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| Open AccessScale-invariant magnetic textures in the strongly correlated oxide NdNiO3
The many strongly interacting degrees of freedom in transition metal oxides make it difficult to capture and describe the nature of their metal-insulator transitions. Li et al. show that a resonant magnetic X-ray nanoprobe gives access to local critical behavior that is difficult to detect otherwise.
- Jiarui Li
- , Jonathan Pelliciari
- & Riccardo Comin
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Article
| Open AccessRobust thermoelastic microactuator based on an organic molecular crystal
Molecular crystals that show a reversible shape change by external stimuli are invaluable for the design of actuators but their strong deformations usually lead to their destruction. Here the authors report a fluorenone derivative showing a strong, reversible and instantaneous shear deformation upon heating due to a structural phase transition.
- Yulong Duan
- , Sergey Semin
- & Theo Rasing
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Article
| Open AccessSynthesis of clathrate cerium superhydride CeH9 at 80-100 GPa with atomic hydrogen sublattice
Hydrogen-rich superhydrides are promising high-temperature superconductors which have been observed only at pressures above 170 GPa. Here the authors show that CeH9 can be synthesized at 80-100 GPa with laser heating, and is characterized by a clathrate structure with a dense 3-dimensional atomic hydrogen sublattice.
- Nilesh P. Salke
- , M. Mahdi Davari Esfahani
- & Jung-Fu Lin
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Article
| Open AccessDome patterns in pelagic size spectra reveal strong trophic cascades
An important question in ecology is how much species at higher trophic levels affect lower levels through top-down cascades. Here the authors show through analyses of pelagic size spectra that such cascades are strong in freshwater systems and can also arise in nutrient rich marine systems.
- Axel G. Rossberg
- , Ursula Gaedke
- & Pavel Kratina
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Article
| Open Access3/2 fractional quantum Hall plateau in confined two-dimensional electron gas
Fractional quantum Hall states in 2D electron gases arise due to strong electron-electron interactions, which makes a general theoretical understanding difficult. Fu et al. present data showing the ν = 5/3 quantum Hall state has a 3/2 plateau in the diagonal resistance that has not been captured by existing models.
- Hailong Fu
- , Yijia Wu
- & Xi Lin
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| Open AccessUnifying description of competing orders in two-dimensional quantum magnets
The Dirac spin liquid is a candidate description for the strongly correlated behaviour of some quantum magnets. Song et al. study the symmetry dependence physics of monopole excitations and argue that the lattice-dependent consequences for magnetic ordering may provide a unifying picture for 2D quantum magnetism.
- Xue-Yang Song
- , Chong Wang
- & Yin-Chen He
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Article
| Open AccessVisualization of supercritical water pseudo-boiling at Widom line crossover
Supercritical water exists in gas- and liquid-like forms, but these have not been distinguished yet at the macroscale. Here the authors investigate supercritical water interacting with microporous carbon by neutron imaging, and observe the coexistence of gas- and liquid-like states upon crossing the Widom line.
- Florentina Maxim
- , Cristian Contescu
- & Christian Ludwig
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| Open AccessUnveiling hidden multipolar orders with magnetostriction
Higher-order multipolar phases are unusual states that can form in correlated materials and are difficult to observe as they do not directly couple to conventional probes. Patri et al. theoretically show that angle-dependent magnetostriction measurements can probe quadrupolar and octupolar ordering.
- Adarsh S. Patri
- , Akito Sakai
- & Yong Baek Kim
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Matters Arising
| Open AccessUltrafast evolution and transient phases of a prototype out-of-equilibrium Mott-Hubbard material
- David Moreno-Mencía
- , Alberto Ramos-Álvarez
- & Simon Wall
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Matters Arising
| Open AccessReply to: Ultrafast evolution and transient phases of a prototype out-of-equilibrium Mott-Hubbard material
- D. Boschetto
- , M. Weis
- & M. Zaghrioui
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Article
| Open AccessTuning high-Q nonlinear dynamics in a disordered quantum magnet
The Ising magnet LiHo0.045Y0.955F4 allows experimental probes of disordered quantum dynamics. Silevitch et al. show that strongly-driven localized spin clusters form effectively decoupled two-level systems whose interactions and coherence can be tuned by external ac and dc magnetic fields.
