Perspective
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Open Access
Featured
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Review Article
| Open AccessSkin-interfacing wearable biosensors for smart health monitoring of infants and neonates
Wearable sensors have been widely studied, but research has tended to focus on their use in adults. This Review explores skin-interfacing smart health systems that are designed with infants and neonates in mind.
- Lauren Zhou
- , Matthew Guess
- & Woon-Hong Yeo
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Article
| Open AccessMicrowave quantum memcapacitor effect
Nonlinear memory devices such as memristors, memcapacitors, and meminductors, are the building blocks of energy-efficient neuromorphic computing. Here, the authors propose a superconducting circuit design acting as a microwave quantum memcapacitor, which could be implemented in neuromorphic quantum computing architectures.
- Xinyu Qiu
- , Shubham Kumar
- & Francisco Albarrán-Arriagada
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Article
| Open Access3D printed titanium carbide MXene-coated polycaprolactone scaffolds for guided neuronal growth and photothermal stimulation
Neural circuitry is important for comprehending computational mechanisms and physiology of the brain but controlling neuronal connectivity and response in 3D is challenging. Here, titanium carbide MXene-coated 3D polycaprolactone scaffolds are demonstrated to effectively control neuronal interconnection.
- Jianfeng Li
- , Payam Hashemi
- & Joyce K. S. Poon
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Article
| Open AccessMartensite decomposition during rapid heating of Ti-6Al-4V studied via in situ synchrotron X-ray diffraction
Martensite in Ti-6Al-4V is known to decompose under heating. This study employs rapid laser heating in situ in a synchrotron to study changes in the diffraction profiles during the martensite decomposition process.
- Seunghee A. Oh
- , Joseph W. Aroh
- & Anthony D. Rollett
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Review Article
| Open AccessMaterial and structural considerations for high-performance electrodes for wearable skin devices
A key aspect of wearable devices used in personal health monitoring are the electrodes that make contact with the skin. This Review discusses how the materials and structure of electrodes used in these devices are vital to their performance, including how altering these factors might optimize their function.
- Kyeonghee Lim
- , Hunkyu Seo
- & Jang-Ung Park
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Review Article
| Open AccessRecent developments in wearable breath sensors for healthcare monitoring
Human breath contains a vast amount of information that might be used to indicate respiratory and cardiovascular health. This Review summarizes and discusses recent advances in wearable breath sensors for monitoring breath temperature, humidity and airflow, as well as biomarker presence.
- Dohyung Kim
- , Jinwoo Lee
- & Seung Hwan Ko
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Review Article
| Open AccessAdvances in 3D silicon-based lithium-ion microbatteries
Three-dimensional silicon-based lithium-ion microbatteries have potential use in miniaturized electronics that require independent energy storage. Here, their developments are discussed in terms of their material compatibility, cell designs, fabrication methods, and performance in various applications.
- Andam Deatama Refino
- , Calvin Eldona
- & Hutomo Suryo Wasisto
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Article
| Open AccessCathodic protection mechanism of iron and steel in porous media
Cathodic protection is widely used in protecting structures from corrosion, but its working mechanism remains unclear. Here, in-situ and ex-situ characterization techniques, coupled with electrochemical measurements, are used to study the spatio-temporal changes at the steel-electrolyte interface.
- Federico Martinelli-Orlando
- , Shishir Mundra
- & Ueli M. Angst
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Article
| Open AccessAdditive manufacturing of defect-free TiZrNbTa refractory high-entropy alloy with enhanced elastic isotropy via in-situ alloying of elemental powders
Refractory high-entropy alloys are attractive for high-temperature applications, but are challenging to process. Here, a method is shown for identifying a processing window that allows the additive manufacturing of a TiZrNbTa refractory alloy with a low defect content and mechanical properties comparable to as-cast samples.
- Shahryar Mooraj
- , George Kim
- & Wen Chen
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Article
| Open AccessCurvature tuning through defect-based 4D printing
4D printing techniques enable the realization of smart materials whose shape or properties can change with time. Here, utilizing the anisotropic deformation of a combination of polymers and the distribution of microdefects formed during the 3D printing process, the authors realize a variety of shape-changing curved structures that can be used in drug delivery systems.
