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Letter |
Epitaxial growth of a 100-square-centimetre single-crystal hexagonal boron nitride monolayer on copper
The epitaxial growth of large single-crystal hexagonal boron nitride monolayers on low-symmetry copper foils is demonstrated.
- Li Wang
- , Xiaozhi Xu
- & Kaihui Liu
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Letter |
Topological superconductivity in a phase-controlled Josephson junction
Majorana bound states are created in a two-dimensional architecture by confining Majorana channels within a planar Josephson junction, using the phase difference across the junction and an in-plane magnetic field.
- Hechen Ren
- , Falko Pientka
- & Amir Yacoby
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Letter |
Chiral twisted van der Waals nanowires
A tunable interlayer twist that evolves naturally during synthesis of van der Waals nanowires made from layered crystals of germanium sulfide could produce new electronic structure and correlation phenomena.
- Peter Sutter
- , Shawn Wimer
- & Eli Sutter
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Letter |
Production of phosphorene nanoribbons
Phosphorene nanoribbons are produced in liquids through the intercalation of black phosphorous crystals with lithium ions, enabling the search for predicted exotic states and applications of these nanoribbons.
- Mitchell C. Watts
- , Loren Picco
- & Christopher A. Howard
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Letter |
Van der Waals contacts between three-dimensional metals and two-dimensional semiconductors
Ultraclean van der Waals bonds between gold-capped indium and a monolayer of the two-dimensional transition-metal dichalcogenide molybdenum disulfide show desirably low contact resistance at the interface, enabling high-performance field-effect transistors.
- Yan Wang
- , Jong Chan Kim
- & Manish Chhowalla
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Perspective |
Van der Waals integration before and beyond two-dimensional materials
Recent advances and future directions in the use of van der Waals integration beyond two-dimensional materials are reviewed.
- Yuan Liu
- , Yu Huang
- & Xiangfeng Duan
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Letter |
Resonantly hybridized excitons in moiré superlattices in van der Waals heterostructures
Excitonic bands in MoSe2/WS2 heterostructures can hybridize, resulting in a resonant enhancement of moiré superlattice effects.
- Evgeny M. Alexeev
- , David A. Ruiz-Tijerina
- & Alexander I. Tartakovskii
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Letter |
Observation of moiré excitons in WSe2/WS2 heterostructure superlattices
Moiré superlattice exciton states are observed in WSe2/WS2 heterostructures with closely aligned layers.
- Chenhao Jin
- , Emma C. Regan
- & Feng Wang
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Letter |
Evidence for moiré excitons in van der Waals heterostructures
Multiple interlayer exciton resonances in a MoSe2/WSe2 heterobilayer with a small twist angle are attributed to excitonic ground and excited states confined within the moiré potential.
- Kha Tran
- , Galan Moody
- & Xiaoqin Li
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Letter |
Signatures of moiré-trapped valley excitons in MoSe2/WSe2 heterobilayers
The trapping of interlayer valley excitons in a moiré potential formed by a molybdenum diselenide/tungsten diselenide heterobilayer with twist angle control is reported.
- Kyle L. Seyler
- , Pasqual Rivera
- & Xiaodong Xu
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Letter |
Observation of the nonlinear Hall effect under time-reversal-symmetric conditions
The nonlinear Hall effect is observed in bilayer WTe2 in the absence of a magnetic field, providing a direct measure of the dipole moment of the Berry curvature.
- Qiong Ma
- , Su-Yang Xu
- & Pablo Jarillo-Herrero
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Letter |
Reversible superdense ordering of lithium between two graphene sheets
Using a double-aberration-corrected transmission electron microscope, intercalation of lithium between two graphene sheets is found to produce a dense, multilayer lithium phase, rather than the expected single layer.
- Matthias Kühne
- , Felix Börrnert
- & Jurgen H. Smet
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Perspective |
Structural superlubricity and ultralow friction across the length scales
The phenomenon of ultralow friction between sliding incommensurate crystal surfaces—structural superlubricity—is examined, and the challenges and opportunities involved in its extension to the macroscale are assessed.
