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| Open AccessSingle-particle mass spectrometry with arrays of frequency-addressed nanomechanical resonators
Nano-electro-mechanical system-based mass spectrometry holds promise for detecting supramolecular assemblies at large molecular weights, but its efficiency is too poor to be practical. Sage et al. overcome this problem using a nanomechanical resonator array, which significantly decreases detection time.
- Eric Sage
- , Marc Sansa
- & Sébastien Hentz
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Article
| Open AccessUphill production of dihydrogen by enzymatic oxidation of glucose without an external energy source
Most chemical reactions proceed downhill without external energy input. Here, authors employ an electronic flyback and a boost converter to store energy and spontaneously drive an uphill reaction. The concept is exhibited by an enzymatic biofuel cell, driving water splitting in a single compartment.
- Emmanuel Suraniti
- , Pascal Merzeau
- & Alexander Kuhn
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| Open AccessBurden on hydropower units for short-term balancing of renewable power systems
Quantifying burden on hydropower units for balancing variable renewable energy sources has been uncertain and difficult. Herein Yang et al. propose a framework and characterize the burden, performance and compensation of hydropower regulation of renewable power systems.
- Weijia Yang
- , Per Norrlund
- & Urban Lundin
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| Open AccessEfficient and self-adaptive in-situ learning in multilayer memristor neural networks
Memristor-based neural networks hold promise for neuromorphic computing, yet large-scale experimental execution remains difficult. Here, Xia et al. create a multi-layer memristor neural network with in-situ machine learning and achieve competitive image classification accuracy on a standard dataset.
- Can Li
- , Daniel Belkin
- & Qiangfei Xia
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Article
| Open AccessImplementation of multilayer perceptron network with highly uniform passive memristive crossbar circuits
Memristive devices used in neuromorphic computing typically need to be accessed using transistors, adding circuit complexity and size. In this work, the authors demonstrate a neural network using a transistor-free passive memristor crossbar array, offering potential circuit miniaturisation and energy savings.
- F. Merrikh Bayat
- , M. Prezioso
- & D. Strukov
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| Open AccessSeamlessly fused digital-analogue reconfigurable computing using memristors
Conventional analogue and digital circuits are mixed at signal level yet remain technologically separate, adding complexity and cost. This work introduces a new design paradigm where the analogue and digital worlds are seamlessly fused via memristors, enabling electronics with reconfigurability.
- Alexantrou Serb
- , Ali Khiat
- & Themistoklis Prodromakis
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| Open AccessSeparation of current density and electric field domains caused by nonlinear electronic instabilities
The usefulness of metal-oxide memristors for memory and brain-inspired computing applications arises from their electronic instabilities, whose details remain limited. In this work, the authors analyze electronic decompositions in several metal oxides, providing new insights for device modeling.
- Suhas Kumar
- & R. Stanley Williams
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| Open AccessTransparent and attachable ionic communicators based on self-cleanable triboelectric nanogenerators
Flexible, transparent wearable electronics harvesting energy from human motion are nearing reality, but stable adhesion while staying clean remains a problem. Here the authors solve both issues with a functionalized organic polymer/hydrogel-based device capable of wireless communication via finger gestures.
- Younghoon Lee
- , Seung Hee Cha
- & Jeong-Yun Sun
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Article
| Open AccessReconfigurable engineered motile semiconductor microparticles
Active particles that demonstrate life-like behavior may find use in bio-inspired technologies, but achieving on-demand reconfiguration remains challenging. Here, the authors demonstrate controllable, collective behavior in silicon microparticles, which are fabricated via conventional semiconductor methods.
- Ugonna Ohiri
- , C. Wyatt Shields IV
- & Nan Jokerst
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Article
| Open AccessMolecular doping enabled scalable blading of efficient hole-transport-layer-free perovskite solar cells
The existing hole-transporting materials cause problems in the cost and scalability of the perovskite solar cells. Here Wu et al. fabricate high efficiency cells by molecularly doping the perovskite layer without using hole-transporting layers, thus simplify the device architecture and processing steps.
- Wu-Qiang Wu
- , Qi Wang
- & Jinsong Huang
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Article
| Open AccessNeural-like computing with populations of superparamagnetic basis functions
Population coding, where populations of artificial neurons process information collectively can facilitate robust data processing, but require high circuit overheads. Here, the authors realize this approach with reduced circuit area and power consumption, by utilizing superparamagnetic tunnel junction based neurons.
- Alice Mizrahi
- , Tifenn Hirtzlin
- & Damien Querlioz
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| Open AccessEnergy-loss return gate via liquid dielectric polarization
One major energy loss in electronics is heat dissipation due to induced polarization in dielectric materials in the presence of electric fields. Kim et al. utilize large polarization in liquids to harvest dielectric loss via an energy-loss return gate design, which converts energy back to electricity.
