Featured
-
-
Article |
High-resolution optical spectroscopy using multimode interference in a compact tapered fibre
While desirable for compact solutions, the miniaturization of spectrometers comes at the cost of spectral resolution and operating range. Here, Wanet al. propose a tapered fibre multimode interference spectrometer exhibiting high spectral resolution from the visible to the near infrared in a compact configuration.
- Noel H. Wan
- , Fan Meng
- & Dirk Englund
-
Article
| Open AccessQuantitative X-ray phase-contrast microtomography from a compact laser-driven betatron source
With excellent resolving power and tissue contrast, X-ray phase-contrast imaging holds great promise but the source requirements have limited its use. Here, Wenz et al. show a phase-contrast microtomogram of a biological sample using X-ray radiation driven by a high-power laser.
- J. Wenz
- , S. Schleede
- & S. Karsch
-
Article
| Open AccessHighly indistinguishable photons from deterministic quantum-dot microlenses utilizing three-dimensional in situ electron-beam lithography
Single indistinguishable photon sources with high flux rates and purity are needed in quantum communications. Here, Gschreyet al. use three-dimensional electron-beam lithography to pattern deterministic quantum-dot microlenses and demonstrate enhanced photon-extraction efficiency and photon indistinguishability.
- M. Gschrey
- , A. Thoma
- & S. Reitzenstein
-
Article
| Open AccessImaging an aligned polyatomic molecule with laser-induced electron diffraction
Laser-induced electron diffraction can provide structural information on gas-phase molecules with high spatial and temporal resolution. Going beyond previous diatomic cases, Pullen et al.apply this approach to acetylene and show that it can be used to measure bond lengths for polyatomic molecules.
- Michael G. Pullen
- , Benjamin Wolter
- & Jens Biegert
-
Article |
Temporal tweezing of light through the trapping and manipulation of temporal cavity solitons
Optical tweezing typically refers to the trapping and manipulation of particles using lasers. Here, Jang et al. demonstrate analogous manipulation of ultrashort cavity soliton-pulses in the time domain, trapped by the phase modulation of a continuous wave laser beam, and moved by modifying the phase profile.
- Jae K. Jang
- , Miro Erkintalo
- & Stuart G. Murdoch
-
Article
| Open AccessSpatial and temporal imaging of long-range charge transport in perovskite thin films by ultrafast microscopy
Determining the mechanism of charge carrier transport in solar cells is important for their development towards higher efficiencies. Here, the authors elucidate the spatial and temporal diffusion of charge carriers in hybrid perovskite thin films through ultrafast transient absorption microscopy.
- Zhi Guo
- , Joseph S. Manser
- & Libai Huang
-
Article
| Open AccessControlling dispersion forces between small particles with artificially created random light fields
Natural dispersion forces acting between molecules and particles arise from electromagnetic fields generated by quantum and thermal fluctuations. Here, Brügger et al.show that isotropic dispersion forces between colloidal particles can be induced, controlled and tuned with artificial, fluctuating laser light fields.
- Georges Brügger
- , Luis S. Froufe-Pérez
- & Juan José Sáenz
-
Article
| Open AccessSTED nanoscopy with fluorescent quantum dots
STED nanoscopy enables sub-diffraction imaging with a wide range of fluorescent probes. Here, the authors show that a bright and very photostable class of fluorescent quantum dots can be super-resolved with STED as biolabels in cellular contexts.
- Janina Hanne
- , Henning J. Falk
- & Stefan W. Hell
-
Article
| Open AccessQuantification of thickness and wrinkling of exfoliated two-dimensional zeolite nanosheets
Two-dimensional sheets of zeolites can function as molecular sieves for applications such as membranes or as catalysts. Here, the authors demonstrate a method using electron diffraction patterns to accurately measure the thickness and wrinkles of thin zeolite nanosheets.
- Prashant Kumar
- , Kumar Varoon Agrawal
- & K. Andre Mkhoyan
-
Article
| Open AccessOptical aperture synthesis with electronically connected telescopes
In astronomy, interferometry between telescopes enables high-resolution imaging but optical links are limited by atmospheric turbulence. Here, the authors show how this can be circumvented, producing diffraction-limited images using an array of electronically connected optical telescopes.
