Featured
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| Open AccessGeometric quenching of orbital pair breaking in a single crystalline superconducting nanomesh network
It is highly desired to maintain superconductivity in presence of magnetic fields but it is by far difficult. Here, Nam et al. create a single crystalline superconducting Pb nanowire network, where critical temperatures are maintained and critical fields are enhanced in either parallel or perpendicular fields.
- Hyoungdo Nam
- , Hua Chen
- & Chih-Kang Shih
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Article
| Open AccessMachine learning plastic deformation of crystals
Predicting plastic deformation in crystals remains challenging owing to the nonlinear nature of stochastic avalanches involved, which resemble the critical phenomena. Salmenjoki et al. use machine learning to predict plastic deformation and show that it works better for those under large strains.
- Henri Salmenjoki
- , Mikko J. Alava
- & Lasse Laurson
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| Open AccessMelt-driven erosion in microparticle impact
Supersonic particle impacts can cause permanent damage to space vehicles and satellites, but how exactly remains unclear. Here, the authors visualise for the first time the high impact of single tin microparticles on a tin substrate and show erosion of ductile metallic materials is melt-driven.
- Mostafa Hassani-Gangaraj
- , David Veysset
- & Christopher A. Schuh
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| Open AccessThermodynamic phases in two-dimensional active matter
Adapting statistical physics tools to study active systems is challenging due to their non-equilibrium nature. Here the authors use simulations to present a phase diagram of a 2D active system, showing a two-step melting scenario far from equilibrium along with gas-liquid motility-induced phase separation.
- Juliane U. Klamser
- , Sebastian C. Kapfer
- & Werner Krauth
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| Open AccessTuning the balance between dispersion and entropy to design temperature-responsive flexible metal-organic frameworks
Rational design of metal organic frameworks (MOFs) with shape-memory nanopores is a formidable challenge. Here the authors use an accurate theoretical approach to design thermo-responsive MOFs based on a balance of van der Waals and entropy contributions.
- J. Wieme
- , K. Lejaeghere
- & V. Van Speybroeck
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| Open AccessUnusually complex phase of dense nitrogen at extreme conditions
Nitrogen has a complex phase diagram with rich polymorphism, which is challenging to characterize due to the extreme conditions and uncertain stability ranges needed to do so. Here the authors resolve one of the most elusive phases of this model system, reporting a crystalline structure with unusual complexity.
- Robin Turnbull
- , Michael Hanfland
- & Eugene Gregoryanz
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| Open AccessThermal transport crossover from crystalline to partial-crystalline partial-liquid state
Phase-change materials are applied as thermoelectric converters and battery electrodes, but underlying mechanisms are not fully understood. Here, the authors comprehensively describe thermal transport mechanisms of lithium sulfide based on molecular dynamics and first-principles simulations.
- Yanguang Zhou
- , Shiyun Xiong
- & Ming Hu
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| Open AccessSignature of quantum Griffiths singularity state in a layered quasi-one-dimensional superconductor
Whether the quantum Griffiths singularity state exists in one-dimensional (1D) systems remains elusive. Here, Zhang et al. report violation of the Pauli limit in the superconducting critical field and multiple phase transitions in the current-voltage hysteresis loops in a Ta2PdS5 nanowire, suggesting signatures of quasi-1D quantum Griffith singularity.
- Enze Zhang
- , Jinhua Zhi
- & Faxian Xiu
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| Open AccessTheory of photoinduced ultrafast switching to a spin-orbital ordered hidden phase
Ultrafast excitation of materials can cause the formation of hidden phases that are not accessible in thermal equilibrium. Li et al. identify and investigate theoretically a hidden phase that can be accessed in systems with intertwined spin and orbital-ordering such as KCuF3.
- Jiajun Li
- , Hugo U. R. Strand
- & Martin Eckstein
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| Open AccessStability and nature of the volume collapse of ε-Fe2O3 under extreme conditions
Iron oxides exist in a variety of polymorphs at different pressure and temperature conditions, displaying important magnetic properties, and are major constituents of the Earth’s interior. Here the authors investigate the structural and electronic changes in the uncommon epsilon phase under compression to deep Mantle pressures.
