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| Open AccessAxion insulator state in hundred-nanometer-thick magnetic topological insulator sandwich heterostructures
A zero Hall conductance plateau has been taken as evidence of the axion insulator state in magnetically doped topological insulator heterostructures, but it can also originate from surface state hybridization. Here the authors establish such a state in a ~106 nm thick sample, where hybridization is negligible.
- Deyi Zhuo
- , Zi-Jie Yan
- & Cui-Zu Chang
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Article
| Open AccessTopotactically transformable antiphase boundaries with enhanced ionic conductivity
Antiphase boundaries (APBs) have been considered major obstacles to optimizing the ionic conductivity of conductors. Here authors reveal that ionic conductivity can be enhanced through engineering APBs by topotactical transformation at the atomic scale.
- Kun Xu
- , Shih-Wei Hung
- & Jing Zhu
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Article
| Open AccessReentrance of interface superconductivity in a high-Tc cuprate heterostructure
The authors study interface superconductivity in over-doped La2-xSrxCuO4/La2CuO4 heterostructures. As x increases, the superconductivity is killed at x = 0.8 but fully recovers at x = 1.0, a “re-entrant” superconductivity.
- J. Y. Shen
- , C. Y. Shi
- & J. Wu
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Article
| Open AccessRotational symmetry breaking in superconducting nickelate Nd0.8Sr0.2NiO2 films
The authors study transport in the superconducting state of infinite-layer nickelate Nd0.8Sr0.2NiO2 films using a Corbino-disk configuration, finding that the magnetoresistance changes from isotropic to four-fold anisotropic with increasing magnetic field. At even higher field, an additional two-fold component emerges, which coincides with an anomalous upturn of the critical field.
- Haoran Ji
- , Yi Liu
- & Jian Wang
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Article
| Open AccessDirac-fermion-assisted interfacial superconductivity in epitaxial topological-insulator/iron-chalcogenide heterostructures
The authors study (Bi,Sb)2Te3/FeTe bilayers, which feature emergent superconductivity at the interface with Tc ~ 12 K. Through angle-resolved photoemission spectroscopy and electrical transport measurements, they argue that the Dirac-fermion-mediated Ruderman-Kittel-Kasuya-Yosida-type interaction weakens antiferromagnetic order in FeTe layer, allowing for superconductivity.
- Hemian Yi
- , Lun-Hui Hu
- & Cui-Zu Chang
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Article
| Open AccessTransport of bound quasiparticle states in a two-dimensional boundary superfluid
Superfluid 3He appears to be composed of two independent superfluid subsystems. Here the authors discuss diffusion of quasiparticles in the two-dimensional boundary superfluid.
- Samuli Autti
- , Richard P. Haley
- & Dmitry E. Zmeev
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Article
| Open AccessEmergent superconductivity in topological-kagome-magnet/metal heterostructures
The authors deposit non-superconducting metallic thin films on surfaces of the kagome Chern magnet TbMn6Sn6 and observe emergent superconductivity even though neither component is a superconductor. Furthermore, the superconducting state is quasi-two-dimensional and coexists with ferromagnetism, consistent with possible spin-triplet pairing and topological superconductivity.
- He Wang
- , Yanzhao Liu
- & Jian Wang
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Article
| Open AccessAnisotropic resistance with a 90° twist in a ferromagnetic Weyl semimetal, Co2MnGa
Weyl semimetals exhibit a rich variety of transport phenomena, but it usually takes low temperatures and a strong magnetic field to realize them. Here, Quirk et al. show that when the ferromagnetic Weyl semimetal Co2MnGa is polished to micron thicknesses, it develops a remarkable resistance anisotropy that has opposite directions on opposing crystal faces. They show that this unusual transport property, which is robust at room temperature and in a strong magnetic field, may be generated by distinct conducting states on the surfaces of these thin crystals.
- Nicholas P. Quirk
- , Guangming Cheng
- & N. P. Ong
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Article
| Open AccessFast and versatile electrostatic disc microprinting for piezoelectric elements
In this work, authors demonstrate a fast and versatile microprinting technique to produce high-performance and customizable piezoelectric elements by employing a conductive spiny disc to electrostatically trigger instability to the liquid-air interface of the ink.
- Xuemu Li
- , Zhuomin Zhang
- & Zhengbao Yang
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Article
| Open AccessFully automatic transfer and measurement system for structural superlubric materials
A critical step to enable practical structural superlubricity (SSL) applications is to enable high throughput to both fabrication and performance evaluation. Here, the authors demonstrate an automated system for efficient and multiple SSL materials transfer and tribological measurement.
