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| Open AccessGiant optomechanical spring effect in plasmonic nano- and picocavities probed by surface-enhanced Raman scattering
Extreme confinement of light in plasmonic nanocavities strongly enhances the optomechanical coupling of light with molecular vibrations. Here, the authors use a giant optical spring effect to reversibly weaken molecular bonds.
- Lukas A. Jakob
- , William M. Deacon
- & Jeremy J. Baumberg
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| Open AccessEye accommodation-inspired neuro-metasurface focusing
Here the authors propose for the first time the concept of supervised-evolving learning (SEL) and a corresponding SEL-driven adaptive focusing (SELAF) system. This metasurface can adaptively realize focusing at any specified position for waves incident from any direction. This work demonstrates unprecedented potential for tasks involving real-time, fast and complex electromagnetic wave manipulation.
- Huan Lu
- , Jiwei Zhao
- & Hongsheng Chen
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| Open AccessDrug screening at single-organoid resolution via bioprinting and interferometry
Traditional 2D cell culture platforms do not accurately reflect the physiology of human tumors. Here, authors combine bioprinting and high-speed live cell interferometry with machine learning to measure drug sensitivity at single-organoid resolution in a label-free manner.
- Peyton J. Tebon
- , Bowen Wang
- & Alice Soragni
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Article
| Open AccessCharacterization of diffusing sub-10 nm nano-objects using single anti-resonant element optical fibers
Characterizing diffusing species is increasingly important for revealing nanoscale processes. Here, the authors uncover the potential of fiber-assisted nanoparticle tracking analysis by characterizing nanoparticles as small as 9 nm at record precision levels, reaching fundamental limits.
- Torsten Wieduwilt
- , Ronny Förster
- & Markus A. Schmidt
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| Open AccessPoint singularity array with metasurfaces
Optical singularities are typically 1D structures like vortices. This study used metasurfaces to position ten identical point singularities with tight confinement. This could miniaturize optical systems for super-resolution microscopy and dark traps.
- Soon Wei Daniel Lim
- , Joon-Suh Park
- & Federico Capasso
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| Open AccessParallel interrogation of the chalcogenide-based micro-ring sensor array for photoacoustic tomography
The authors report a highly sensitive chalcogenide-based micro-ring sensor array for photoacoustic tomography and develops a compatible parallel interrogation means by synthesizing a digital optical frequency comb. Imaging is demonstrated on fast-moving objects, leaf veins, and live zebrafish.
- Jingshun Pan
- , Qiang Li
- & Zhaohui Li
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Article
| Open AccessNanowire-based smart windows combining electro- and thermochromics for dynamic regulation of solar radiation
Smart windows offer more efficient sunlight modulation and heat management. Here, the authors propose a co-assembly strategy to produce smart windows that combine electrochromic and thermochromic functions with tunable components and ordered structures for dynamic solar radiation regulation.
- Si-Zhe Sheng
- , Jin-Long Wang
- & Shu-Hong Yu
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Article
| Open AccessNon-line-of-sight imaging with arbitrary illumination and detection pattern
The authors propose a confocal complemented signal-object collaborative regularization method for non-line-of-sight (NLOS) imaging without specific requirements on the spatial pattern of measurement points. The method extends the application range of NLOS imaging.
- Xintong Liu
- , Jianyu Wang
- & Lingyun Qiu
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| Open AccessUnique Huygens-Fresnel electromagnetic transportation of chiral Dirac wavelet in topological photonic crystal
Huygens-Fresnel features are useful for harnessing light in unique ways. Here the authors demonstrate a chiral light source that induces globally a counter energy flow in a topological photonics structure with Dirac-type frequency dispersion.
- Xing-Xiang Wang
- , Zhiwei Guo
- & Xiao Hu
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Article
| Open AccessTopological quadratic-node semimetal in a photonic microring lattice
Topological semimetals can host coexisting higher-order topological nodes that may enable unique physical properties. Here, based on these topological principles, authors design and experimentally realise simultaneous massive and massless chiral quasiparticles in a photonic microring lattice.