- J. A. Sans
- , V. Monteseguro
- & C. Popescu
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| Open AccessIn situ strain tuning of the metal-insulator-transition of Ca2RuO4 in angle-resolved photoemission experiments
The role of the lattice in the correlated metal-insulator transition of Ca2RuO4 has led to significant interest but experiments that are at the same time sensitive to crystal and electronic structure are difficult. Riccò et al. successfully combine ARPES measurements with in situ strain tuning across the Mott transition.
- S. Riccò
- , M. Kim
- & F. Baumberger
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| Open AccessScaling and data collapse from local moments in frustrated disordered quantum spin systems
There are many proposals for new forms of quantum matter in frustrated magnets but in practice disorder prevents the realisation of theoretically-tractable idealised models. Kimchi et al. show that recently observed scaling behavior common to several disordered quantum magnets can be understood as the emergence of a universal random-singlet regime.
- Itamar Kimchi
- , John P. Sheckelton
- & Patrick A. Lee
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Article
| Open AccessComposite fermion liquid to Wigner solid transition in the lowest Landau level of zinc oxide
In two-dimensional electron systems, strong Coulomb interactions lead to the formation of new phases. Here the authors observe a transition between two of these correlated phases, a composite fermion liquid and Wigner solid, in a zinc oxide heterostructure.
- D. Maryenko
- , A. McCollam
- & M. Kawasaki
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| Open AccessEmergence of superconductivity in the cuprates via a universal percolation process
The emergence of superconductivity from the normal state in the cuprates above the transition temperature (Tc) has been controversial. Here, Pelc et al. report nonlinear conductivity, resulting from superconducting precursors only, vanishing exponentially above Tc both with temperature and with magnetic field.
- Damjan Pelc
- , Marija Vučković
- & Neven Barišić
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| Open AccessPhoto-induced semimetallic states realised in electron–hole coupled insulators
Ultrafast light pulses can manipulate and probe materials faster than relaxation timescales, leading to new electronic states and insights into equilibrium properties. Okazaki et al. use the properties of photo-induced metallic states to investigate unconventional correlated behaviour in Ta2NiSe5 and Ta2NiS5.
- Kozo Okazaki
- , Yu Ogawa
- & Shik Shin
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| Open AccessPressure tuning of charge ordering in iron oxide
The charge order transition of commonly known magnetite has only recently been unraveled. Here, the measurement of the low-temperature high-pressure phase diagram of a related material (Fe4O5) elucidates the interplay of average oxidation state and charge-ordering phenomena in the iron oxide family.
- Sergey V. Ovsyannikov
- , Maxim Bykov
- & Leonid S. Dubrovinsky
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| Open AccessUltra-low-field magneto-elastocaloric cooling in a multiferroic composite device
The broad use of elastocaloric materials in cooling applications is hindered by the need to exert large forces onto the material. Compressing a magnetostrictive-elastocaloric composite using a low magnetic field of 0.16 T, temperature changes up to 4 K are achieved without applying external forces.
- Huilong Hou
- , Peter Finkel
- & Ichiro Takeuchi
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| Open AccessResonant torsion magnetometry in anisotropic quantum materials
Insights into the behavior of quantum materials are only possible because of the development of suitable experimental probes. Modic et. al. develop the theoretical and experimental basis for resonant torsion magnetometry—a technique to measure anisotropic magnetic responses with high sensitivity.
- K. A. Modic
- , Maja D. Bachmann
- & Philip J. W. Moll
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| Open AccessTransport evidence for a sliding two-dimensional quantum electron solid
At low densities, it is understood that the physics of two-dimensional electron gases becomes dominated by interactions but the nature of the state that forms remains controversial. Here the authors present transport measurements that indicate the existence of a Wigner crystal in silicon MOSFETs.
- Pedro Brussarski
- , S. Li
- & M. P. Sarachik
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| Open AccessImaging the nanoscale phase separation in vanadium dioxide thin films at terahertz frequencies
The insulator-to-metal transition in vanadium dioxide still has many unexplored properties. Here the authors use multi-modal THz and mid-IR nano-imaging to examine the phase transition in VO2 thin films, and discuss the unexpectedly smooth transition at THz frequencies in the context of a dimer Hubbard model.