- Li Chen
- , Cong Lin
- & Ming Ma
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Article
| Open AccessElectronic Janus lattice and kagome-like bands in coloring-triangular MoTe2 monolayers
2D materials with Kagome lattices have attracted significant interest due to their exotic electronic properties. Here, the authors report the synthesis and characterization of a 2D MoTe2 phase characterized by a colouring-triangular lattice (a Kagome variant), showing evidence of Dirac-like and flat electronic bands.
- Le Lei
- , Jiaqi Dai
- & Wei Ji
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| Open AccessVisualizing symmetry-breaking electronic orders in epitaxial Kagome magnet FeSn films
The Kagome lattice consists of equilateral triangles occupying each edge of a hexagon, resembling a star with six-fold rotation symmetry. Here, using scanning tunnelling microscopy, Zhang et al observe the breaking of this six-fold rotation symmetry in the Kagome lattice plane of the planar antiferromagnet, FeSn.
- Huimin Zhang
- , Basu Dev Oli
- & Lian Li
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Article
| Open AccessUnraveling bilayer interfacial features and their effects in polar polymer nanocomposites
The nanoparticle-polymer interface plays a key role in nanoparticle-polymer composites but understanding the structures and properties of the interfacial region remains challenging. Here, the authors directly observe the presence of two interfacial polymer layers around a nanoparticle in polar polymers with different polar molecular conformations from the bulk polymer leading to an enhancement in polarity-related properties of polymer nanocomposites
- Xinhui Li
- , Shan He
- & Ce-Wen Nan
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Article
| Open AccessCharge density wave surface reconstruction in a van der Waals layered material
Recent work has reported puzzling results on the surface of 1T-TaS2. Based on first-principles calculations, the authors show that charge density wave order undergoes surface reconstruction, leading to modifications in the surface electronic structure, which can explain recent experiments.
- Sung-Hoon Lee
- & Doohee Cho
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Article
| Open AccessAn anisotropic van der Waals dielectric for symmetry engineering in functionalized heterointerfaces
Here, the authors demonstrate that a layered anisotropic dielectric material, SiP2, can break the rotational symmetry of 2D MoS2, leading to linearly polarized photoluminescence emission and conductance anisotropy ratios up to 1000 in gated SiP2/MoS2 heterostructures.
- Zeya Li
- , Junwei Huang
- & Hongtao Yuan
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Article
| Open AccessSynergistic correlated states and nontrivial topology in coupled graphene-insulator heterostructures
Here, the authors theoretically predict the formation of synergistic correlated and topological states in Coulomb-coupled and gate-tunable graphene/insulator heterostructures, proposing a number of promising substrate candidates and a possible explanation for recent experimental observations in graphene/CrOCl heterostructures.
- Xin Lu
- , Shihao Zhang
- & Jianpeng Liu
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| Open AccessFrom Stoner to local moment magnetism in atomically thin Cr2Te3
Over the last few years, several van der Waals materials have been found that retain magnetic ordering down to monolayer thickness. These materials provide a simple platform for studying the magnetism in reduced dimensions. Here, Zhong et al study the thickness dependence of magnetic ordering in Cr2Te3, and find a crossover from Stoner to Heisenberg-type magnetism as thicknesses are reduced.
- Yong Zhong
- , Cheng Peng
- & Zhi-Xun Shen
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Article
| Open AccessIdentifying s-wave pairing symmetry in single-layer FeSe from topologically trivial edge states
The nature of the pairing symmetry in superconducting single-layer FeSe has been the subject of intense debate. Here, the authors use scanning tunneling microscopy/spectroscopy to show the absence of topological edge/corner modes, providing evidence for sign-preserving s-wave pairing.
- Zhongxu Wei
- , Shengshan Qin
- & Qi-Kun Xue
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| Open AccessDiscovery and construction of surface kagome electronic states induced by p-d electronic hybridization in Co3Sn2S2
Kagome materials host 2D planes which give rise to kagome physics, but these are typically embedded in the bulk. Huang et al. demonstrate a strategy for generating surface kagome electronic states by vertical p-d electronic hybridization between surface atoms and the buried Co kagome network in Co3Sn2S2.