- Zihe Gao
- , Haoqi Zhao
- & Liang Feng
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Article
| Open AccessCASPI: collaborative photon processing for active single-photon imaging
The sparse, noisy, and distorted raw photon data captured by single-photon cameras make it difficult to estimate scene properties under challenging illumination conditions. Here, the authors present Collaborative photon processing for Active Single-Photon Imaging (CASPI), a technology-agnostic, application-agnostic, and training-free photon processing pipeline for high-resolution single-photon cameras.
- Jongho Lee
- , Atul Ingle
- & Mohit Gupta
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Article
| Open AccessHybrid achromatic microlenses with high numerical apertures and focusing efficiencies across the visible
Creating compact, lightweight and powerful optics that work well under visible light has been challenging. Here, the authors 3D print optically transparent polymers inside nanoporous glass in order to densely integrate refractive and diffractive elements, forming thin, high-performance hybrid achromatic imaging micro-optics.
- Corey A. Richards
- , Christian R. Ocier
- & Paul V. Braun
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| Open AccessUnraveling chirality transfer mechanism by structural isomer-derived hydrogen bonding interaction in 2D chiral perovskite
Chiral Ruddlesden-Popper perovskites are of interest as they exhibit circular dichroism in the visible light region. Here authors demonstrate the effect of asymmetric hydrogen bonding on the spin-polarization-based phenomena in chiral 2D perovskites by using structural isomer organic spacers.
- Jaehyun Son
- , Sunihl Ma
- & Jooho Moon
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Article
| Open AccessPhotonic integrated beam delivery for a rubidium 3D magneto-optical trap
Ultracold atoms are generated in the lab using optical trapping and cooling. Here the authors implement a fiber-coupled photonic integrated circuit for a beam delivery to a three-dimensional magneto-optical trap where greater than 1 million rubidium atoms are cooled near 200 μK.
- Andrei Isichenko
- , Nitesh Chauhan
- & Daniel J. Blumenthal
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| Open AccessA biodegradable, flexible photonic patch for in vivo phototherapy
Illuminating internal organs and tissues with high controllability and adaptability remains challenging. Here the authors present a flexible, biodegradable photonic device called iCarP for large area, high intensity, wide spectrum, deeply penetrating, continuous or pulsatile illumination.
- Kaicheng Deng
- , Yao Tang
- & Yang Zhu
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| Open AccessDeep learning enables satellite-based monitoring of large populations of terrestrial mammals across heterogeneous landscape
This study presents a deep learning pipeline to automatically locate and count large herds of migratory ungulates (wildebeest and zebra) in the Serengeti-Mara ecosystem using fine resolution satellite imagery. The results achieve accurate detection of nearly 500,000 individuals across thousands of square kilometers and multiple habitat types.
- Zijing Wu
- , Ce Zhang
- & Tiejun Wang
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| Open AccessPhoto-triggered full-color circularly polarized luminescence based on photonic capsules for multilevel information encryption
Phototunable full-color circularly polarized luminescence (CPL) features large storage density which is important for the field of information encryption and decryption. Here, the authors present a device-friendly solid film with color-tunability by employing Förster resonance energy transfer among a chiral donor and achiral molecular switches in a liquid crystal photonic capsules.
- Siyang Lin
- , Yuqi Tang
- & Quan Li
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| Open AccessCompact optical convolution processing unit based on multimode interference
In most optical computing schemes, the size of the chip increases quadratically with the problem size. Here, the authors demonstrate an architecture for optical convolutional neural networks which, while losing the independent reconfigurability of the kernels, allows for linear scaling of the circuit size.
- Xiangyan Meng
- , Guojie Zhang
- & Ming Li
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Article
| Open AccessImaging quantized vortex rings in superfluid helium to evaluate quantum dissipation
Quantum vortices exist in superfluid and play important role in superfluid characteristics. Here the authors determine quantum dissipation caused by mutual friction in superfluid by filming the motion of quantized vortex rings in superfluid helium.
- Yuan Tang
- , Wei Guo
- & Toshiaki Kanai
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| Open AccessIntramolecular charge transfer enables highly-efficient X-ray luminescence in cluster scintillators
X-ray luminescence efficiency of copper halide clusters is limited by nonradiative charge transfer. Here, Zhang et al. report highly emissive radioluminescence of Cu4I4 cubes by functionalizing biphosphine ligands with acridine, unlocking the potential use as low-cost and eco-friendly scintillators.