- H. T. Stinson
- , A. Sternbach
- & D. N. Basov
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| Open AccessPeritectic titanium alloys for 3D printing
3D printing of titanium alloys today is based on known alloy compositions that result in anisotropic structural properties. Here, the authors add lanthanum to commercially pure titanium and exploit a solidification path that reduces texture and anisotropy.
- Pere Barriobero-Vila
- , Joachim Gussone
- & Guillermo Requena
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| Open AccessEfficient non-Markovian quantum dynamics using time-evolving matrix product operators
In general the computational requirements for simulating quantum systems scale exponentially but in some cases it is possible to formulate more efficient schemes. Here the authors present an efficient approach to calculate non-Markovian quantum dynamics using matrix product operator methods.
- A. Strathearn
- , P. Kirton
- & B. W. Lovett
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| Open AccessEvolution of the Kondo lattice and non-Fermi liquid excitations in a heavy-fermion metal
The competition between Kondo correlations and magnetic ordering in heavy fermion materials leads to emergent physics that is not fully understood. Seiro et al. show inter-site Kondo correlations only dominate over local ones at temperatures well below the single-ion Kondo temperature but this is a prerequisite for quantum critical behavior.
- S. Seiro
- , L. Jiao
- & S. Wirth
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| Open AccessMechanical glass transition revealed by the fracture toughness of metallic glasses
Understanding the fracture toughness of metallic glasses remains challenging. Here, the authors show that a fictive temperature controls an abrupt mechanical toughening transition in metallic glasses, and can explain the scatter in previously reported fracture toughness data.
- Jittisa Ketkaew
- , Wen Chen
- & Jan Schroers
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| Open AccessLocal structure in deeply supercooled liquids exhibits growing lengthscales and dynamical correlations
The glass transition remains an unsolved problem due to the scarcity of particle-resolved data over a large dynamic range. Hallett et al. probe an unprecedented time window and show a strong correlation between local structure and slow dynamics in a deeply supercooled liquid of colloids.
- James E. Hallett
- , Francesco Turci
- & C. Patrick Royall
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| Open AccessSimulations tackle abrupt massive migrations of energetic beam ions in a tokamak plasma
Understanding the occurrence of sudden changes in plasma parameters is important for the operation of magnetically confined fusion devices. Here the authors use simulation to shed light on the formation of abrupt large-amplitude events and the associated redistribution of energetic ions in a tokamak.
- Andreas Bierwage
- , Kouji Shinohara
- & Masatoshi Yagi
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| Open AccessStrongly-coupled quantum critical point in an all-in-all-out antiferromagnet
The critical behavior of a continuous phase transition is determined by both symmetry and dimensionality. Wang et al. present evidence that the cubic all-in-all-out spin order in Cd2Os2O7 leads to a realization of a non-mean-field strongly-coupled quantum phase transition in three dimensions.
- Yishu Wang
- , T. F. Rosenbaum
- & Yejun Feng
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| Open AccessNon-hysteretic first-order phase transition with large latent heat and giant low-field magnetocaloric effect
First order magnetic phase transitions have many practical applications but they often involve structural changes that make it difficult to control energy losses. Guillou et al. show that Eu2In has an isostructural transition with a mechanism distinct from other known magnetoelastic transitions.
- F. Guillou
- , A. K. Pathak
- & V. K. Pecharsky
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| Open AccessCollective magnetism in an artificial 2D XY spin system
Magnetic metamaterials can be designed to provide models of frustrated systems that allow theoretical predictions to be experimentally tested. Here the authors realise a 2D XY model with dipolar interactions and find behaviour consistent with predictions of a low-temperature ordered state.
- Naëmi Leo
- , Stefan Holenstein
- & Laura J. Heyderman
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| Open AccessObservation of nuclear quantum effects and hydrogen bond symmetrisation in high pressure ice
Hydrogen atoms in water ices, under pressures at which they might exist in ocean exoplanets and icy moons, exhibit dynamics that are still poorly understood. Here, 1H-NMR experiments approaching the Mbar range shed light on the symmetrisation of hydrogen bonds preceding and accompanying the transformation of ice VII into ice X.