- Li Huang
- , Xianghua Kong
- & Hong-Jun Gao
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Article
| Open AccessSpin-orbit driven superconducting proximity effects in Pt/Nb thin films
The authors study a Pt/Nb hybrid structure by scanning microscopy and muon spin rotation. They find an anomalous absence of Meissner screening near the Pt/Nb interface due to spin-triplet pair correlations driven by spin-orbit coupling alone with no ferromagnetic layer necessary.
- Machiel Flokstra
- , Rhea Stewart
- & Stephen Lee
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| Open AccessObservation of ultrafast interfacial Meitner-Auger energy transfer in a Van der Waals heterostructure
Here, the authors investigate the interfacial charge/energy transfer dynamics in a WSe2/graphene heterostructure. They unveil an energy transfer mechanism from WSe2 to graphene mediated by an interfacial Meitner-Auger process, resulting in a transient hole distribution in the Dirac cone at energies larger than the photon energy of the optical excitation.
- Shuo Dong
- , Samuel Beaulieu
- & Ralph Ernstorfer
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Article
| Open AccessCharge-state lifetimes of single molecules on few monolayers of NaCl
Resonant charge transport to and from molecules and their corresponding charge-state transitions are critical to understanding electrically driven processes. Here, the authors investigate the charge-state lifetimes of single molecules through NaCl films of 3 to 5 monolayers thickness.
- Katharina Kaiser
- , Leonard-Alexander Lieske
- & Leo Gross
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Article
| Open AccessTowards layer-selective quantum spin hall channels in weak topological insulator Bi4Br2I2
Weak topological insulators offer promising topological state tunability for devices. Here, the authors use ARPES and first-principles calculations to evidence signatures of layer-selective quantum spin Hall channels that may be tunable with chemical potential for future applications.
- Jingyuan Zhong
- , Ming Yang
- & Yi Du
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Article
| Open AccessUltra-thin lithium aluminate spinel ferrite films with perpendicular magnetic anisotropy and low damping
Ferromagnetic insulators offer low magnetic damping, and potentially efficient magnetic switching, making them ideal candidates for spin-based information processing. Here, Zheng et al introduce a ferromagnetic insulator spinel, Li0.5Al1.0Fe1.5O4, with low magnetic damping, perpendicular magnetic anisotropy, and no magnetic dead layer.
- Xin Yu Zheng
- , Sanyum Channa
- & Yuri Suzuki
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Article
| Open AccessBamboo-like dual-phase nanostructured copper composite strengthened by amorphous boron framework
Achieving strength and toughness synergy via microstructure design is challenging in materials science. Here, the authors construct a bamboo-like dual-phase copper-boron structure that has unique mechanical response resulting in simultaneous increase in hardness, strength, and ductility.
- Hang Lv
- , Xinxin Gao
- & Weitao Zheng
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Article
| Open AccessKinetic drop friction
Sliding of drops over solid surface is a common phenomenon, but it remains impossible to predict the sliding velocity due to numerous dissipation channels causing drop friction. Li et al. show that dynamic wetting is determined by a dimensionless friction coefficient, which is a material parameter.
- Xiaomei Li
- , Francisco Bodziony
- & Hans-Jürgen Butt
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Article
| Open AccessGeneration of out-of-plane polarized spin current by spin swapping
Controlling the magnetization of a material is a major goal of spin-based information processing. One extensively studied method is to use spin-currents, generated from charge currents via the spin hall effect, however, the resulting spin polarization is typically limited to in-plane orientations. Here, Hazra et al demonstrate the presence of out-of-plane polarized spin-currents, which arise due to spin swapping at the Mn3Sn/permalloy interface.
- Binoy K. Hazra
- , Banabir Pal
- & Stuart S. P. Parkin
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| Open AccessSurface coupling in Bi2Se3 ultrathin films by screened Coulomb interaction
Single-particle band theory is facing limitations in describing the physics of ultrathin topological insulator films. Here, the authors investigate the coupling between top and bottom surfaces of a topological insulator and analyse their interaction in the framework of screened Coulomb interactions.
- Jia-nan Liu
- , Xu Yang
- & Zhao-Hua Cheng
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| Open AccessWater nanolayer facilitated solitary-wave-like blisters in MoS2 thin films
‘Solitary waves are unique in nonlinear systems. Here, the authors report on an anomalous, solitary wave-like blister (SWLB) of MoS2 thin films, which propagates forward like solitary waves appearing in fluids. The SWLB results from fluid structure interaction due to an interfacial water nanolayer.’