- D. M. Silevitch
- , C. Tang
- & T. F. Rosenbaum
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Article
| Open AccessEquivalence and its invalidation between non-Markovian and Markovian spreading dynamics on complex networks
When modelling epidemic spreading on complex networks, one useful simplification is to assume that the dynamics are Markovian, i.e. memoryless. Here the authors present a more general non-Markovian approach which is able to accurately reproduce the transient and stationary regime on different substrates.
- Mi Feng
- , Shi-Min Cai
- & Ying-Cheng Lai
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Article
| Open AccessDirect atomic insight into the role of dopants in phase-change materials
Quantitative imaging on the doping in phase-change materials for data storage remains scarce. Here, the authors combine electron microscopy, atom probe tomography, and simulations to determine the role of indium and silver dopants during recrystallization.
- Min Zhu
- , Wenxiong Song
- & Richard Dronskowski
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Article
| Open AccessTopological Lifshitz transitions and Fermi arc manipulation in Weyl semimetal NbAs
Surface Fermi arcs (SFAs) are characteristic features of a topological Weyl semimetal but there is no easy way to manipulate them so far. Here, the authors report manipulation of the shape, size and connections of SFAs in a Weyl semimetal NbAs, leading to an unusual topological Lifshitz transition.
- H. F. Yang
- , L. X. Yang
- & Y. L. Chen
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Article
| Open AccessA first-principles phase field method for quantitatively predicting multi-composition phase separation without thermodynamic empirical parameter
Predicting alloy microstructures with parameter-free theoretical schemes remains a challenge. Here the authors derive a general phase field approach to reproduce the microstructural evolution of a nickel-aluminum alloy as a function of composition only and without empirical thermodynamic parameters.
- Swastibrata Bhattacharyya
- , Ryoji Sahara
- & Kaoru Ohno
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| Open AccessDiagonal nematicity in the pseudogap phase of HgBa2CuO4+δ
One of the proposed explanations for the unusual pseudogap behaviour of cuprate superconductors is the formation of an electron nematic phase. Murayama et al. find magnetic anisotropy in the pseudogap regime of HgBa2CuO4+δ, providing evidence for anomalous nematic ordering.
- H. Murayama
- , Y. Sato
- & Y. Matsuda
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Article
| Open AccessEvidence for the weakly coupled electron mechanism in an Anderson-Blount polar metal
A ferroelectric metal is a peculiar state proposed by Anderson and Blunt half a century ago, but is not fully understood. Here, the authors present a time-resolved reflectivity study of LiOsO3 demonstrating evidence for decoupling of itinerant electrons and phonons in the polar transition of the material.
- N. J. Laurita
- , A. Ron
- & D. Hsieh
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Article
| Open AccessCo-emergence of magnetic order and structural fluctuations in magnetite
The Verwey transition in magnetite was reported 80 years ago but identifying the underlying mechanism has been difficult. Here the authors show that structural distortions associated with the Verwey transition emerge as local fluctuations at the Curie temperature, confirming their link with magnetic order.
- Giuditta Perversi
- , Elise Pachoud
- & J. Paul Attfield
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Article
| Open AccessIntertwined topological phases induced by emergent symmetry protection
The still-developing understanding of topologically non-trivial phases of matter has led to new mechanisms for unconventional many-body behaviour. Here the authors present a model where the symmetry needed for a symmetry-protected topological phase only emerges after the formation of long-range order.
- Daniel González-Cuadra
- , Alejandro Bermudez
- & Alexandre Dauphin
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| Open AccessSuperconductivity from the condensation of topological defects in a quantum spin-Hall insulator
Deconfined quantum critical points separate two phases with different broken symmetries, which puts them beyond the standard Landau theory of phase transitions. Here the authors present a model with a monopole-free deconfined quantum critical point, making it more amenable to detailed numerical studies.