- Vahid Moosabeiki
- , Ebrahim Yarali
- & Amir A. Zadpoor
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Perspective
| Open AccessTowards a digitally connected body for holistic and continuous health insight
Wearable electronics provide opportunities for personalized health monitoring and treatment. This Perspective addresses challenges in the field, including material selection for devices, device integration strategies, and public adoption factors.
- Philipp Gutruf
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Article
| Open AccessDeformation twins as a probe for tribologically induced stress states
A complex relationship exists between microstructure development and stress field during tribological loading of a metal. Here, twinning in a high-entropy alloy is used as a model system to understand stress fields during tribological experiments, supported by molecular dynamics simulations.
- Antje Dollmann
- , Christian Kübel
- & Christian Greiner
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Article
| Open AccessA magnetically actuated dynamic labyrinthine transmissive ultrasonic metamaterial
Space-coiling acoustic metamaterials, where sound travels through labyrinthine geometries, are interesting for their high energy transmission and broad modulation characteristics. Here, the authors demonstrate an active approach to acoustic metamaterial reconfiguration based on dynamic space-coiling unit cells and soft robotic-inspired actuators.
- Christabel Choi
- , Shubhi Bansal
- & Sriram Subramanian
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Article
| Open AccessAnticounterfeiting tags based on randomly oriented MoSx clusters enabled by capillary and Marangoni flow
There is an ongoing need for new anticounterfeiting technologies. Here, the combined effects of capillary and Marangoni flow create randomly oriented MoSx clusters on a surface, which are used as anticounterfeiting tags.
- Changgyun Moon
- , Pavan Pujar
- & Sunkook Kim
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Article
| Open AccessLocal resonance bandgap control in a particle-aligned magnetorheological metamaterial
Stimuli-responsive elastic metamaterials enable a high degree of tunability of resonance-based features. Here, a magnetically programmable metamaterial based on magnetorheological elastomers is designed and fabricated, demonstrating robust local resonance bandgap control.
- Mohammadreza Moghaddaszadeh
- , Andrew Ragonese
- & Mostafa Nouh
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Article
| Open AccessStress–strain relationships and yielding of metal-organic framework monoliths
Mechanical characterizations of metal-organic framework monoliths are often overlooked. Here, the stress-strain behaviour of ZIF-8 and MIL-68 monoliths was investigated with flat punch nanoindentation, micropillar compression and Raman microspectroscopy.
- Michele Tricarico
- , Cyril Besnard
- & Jin-Chong Tan
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Article
| Open AccessDendritic deformation modes in additive manufacturing revealed by operando x-ray diffraction
In-situ x-ray studies have proven to be vital in understanding solidification behavior during additive manufacturing of alloys. Here, operando synchrotron diffraction of a superalloy reveals the effects of solidification dynamics on dendrite deformation mechanisms during laser melting.
- Adrita Dass
- , Chenxi Tian
- & Atieh Moridi
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Article
| Open AccessA multibody kinematic system approach for the design of shape-morphing mechanism-based metamaterials
The ability of a structure to reliably change its shape is key to the function of various organisms in nature, as well as for applications such as implants and robotics. Here, a methodology is shown to predict shape-morphing in kinematic structures, based on geometrical multibody design of connecting elements and joints.
- Pier H. de Jong
- , A. L. Schwab
- & Amir A. Zadpoor
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Article
| Open AccessIntegrating stability metrics with high-throughput computational screening of metal–organic frameworks for CO2 capture
High-throughput computational screening accelerates the search for promising metal-organic frameworks but often neglects stability. Here, four stability metrics are integrated with high-throughput computational screening to identify top-performing metal-organic frameworks for carbon dioxide capture.
- Saad Aldin Mohamed
- , Daohui Zhao
- & Jianwen Jiang
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Review Article
| Open AccessMultiscale mechanics and molecular dynamics simulations of the durability of fiber-reinforced polymer composites
Fiber-reinforced polymer composites have found widespread use in critical engineering applications. Here, the use of simulations to understand the mechanical durability of polymer composites across a range of length scales is reviewed, with a focus on molecular dynamics simulations.