- Thomas Meier
- , Sylvain Petitgirard
- & Leonid Dubrovinsky
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| Open AccessRole of disordered bipolar complexions on the sulfur embrittlement of nickel general grain boundaries
Sulfur at nickel grain boundaries can cause catastrophic failure, but the mechanisms behind that embrittlement remain poorly understood. Here, the authors image and model bipolar sulfur–nickel structures at amorphous-like and bilayer-like facets of general grain boundaries that cause embrittlement.
- Tao Hu
- , Shengfeng Yang
- & Jian Luo
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| Open AccessA quantitative criterion for determining the order of magnetic phase transitions using the magnetocaloric effect
Magnetocaloric materials often perform best when their magnetic transitions are at the boundary between first- and second-order behavior. Here the authors propose a simple criterion to determine the order of a transition, which may accelerate future magnetocaloric material searches.
- Jia Yan Law
- , Victorino Franco
- & Oliver Gutfleisch
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| Open AccessMetallization and molecular dissociation of dense fluid nitrogen
Nitrogen is a model system still presenting unknown behaviors at the pressures and temperatures typical of deep planets’ interiors. Here the authors explore, by pulsed laser heating in a diamond anvil cell and optical measurements, the metallization and non-molecular states of nitrogen in a previously unexplored domain above 1 Mbar and at 2000-7000K.
- Shuqing Jiang
- , Nicholas Holtgrewe
- & Alexander F. Goncharov
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| Open AccessElectron–electron interactions and the paired-to-nematic quantum phase transition in the second Landau level
Two-dimensional electron systems at half-filled Landau levels can form unusual electronic states such as paired fractional quantum Hall and nematic phases. Here the authors observe the transition between these two phases at filling factors 5/2 and 7/2 and demonstrate the important influence of interactions.
- K. A. Schreiber
- , N. Samkharadze
- & G. A. Csáthy
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| Open AccessNature of the metal-insulator transition in few-unit-cell-thick LaNiO3 films
The electronic behaviour of complex oxides such as LaNiO3 depends on many intrinsic and extrinsic factors, making it challenging to identify microscopic mechanisms. Here the authors demonstrate the influence of oxygen vacancies on the thickness-dependent metal-insulator transition of LaNiO3 films.
- M. Golalikhani
- , Q. Lei
- & X. X. Xi
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| Open AccessQuantum limit transport and destruction of the Weyl nodes in TaAs
Weyl semimetals should exhibit unusual electronic behaviour but conditions where these effects dominate are difficult to achieve. Ramshaw et al. use high magnetic fields to drive TaAs into the quantum limit, finding evidence for the predicted chiral anomaly and an unanticipated increase in resistivity at the highest fields.
- B. J. Ramshaw
- , K. A. Modic
- & R. D. McDonald
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| Open AccessTuning the interplay between nematicity and spin fluctuations in Na1−xLi x FeAs superconductors
Whether the spin, charge and orbital degrees of freedom could drive an iron-based superconductor to the nematic state remains elusive. Here, Baek et al. report the doping-temperature phase diagram of Na1−xLi x FeAs and show a subtle relationship between nematicity and spin fluctuations with respect to doping.
- S.-H. Baek
- , Dilip Bhoi
- & Kee Hoon Kim
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| Open AccessSoft Coulomb gap and asymmetric scaling towards metal-insulator quantum criticality in multilayer MoS2
The interplay between strong interactions and presence of disorder makes atomically thin transition metal dichalcogenides an ideal platform to study phase transitions and critical phenomena. Here, the authors observe asymmetric critical exponents around the metal-insulator-transition of multilayer MoS2.
- Byoung Hee Moon
- , Jung Jun Bae
- & Young Hee Lee
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| Open AccessSimilar temperature scale for valence changes in Kondo lattices with different Kondo temperatures
The competition between interactions promoting magnetic order and those suppressing magnetism causes unusual electronic behaviour in Kondo lattice materials. Here, the authors show the energy scale for valence fluctuations is not controlled by the Kondo scale, contrary to expectations from single-site models.