- Oded Hod
- , Ernst Meyer
- & Michael Urbakh
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Letter |
Gate-tunable room-temperature ferromagnetism in two-dimensional Fe3GeTe2
Monolayers of Fe3GeTe2 exhibit itinerant ferromagnetism with an out-of-plane magnetocrystalline anisotropy; ionic gating raises the ferromagnetic transition temperature of few-layer Fe3GeTe2 to room temperature.
- Yujun Deng
- , Yijun Yu
- & Yuanbo Zhang
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Letter |
Solution-processable 2D semiconductors for high-performance large-area electronics
By intercalating large ammonium molecules to exfoliate MoS2 with preservation of the 2H-phase, highly uniform solutionprocessable 2D semiconductor nanosheets are obtained for the scalable fabrication of large-area thin-film electronics.
- Zhaoyang Lin
- , Yuan Liu
- & Xiangfeng Duan
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Letter |
Observation of topological phenomena in a programmable lattice of 1,800 qubits
A large-scale programmable quantum simulation is described, using a D-Wave quantum processor to simulate a two-dimensional magnetic lattice in the vicinity of a topological phase transition.
- Andrew D. King
- , Juan Carrasquilla
- & Mohammad H. Amin
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Letter |
Room-temperature electrical control of exciton flux in a van der Waals heterostructure
Heterobilayer excitonic devices consisting of two different van der Waals materials, in which excitons are shared between the layers, exhibit electrically controlled switching actions at room temperature.
- Dmitrii Unuchek
- , Alberto Ciarrocchi
- & Andras Kis
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Letter |
Ferroelectric switching of a two-dimensional metal
Two- and three-layer WTe2 exhibits spontaneous out-of-plane electric polarization that can be switched electrically at room temperature and is sufficiently robust for use in applications with other two-dimensional materials.
- Zaiyao Fei
- , Wenjin Zhao
- & David H. Cobden
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Article |
Electron ptychography of 2D materials to deep sub-ångström resolution
Combining an electron microscope pixel-array detector that collects the entire distribution of scattered electrons with full-field ptychography greatly improves image resolution and contrast compared to traditional techniques, even at low beam energies.
- Yi Jiang
- , Zhen Chen
- & David A. Muller
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Letter |
Electrically controlled water permeation through graphene oxide membranes
The rapid water transport through graphene oxide membranes can be switched off by introducing localized electric fields within the membranes that ionize surrounding water molecules and thus block transport.
- K.-G. Zhou
- , K. S. Vasu
- & R. R. Nair
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Letter |
Heterointerface effects in the electrointercalation of van der Waals heterostructures
The electrointercalation of lithium into van der Waals heterostructures of graphene, hexagonal boron nitride and molybdenum dichalcogenides is studied at the level of individual atomic interfaces.
- D. Kwabena Bediako
- , Mehdi Rezaee
- & Philip Kim
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Letter |
Thickness-independent capacitance of vertically aligned liquid-crystalline MXenes
Electrode films prepared from a liquid-crystal phase of vertically aligned two-dimensional titanium carbide show electrochemical energy storage that is nearly independent of film thickness.
- Yu Xia
- , Tyler S. Mathis
- & Shu Yang
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Letter |
Approaching the Schottky–Mott limit in van der Waals metal–semiconductor junctions
In metal–semiconductor junctions, interfacial bonding and disorder cause deviations from theoretical predictions for the energy barrier, but delicately transferring pre-fabricated metal films onto two-dimensional semiconductors can overcome this challenge.
- Yuan Liu
- , Jian Guo
- & Xiangfeng Duan
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Letter |
Dynamic band-structure tuning of graphene moiré superlattices with pressure
For appropriately aligned layers of different two-dimensional materials, the separation between layers—and hence the interlayer coupling—is very sensitive to pressure, leading to pressure-induced changes in the electronic properties of the heterostructures.
- Matthew Yankowitz
- , Jeil Jung
- & Cory R. Dean
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Letter |
Lightwave valleytronics in a monolayer of tungsten diselenide
A strong lightwave in a monolayer of tungsten diselenide drives changes in the valley pseudospin, making valley pseudospin an information carrier that is switchable faster than a single light cycle.
- F. Langer
- , C. P. Schmid
- & R. Huber
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Letter |
A library of atomically thin metal chalcogenides
Molten-salt-assisted chemical vapour deposition is used to synthesize a wide variety of two-dimensional transition-metal chalcogenides.