- Kui Lin
- & Zhanlong Wang
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Review Article
| Open AccessEngineering receptor-mediated transmembrane signaling in artificial and living cells
Transmembrane signaling systems are present in living cells which receive cues from the environment and produce a cellular response. Here, recent advances in the design of bioinspired systems that mimic transmembrane signaling in synthetic and living cells are reviewed.
- Ke Shi
- , Chuwen Song
- & Yiyang Lin
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Article
| Open AccessRandomly stacked open cylindrical shells as functional mechanical energy absorber
Mechanical metamaterials are artificially designed structures with tunable behavior, typically obeying precisely programmed dynamics. Here, a metamaterial based on randomly stacked flexible cylindrical shells provides a disordered yet statistically robust and controllable structure for mechanical energy dissipation and storage.
- Tomohiko G. Sano
- , Emile Hohnadel
- & Florence Bertails-Descoubes
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Article
| Open AccessImaging Fermi-level hysteresis in nanoscale bubbles of few-layer MoS2
Nanobubbles are sources of charge trapping that influence the performance and stability of devices based on 2D materials. Here, Kelvin probe force microscopy is used to study the origin and mechanism of charge trapping in nanobubbles of MoS2 on a SiO2 substrate.
- Dohyeon Jeon
- , Haesol Kim
- & Taekyeong Kim
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Article
| Open AccessA catch bond mechanism with looped adhesive tethers for self-strengthening materials
Catch bonds exist in some protein-ligand complexes and are of interest for their increased lifetime under greater mechanical force. Here, a mathematical model for nanoparticles tethered with macromolecules shows catch-bond behavior, which may be useful for designing synthetic materials.
- Kerim C. Dansuk
- , Subhadeep Pal
- & Sinan Keten
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Article
| Open AccessNeon encapsulation by a hydroquinone organic crystalline clathrate under ambient conditions
It is difficult to store noble gases in solids due to their chemical inertness and relative lightness. Here, a hydroquinone organic clathrate can stably capture neon at atmospheric pressure and room temperature and be released at elevated temperatures.
- Sol Geo Lim
- , Jong-Won Lee
- & Ji-Ho Yoon
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Article
| Open AccessDesign of acoustic absorbing metasurfaces using a data-driven approach
Designing artificial acoustic metasurfaces via traditional numerical simulations is computationally challenging. Here, the authors introduce a data-driven neural network approach for the inverse design of membrane-type sound absorbers, testing the desired properties on two devices fabricated using model-estimated parameters.
- Hamza Baali
- , Mahmoud Addouche
- & Abdelkrim Khelif
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Article
| Open AccessMillimeter-wave to near-terahertz sensors based on reversible insulator-to-metal transition in VO2
Vanadium dioxide is a strongly correlated material interesting for its ultra-fast resistive switching controlled by an electric-field-driven insulator-metal transition. Here, VO2 stochastic oscillator power sensors for mm-wave to sub-THz radiation are demonstrated, displaying high responsivities, low noise, and a small scalable footprint.
- Fatemeh Qaderi
- , Teodor Rosca
- & Adrian M. Ionescu
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Article
| Open AccessStrong conformable structure via tension activated kirigami
Kirigami, the art of deploying flat sheets to create three-dimensional structures, relies often on complex folding processes that hinder industrial applications. Here, the authors develop a folding-wall kirigami pattern that deploys easily under tension, demonstrating its strength, stiffness, energy absorption, and interlocking properties.
- Tom Corrigan
- , Patrick Fleming
- & Delony Langer-Anderson
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Article
| Open AccessFabrication of helix–fiber composites with mechanically coupled core-wrapping for programmable properties
Helix-fiber composites are used in intelligent stretchable materials but current understanding is still lacking. Here, we show that mechanical coupling plays a critical role in controlling structural properties and demonstrate use as an elastic conductor, sensor, and structure transplantation.
- Dan Li
- , Zhiwei Zhu
- & Yu Wang
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Article
| Open AccessEffect of grip-enhancing agents on sliding friction between a fingertip and a baseball
Foreign substances on the surface of a baseball can alter its delivery and enhance pitching performance. Here, sticky substances are found to increase finger-ball friction which can positively affect spin rate, whereas rosin powder can ensure consistent friction across pitchers, with results differing between baseballs used in the United States and Japan.