- Nan Zhang
- , Lei Qu
- & Hui Xu
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| Open AccessIn-memory photonic dot-product engine with electrically programmable weight banks
Hybrid photonic–electronic systems are essential for high-throughput neuromorphic computing. Here, the authors report an in-memory photonic–electronic dot-product engine with decoupled electronic programming of the phase-change memory cells and parallel photonic computation with high-bit operation, low energy consumption, and high accuracy.
- Wen Zhou
- , Bowei Dong
- & Harish Bhaskaran
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| Open AccessObservation of directional leaky polaritons at anisotropic crystal interfaces
A new form of directional polaritons, leaky in nature and featuring lenticular dispersion contours, is experimentally observed both in near-field and through prism excitation, unveiling opportunities stemming from the interplay of extreme anisotropic responses, light confinement and directional radiation leakage.
- Xiang Ni
- , Giulia Carini
- & Andrea Alù
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| Open AccessSingle-frame deep-learning super-resolution microscopy for intracellular dynamics imaging
Multi-frame super-resolution microscopy is hampered by long acquisition times and phototoxicity, which hinder its use for live-cell imaging. Here, authors propose a deep-learning-based single-frame super-resolution approach to image cellular dynamics with high spatiotemporal resolution.
- Rong Chen
- , Xiao Tang
- & Shuhuai Yao
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Article
| Open AccessMeasurement-induced collective vibrational quantum coherence under spontaneous Raman scattering in a liquid
Spontaneous Raman scattering is classically understood as an incoherent process. Here, the authors demonstrate that macroscopic quantum coherence among billions of vibrating molecules in a liquid is generated when single photon detection and single spatio-temporal mode excitation are implemented.
- Valeria Vento
- , Santiago Tarrago Velez
- & Christophe Galland
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| Open AccessSelf-wavelength shifting in two-dimensional perovskite for sensitive and fast gamma-ray detection
Efficient light extraction in perovskite X/γ-ray scintillators is hindered by the small Stokes shift of exciton luminescence. Here, Jin et al. exploit the intrinsic strain in 2D perovskite as “self-wavelength shifting” to reduce the self-absorption effect without sacrificing the device response speed.
- Tong Jin
- , Zheng Liu
- & Guangda Niu
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Article
| Open AccessBrillouin zone folding driven bound states in the continuum
Periodic perturbations and guided mode engineering into Brillouin zone folding-induced bound states in the continuum resulted in ultrahigh Q factors that are both robust and sustainable across a broad range of tunable momentum space.
- Wenhao Wang
- , Yogesh Kumar Srivastava
- & Ranjan Singh
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Article
| Open AccessTwo-colour dissipative solitons and breathers in microresonator second-harmonic generation
Boosting conversion efficiency, coherence and spectral bandwidth of optical signals generated in integrated photonic devices is an important current challenge. Here, the authors present their observations of two-colour dissipative solitons, breathers and frequency combs resulting from second-harmonic generation in lithium-niobate ring microresonators.
- Juanjuan Lu
- , Danila N. Puzyrev
- & Hong X. Tang
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Article
| Open Access3D-patterned inverse-designed mid-infrared metaoptics
The authors show computationally optimized, multilayer scattering structures in the mid-infrared for high efficiency imaging. Multispectral and polarization sorting devices are fabricated via two-photon lithography and characterized optically.
- Gregory Roberts
- , Conner Ballew
- & Andrei Faraon
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Article
| Open AccessComputational study on the catalytic control of endo/exo Diels-Alder reactions by cavity quantum vacuum fluctuations
Strong light-matter interactions are a pathway to chemical control at the molecular level. Here, authors theoretically show that an optical cavity allows to control catalysis, inhibition, and endo/exo stereoselectivity in Diels-Alder reactions.
- Fabijan Pavošević
- , Robert L. Smith
- & Angel Rubio
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| Open AccessEmission enhancement of erbium in a reverse nanofocusing waveguide
Emission enhancement and extraction from quantum emitters is a major challenge for photon sources in e.g. quantum photonic networks. Here the authors propose a broadband waveguide platform which allows to boost, extract, and guide quantum emission within integrated photonic networks.