- Dainis Dravins
- , Tiphaine Lagadec
- & Paul D. Nuñez
-
Article
| Open AccessCavity ring-up spectroscopy for ultrafast sensing with optical microresonators
Whispering-gallery mode microresonators are powerful sensing tools, but spectrum acquisition has taken milliseconds or longer. Here, Rosenblum et al.introduce cavity ring-up spectroscopy, in which sharply rising detuned probe pulses capture spectra of microresonators on nanosecond timescales.
- Serge Rosenblum
- , Yulia Lovsky
- & Barak Dayan
-
Article
| Open AccessUltra-sensitive all-fibre photothermal spectroscopy with large dynamic range
Photothermal interferometry systems using free-space optics have limits in terms of light–matter interaction efficiency, size, optical alignment and integration. Here, Jin et al. use a gas-filled hollow-core photonic bandgap fibre to demonstrate an all-fibre gas sensor with ultrahigh sensitivity and dynamic range.
- Wei Jin
- , Yingchun Cao
- & Hoi Lut Ho
-
Article
| Open AccessEncoding and decoding spatio-temporal information for super-resolution microscopy
Increasing the resolution of fluorescence microscopy is a fundamental need for modern cell biology. Lanzanò et al.demonstrate that arbitrary spatial resolution is, in principle, possible by encoding the fluorophore's spatial distribution information in the temporal dynamics of the fluorophore's transition.
- Luca Lanzanò
- , Iván Coto Hernández
- & Giuseppe Vicidomini
-
Article
| Open AccessNanoscale probing of image-dipole interactions in a metallic nanostructure
An emitter near a surface induces an image dipole that alters the emission pattern and creates errors in single-particle imaging applications. Here, Ropp et al.show that an image dipole can distort the polarization and measured position of an emitter, and that these distortions can be corrected.
- Chad Ropp
- , Zachary Cummins
- & Edo Waks
-
Article
| Open AccessPartially coherent ultrafast spectrography
Ultrafast metrology typically relies on pulse coherence, but full coherence is not always possible in emerging attosecond and ultrashort X-ray technologies. Here, Bourassin-Bouchet and Couprie adapt frequency-resolved optical gating (FROG) to measure partially coherent optical pulses in the attosecond scale.
- C. Bourassin-Bouchet
- & M.-E. Couprie
-
Article |
Single-pixel imaging by means of Fourier spectrum acquisition
Single-pixel imaging can capture a scene without a direct line of sight to the object but high-quality imaging has proven challenging. Here, by acquiring their Fourier spectrum, Zhang et al. demonstrate indirect, high-quality single-pixel imaging in the presence of noisy environmental illumination.
- Zibang Zhang
- , Xiao Ma
- & Jingang Zhong
-
Article |
Seeded growth of highly crystalline molybdenum disulphide monolayers at controlled locations
Although synthesis of high-quality MoS2 has been demonstrated, growth of monolayer MoS2at controlled locations is highly desirable for applications. Here, the authors introduce a method where patterned seeds of molybdenum source material are used to grow isolated flakes at predetermined locations.
- Gang Hee Han
- , Nicholas J. Kybert
- & A. T. Charlie Johnson
-
Article |
Forbidden atomic transitions driven by an intensity-modulated laser trap
Atomic spectroscopy is typically based on multipole atom-field interactions that obey established selection rules. Using Rydberg atoms as an example, Moore et al. show that the quadratic (ponderomotive) interaction can provide both more flexible selection rules and greater spatial addressability.
- Kaitlin R. Moore
- , Sarah E. Anderson
- & Georg Raithel
-
Article
| Open AccessDip-pen patterning of poly(9,9-dioctylfluorene) chain-conformation-based nano-photonic elements
The optoelectronic properties of semiconducting polymers are controlled by altering chemical structure and/or inter-chain order. Perevedentsev et al. propose a nanopatterning approach whereby the geometry of polymer chain segments is modified to engineer metamaterial structures for visible light.