- Enze Wang
- , Zixin Xiong
- & Kai Liu
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Article
| Open AccessFerroelectric solitons crafted in epitaxial bismuth ferrite superlattices
Topological structures could spark promising functionalities in next generation nanoelectronics. Here, the authors report the realization of complex topological polar textures in epitaxial multiferroic BiFeO3 –SrTiO3 superlattices induced by competing electrical and mechanical boundary conditions.
- Vivasha Govinden
- , Peiran Tong
- & Daniel Sando
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Article
| Open AccessMolecular conformation of polyelectrolytes inside Layer-by-Layer assembled films
’Layer-by-layer (LbL) assembly is currently one of the most widely used techniques for the fabrication of multicomponent architectures with nanometer scale control but achieving control over the 3D structure, and thus the ability to predict and understand the device performance, is challenging. Here, the authors use neutron scattering to determine the average conformation of individual deuterated polyelectrolyte chains inside LbL assembled films.
- Philipp Gutfreund
- , Christophe Higy
- & Gero Decher
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Article
| Open AccessArtificially controlled nanoscale chemical reduction in VO2 through electron beam illumination
The authors demonstrate a nanoscale chemical reduction for VO2 into V2O3 through electron-beam illumination, showcasing potential for nanoscale manipulation of oxygen ionic evolution for advanced harvesting functionalities.
- Yang Zhang
- , Yupu Wang
- & Pu Yu
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| Open AccessDirect measurements of the colloidal Debye force
The Debye interaction is defined as the attraction between a polar molecule and a nonpolar molecule, which governs many self-assembling processes in materials. Here, Lee et al. design a like-charged colloidal model at the water-oil interface to characterize the Debye interaction for the first time.
- Hyang Mi Lee
- , Yong Woo Kim
- & Bum Jun Park
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| Open AccessAtomic-scale manipulation of single-polaron in a two-dimensional semiconductor
Herein, using scanning tunnelling microscopy, the authors create single polarons in a monolayer two-dimensional semiconductor, CoCl2. They show that a series of manipulation progresses — from creation, erasure, to transition — can be accurately implemented on individual polarons.
- Huiru Liu
- , Aolei Wang
- & Kehui Wu
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| Open AccessTuning orbital-selective phase transitions in a two-dimensional Hund’s correlated system
Hund’s coupling, or the intra-atomic exchange, can drive novel quantum phases in multi-orbital systems, but this requires precise control of orbital occupancy. Ko et al. report an orbital-selective metal-to-insulator transition driven by Hund´s physics via symmetry-preserving strain tuning in monolayer SrRuO3.
- Eun Kyo Ko
- , Sungsoo Hahn
- & Tae Won Noh
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Article
| Open AccessAtomic motifs govern the decoration of grain boundaries by interstitial solutes
Interplay between structure and composition of grain boundaries remains elusive, particularly at the atomic level. Here, the authors discover the atomic motifs, which is the smallest structural unit, control the most important chemical properties of grain boundaries.
- Xuyang Zhou
- , Ali Ahmadian
- & Dierk Raabe
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Article
| Open AccessQuantum bath suppression in a superconducting circuit by immersion cooling
Removing excess energy (cooling) and reducing noise in superconducting quantum circuits is central to improved coherence. Lucas et al. demonstrate cooling of a superconducting resonator and its noisy environment to sub-mK temperatures by immersion in liquid 3He.
- M. Lucas
- , A. V. Danilov
- & S. E. de Graaf
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Article
| Open AccessBerry curvature contributions of kagome-lattice fragments in amorphous Fe–Sn thin films
The topological character of solids is usually revealed by considering the Berry curvature of electronic bands in a periodic crystal. Here, authors demonstrate the influence of the Berry curvature on the electronic properties of an amorphous thin film.
- Kohei Fujiwara
- , Yasuyuki Kato
- & Atsushi Tsukazaki
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Article
| Open AccessAbsence of critical thickness for polar skyrmions with breaking the Kittel’s law
Here, the authors find that ferroelectric skyrmions can be sustained in [(PbTiO3)2/(SrTiO3)2]m ultrathin superlattices. The period-thickness relationship of skyrmions in the ultrathin PbTiO3 layers breaks Kittel’s law.