- Takeshi Yamaguchi
- , Daiki Nasu
- & Kei Masani
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Article
| Open AccessSelective hinge removal strategy for architecting hierarchical auxetic metamaterials
Pivotally interconnected polygons are capable of auxetic behavior, but have not been fully explored. Here, a design method is demonstrated based on the selective removal of rotational hinges in pivotally interconnected polygons with even-numbered modules, leading to fully-deployable structures.
- Ehsan Jalali
- , Hadi Soltanizadeh
- & Pooya Sareh
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Article
| Open AccessGradient droplet distribution promotes spontaneous formation of frost-free zone
Preventing the condensation of water is key for anti-icing applications. Here, a macro-ridged surface is found to prevent frost formation either side of each ridge, attributed to a change in water vapor distribution preventing ice bridge formation.
- Chenguang Lu
- , Cong Liu
- & Yahua Liu
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Article
| Open AccessUnraveling the effect of collagen damage on bone fracture using in situ synchrotron microtomography with deep learning
Collagen is known to play a key role in the fracture resistance of bone. Here, in situ synchrotron tomography during the mechanical testing of bone is combined with deep learning to mitigate radiation damage, revealing that a compromised collagen network lowers the efficacy of crack deflection.
- Michael Sieverts
- , Yoshihiro Obata
- & Claire Acevedo
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Article
| Open AccessNon-Hermitian elastodynamics in gyro-odd continuum media
Active metamaterials can host non-Hermitian interactions that defy the conservation laws of linear elasticity, leading to unusual phenomena such as one-way energy transmission and odd-elastic moduli. Here, robust unidirectional Rayleigh surface waves are found in active media comprising both gyroscopic and odd-elastic effects.
- Penglin Gao
- , Yegao Qu
- & Johan Christensen
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Article
| Open AccessTopological state transfer in Kresling origami
Topological mechanical metamaterials have been considered effective for energy manipulation via edge states, but manipulating these states remains challenging. Here, a Kresling origami mechanical metamaterial hosts multiple topological edge states at finite frequencies, which can be manipulated and transferred across the boundaries of the system by adjusting the lattice torsion.
- Yasuhiro Miyazawa
- , Chun-Wei Chen
- & Jinkyu Yang
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Perspective
| Open AccessProbing process kinetics in batteries with electrochemical impedance spectroscopy
Electrochemical impedance spectroscopy is a powerful and increasingly accessible approach for studying kinetic processes in batteries. Here, key factors for using impedance to obtain accurate and reproducible data from batteries are discussed, providing guidance for researchers.
- Deyang Qu
- , Weixiao Ji
- & Huainan Qu
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Article
| Open AccessLearning the dynamics of metamaterials from diffracted waves with convolutional neural networks
Scattered elastic waves provide non-invasive diagnostics and dynamic characterization of metamaterials, but extracting information from small-size samples is challenging. Here, convolutional neural networks are used to interpret diffracted waves, revealing how sample-edge scattering provides the most significant information on macroscopic metamaterial properties.
- Yuxin Zhai
- , Hyung-Suk Kwon
- & Bogdan-Ioan Popa
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Article
| Open AccessDeep learning for the rare-event rational design of 3D printed multi-material mechanical metamaterials
Multi-material 3D printing techniques are now enabling the rational design of metamaterials with both complex geometries and multiple materials compositions. Here, deep-learning methods are used to identify, among planar network structures, the rare designs that yield very unusual and desirable combinations of materials properties.
- Helda Pahlavani
- , Muhamad Amani
- & Amir A. Zadpoor
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Article
| Open AccessTheoretical stiffness limits of 4D printed self-folding metamaterials
The 3D stiffness of a self-folded metamaterial structure is limited by the low stiffness required by the folding process. Here, the stiffness limits of self-folding bilayers are theoretically established by a nonlinear model and experimentally validated on polymer-metal composites, providing the optimal combinations of geometrical and mechanical properties of folded constructs.