- Aleksandr Perevedentsev
- , Yannick Sonnefraud
- & Donal D. C. Bradley
-
Article
| Open AccessImaging with a small number of photons
Advances in low-light-level imaging techniques have shown that imaging in the one photon per pixel regime is possible. Here, Morris et al. demonstrate high-quality image reconstruction using ghost and heralded imaging with less than one photon per image pixel with a time-gated intensified camera.
- Peter A. Morris
- , Reuben S. Aspden
- & Miles J. Padgett
-
Article
| Open AccessAssembling programmable FRET-based photonic networks using designer DNA scaffolds
DNA is a useful molecule with which to construct nanomaterials with controllable functionalities. Here, the authors fabricate photonic wires by appending dye molecules at set positions along DNA structures, and show how FRET performance can be tuned by modifying dye separation.
- Susan Buckhout-White
- , Christopher M Spillmann
- & Igor L. Medintz
-
Article |
A far-off-resonance optical trap for a Ba+ ion
Trapped ions are promising for studies of atomic and quantum physics, but their need for radiofrequency fields poses numerous technical limitations. Huber et al.present an approach using far-off-resonance optical traps, circumventing radiofrequency fields to improve on photon scattering and recoil heating.
- Thomas Huber
- , Alexander Lambrecht
- & Tobias Schaetz
-
Article |
High-throughput imaging of self-luminous objects through a single optical fibre
Imaging through a single optical fibre offers attractive possibilities in applications such as micro-endoscopy or remote sensing. Using spread-spectrum encoding, Barankov and Mertz demonstrate two-dimensional imaging of self-luminous objects with high throughput, in theory independent of pixel number.
- Roman Barankov
- & Jerome Mertz
-
Article |
High-resolution nanotransfer printing applicable to diverse surfaces via interface-targeted adhesion switching
There is an ongoing need for high resolution, versatile and simplistic nanoscale lithography and transfer. Here the authors report a solvent-assisted nanotransfer printing route, which allows for the easy release of 8–20 nm scale features on to a range of substrates.
- Jae Won Jeong
- , Se Ryeun Yang
- & Yeon Sik Jung
-
Article |
Generation of ultra-short hydrogen atom pulses by bunch-compression photolysis
Short pulses of atoms or molecules can act as sensitive probes for numerous physical and chemical systems, but they are typically limited to the microsecond scale. By exploiting short pulse laser photolysis, Kaufmann et al. present a method that can produce pulses of hydrogen atoms on sub-nanosecond scales.
- Sven Kaufmann
- , Dirk Schwarzer
- & Oliver Bünermann
-
Article |
Three-dimensional plasmonic stereoscopic prints in full colour
Plasmonic nanostructures enable control over the spatial and spectral dependence of scattered light. Here, the authors use pixels formed of nanoellipse or nanosquare dimers to show polarization-dependent full-colour scattering in reflection, and build 3D stereoscopic colour microprints from them.
- Xiao Ming Goh
- , Yihan Zheng
- & Joel K. W. Yang
-
Article |
Enhanced acoustic sensing through wave compression and pressure amplification in anisotropic metamaterials
Acoustic sensors have myriad important applications, but they are limited by their pressure sensitivity. Chen et al.show how the use of graded anisotropic acoustic metamaterial structures can help overcome this by amplifying the acoustic waves via compression effects.
- Yongyao Chen
- , Haijun Liu
- & Miao Yu
-
Article |
Dual-comb spectroscopy based on quantum-cascade-laser frequency combs
The fundamental vibrational bands of many molecules lie on the mid-infrared, so generating all solid-state, compact frequency combs in that region is important for molecular spectroscopy. Here, Villares et al.use quantum-cascade-laser frequency combs to demonstrate a high resolution, broadband dual-comb spectrometer.
- Gustavo Villares
- , Andreas Hugi
- & Jérôme Faist
-
Article |
Nanomotor lithography
Miniaturization of devices and machines requires advanced lithographic techniques, whilst the high cost and complexity are the bottlenecks. Li et al.now show an approach for direct, arbitrary nano-patterning using self-propelled nanomotors acting as mobile nanomasks and near-field lenses.
- Jinxing Li
- , Wei Gao
- & Joseph Wang
-
Article |
Germanium avalanche receiver for low power interconnects
Despite many recent advances in silicon photonics for optical telecommunications and on-chip optical interconnects, the issue of power consumption has not been fully addressed. Here, Virot et al. propose a waveguide avalanche germanium photodiode suitable for low power consumption interconnects.
