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Article |
Direct observation of Landau levels in silicon photonic crystals
Photonic Landau levels are demonstrated via a strain-induced pseudomagnetic field in a silicon photonic crystal slab.
- Maria Barsukova
- , Fabien Grisé
- & Mikael C. Rechtsman
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Article |
Epsilon-near-zero regime enables permanent ultrafast all-optical reversal of ferroelectric polarization
Researchers reveal that naturally emerging epsilon-near-zero conditions in BaTiO3 can be exploited to drive permanent all-optical switching of ferroelectric polarization. The general nature of the epsilon-near-zero regime means that the approach could be used to switch spontaneous order parameters in other systems.
- M. Kwaaitaal
- , D. G. Lourens
- & A. Kirilyuk
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Article
| Open AccessA high-efficiency programmable modulator for extreme ultraviolet light with nanometre feature size based on an electronic phase transition
A reflective spatial light modulator for extreme ultraviolet (EUV) or soft X-ray light is demonstrated in an electronic Wigner crystal material with a sub-90-nm feature size. The diffraction grating imprinted by sub-picosecond EUV beams is rewritable. The projected efficiency according to the modelling exceeds 1%.
- Igor Vaskivskyi
- , Anze Mraz
- & Dragan Mihailovic
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Article |
Optical readout of the chemical potential of two-dimensional electrons
An optical readout technique for the chemical potential of an arbitrary two-dimensional material is realized using a monolayer transition metal dichalcogenide semiconductor sensor whose optical response sharply depends on the chemical potential.
- Zhengchao Xia
- , Yihang Zeng
- & Kin Fai Mak
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Article
| Open AccessSub-cycle multidimensional spectroscopy of strongly correlated materials
Nonlinear multidimensional spectroscopy that can image the sub-cycle dynamics of strongly correlated systems on the sub-femtosecond timescale is demonstrated by using the carrier–envelope-phase dependence of the correlated multielectron response to decode the complex interplay between different many-body states.
- V. N. Valmispild
- , E. Gorelov
- & O. Smirnova
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News & Views |
Spin-selective transitions between quantum Hall states
Platforms enabling control over strong light–matter interactions in optical cavities provide a challenging but promising way to manipulate emergent light–matter hybrids. Spin selectivity of transitions has now been demonstrated in a two-dimensional hole gas microcavity system, paving the way towards the study of new spin physics phenomena in hybrid excitations.
- Hrvoje Buljan
- & Zhigang Chen
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Article |
Electric quadrupole second-harmonic generation revealing dual magnetic orders in a magnetic Weyl semimetal
Optical second-harmonic waves are generated from the electric quadrupole contribution in a centrosymmetric magnetic Weyl semimetal Co3Sn2S2. Two magnetic orders and phase transitions are explored in temperature-dependent rotational anisotropy measurements by second-harmonic generation.
- Youngjun Ahn
- , Xiaoyu Guo
- & Liuyan Zhao
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Article |
Field-driven attosecond charge dynamics in germanium
Attosecond transient reflectivity spectroscopy, in combination with extensive time-dependent density functional theory calculations, is used to study field-driven carrier injection in germanium in the time window of few femtoseconds around pulse overlap, paving a route towards achieving full optical control over charge carriers in semiconductors.
- Giacomo Inzani
- , Lyudmyla Adamska
- & Matteo Lucchini
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Article |
Spin-selective strong light–matter coupling in a 2D hole gas-microcavity system
Strong coupling of a 2D hole gas in the quantum Hall state dressed with a microcavity mode is studied, showing that tuning the strength of the magnetic field, and therefore the density of states in the system, can select specific spin-dependent light–matter coupling.
- D. G. Suárez-Forero
- , D. W. Session
- & M. Hafezi
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Article |
Onset of vortex clustering and inverse energy cascade in dissipative quantum fluids
The turbulent dynamics of a 2D quantum fluid of exciton–polaritons is measured in a planar AlGaAs microcavity after a pulsed optical excitation. Clear evidence of both the onset of vortex clustering and inverse energy cascade is provided.
- R. Panico
- , P. Comaron
- & D. Ballarini
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Article |
Terahertz cyclotron emission from two-dimensional Dirac fermions
Two-dimensional massive and massless Dirac fermions in HgTe/CdHgTe quantum wells yield terahertz Landau emission. The emission frequency is continuously tunable with magnetic field or carrier concentration, over the range from 0.5 to 3 THz.