- Jiadong Zhou
- , Junhao Lin
- & Zheng Liu
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Letter |
Monolayer atomic crystal molecular superlattices
Superlattices consisting of alternating monolayer atomic crystals and molecular layers allow access to stable phosphorene monolayers with competitive transistor performance and to bulk monolayer materials with tunable optoelectronic properties.
- Chen Wang
- , Qiyuan He
- & Xiangfeng Duan
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Letter |
Multi-terminal memtransistors from polycrystalline monolayer molybdenum disulfide
Polycrystalline monolayer molybdenum disulfide is used to fabricate a multi-terminal device combining a memristor and a transistor, which can mimic biological neurons with multiple synapses for neuromorphic computing applications.
- Vinod K. Sangwan
- , Hong-Sub Lee
- & Mark C. Hersam
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Letter |
One-pot growth of two-dimensional lateral heterostructures via sequential edge-epitaxy
An approach is developed for the continuous fabrication of lateral multi-junction heterostructures of transition-metal dichalcogenides, in which the sequential formation of heterojunctions is achieved solely by changing the composition of the reactive gas environment in the presence of water vapour.
- Prasana K. Sahoo
- , Shahriar Memaran
- & Humberto R. Gutiérrez
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Letter |
Structural phase transition in monolayer MoTe2 driven by electrostatic doping
A structural phase transition in a monolayer of molybdenum ditelluride has been shown experimentally to be driven forwards and backwards by electrostatic doping.
- Ying Wang
- , Jun Xiao
- & Xiang Zhang
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Letter |
Layer-by-layer assembly of two-dimensional materials into wafer-scale heterostructures
Layer-by-layer stacking enables the construction of transition-metal dichalcogenide van der Waals heterostructures with high-quality, uniform interfaces and tunable electrical properties.
- Kibum Kang
- , Kan-Heng Lee
- & Jiwoong Park
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Letter |
Layer-dependent ferromagnetism in a van der Waals crystal down to the monolayer limit
Magneto-optical Kerr effect microscopy is used to show that monolayer chromium triiodide is an Ising ferromagnet with out-of-plane spin orientation.
- Bevin Huang
- , Genevieve Clark
- & Xiaodong Xu
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Letter |
Discovery of intrinsic ferromagnetism in two-dimensional van der Waals crystals
Intrinsic long-range ferromagnetic order is observed in few-layer Cr2Ge2Te6 crystals, with a transition temperature that can be controlled using small magnetic fields.
- Cheng Gong
- , Lin Li
- & Xiang Zhang
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Letter |
Ultra-selective high-flux membranes from directly synthesized zeolite nanosheets
A direct synthesis of high-aspect-ratio microporous zeolite nanosheets and the use of such nanosheets in separation membranes are described.
- Mi Young Jeon
- , Donghun Kim
- & Michael Tsapatsis
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Letter |
Controlling charge quantization with quantum fluctuations
A device consisting of a metallic island connected to electrodes via tunable semiconductor-based conduction channels is used to explore the evolution of charge quantization in the presence of quantum fluctuations; the measurements reveal a robust scaling of charge quantization as the square root of the residual electron reflection probability across a quantum channel, consistent with theoretical predictions.
- S. Jezouin
- , Z. Iftikhar
- & F. Pierre
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Letter |
Single-layer MoS2 nanopores as nanopower generators
Blue energy is a desirable renewable resource, involving the osmotic transport of ions through a membrane from seawater to fresh water; here, nanopores have been created in two-dimensional molybdenum-disulfide membranes, and shown to generate a substantial osmotic power output.
- Jiandong Feng
- , Michael Graf
- & Aleksandra Radenovic
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Letter |
Self-assembly of graphene ribbons by spontaneous self-tearing and peeling from a substrate
The controllable self-assembly of graphene ribbons on a substrate is shown, demonstrating an effect which could be applied to patterning and actuating devices made from two-dimensional materials.
- James Annett
- & Graham L. W. Cross
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Letter |
High-efficiency two-dimensional Ruddlesden–Popper perovskite solar cells
Thin-film solar cells were fabricated using layered two-dimensional perovskites with near-single-crystalline out-of-plane alignment, which facilitates efficient charge transport leading to greatly improved power conversion efficiency with technologically relevant stability to light exposure, humidity and heat stress.