- Léopold Virot
- , Paul Crozat
- & Laurent Vivien
-
Article |
Two-colour spin noise spectroscopy and fluctuation correlations reveal homogeneous linewidths within quantum-dot ensembles
Conventional linear optical methods cannot probe within an inhomogeneously broadened ensemble of particles. Yang et al.demonstrate a spectroscopic technique based on fluctuation correlations that can reveal the underlying homogeneous linewidths of quantum dots in a low-power ensemble measurement.
- Luyi Yang
- , P. Glasenapp
- & S. A. Crooker
-
Article |
Angular momentum-induced circular dichroism in non-chiral nanostructures
The differential absorption of left and right handed light, circular dichroism, is typically observed only in chiral objects. Here, the authors demonstrate that giant circular dichroism can be induced in non-chiral objects when the left and right handed circularly polarized modes used are vortex beams.
- Xavier Zambrana-Puyalto
- , Xavier Vidal
- & Gabriel Molina-Terriza
-
Article
| Open AccessImaging the dynamics of free-electron Landau states
Landau states are associated with the quantised orbits of charged particles in magnetic fields. By manipulating electron vortex beams in a magnetic field, this study reconstructs the internal quantum dynamics of free-electron Landau states, which differs strongly from the classical cyclotron rotation.
- P. Schattschneider
- , Th. Schachinger
- & Franco Nori
-
Article |
Helicity-dependent three-dimensional optical trapping of chiral microparticles
It is known that light can be used for the optical trapping of microparticles. Here, the authors demonstrate that the interplay between helicity of the light and chirality of the matter can be applied for using the photon spin angular momentum as a tool for selective trapping of chiral particles.
- Georgiy Tkachenko
- & Etienne Brasselet
-
Article
| Open AccessObservation of a quantum Cheshire Cat in a matter-wave interferometer experiment
One of the paradoxical phenomena of quantum mechanics is the quantum Cheshire Cat, consisting of the apparent spatial separation of a particle and one of its properties. Denkmayr et al.use neutron interferometry to prepare and evaluate the Cheshire Cat state of a neutron and its magnetic moment.
- Tobias Denkmayr
- , Hermann Geppert
- & Yuji Hasegawa
-
Article |
Direct optical sensing of single unlabelled proteins and super-resolution imaging of their binding sites
The development of biosensors with improved sensitivity for the detection of biological molecules presents obvious possibilities for improved diagnostic tools in healthcare. Here, the authors present a technique for the label-free detection and super-resolution imaging of single proteins.
- Marek Piliarik
- & Vahid Sandoghdar
-
Article
| Open AccessSuper-resolution imaging and tracking of protein–protein interactions in sub-diffraction cellular space
Protein–protein interactions are ubiquitous in cells and these contacts are crucial for a wide number of cellular processes. Here, the authors present a technique for the super-resolution imaging and tracking of protein–protein interactions in cells.
- Zhen Liu
- , Dong Xing
- & Yujie Sun
-
Article |
Plasmofluidic single-molecule surface-enhanced Raman scattering from dynamic assembly of plasmonic nanoparticles
Plasmonic hot-spot generation in solution is not reversible for single-molecule surface-enhanced Raman scattering, which limits its applications. Patra et al.tackle this problem by integrating this technique with thermo-plasmon-assisted reconfiguration of nanoparticles at a metal–fluid interface.
- Partha Pratim Patra
- , Rohit Chikkaraddy
- & G. V. Pavan Kumar
-
Article
| Open AccessImaging and steering an optical wireless nanoantenna link
Like conventional antennas, optical nanoantennas can transmit and receive signals but on much smaller length scales. Dregely et al.measure the optical power transmitted and received in the far-field by plasmonic nanoantennas and show that they can control the direction of transmission over a broad range.
- Daniel Dregely
- , Klas Lindfors
- & Harald Giessen
-
Article
| Open AccessHigh-contrast sub-millivolt inelastic X-ray scattering for nano- and mesoscale science
Inelastic X-ray scattering suffers from not being able to access high-frequency collective excitations in condensed matter on the nano- to mesoscales. Here, the authors report a new spectrometer that allows these regimes to be accessed, and demonstrate its advances by studying an organic glass-forming liquid.
