian Xie
- & Hailin Peng
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Article
| Open AccessUltra-sensitive all-fibre photothermal spectroscopy with large dynamic range
Photothermal interferometry systems using free-space optics have limits in terms of light–matter interaction efficiency, size, optical alignment and integration. Here, Jin et al. use a gas-filled hollow-core photonic bandgap fibre to demonstrate an all-fibre gas sensor with ultrahigh sensitivity and dynamic range.
- Wei Jin
- , Yingchun Cao
- & Hoi Lut Ho
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Article
| Open AccessPositioning and joining of organic single-crystalline wires
Aligned, one-dimensional, single-crystal materials may allow on-demand photon/electron transfer. Here, the authors use a physical vapour transport technique to grow organic single-crystal wires with the guidance of pillar-structured substrates, and perform proof of concept waveguide experiments.
- Yuchen Wu
- , Jiangang Feng
- & Lei Jiang
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Article
| Open AccessUltrafast helicity control of surface currents in topological insulators with near-unity fidelity
Bulk contributions to transport measurements often inhibit the study of the surface states of topological insulators. Here, Kastl et al. demonstrate high-fidelity helicity-dependent photocurrents in the surface states of Bi2Se3, controlled via circularly polarized light with a picosecond time-resolution.
- Christoph Kastl
- , Christoph Karnetzky
- & Alexander W. Holleitner
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Article
| Open AccessUltimate thin vertical p–n junction composed of two-dimensional layered molybdenum disulfide
Molybdenum disulfide is a two-dimensional semiconducting material that has properties that make it useful for compact electronic devices. Here, the authors use molybdenum disulfide in an ultra-thin p–n junction that demonstrate ambipolar carrier transport and current rectification.
- Hua-Min Li
- , Daeyeong Lee
- & Won Jong Yoo
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Efficient hole-blocking layer-free planar halide perovskite thin-film solar cells
Lead halide perovskite solar cells use hole-blocking layers to allow a separate collection of positive and negative charge carriers and to achieve high-operation voltages. Here, the authors demonstrate efficient lead halide perovskite solar cells that avoid using this extra layer.
- Weijun Ke
- , Guojia Fang
- & Yanfa Yan
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Graphene-enabled electrically switchable radar-absorbing surfaces
Controlling the electrical properties of radar absorbing materials is required for active camouflage systems in the microwave. Here, Balci et al.use large-area graphene electrodes to demonstrate electrical control of microwave reflection, transmission and absorption by electrostatic tuning of the charge density.
- Osman Balci
- , Emre O. Polat
- & Coskun Kocabas
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Spin-dependent charge transfer state design rules in organic photovoltaics
An important source of loss in solar cells is the recombination of the photogenerated charge carriers before they are extracted from the device. Chang et al. now show that such recombination can be reduced in organic solar cells by increasing the separation between donors and acceptors.
- Wendi Chang
- , Daniel N. Congreve
- & Marc A. Baldo
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Surface transfer doping induced effective modulation on ambipolar characteristics of few-layer black phosphorus
Black phosphorus is a graphene-like material that can be harnessed for two-dimensional electronic devices. Here, Xiang et al. demonstrate that adding caesium carbonate or molybdenum trioxide can significantly enhance the electron or hole conduction, respectively, of this promising material.
- Du Xiang
- , Cheng Han
- & Wei Chen
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Article
| Open AccessEnhancing and inhibiting stimulated Brillouin scattering in photonic integrated circuits
On-chip nonlinear optics can be used to manipulate classical or quantum signals but enhancement of competing nonlinear processes can cause signal distortion. Here, Merklein et al. enhance and inhibit nonlinear scattering on a chip by tailoring the optical density-of-states at the edge of a photonic bandgap.
- Moritz Merklein
- , Irina V. Kabakova
- & Benjamin J. Eggleton
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10.5% efficient polymer and amorphous silicon hybrid tandem photovoltaic cell
Ultrathin film photovoltaic cells are a promising energy device, but suffer from low power conversion efficiency. Here, the authors construct a double-junction tandem cell using a hydrogenated amorphous silicon and a polymer as the front and back cell, respectively, which achieves 10.5% efficiency.