- S. Gebert
- , C. Consejo
- & F. Teppe
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Article |
Excitonic resonances control the temporal dynamics of nonlinear optical wave mixing in monolayer semiconductors
Researchers show that resonant coupling of light pulses with excitonic transitions affects the optimal time difference between pulses for sum-frequency generation and four-wave mixing in monolayer WSe2.
- Jonas M. Bauer
- , Lijue Chen
- & Kai-Qiang Lin
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Letter |
Probing topological phase transitions using high-harmonic generation
Researchers demonstrate a method based on circularly polarized laser-field-driven high-harmonic generation for probing non-trivial and trivial topological phases in a three-dimensional topological insulator.
- Christian Heide
- , Yuki Kobayashi
- & Shambhu Ghimire
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Letter |
Few-photon all-optical phase rotation in a quantum-well micropillar cavity
Giant effective photon–photon interactions are achieved by hybridizing light with excitons in an InGaAs-based quantum well micropillar cavity. Cross-phase modulation of up to 3 mrad per polariton is observed at the laser intensity below the single-photon level.
- Tintu Kuriakose
- , Paul M. Walker
- & Dmitry N. Krizhanovskii
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Article |
Spontaneous-polarization-induced photovoltaic effect in rhombohedrally stacked MoS2
It is shown that rhombohedral stacked MoS2 can enable scalable photovoltaic effects induced by spontaneous polarization throughout few-micrometre-sized exfoliated flakes. This is exploited in a graphene–MoS2-based photovoltaic device.
- Dongyang Yang
- , Jingda Wu
- & Ziliang Ye
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Article |
Room-temperature superfluorescence in hybrid perovskites and its origins
Superfluorescence—the collective emission of fluorescent light—is observed at temperatures up to 330 K in lead halide perovskite thin films. This finding suggests an intrinsic mechanism for protecting the electronic coherence in these materials.
- Melike Biliroglu
- , Gamze Findik
- & Kenan Gundogdu
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Article |
Cavity-enhanced linear dichroism in a van der Waals antiferromagnet
Researchers use spin-charge coupling and FePS3 crystals to induce large in-plane optical anisotropy and near-unity linear dichroism in the visible–near-infrared range.
- Huiqin Zhang
- , Zhuoliang Ni
- & Deep Jariwala
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Article |
Spatiotemporally controlled room-temperature exciton transport under dynamic strain
Researchers exploit Rayleigh waves and associated dynamic strains to control exciton transport in the weak coupling regime at room temperature. The findings may pave the way for new types of excitonic device for applications ranging from communications to energy.
- Kanak Datta
- , Zhengyang Lyu
- & Parag B. Deotare
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Article
| Open AccessReal-space subfemtosecond imaging of quantum electronic coherences in molecules
By combining scanning tunnelling microscopy and attosecond technologies, the coherent electronic motion generated in molecules by carrier-envelope-phase-stable laser pulses is visualized at ångström-scale spatial resolution and subfemtosecond temporal resolution.
- M. Garg
- , A. Martin-Jimenez
- & K. Kern
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Article |
Slow carrier relaxation in tin-based perovskite nanocrystals
Tin-based perovskite nanocrystals with slower than usual relaxation dynamics holds promise for superior lead-free perovskite optoelectronic devices.
- Linjie Dai
- , Zeyu Deng
- & Neil C. Greenham
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Article |
Quantum transport in fractal networks
Quantum transport in fractal networks is experimentally investigated by performing continuous-time quantum walks in fractal photonic lattices. Contrarily to classical fractals, anomalous transport governed solely by the fractal dimension is observed.
- Xiao-Yun Xu
- , Xiao-Wei Wang
- & Xian-Min Jin
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Letter |
High-temperature superfluorescence in methyl ammonium lead iodide
A collective coherent quantum many-body phase, namely superfluorescence, is observed in CH3NH3PbI3 at 78 K. The excitation fluence dependence of the spectroscopic features and the population kinetics confirm all its well-known characteristics.
- Gamze Findik
- , Melike Biliroglu
- & Kenan Gundogdu
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Article |
Subcycle contact-free nanoscopy of ultrafast interlayer transport in atomically thin heterostructures
Subcycle nano-videography of charge-transfer dynamics in WSe2/WS2 heterostructures is obtained by using a terahertz near-field microscopy. The central idea is to probe the local polarizability of electron–hole pairs with evanescent terahertz fields.