- Yuhai Liu
- , Zhenjiu Wang
- & Fakher F. Assaad
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| Open AccessCritical spin liquid versus valence-bond glass in a triangular-lattice organic antiferromagnet
The low temperature magnetic properties of organic Mott insulator κ-(ET)2-Cu2(CN)3 a quantum spin liquid candidate is notoriously difficult to understand. Here, a model based on defect spins is introduced that allows to describe results of complementary experiments on the same theoretical footing.
- Kira Riedl
- , Roser Valentí
- & Stephen M. Winter
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Article
| Open AccessTheory of the field-revealed Kitaev spin liquid
α-RuCl3 is a candidate material for studying Kitaev physics but a microscopic theory consistent with experiments has not yet been established. Here the authors present a theory with an intermediate-field spin liquid phase that can explain recent results indicating anyonic behaviour.
- Jacob S. Gordon
- , Andrei Catuneanu
- & Hae-Young Kee
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| Open AccessPhase transition in the cuprates from a magnetic-field-free stiffness meter viewpoint
Precise measurements of the superconducting stiffness tensor can give detailed insights into the superconductor-normal phase transition. Kapon et al. introduce the Stiffnessometer approach for sensitive magnetic-field-free measurements and find two transition temperatures in LSCO rings.
- Itzik Kapon
- , Zaher Salman
- & Amit Keren
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Article
| Open AccessEmergent bound states and impurity pairs in chemically doped Shastry-Sutherland system
Exploring the impurity-induced phenomena facilitates the understanding of emergent quantum materials. Here the authors show the anomalous magnetization transitions as well as demonstrate the relation between the impurities and the excited spin states in the Mg doped Shastry-Sutherland compound SrCu2(BO3)2.
- Zhenzhong Shi
- , William Steinhardt
- & Sara Haravifard
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Article
| Open AccessDirect observation of picosecond melting and disintegration of metallic nanoparticles
Laser-matter interaction has been intensively studied in equilibrium states, but irreversible processes in a highly nonequilibrium state at nanoscales remains elusive due to experimental challenges. Here, Ihm et al. image heterogeneous melting of gold nanoparticles with nanometer and picosecond resolution.
- Yungok Ihm
- , Do Hyung Cho
- & Changyong Song
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Article
| Open AccessThe Kibble-Zurek mechanism at exceptional points
Universal non-equilibrium behaviour can emerge in physical systems when they are driven through a parameter regime where their energy gap closes. Dóra et al. show that the Kibble-Zurek scaling associated with exceptional points in non-Hermitian systems is distinct from the conventional Hermitian result.
- Balázs Dóra
- , Markus Heyl
- & Roderich Moessner
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Article
| Open AccessScaling of domain cascades in stripe and skyrmion phases
Switching of magnetic materials often occurs through discrete random avalanches. Singh et al. observe sharply reduced avalanches in the topologically protected skyrmion phase of a Fe/Gd heterostructure and obtain different critical behaviour in the stripe and skyrmion phases, suggesting distinct universality classes.
- A. Singh
- , J. C. T Lee
- & S. Roy
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Article
| Open AccessConcomitant opening of a bulk-gap with an emerging possible Majorana zero mode
A quantized zero-bias conductance peak (ZBCP) is potentially a signature of Majorana edge mode provided that a topological gap opens in the bulk. Here, Grivnin et al. observe ZBCP at the edge both with and without a superconducting bulk-gap in an InAs nanowire coated with epitaxial Al.
- Anna Grivnin
- , Ella Bor
- & Hadas Shtrikman
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Article
| Open AccessUltrafast nematic-orbital excitation in FeSe
Several experiments have shown evidence for unusual nematic electronic behaviour in unconventional superconductors. Here the authors use pump-probe spectroscopy to observe out-of-equilibrium behaviour of coupled nematic-orbital excitations in iron selenide.
- T. Shimojima
- , Y. Suzuki
- & K. Ishizaka
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Article
| Open AccessRoom temperature electrofreezing of water yields a missing dense ice phase in the phase diagram
Water can crystallize in different ice polymorphs according to temperature and pressure conditions. Here the authors predict by molecular dynamics simulations a new ice phase spontaneously forming at room temperature under high pressure and high electric field.