- Jeehwan Kim
- , Ziruo Hong
- & Yang Yang
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Crystalline silicon core fibres from aluminium core preforms
The integration of silicon optoelectronic devices in a fibre platform has great potential, but drawing such fibres is difficult. Using a simple, low cost and scalable method, Hou et al. fabricate a metre-long crystalline silicon-core, silica-clad fibre from a preform not containing elemental silicon.
- Chong Hou
- , Xiaoting Jia
- & Yoel Fink
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Considerably improved photovoltaic performance of carbon nanotube-based solar cells using metal oxide layers
The interface between electrodes and active layers of electronic devices such as solar cells is crucial for the device performance. Here, the authors show that metal oxides MoOxand ZnO play an important role in reducing the electronic barrier at the interface in photovoltaic devices based on carbon nanotubes.
- Feijiu Wang
- , Daichi Kozawa
- & Kazunari Matsuda
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Bandgap tunability at single-layer molybdenum disulphide grain boundaries
Molybdenum disulphide is a two-dimensional material that, unlike graphene, has a nonzero bandgap. Here, the authors demonstrate that the bandgap of single-layer molybdenum disulphide grown on graphite by chemical vapour deposition changes with distance from the grain boundary
- Yu Li Huang
- , Yifeng Chen
- & Andrew T. S. Wee
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Wide-angle planar microtracking for quasi-static microcell concentrating photovoltaics
Concentrating photovoltaics (PVs) offer a route to lower the cost of solar power, but their scale has been incompatible with roof top installation. Here, Price et al.demonstrate quasi-static concentrating PVs that achieve >200 × flux concentration over a full day in the form factor of a standard PV panel.
- Jared S. Price
- , Xing Sheng
- & Noel C. Giebink
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Seeded growth of highly crystalline molybdenum disulphide monolayers at controlled locations
Although synthesis of high-quality MoS2 has been demonstrated, growth of monolayer MoS2at controlled locations is highly desirable for applications. Here, the authors introduce a method where patterned seeds of molybdenum source material are used to grow isolated flakes at predetermined locations.
- Gang Hee Han
- , Nicholas J. Kybert
- & A. T. Charlie Johnson
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Detecting noise with shot noise using on-chip photon detector
The detection of high-frequency radiation emitted by a quantum conductor is promising but current approaches exhibit limited sensitivity. Here, Jompol et al. propose on-chip radiation detection based on photo-assisted shot noise and show the response to be independent of the nature and geometry of the quantum conductor.
- Y. Jompol
- , P. Roulleau
- & D. C. Glattli
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Experimental evidence of replica symmetry breaking in random lasers
Replica symmetry breaking, in which identical systems subject to identical conditions evolve to different end states, has been predicted to occur in many contexts but has yet to be observed experimentally. Ghofraniha et al.report evidence for its occurrence in the pulse-to-pulse variations of a random laser.
- N. Ghofraniha
- , I. Viola
- & C. Conti
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Article
| Open AccessReconfigurable radio-frequency arbitrary waveforms synthesized in a silicon photonic chip
Performing radio-frequency arbitrary waveform generation in the optical domain offers advantages over electronic-based methods but suffers from lack of integration and slow speed. Here, Wang et al. propose a fast-reconfigurable, radio-frequency arbitrary waveform generator fully integrated in a silicon chip.
- Jian Wang
- , Hao Shen
- & Minghao Qi
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Tunable ferroelectric polarization and its interplay with spin–orbit coupling in tin iodide perovskites
Halide perovskites are widely studied as components in photovoltaic cells. Here, the authors show that these materials also possess a tunable ferroelectric polarization as well as relativistic spin-splitting effects suggesting additional functionalities, for example, as spintronic and optoelectronic devices.