- Teunis van Manen
- , Vahid Moosabeiki Dehabadi
- & Amir A. Zadpoor
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Article
| Open AccessFlexible thermoelectric generator with high Seebeck coefficients made from polymer composites and heat-sink fabrics
Light and flexible thermoelectric generators operating at room temperature are highly desirable for wearable microelectronics. Here, flexible thermoelectric composites comprising semiconducting Bi2Te3 particles and conductive polymers exhibit a high output power within a small temperature window around room temperature.
- Shuping Lin
- , Lisha Zhang
- & Xiaoming Tao
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Article
| Open AccessMulti-functional multi-gate one-transistor process-in-memory electronics with foundry processing and footprint reduction
Developing scalable strategies of miniaturization and integration is key for achieving high-density integrated circuit devices. Here, the authors propose a silicon-based one-transistor device with a 40% reduction in circuit footprint, which combines the functionalities of logic gates, memory, and artificial synapses for mass production.
- Mingzhi Dai
- , Zhitang Song
- & Junhao Chu
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Article
| Open AccessAerosol capture and coronavirus spike protein deactivation by enzyme functionalized antiviral membranes
The COVID-19 pandemic highlights the importance of materials that block airborne virus transmission. Here, a nanostructured membrane is shown to filter coronavirus-sized particles, while the membrane surface incorporates enzymes that denature the SARS-CoV-2 spike protein within 30 s.
- Rollie Mills
- , Ronald J. Vogler
- & Dibakar Bhattacharyya
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Article
| Open AccessIn vivo engraftment into the cornea endothelium using extracellular matrix shrink-wrapped cells
Tissue regeneration by injecting cells into the damaged area is a common clinical treatment, but is not always affective. Here, a shrink-wrap-like process is reported for corneal endothelial cells, allowing them to be engrafted into the corneal endothelium of a rabbit animal model.
- Rachelle N. Palchesko
- , Yiqin Du
- & Adam W. Feinberg
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Article
| Open AccessMultilayers for directed energy accelerated lightsails
Lightsails accelerated by ground-based laser arrays are a candidate technology to send probes into deep space in a timeframe compatible with human life. Here, an optimization study identifies the most promising multilayer structures that maximize propulsion efficiency, thermal stability, and mechanical stiffness.
- Giovanni Santi
- , Giulio Favaro
- & Maria G. Pelizzo
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Article
| Open AccessAlgorithmic design of origami mechanisms and tessellations
Origami is a promising source of inspiration in designing foldable structures and reconfigurable metamaterials. Here, building on exact folding kinematic conditions, an algorithmic design of rigidly-foldable origami structures is presented, allowing the engineering of metamaterials with arbitrary complex crease patterns.
- Andreas Walker
- & Tino Stankovic
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Perspective
| Open AccessOrganic semiconductors for light-mediated neuromodulation
There is growing interest in organic semiconductor devices for light-mediated neuromodulation, such as for retinal stimulation. Here, the key working principles of these devices are discussed, as well as promising applications and outstanding challenges for the field.
- Danashi Imani Medagoda
- & Diego Ghezzi
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Article
| Open AccessHeterogeneous origami-architected materials with variable stiffness
Origami-inspired metamaterials are attractive for their programmable shape-shifting properties but are typically characterized by low structural rigidity. Here, 3D heterogeneous origami structures display highly reconfigurable mechanical properties, including finely controllable and reversible stiffness variation.
- Yasuhiro Miyazawa
- , Hiromi Yasuda
- & Jinkyu Yang
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Review Article
| Open AccessDesign principles and biological applications of red-emissive two-photon carbon dots
Carbon dots are suitable for a range of biological applications due to their unique physicochemical properties and biological behavior. This Review summarizes research related to the emerging field of red-emissive two-photon carbon dots for bioimaging, biosensing, and phototherapeutic applications.
- Pooria Lesani
- , Aina Hazeera Mohamad Hadi
- & Hala Zreiqat
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Article
| Open AccessCavity vat photopolymerisation for additive manufacturing of polymer-composite 3D objects
There is an ongoing drive for new additive manufacturing processes that produce complex parts. Here, cavity vat polymerisation is introduced, in which cavities are filled with a dual-curing resin that forms an elastomer/thermoset covalently bonded interface, creating hard-shell/soft-core parts.
- Joel Bachmann
- , Philip Obst
- & Olaf Hinrichsen