- Weiduo Zhu
- , Yingying Huang
- & Xiao Cheng Zeng
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Article
| Open AccessModel states for a class of chiral topological order interfaces
Interfaces between topologically distinct phases are often described by effective field theories. Here, Crépel et al. propose a family of model wave functions based on matrix product states which not only unveils the universal properties of the whole system but also unprecedented captures low energy physics.
- V. Crépel
- , N. Claussen
- & N. Regnault
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| Open AccessMicroscopic study of the Halperin–Laughlin interface through matrix product states
Interfaces between topologically distinct phases reveal rich phenomenology. Here, Crépel et al. present a microscopic study on the low energy physics, interface gapless mode, identification of spin and charge excitations, etc. of the Halperin–Laughlin interface using recently proposed model wavefunctions.
- V. Crépel
- , N. Claussen
- & B. Estienne
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Article
| Open AccessColossal barocaloric effects near room temperature in plastic crystals of neopentylglycol
There is great interest, in refrigeration technology, in replacing harmful volatile hydrofluorocarbons with solid materials. Here the authors show that commercially available plastic crystal neopentylglycol displays colossal and reversible barocaloric effects comparable with those exploited in hydrofluorocarbons, which make it suitable for application.
- P. Lloveras
- , A. Aznar
- & J.-Ll. Tamarit
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Article
| Open AccessSpin-current-mediated rapid magnon localisation and coalescence after ultrafast optical pumping of ferrimagnetic alloys
The understanding of the magnetisation evolution upon femtosecond optical pumping remains elusive. The authors perform resonant X-ray magnetic scattering measurements and multiscale simulations that reveal rapid magnetic order recovery in ferrimagnets via nonlinear magnon processes.
- E. Iacocca
- , T.-M. Liu
- & H. A. Dürr
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| Open AccessDimensional crossover in a layered ferromagnet detected by spin correlation driven distortions
Exploring lattice distortions from magnetic short-range ordering (SRO) facilitates the understanding of magnetic long-range ordering (LRO). Here the authors apply high-multipole nonlinear optical polarimetry to track SRO induced distortions in CrSiTe3, showing that LRO is established via a crossover from two- to three-dimensional SRO.
- A. Ron
- , E. Zoghlin
- & D. Hsieh
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Article
| Open AccessZero-temperature glass transition in two dimensions
Identifying the nature of the glass transition is challenging because relevant experiments or analytical descriptions are hard to achieve. Here, Berthier et al. develop a Monte Carlo numerical tool to investigate two-dimensional glasses and find a zero-temperature thermodynamic glass transition.
- Ludovic Berthier
- , Patrick Charbonneau
- & Sho Yaida
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| Open AccessA series of magnon crystals appearing under ultrahigh magnetic fields in a kagomé antiferromagnet
In many quantum magnets, an applied magnetic field competes with the expected zero-field state, leading to complex magnetic behavior. Okuma et al. observe the formation of quantum magnetization plateaus in a kagomé antiferromagnet and argue they form due to the crystallization of magnon excitations.
- R. Okuma
- , D. Nakamura
- & Z. Hiroi
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Article
| Open AccessPhase transitions in few-monolayer spin ice films
Magnetic spin ice compounds are described by vertex models, which have been intensively studied for their exotic properties. Bovo et al. show thin films of Dy2Ti2O7 have structures distinct from bulk crystals and come close to realising the two-dimensional F-model, which has an unusual ordering transition in the Berezinskii–Kosterlitz–Thouless class.
- L. Bovo
- , C. M. Rouleau
- & S. T. Bramwell
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Article
| Open AccessOvercoming the thermal regime for the electric-field driven Mott transition in vanadium sesquioxide
Thermal effects limit the speed of the electrically driven insulator-metal transition in V2O3 to tens of picoseconds. Here the authors show that under an intense THz-electric-field excitation the thermal regime can be overcome, achieving a purely electronic transition on ultrafast timescales.
- Flavio Giorgianni
- , Joe Sakai
- & Stefano Lupi
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Article
| Open AccessBand gap closure, incommensurability and molecular dissociation of dense chlorine
Molecular systems are predicted to transform into atomic solids and be metallic at high pressure; this was observed for the diatomic elements iodine and bromine. Here the authors access the higher pressures needed to observe the dissociation in chlorine, through an incommensurate phase, and provide evidence for metallization.