- Alessandro Stroppa
- , Domenico Di Sante
- & Silvia Picozzi
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Article
| Open AccessModulator-free quadrature amplitude modulation signal synthesis
Quadrature amplitude modulation signalling is currently enabling rapid data transfer capacity growth, but it still has associated drawbacks. Here, Liu et al.use optical injection locking to generate complex modulation format signals with reduced consumption, small footprint and easy integration.
- Zhixin Liu
- , Joseph Kakande
- & Radan Slavík
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Solution-processed multilayer small-molecule light-emitting devices with high-efficiency white-light emission
High-efficiency organic light-emitting devices usually require the growth of many layers of different materials by vapour deposition in vacuum. Naoya Aizawa et al. demonstrate the fabrication of high-efficiency multilayer organic LEDs from solution.
- Naoya Aizawa
- , Yong-Jin Pu
- & Junji Kido
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Coherent two-dimensional photocurrent spectroscopy in a PbS quantum dot photocell
Two-dimensional photocurrent spectroscopy can identify coherent electronic dynamics and offers promise for studies of numerous material systems. Karki et al. now show that the method can be used to study ultrafast carrier processes in lead sulphide quantum dots, such as multiple exciton generation.
- Khadga J. Karki
- , Julia R. Widom
- & Andrew H. Marcus
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Experimental realization of photonic topological insulator in a uniaxial metacrystal waveguide
Photonic topological insulators have been theoretically predicted but their experimental demonstration has proven challenging. Here, Chen et al.experimentally realize a photonic topological insulator by embedding a non-bianisotropic and a non-resonant metacrystal into a waveguide.
- Wen-Jie Chen
- , Shao-Ji Jiang
- & C. T. Chan
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High quality-factor optical nanocavities in bulk single-crystal diamond
Single-crystal diamond is a promising material for applications in classical and quantum optics, but the lack of scalable fabrication remains an issue. Here, Burek et al. adapt angle-etching nanofabrication techniques to realize ring resonators and photonic crystal cavities in single crystal diamond with quality factors in excess of 105.
- Michael J. Burek
- , Yiwen Chu
- & Marko Lončar
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Long-term stable polymer solar cells with significantly reduced burn-in loss
Efficiency and stability are two major concerns in polymer-based solar cell development. Here Kong et al.report that the lifetime of a bulk heterojunction polymer can be improved by removing its low-molecular-weight components, which leads to a substantially reduced burn-in loss under photo-aging conditions.
- Jaemin Kong
- , Suhee Song
- & Kwanghee Lee
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Article |
Bio-inspired networks for optoelectronic applications
Biological systems, subject to evolutionary optimization over millions of years, have been a source of ingenious solutions in many areas of science. Here, Han et al. develop transparent electrodes inspired by two such systems: a leaf venation and a spider’s web.
- Bing Han
- , Yuanlin Huang
- & Jinwei Gao
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Photon energy upconversion through thermal radiation with the power efficiency reaching 16%
Energy transfer upconversion can increase the absorption efficiency but has been limited by multiphonon relaxation. Here, Wang et al. demonstrate that photon energy upconversion by thermal radiation benefits from multiphonon relaxation and achieves efficiencies as high as 16%.
- Junxin Wang
- , Tian Ming
- & Chun-Hua Yan
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Article
| Open AccessPhoton-assisted tunnelling with nonclassical light
Coherently coupling microwave photons to quantum electronic conductors could provide a useful platform for quantum information processing. Souquet et al. now theoretically demonstrate that such systems can also act as sensitive probes of the quantum properties of non-classical microwave radiation.
- J. -R. Souquet
- , M. J. Woolley
- & A. A. Clerk
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Article
| Open AccessUltralow mode-volume photonic crystal nanobeam cavities for high-efficiency coupling to individual carbon nanotube emitters
Efficient coupling to photonic structures is essential to exploit the emission properties of carbon nanotubes (CNTs). Here, Miura et al.demonstrate spontaneous emission coupling efficiency exceeding 85% from a single CNT to a silicon photonic crystal nanobeam cavity with an ultralow mode-volume.
- R. Miura
- , S. Imamura
- & Y. K. Kato
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