- K. Kummer
- , C. Geibel
- & D. V. Vyalikh
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Article
| Open AccessUnconventional slowing down of electronic recovery in photoexcited charge-ordered La1/3Sr2/3FeO3
Unusual electronic behavior can emerge in complex oxides due to strong coupling between charge, magnetic and lattice degrees of freedom. Zhu et al. observe separation of electronic and lattice equilibration times in La1/3Sr2/3FeO3 as magnetic interactions make the recovery of charge order much slower than lattice relaxation.
- Yi Zhu
- , Jason Hoffman
- & Haidan Wen
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Article
| Open AccessSpin-lattice decoupling in a triangular-lattice quantum spin liquid
A number of materials have been proposed as realizations of exotic quantum spin liquids but many important properties are difficult to establish. Isono et al. show evidence for spin-lattice decoupling in an organic material, which may help resolve conflicting results about the existence of a spin-excitation gap.
- Takayuki Isono
- , Shiori Sugiura
- & Shinya Uji
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Article
| Open AccessSnap evaporation of droplets on smooth topographies
Droplet evaporation control has applications in inkjet printing and surface patterning. Here, the authors show that on slippery curved substrates droplets evaporate by slowly retracting and then suddenly snapping, which can be exploited to design surfaces that control an evaporation sequence.
- Gary G. Wells
- , Élfego Ruiz-Gutiérrez
- & Rodrigo Ledesma-Aguilar
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Article
| Open AccessMagnetically-driven phase transformation strengthening in high entropy alloys
Medium entropy alloy CoCrNi has better mechanical properties than high entropy alloys such as CrMnFeCoNi, but why that is remains unclear. Here, the authors show that a nanostructured phase at lattice defects in CoCrNi causes its extraordinary properties, while it is magnetically frustrated and suppressed in CrMnFeCoNi.
- Changning Niu
- , Carlyn R. LaRosa
- & Maryam Ghazisaeidi
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Article
| Open AccessEntropy favors heterogeneous structures of networks near the rigidity threshold
The mechanical and thermodynamic properties of amorphous materials are governed by their disordered network at microscales, but the detail remains elusive. Yan shows that the vibrational entropy induces a floppy-rigid phase separation near the rigidity onset and thus favors heterogeneous structures.
- Le Yan
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Article
| Open AccessPhase nucleation through confined spinodal fluctuations at crystal defects evidenced in Fe-Mn alloys
Solid-state phase transitions often involve nucleation of the new phase on defects but a detailed mechanistic understanding has not been established. Here the authors observe spinodal fluctuations at dislocations and grain boundaries in an iron alloy, which may be precursors in a multistep nucleation process.
- A. Kwiatkowski da Silva
- , D. Ponge
- & D. Raabe
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| Open AccessUniaxial strain control of spin-polarization in multicomponent nematic order of BaFe2As2
A fundamental understanding of nematic order is one of the most important issues to explore in the high temperature superconductors. Here, the authors unveil an internal spin structure of the nematic order in BaFe2As2 by using nuclear magnetic resonance under precisely controlled tunable strain.
- T. Kissikov
- , R. Sarkar
- & N. J. Curro
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Article
| Open AccessRotating robots move collectively and self-organize
Active rotating particles were shown to undergo a phase separation through numerical simulations. Here the authors provide an experimental realization of this phenomenon by presenting an ensemble of 3D-printed robots that rotate in different directions and interact with each other.
- Christian Scholz
- , Michael Engel
- & Thorsten Pöschel
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| Open AccessNon-catalytic hydrogenation of VO2 in acid solution
Hydrogenation is an effective way to tune the property of metal oxides. Here, the authors report a simple approach to hydrogenate VO2 in acid solution under ambient conditions by placing a small piece of low workfunction metal on VO2 surface.
- Yuliang Chen
- , Zhaowu Wang
- & Yi Luo
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| Open AccessQuantum phase transitions in highly crystalline two-dimensional superconductors
Superconductor-insulator transitions predominantly occur in highly disordered thin films. Here, Saito et al. report that a quantum metallic state transforms via the quantum Griffiths state to a weakly localized metal at high magnetic fields in a crystalline two-dimensional superconductor.
- Yu Saito
- , Tsutomu Nojima
- & Yoshihiro Iwasa