- M. Plankl
- , P. E. Faria Junior
- & R. Huber
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Article |
Room-temperature electron spin polarization exceeding 90% in an opto-spintronic semiconductor nanostructure via remote spin filtering
An electron spin polarization of 90% is achieved in a non-magnetic nanostructure at room temperature without magnetic field. This is accomplished by remote spin filtering of InAs quantum-dot electrons via an adjacent tunnelling-coupled GaNAs spin filter.
- Yuqing Huang
- , Ville Polojärvi
- & Weimin M. Chen
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Article |
High-power portable terahertz laser systems
GaAs-based terahertz quantum cascade lasers emitting around 4 THz are demonstrated up to 250 K without a magnetic field. To elevate the operation temperature, carrier leakage channels are reduced by carefully designing the quantum well structures.
- Ali Khalatpour
- , Andrew K. Paulsen
- & Qing Hu
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Article |
Dynamics of the Berezinskii–Kosterlitz–Thouless transition in a photon fluid
A topological transition in a nonlinear photonic lattice results in new vortex dynamics and a change from photonic fluid behaviour to that of a plasma-like gas.
- Guohai Situ
- & Jason W. Fleischer
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Comment |
In memory of Philip W. Anderson
Philip Warren Anderson is one of the founding fathers of modern condensed-matter physics. With his death on 29 March 2020, we have lost one of the most influential physicists of the twentieth century.
- Diederik S. Wiersma
- , Bart A. van Tiggelen
- & Ad Lagendijk
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Article |
Dynamics and efficient conversion of excitons to trions in non-uniformly strained monolayer WS2
The photoluminescence spectrum of WS2 is modified under strain applied by an atomic force microscope probe. The free carrier redistribution yields conversion of excitons to trions with conversion efficiency approaching 100%.
- Moshe G. Harats
- , Jan N. Kirchhof
- & Kirill I. Bolotin
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Letter |
High-efficiency organic solar cells with low non-radiative recombination loss and low energetic disorder
An organic solar cell designed with minimal energetic disorder exhibits very low energy loss due to non-radiative recombination and highly efficient operation.
- Sha Liu
- , Jun Yuan
- & Yong Cao
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Article |
Attosecond spectral singularities in solid-state high-harmonic generation
High-harmonic waves are generated from a MgO crystal under experimental conditions where the simple semi-classical analysis fails. High-harmonic generation spectroscopy directly probes the strong-field attosecond dynamics over multiple bands.
- Ayelet Julie Uzan
- , Gal Orenstein
- & Nirit Dudovich
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Letter |
Photonic quadrupole topological phases
A higher-order topological phase is demonstrated, manifesting as robust, topologically protected corner modes in a silicon photonics system.
- Sunil Mittal
- , Venkata Vikram Orre
- & Mohammad Hafezi
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Article |
Josephson vortices induced by phase twisting a polariton superfluid
All-optical control of the topological excitations of a superfluid of light is demonstrated in a high-quality-factor semiconductor microcavity. Recovery of superfluid behaviour at high polariton densities and bosonic Josephson vortices are observed.
- Davide Caputo
- , Nataliya Bobrovska
- & Daniele Sanvitto
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News & Views |
Quasi-two-dimensional electron–hole droplets
The observation of a room-temperature stable liquid phase of electrons and holes in a quasi-two-dimensional photocell paves the way towards optoelectronic devices that harness collective phenomena.
- Stéphane Berciaud
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Letter |
Electron–hole liquid in a van der Waals heterostructure photocell at room temperature
Photoexcited charge carriers are typically approximated as a gas, but now it is shown that electrons and holes can behave as a liquid in MoTe2 photocells.
- Trevor B. Arp
- , Dennis Pleskot
- & Nathaniel M. Gabor
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Letter |
Laguerre–Gauss and Hermite–Gauss soft X-ray states generated using diffractive optics
Robust methods for creating and analysing soft X-ray modes, with as much as 30ħ angular momentum per photon, are demonstrated.
- J. C. T Lee
- , S. J. Alexander
- & B. J. McMorran
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Article |
High-efficiency perovskite–polymer bulk heterostructure light-emitting diodes
Near-infrared perovskite–polymer light-emitting diodes (LEDs) with external quantum efficiencies of up to 20.1% are reported.