- Taehun Kim
- , Hyungseok Yong
- & Sangmin Lee
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| Open AccessHigh-sensitivity ion detection at low voltages with current-driven organic electrochemical transistors
The organic electrochemical transistor is a type of transistor that modulates the channel current by the ion concentration and is thus explored for bio-applications. Here Ghittorelli et al. show a current-driven device configuration to increase the sensitivity by ten times than conventional approaches.
- Matteo Ghittorelli
- , Leona Lingstedt
- & Fabrizio Torricelli
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| Open AccessA high-brightness large-diameter graphene coated point cathode field emission electron source
Traditional cold field emission electron sources rely on single crystal tungsten sharpened wires. Here, the authors use graphene-coated nickel point cathodes to devise alternative cold field emission electron sources for electron microscopy and lithography applications.
- Xiuyuan Shao
- , Avinash Srinivasan
- & Anjam Khursheed
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| Open AccessLarge-area and bright pulsed electroluminescence in monolayer semiconductors
Atomically thin monolayers with high photoluminescence quantum yield are promising for optoelectronic and lighting applications. Here, the authors fabricate a transient-mode electroluminescent device to bypass the requirement of ohmic contacts for electrons and holes, and observe millimetre-scale light emission from a transparent 2D display.
- Der-Hsien Lien
- , Matin Amani
- & Ali Javey
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Article
| Open AccessDecomposing the Bragg glass and the peak effect in a Type-II superconductor
The disordering of the vortex lattice in a type-II superconductor is widely perceived to underpin unusual peaks in the temperature and field dependence of critical current. By contrast, here Toft-Petersen et al. find an order-disorder transition in a superconducting vanadium sample that is unconnected with peaks observed in critical current.
- Rasmus Toft-Petersen
- , Asger B. Abrahamsen
- & Mark Laver
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| Open AccessShape anisotropy revisited in single-digit nanometer magnetic tunnel junctions
The thermal stability impedes the application of nanoscale magnetic tunnel junctions in electronic and spintronics devices. Here the authors achieved current-induced magnetization switching in magnetic tunnel junctions smaller than 10 nm with sufficient thermal stability due to the shape anisotropy without adding new material systems.
- K. Watanabe
- , B. Jinnai
- & H. Ohno
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| Open AccessAn artificial nociceptor based on a diffusive memristor
The development of humanoid robots with artificial intelligence calls for smart solutions for tactile sensing systems that respond to dynamic changes in the environment. Here, Yoon et al. emulate non-adaption and sensitization function of a nociceptor—a sensory neuron—using diffusive oxide-based memristors.
- Jung Ho Yoon
- , Zhongrui Wang
- & J. Joshua Yang
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Article
| Open AccessDNA multi-bit non-volatile memory and bit-shifting operations using addressable electrode arrays and electric field-induced hybridization
DNA based technology holds promise for non-volatile memory and computational tasks, yet the relatively slow hybridization kinetics remain a bottleneck. Here, Song et al. have developed an electric field-induced hybridization platform that can speed up multi-bit memory and logic operations.
- Youngjun Song
- , Sejung Kim
- & Xiaohua Huang
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| Open AccessSkin-inspired highly stretchable and conformable matrix networks for multifunctional sensing
Electronic skins have been developed to emulate human sensory systems, but simultaneous detection of multiple stimuli remains a big challenge due to coupling of electronic signals. Here, Hua et al. overcome this problem in a stretchable and conformable matrix network integrated with seven different modes.
- Qilin Hua
- , Junlu Sun
- & Zhong Lin Wang
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| Open AccessUnidirectional spin-Hall and Rashba−Edelstein magnetoresistance in topological insulator-ferromagnet layer heterostructures
Unidirectional spin Hall magnetoresistance enables the new spintronic devices but is limited by the low amplitude or working temperature. Here, the authors report the large unidirectional spin Hall magnetoresistance in a topological insulator and ferromagnetic metal bilayer system at relatively higher temperature.
- Yang Lv
- , James Kally
- & Jian-Ping Wang
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| Open AccessSolving for ambiguities in radar geophysical exploration of planetary bodies by mimicking bats echolocation
Radar sounders, used for the geophysical exploration of celestial objects in the solar system, possess striking similarities to bat sonars. Here, the authors adapt and implement the bat clutter mitigation mechanism to radar geophysical exploration of planetary bodies.
- Leonardo Carrer
- & Lorenzo Bruzzone
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| Open AccessReservoir computing using dynamic memristors for temporal information processing
Reservoir computing facilitates the projection of temporal input signals onto a high-dimensional feature space via a dynamic system, known as the reservoir. Du et al. realise this concept using metal-oxide-based memristors with short-term memory to perform digit recognition tasks and solve non-linear problems.