- Feng-Hui Gong
- , Yun-Long Tang
- & Xiu-Liang Ma
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Article
| Open AccessStrain-tunable Berry curvature in quasi-two-dimensional chromium telluride
Chromium tellurides are a particularly promising family of quasi-2D magnetic materials; towards the single van der Waals layer limit, they preserve magnetic ordering, some even above room temperature, and exhibit a variety of intrinsic topological properties. Here, Hang Chi, Yunbo Ou and co-authors demonstrate a strain tunable Berry curvature induced reversal of the anomalous Hall effect in Cr2Te3.
- Hang Chi
- , Yunbo Ou
- & Jagadeesh S. Moodera
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Article
| Open AccessCryogenic characteristics of graphene composites—evolution from thermal conductors to thermal insulators
Graphene composites can serve both as efficient thermal insulators at low temperatures and thermal conductors at high temperatures. Here, the authors report the evolution of thermal conductivity of composites with graphene fillers from cryogenic to room temperature.
- Zahra Ebrahim Nataj
- , Youming Xu
- & Alexander A. Balandin
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Article
| Open AccessSpontaneous rotational symmetry breaking in KTaO3 heterointerface superconductors
Superconducting interfaces involving KTaO3 have recently attracted attention due to their relatively high transition temperature. Here, the authors study amorphous-YAlO3/KTaO3 interfaces and find two-fold symmetry in the superconducting regime, possibly due to a mixed-parity superconducting state.
- Guanqun Zhang
- , Lijie Wang
- & Wei Li
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Article
| Open AccessBimodal ionic photomemristor based on a high-temperature oxide superconductor/semiconductor junction
Designing efficient photonic neuromorphic systems remains a challenge. Here, the authors develop a new class of memristor sensitive to the dual electro-optical history obtained by exploiting electrochemical, photovoltaic and photo-assisted oxygen ion motion effects at a high temperature superconductor / semiconductor interface.
- Ralph El Hage
- , Vincent Humbert
- & Javier E. Villegas
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Article
| Open AccessLithium crystallization at solid interfaces
In solid-state lithium metal batteries, the crystallization of Li-ions deposited at interfaces remains unclear. Here, authors use molecular dynamics simulations to reveal lithium crystallization pathways and energy barriers, guiding improved interfacial engineering and accelerated crystal growth.
- Menghao Yang
- , Yunsheng Liu
- & Yifei Mo
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Article
| Open AccessSpectroscopic signature of obstructed surface states in SrIn2P2
The authors observe spectroscopic signature of obstructed surface states on the (0001) plane of SrIn2P2. Due to structural reconstruction, the surface state undergoes an adiabatic evolution and split into two branches, the upper of which being spatially localized with unusual negative differential conductance.
- Xiang-Rui Liu
- , Hanbin Deng
- & Chang Liu
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Article
| Open AccessInterfacial interaction and intense interfacial ultraviolet light emission at an incoherent interface
Incoherent interfaces usually have weak interfacial interactions and lack of unique properties. Here, Yan et al. demonstrate unexpected strong interfacial interactions and intense ultraviolet light emission at an incoherent AlN/Al2O3 interface.
- Xuexi Yan
- , Yixiao Jiang
- & Xiu-Liang Ma
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Article
| Open AccessAnomalous enhancement of charge density wave in kagome superconductor CsV3Sb5 approaching the 2D limit
The kagome superconductor CsV3Sb5 exhibits a charge density wave (CDW) as well as superconductivity (SC). Here, the authors find that the CDW transition temperature decreases with decreasing sample thickness to 72 K at 27 atomic layers, but then unexpectedly increases to 120 K at 5 layers, an opposite trend to SC.
- Boqin Song
- , Tianping Ying
- & Shiyan Li
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Article
| Open AccessPhonon transition across an isotopic interface
Here, the authors probe the phonon changes across an atomically sharp h-10BN/h-11BN isotope interface with sub-unit-cell spatial resolution and momentum resolution. The observed phonon delocalization suggests strong electron-phonon coupling at isotopic interface.
- Ning Li
- , Ruochen Shi
- & Peng Gao
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Article
| Open AccessPara-hydrodynamics from weak surface scattering in ultraclean thin flakes
Classical hydrodynamics applies to electron fluids as well, provided the system has a high electron–electron collision rate. Now, model calculations show that regimes in which other scattering processes are at play can explain hydrodynamic electron transport in thin flakes of the 2D material WTe2.
- Yotam Wolf
- , Amit Aharon-Steinberg
- & Tobias Holder