- Yuri Shvyd’ko
- , Stanislav Stoupin
- & Martin Tolkiehn
-
Article |
Ultrafast fluorescence imaging in vivo with conjugated polymer fluorophores in the second near-infrared window
In vivofluorescence imaging in the second near-infrared window allows high resolution and tissue penetration. Here, using conjugated polymers, the authors achieve imaging with high spatial and time resolutions capable of resolving mouse femoral artery blood-flow variations within a single cardiac cycle.
- Guosong Hong
- , Yingping Zou
- & Hongjie Dai
-
Article
| Open AccessLamb-Dicke spectroscopy of atoms in a hollow-core photonic crystal fibre
Atoms lose coherence via interactions with each other and the walls of their environment, which degrades the performance of atomic systems. As a route to minimize such effects, Okaba et al.use kagome-lattice hollow-core photonic crystal fibres to confine atoms, preventing them interacting with the wall.
- Shoichi Okaba
- , Tetsushi Takano
- & Hidetoshi Katori
-
Article
| Open AccessMonolithically integrated mid-infrared lab-on-a-chip using plasmonics and quantum cascade structures
Quantum cascade lasers and detectors enable photonic integration of semiconductor devices across a broad spectral range. Here, Schwarz et al.present a bi-functional laser and detector structure, monolithically integrated with plasmonic waveguides for mid-infrared chemical sensors on a chip.
- Benedikt Schwarz
- , Peter Reininger
- & Gottfried Strasser
-
Article
| Open AccessAll-printable band-edge modulated ZnO nanowire photodetectors with ultra-high detectivity
Nanowire photodetectors offer a high sensitivity arising from their geometry that makes them of interest for optoelectronic devices. Here, the authors demonstrate the printable fabrication of ZnO nanowires with high detectivity, making them suitable for high-performance flexible electronics applications.
- Xi Liu
- , Leilei Gu
- & Zhiyong Fan
-
Article |
Hybrid multiphoton volumetric functional imaging of large-scale bioengineered neuronal networks
Three-dimensional neural networks are promising models of nervous tissues, which could aid our understanding of their structure and function. Here, the authors present advanced methods for studying volumetric activity in three-dimensional cultures of neural cells in hydrogels.
- Hod Dana
- , Anat Marom
- & Shy Shoham
-
Article |
Ultrafast acousto-plasmonic control and sensing in complex nanostructures
The nanometre length scale of plasmonic structures leads to vibrational dynamics at high frequencies, which could be exploited for sensitive optical detectors. O'Brien et al. show that they can detect spatial properties of phonon modes in multimodal plasmonic structures, revealing complex nanomechanical dynamics.
- Kevin O’Brien
- , N. D. Lanzillotti-Kimura
- & Xiang Zhang
-
Article
| Open AccessInterferometry with non-classical motional states of a Bose–Einstein condensate
Ramsey interferometers are used to measure minute energy shifts, but they are usually only applied to simple, non-interacting ensembles. Here, the authors demonstrate a two-pulse Ramsey-type interferometer built on the motional states of an interacting Bose–Einstein condensate using optimal control.
- S. van Frank
- , A. Negretti
- & J. Schmiedmayer
-
Article |
In vivo imaging of specific drug–target binding at subcellular resolution
The ability to image the action of drugs in cells in real time could yield valuable information on their efficacy and mode of action. Here, the authors use multiphoton fluorescence anisotropy microscopy to image drug distribution and target engagement in real time at the cellular level in vivo.
- J. M. Dubach
- , C. Vinegoni
- & R. Weissleder
-
Article
| Open AccessOn-the-fly decoding luminescence lifetimes in the microsecond region for lanthanide-encoded suspension arrays
Accurately determining luminescence lifetimes for slow-decaying signals can be challenging. Here, the authors report a fitting algorithm and subsequently experimentally show a method for the rapid measurement of luminescence lifetimes in the microsecond region.
- Yiqing Lu
- , Jie Lu
- & Dayong Jin