- Chao Du
- , Fuxi Cai
- & Wei D. Lu
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Article
| Open AccessStateful characterization of resistive switching TiO2 with electron beam induced currents
Oxide-based memristors hold promise for artificial neuromorphic computing, yet the detail of the switching mechanism—filament formation—remains largely unknown. Hoskins et al. provide nanoscale imaging of this process using electron beam induced current microscopy and relate it to resistive states.
- Brian D. Hoskins
- , Gina C. Adam
- & Jabez J. McClelland
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| Open AccessOrigami silicon optoelectronics for hemispherical electronic eye systems
Hemispherical format has been adopted in camera systems to better mimic human eyes, yet the current designs rely on complicated fabrications. Here, Zhang et al. show an origami-inspired approach that enables planar silicon-based photodetector arrays to reshape into concave or convex geometries.
- Kan Zhang
- , Yei Hwan Jung
- & Zhenqiang Ma
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Article
| Open AccessBenchmarking organic mixed conductors for transistors
Organic materials that support both electronic and ionic transport hold promise for applications in bioelectronics and energy storage. Here, Inal et al. use transistors to quantify the materials performance of organic mixed conductors in terms of the product of charge mobility and volumetric capacitance.
- Sahika Inal
- , George G. Malliaras
- & Jonathan Rivnay
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| Open AccessElectrostrictive microelectromechanical fibres and textiles
Micro-electromechanical systems fabrication techniques are based on silicon micromachining processes, resulting in rigid and low aspect ratio structures. Here the authors demonstrate a flexible, high aspect ratio micro-electromechanical system in fibre enabled by an electrostrictive ferrorelaxor terpolymer layer.
- Tural Khudiyev
- , Jefferson Clayton
- & Yoel Fink
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| Open AccessFully inkjet-printed two-dimensional material field-effect heterojunctions for wearable and textile electronics
Heterojunction structures based on 2D materials show promise for wearable and textile electronics. Here, the authors demonstrate fully inkjet-printed hetero junctions of graphene and h-BN as a platform for FET-based smart electronics on wearable and washable textile substrates.
- Tian Carey
- , Stefania Cacovich
- & Felice Torrisi
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| Open AccessBidirectional wavelength-division multiplexing transmission over installed fibre using a simplified optical coherent access transceiver
The signalling scheme used in access networks require electrical bandwidths many times greater than subscribers can utilise. Here, the authors describe a promising approach to achieve bidirectional transmission with bandwidth-efficient yet low-complexity coherent optical network unit transceiver.
- M. S. Erkılınç
- , D. Lavery
- & P. Bayvel
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| Open AccessA novel true random number generator based on a stochastic diffusive memristor
Memristors can switch between high and low electrical-resistance states, but the switching behaviour can be unpredictable. Here, the authors harness this unpredictability to develop a memristor-based true random number generator that uses the stochastic delay time of threshold switching
- Hao Jiang
- , Daniel Belkin
- & Qiangfei Xia
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Article
| Open AccessSynchronized conductivity modulation to realize broadband lossless magnetic-free non-reciprocity
Optical non-reciprocity achieved through refractive index modulation can have its challenges and limitations. Here, Dinc et al. introduce the concept of non-reciprocity based on synchronized spatio-temporal modulation of conductivity to achieve different types of non-reciprocal functionality.
- Tolga Dinc
- , Mykhailo Tymchenko
- & Harish Krishnaswamy
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| Open AccessFrequency-division multiplexer and demultiplexer for terahertz wireless links
There is growing interest in the development of components to facilitate wireless communications in the terahertz but the characterization of these systems involve an unmodulated input. Here the authors demonstrate multiplexing and demultiplexing of data streams in the terahertz range using a real data link.
- Jianjun Ma
- , Nicholas J. Karl
- & Daniel M. Mittleman
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| Open AccessOrganic flash memory on various flexible substrates for foldable and disposable electronics
Flexible flash memory is crucial to modern electronics, but its fabrication is challenging in the absence of suitable dielectric materials. Here, Lee et al. realize organic memory with retention over 10 years using tunneling and blocking dielectric layers prepared by initiated chemical vapor deposition.
- Seungwon Lee
- , Hyejeong Seong
- & Seunghyup Yoo
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| Open AccessPhysical origins of current and temperature controlled negative differential resistances in NbO2
The development of future computation devices will be aided by a better understanding of the physics underlying material behaviors. Using thermoreflectance and spatially resolved X-ray microscopy, Kumar et al. elucidate the origin of two types of negative differential resistance in NbO2 memristors.