- Baodan Zhao
- , Sai Bai
- & Dawei Di
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Letter |
Nonlinear charge oscillation driven by a single-cycle light field in an organic superconductor
A nonlinear charge oscillation driven by a 6 fs light field of 11 MV cm–1 is observed in a layered organic superconductor. The initial response time of the oscillation on the timescale of 10 fs clarifies that Coulomb repulsion is essential for the superconductivity.
- Y. Kawakami
- , T. Amano
- & S. Iwai
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Article |
Continuous transition between weak and ultrastrong coupling through exceptional points in carbon nanotube microcavity exciton–polaritons
A microcavity exciton–polariton system based on aligned and packed single-walled carbon nanotubes exhibits ultrastrong coupling. The coupling strength is polarization sensitive. The record high value of vacuum Rabi splitting, 329 meV, is reported.
- Weilu Gao
- , Xinwei Li
- & Junichiro Kono
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Vacuum Bloch–Siegert shift in Landau polaritons with ultra-high cooperativity
The Bloch–Siegert shift—a strong-field phenomenon that implies a failure of the rotating-wave approximation—is observed in the polariton dispersion diagram of a two-dimensional electron gas system inside a high-Q terahertz photonic crystal cavity.
- Xinwei Li
- , Motoaki Bamba
- & Junichiro Kono
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Letter |
High-harmonic spectroscopy of ultrafast many-body dynamics in strongly correlated systems
A highly nonlinear optical response can be used to time-resolve light-induced phase transitions with few-femtosecond to sub-femtosecond accuracy, paving the way for time-resolving highly correlated many-body dynamics in strongly correlated systems with few-femtosecond accuracy.
- R. E. F. Silva
- , Igor V. Blinov
- & M. Ivanov
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Letter |
Large magneto-optical Kerr effect and imaging of magnetic octupole domains in an antiferromagnetic metal
The magneto-optical Kerr effect is demonstrated in an antiferromagnetic metal. Large rotation angles, magnetic octupole domain imaging was enabled.
- Tomoya Higo
- , Huiyuan Man
- & Satoru Nakatsuji
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Letter |
Reversible optical control of macroscopic polarization in ferroelectrics
Ferroelectric domains are optically reconfigured by a reversible process. The tuning is sufficient to enable macroscopically observable responses and the findings may help lead to the development of photo-stimulated ferroelectric devices.
- Fernando Rubio-Marcos
- , Diego A. Ochoa
- & José E. García
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Article |
Valley-polarized exciton–polaritons in a monolayer semiconductor
Exploitation of the valley electronic structure of transition metal dichalcogenides with exciton–polaritons is an elusive challenge. Now, valley-polarized exciton–polaritons in monolayers of MoS2 have been demonstrated.
- Yen-Jung Chen
- , Jeffrey D. Cain
- & Nathaniel P. Stern
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Letter |
Optical determination of the Néel vector in a CuMnAs thin-film antiferromagnet
Due to their nature antiferromagnets are difficult to probe with conventional magnetometers. The Néel vector of a practically important antiferromagnet, CuMnAs, has now been determined by a femtosecond pump–probe magneto-optical experiment.
- V. Saidl
- , P. Němec
- & T. Jungwirth
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Article |
Large-scale Ising spin network based on degenerate optical parametric oscillators
More than 10,000 time-division-multiplexed degenerate parametric oscillators are generated using phase-sensitive amplification in a nonlinear optical fibre. They can be used to simulate a coherent Ising machine that could solve difficult computing problems.
- Takahiro Inagaki
- , Kensuke Inaba
- & Hiroki Takesue
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Article |
Optical manipulation of the Berry phase in a solid-state spin qubit
An all-optical manipulation of the Berry phase based on stimulated Raman adiabatic passage is demonstrated in an individual nitrogen–vacancy centre in diamond. The adiabatic control is 100 times faster than that demonstrated before in atomic systems.
- Christopher G. Yale
- , F. Joseph Heremans
- & David D. Awschalom
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Article |
Hexagonal boron nitride is an indirect bandgap semiconductor
Scientists resolve the long-debated issue of the nature and value of the bandgap in hexagonal boron nitride by providing evidence for an indirect bandgap at 5.955 eV and an exciton binding energy of about 130 meV by means of optical spectroscopy.
- G. Cassabois
- , P. Valvin
- & B. Gil
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