- Philip Dalladay-Simpson
- , Jack Binns
- & Ross T. Howie
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Article
| Open AccessPressure-tuning the quantum spin Hamiltonian of the triangular lattice antiferromagnet Cs2CuCl4
Theoretical studies of quantum magnetism typically assume idealised lattices with freely tunable parameters, which are difficult to realise experimentally. Zvyagin et al. perform challenging measurements at high pressures to tune and to accurately monitor the exchange parameters of a triangular lattice antiferromagnet.
- S. A. Zvyagin
- , D. Graf
- & H. Tanaka
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Article
| Open AccessDivalent EuRh2Si2 as a reference for the Luttinger theorem and antiferromagnetism in trivalent heavy-fermion YbRh2Si2
Heavy-fermion materials have unusual electronic behavior due to a dual localized-itinerant character of 4f electrons. Here, by studying divalent EuRh2Si2, the authors gain insight into the electronic states of the trivalent heavy fermion system YbRh2Si2 and show that it experimentally demonstrates Luttinger’s theorem.
- M. Güttler
- , A. Generalov
- & D. V. Vyalikh
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Article
| Open AccessEnhanced superconductivity close to a non-magnetic quantum critical point in electron-doped strontium titanate
Among its interesting properties, SrTiO3 can show both superconductivity and ferroelectric quantum criticality at low temperatures. Tomioka et al. use La and oxygen-isotope doping to tune electron-doped SrTiO3 to the critical region and observe enhanced superconductivity, suggesting a link between them.
- Yasuhide Tomioka
- , Naoki Shirakawa
- & Isao H. Inoue
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Article
| Open AccessRevealing the role of lattice distortions in the hydrogen-induced metal-insulator transition of SmNiO3
Proton doping can induce metal-insulator transitions in rare-earth nickelates, demonstrating the complex interplay between dopants and electronic degrees of freedom. Chen et al. use results on strained films to argue that local proton-induced lattice distortions strongly influence the transition.
- Jikun Chen
- , Wei Mao
- & Yong Jiang
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Article
| Open AccessRole of defects in determining the magnetic ground state of ytterbium titanate
Exploring the role of structural defect is essential to understand the exotic quantum spin phenoma in rare earth pyrochlores. Here the authors show oxygen vacancies can stabilise the spin liquid phase and reveal the ferromagnetic ground state when oxygen vacancies are eliminated in Yb2Ti2O7.
- D. F. Bowman
- , E. Cemal
- & J. P. Goff
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Article
| Open AccessHigh temperature singlet-based magnetism from Hund’s rule correlations
Electrons in uranium-based materials are often on the border between localised and itinerant behaviour, which can lead to unusual magnetic behaviour. Here the authors combine experiment and theory to show that USb2 may be an unusually high temperature example of a singlet-ground-state magnet.
- Lin Miao
- , Rourav Basak
- & L. Andrew Wray
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| Open AccessReconstructing the quantum critical fan of strongly correlated systems using quantum correlations
At a zero-temperature phase transition, quantum, rather than thermal, fluctuations determine the behaviour both at the transition and in a finite temperature ‘quantum critical’ region. Here the authors give a quantitative definition of the quantum critical region that could be applied to experimental data.
- Irénée Frérot
- & Tommaso Roscilde
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| Open AccessEmergence of a field-driven U(1) spin liquid in the Kitaev honeycomb model
The Kitaev model is intensively studied as an exactly-solvable starting point for theoretical studies of quantum spin liquid states. Hickey and Trebst show that magnetic fields can destabilize the well-known gapped Kitaev spin liquid and induce a new gapless spin liquid, with a distinct gauge structure and neutral Fermi surface.
- Ciarán Hickey
- & Simon Trebst
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| Open AccessLithium intercalation into bilayer graphene
The mechanism of lithium storage in graphenic carbon remains a fundamental question to be addressed. Here the authors employ suitable bilayer graphene foam to investigate various physiochemical phenomena of lithium intercalation and propose a storage model.
- Kemeng Ji
- , Jiuhui Han
- & Yutaka Oyama