- Nicholas A. Güsken
- , Ming Fu
- & Rupert F. Oulton
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Article
| Open AccessIn-plane hyperbolic polariton tuners in terahertz and long-wave infrared regimes
In-plane hyperbolic phonon polaritons in α-MoO3 crystals hold promise for terahertz (THz) and longwave infrared (LWIR) photonic applications, but their coupling with far-field excitations remains challenging. Here, the authors report the fabrication of α-MoO3 ribbon arrays that can be applied as tunable THz and LWIR filters and polarizers.
- Wuchao Huang
- , Thomas G. Folland
- & Shaozhi Deng
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Article
| Open AccessDirect nano-imaging of light-matter interactions in nanoscale excitonic emitters
Authors investigate quasi-2D nanoscale emitters on different substrates with tapping mode tip-enhanced spectroscopy. They visualize in-plane near-field and radiative energy propagation via Surface plasmon polaritons launched by the nanoscale emitters on dielectric/Au or SiO2/Si substrates.
- Kiyoung Jo
- , Emanuele Marino
- & Deep Jariwala
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| Open AccessMicrocantilever-integrated photonic circuits for broadband laser beam scanning
This work presents ultracompact and low-power laser beam scanners using microcantilevers embedded with nanophotonic circuits. These chip-scale devices are made in a semiconductor foundry and project visible light patterns in one or two dimensions.
- Saeed Sharif Azadeh
- , Jason C. C. Mak
- & Joyce K. S. Poon
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Article
| Open AccessA sensory memory processing system with multi-wavelength synaptic-polychromatic light emission for multi-modal information recognition
Multimodal cognitive computing task is an important research content in the field of AI. Here, the authors propose an efficient sensory memory processing system, which can process sensory information and generate synapse-like and multiwavelength light-emitting output for efficient multimodal information recognition.
- Liuting Shan
- , Qizhen Chen
- & Huipeng Chen
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| Open AccessStructured transverse orbital angular momentum probed by a levitated optomechanical sensor
A new polarization structure of light is synthesized in a straightforward and robust way. The light field is probed using a levitated nanoparticle as a sensor. Optical angular momentum is used to control the particle in a novel way, with applications in sensing and quantum optomechanics.
- Yanhui Hu
- , Jack J. Kingsley-Smith
- & James Millen
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| Open AccessSingle-pulse terahertz spectroscopy monitoring sub-millisecond time dynamics at a rate of 50 kHz
Single-pulse THz spectroscopy at 50 kHz is performed with a table-top system to extract rapid changes of a material’s complex dielectric function. This technique is demonstrated by monitoring carrier accumulation and relaxation dynamics in silicon.
- Nicolas Couture
- , Wei Cui
- & Jean-Michel Ménard
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| Open AccessStrong second-harmonic generation by sublattice polarization in non-uniformly strained monolayer graphene
Nanostructured platforms for efficient nonlinear optics are the building block of next generation integrated photonic devices. Here the authors provide a straightforward method to engineer the lattice symmetry of monolayer graphene, boosting the SHG signal at low temperature.
- Kunze Lu
- , Manlin Luo
- & Donguk Nam
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| Open AccessDispersion-engineered metasurfaces reaching broadband 90% relative diffraction efficiency
Authors demonstrate a dispersion engineered set of eight nanostructures capable of providing 0 to 2π full-phase coverage. Their design offers a broadband and polarization-insensitive 90% relative diffraction efficiency from 450 nm to 700 nm in wavelength.
- Wei Ting Chen
- , Joon-Suh Park
- & Federico Capasso
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Article
| Open AccessMid-infrared analogue polaritonic reversed Cherenkov radiation in natural anisotropic crystals
Here, the authors demonstrate an analogue reversed Cherenkov radiation at mid-infrared frequencies in MoO3, a natural hyperbolic material, and show that the radiation angle and the quality factor can be increased by stacking hBN layers on the MoO3 surface.
- Xiangdong Guo
- , Chenchen Wu
- & Qing Dai
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Article
| Open AccessOptical neural network via loose neuron array and functional learning
Here the authors have realized a programmable incoherent optical neural network that delivers light-speed, high-bandwidth, and power-efficient neural network inference via processing parallel visible light signals in the free space.