- Hsinhan Tsai
- , Wanyi Nie
- & Aditya D. Mohite
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Letter |
Switching stiction and adhesion of a liquid on a solid
Switching of static friction and adhesion of a liquid drop on a corrugated solid boron nitride surface is linked to the intercalation of hydrogen, which changes the electric field of in-plane dipole rings and thus reduces the adsorption energy.
- Stijn F. L. Mertens
- , Adrian Hemmi
- & Thomas Greber
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Letter |
Graphene kirigami
The ratio of in-plane stiffness to out-of-plane bending stiffness of graphene is shown to be similar to that of a piece of paper, which allows ideas from kirigami (a variation of origami that allows cutting) to be applied to micrometre-scale graphene sheets to build mechanically stretchable yet robust electrodes, springs and hinges.
- Melina K. Blees
- , Arthur W. Barnard
- & Paul L. McEuen
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Letter |
High-mobility three-atom-thick semiconducting films with wafer-scale homogeneity
A new chemical vapour deposition method enables transition-metal dichalcogenide (TMD) monolayers to be grown directly on insulating silicon dioxide wafers, demonstrating the possibility of wafer-scale batch fabrication of high-performance devices with TMD monolayers.
- Kibum Kang
- , Saien Xie
- & Jiwoong Park
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Letter |
Square ice in graphene nanocapillaries
The structure of the low-dimensional water confined in hydrophobic pores is shown, using electron microscopy and supported by molecular dynamics simulations, to be ‘square ice’, which does not have the conventional tetrahedral hydrogen bonding.
- G. Algara-Siller
- , O. Lehtinen
- & I. V. Grigorieva
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Letter |
Monolayer semiconductor nanocavity lasers with ultralow thresholds
A miniature laser is reported that uses two-dimensional tungsten diselenide as the active medium, which is placed on a photonic crystal membrane that acts as the laser cavity; the laser emits visible light, with an ultralow pump threshold.
- Sanfeng Wu
- , Sonia Buckley
- & Xiaodong Xu
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Letter |
Proton transport through one-atom-thick crystals
Measurements show that monolayers of graphene and hexagonal boron nitride are unexpectedly highly permeable to thermal protons and that their conductivity rapidly increases with temperature, but that no proton transport is detected for few-layer crystals.
- S. Hu
- , M. Lozada-Hidalgo
- & A. K. Geim
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Letter |
Conductive two-dimensional titanium carbide ‘clay’ with high volumetric capacitance
Two-dimensional titanium carbide has been produced by etching out aluminium in a lithium fluoride and hydrochloric acid mixture; it is hydrophilic and mouldable like clay and has excellent volumetric capacitance and cyclability, properties that are desirable for portable electronics.
- Michael Ghidiu
- , Maria R. Lukatskaya
- & Michel W. Barsoum
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Letter |
Artificial chemical and magnetic structure at the domain walls of an epitaxial oxide
The strain induced on the walls between ferroelastic domains of a thin film of terbium manganite grown on a substrate of strontium titanate can generate an unusual two-dimensional ferromagnetic phase that is yet to be produced by conventional chemical means.
- S. Farokhipoor
- , C. Magén
- & B. Noheda
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Letter |
Probing excitonic dark states in single-layer tungsten disulphide
A series of long-lived excitons in a monolayer of tungsten disulphide are found to have strong binding energy and an energy dependence on orbital momentum that significantly deviates from conventional, three-dimensional, behaviour.
- Ziliang Ye
- , Ting Cao
- & Xiang Zhang
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Letter |
Quantum droplets of electrons and holes
Fast optical pulses create a plasma of electrons and holes in a semiconductor in which excitons (pairs of holes and electrons) and combinations of two excitons emerge; now a stable liquid-like droplet of electrons and holes has been detected and called a ‘dropleton’.
- A. E. Almand-Hunter
- , H. Li
- & S. W. Koch
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Letter |
Dislocations in bilayer graphene
Basal-plane dislocations, identified as fundamental defects in bilayer graphene by transmission electron microscopy and atomistic simulations, reveal striking size effects, most notably a pronounced buckling of the graphene membrane, which drastically alters the strain state and is of key importance for the material’s mechanical and electronic properties.
- Benjamin Butz
- , Christian Dolle
- & Erdmann Spiecker