- Yuchi Huo
- , Hujun Bao
- & Sung-Eui Yoon
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Article
| Open AccessTriboelectric-induced ion mobility for artificial intelligence-enhanced mid-infrared gas spectroscopy
Isopropyl alcohol can play a significant role in anti-virus diagnosis but generally yields limited response in conventional detection. Here, authors propose a methodology of AI-enhanced ion mobility and mid-infrared spectroscopy for accurate gas identification despite presence different carbon-based gases.
- Jianxiong Zhu
- , Shanling Ji
- & Chengkuo Lee
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Article
| Open AccessMultimodal dynamic and unclonable anti-counterfeiting using robust diamond microparticles on heterogeneous substrate
Practical anticounterfeiting labels should possess both high-capacity and robustness, and should allow easy fabrication and readout. Here, the authors show how to heterogeneously grow robust and stable chaotic pattern of diamond microparticles - containing SiV defects - on silicon substrates.
- Tongtong Zhang
- , Lingzhi Wang
- & Zhiqin Chu
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Article
| Open AccessTwo-dimensional semiconducting SnP2Se6 with giant second-harmonic-generation for monolithic on-chip electronic-photonic integration
2D semiconductors with nonlinear optical properties hold promise for multifunction integration in electronic-photonic integrated circuits. Here, the authors report the synthesis of 2D SnP2Se6 and its integration with a SiN photonic platform, showing strong odd-even layer-independent second harmonic generation activity at 1550 nm and broadband photoresponse.
- Cheng-Yi Zhu
- , Zimeng Zhang
- & Cheng-Yan Xu
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Article
| Open AccessA sensitive high repetition rate arrival time monitor for X-ray free electron lasers
In time-resolved measurements it is crucial to know the time delay between the exciting and probing light pulses. Here the authors demonstrate a self-referencing common-path interferometer method measuring the arrival time between the X-ray free electron laser and the optical pulse to the target and thus their inherent timing jitter.
- Michael Diez
- , Henning Kirchberg
- & Christian Bressler
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Article
| Open AccessZero-field quantum beats and spin decoherence mechanisms in CsPbBr3 perovskite nanocrystals
Lead halide perovskites host bright triplet excitons which have applications in optospintronic devices. Here the authors observe quantum coherence between exciton sublevels without magnetic field and clarify the mechanisms of exciton spin relaxation in ensembles of CsPbBr3 nanocrystals.
- Rui Cai
- , Indrajit Wadgaonkar
- & Tze Chien Sum
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Article
| Open AccessQuantum microscopy of cells at the Heisenberg limit
The authors present a method for super-resolution quantum microscopy at the Heisenberg limit by using pairs of entangled photons with balanced pathlengths. They improve the spatial resolution, imaging speed, and contrast-to-noise ratio in practice while providing a theoretical interpretation of the super-resolution feature.
- Zhe He
- , Yide Zhang
- & Lihong V. Wang
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| Open AccessUncovering temperature-dependent exciton-polariton relaxation mechanisms in hybrid organic-inorganic perovskites
Exciton-polaritons present opportunities for quantum photonics, next generation qubits, and tuning material photophysics. Here Laitz et al. study the temperature dependence of 2D perovskite microcavity polaritons, revealing material-specific relaxation mechanisms towards the control of polariton momentum.
- Madeleine Laitz
- , Alexander E. K. Kaplan
- & Vladimir Bulović
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Article
| Open AccessHigh-efficiency and stable short-delayed fluorescence emitters with hybrid long- and short-range charge-transfer excitations
To possess a small singlet-triplet energy gap and a large oscillator strength simultaneously is critical for efficient thermally activated delayed fluorescent emitters. Here, the authors attach an multiresonance-acceptor onto a sterically-uncrowded donor for realizing a device efficiency of 40.4%.
- Guoyun Meng
- , Hengyi Dai
- & Lian Duan
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Article
| Open AccessIndividually addressable and spectrally programmable artificial atoms in silicon photonics
Realising integrated photonic circuits containing isolated telecommunications-wavelength artificial atom single photon emitters is an outstanding challenge in quantum technologies. Here, the authors demonstrate how to embed optically tunable G-centers in silicon-on-insulator integrated circuits.
- Mihika Prabhu
- , Carlos Errando-Herranz
- & Dirk Englund