- Suhas Kumar
- , Ziwen Wang
- & R. Stanley Williams
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| Open AccessMergeable nervous systems for robots
Robots that can self-assemble into different morphologies are desired to perform tasks that require different physical capabilities. Mathews et al. design robots whose bodies and control systems can merge and split to form new robots that retain full sensorimotor control and act as a single entity.
- Nithin Mathews
- , Anders Lyhne Christensen
- & Marco Dorigo
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| Open AccessConformal metasurface-coated dielectric waveguides for highly confined broadband optical activity with simultaneous low-visibility and reduced crosstalk
Controlling all the optical properties of dielectric waveguides is a challenging task and often requires complicated core- and cladding designs. Here, Jiang et al. demonstrate that a thin metasurface coating can control several optical properties simultaneously over a broad frequency range.
- Zhi Hao Jiang
- , Lei Kang
- & Douglas H. Werner
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| Open AccessAcoustically actuated ultra-compact NEMS magnetoelectric antennas
The miniaturization of antennas beyond a wavelength is limited by designs which rely on electromagnetic resonances. Here, Nan et al. have developed acoustically actuated antennas that couple the acoustic resonance of the antenna with the electromagnetic wave, reducing the antenna footprint by up to 100.
- Tianxiang Nan
- , Hwaider Lin
- & Nian Xiang Sun
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| Open AccessElectromagnetic reprogrammable coding-metasurface holograms
Realizing metasurfaces with reconfigurability, high efficiency, and control over phase and amplitude is a challenge. Here, Li et al. introduce a reprogrammable hologram based on a 1-bit coding metasurface, where the state of each unit cell of the coding metasurface can be switched electrically.
- Lianlin Li
- , Tie Jun Cui
- & Shuang Zhang
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Article
| Open AccessRewritable ghost floating gates by tunnelling triboelectrification for two-dimensional electronics
Once fabricated, the gates of conventional electronic devices are spatially fixed. Here, the authors introduce tunnelling triboelectrification to create, modify and destroy on-demand ghost floating gates underneath 2D materials, with the spatial resolution of an atomic force microscope.
- Seongsu Kim
- , Tae Yun Kim
- & Christian Falconi
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Article
| Open AccessDiffusion engineering of ions and charge carriers for stable efficient perovskite solar cells
Ion migration in perovskite solar cells are known to cause hysteresis and instability. Biet al., report a charge extraction layer based on graphene, fullerenes and carbon quantum dots which suppresses ion diffusion and enhances charge carrier diffusion leading to efficient devices with improved stability.
- Enbing Bi
- , Han Chen
- & Liyuan Han
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Article
| Open AccessQuantum tunnelling and charge accumulation in organic ferroelectric memory diodes
Organic non-volatile memories based on ferroelectric and semiconductor polymers are one of promising candidates for flexible electronics, yet the relevant device physics remains elusive. Ghittorelliet al. show that quantum tunnelling and charge accumulation govern the ferroelectric memory operation.
- Matteo Ghittorelli
- , Thomas Lenz
- & Fabrizio Torricelli
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| Open AccessThree-dimensional crossbar arrays of self-rectifying Si/SiO2/Si memristors
Memristors are key structural units of complex memory and computing systems, yet most currently available memristors are based on materials that are not compatible with silicon technology. Here, the authors demonstrate a CMOS-compatible, self-rectifying memristor and arrays entirely based on p-Si/SiO2/n-Si.
- Can Li
- , Lili Han
- & Qiangfei Xia
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Article
| Open AccessNeuromorphic device architectures with global connectivity through electrolyte gating
Global regulation of synaptic strengths in neural systems is known as homeoplasticity. Here, Gkoupideniset al. use an electrolyte to connect and control an array of organic electrochemical devices, in order to demonstrate behaviour that resembles homeoplasticity phenomena in the brain.
- Paschalis Gkoupidenis
- , Dimitrios A. Koutsouras
- & George G. Malliaras
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Article
| Open AccessFace classification using electronic synapses
Using chips that mimic the human brain to perform cognitive tasks, namely neuromorphic computing, calls for low power and high efficiency hardware. Here, Yaoet al. show on-chip analogue weight storage by integrating non-volatile resistive memory into a CMOS platform and test it in facial recognition.
- Peng Yao
- , Huaqiang Wu
- & He Qian
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Article
| Open AccessCharge carrier mobility in thin films of organic semiconductors by the gated van der Pauw method
Charge carrier mobility is one of the key parameters that are used to evaluate the electrical quality of thin film semiconductors, whilst it is easily overestimated. Here, Rolinet al. use the gated van der Pauw method to extract charge mobility independent of contact resistance and device dimensions.
- Cedric Rolin
- , Enpu Kang
- & Jan Genoe
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Article
| Open AccessMultiplexed single-mode wavelength-to-time mapping of multimode light
Photonic lanterns are made by merging several single-mode cores into one multimode core. Here, the authors show this type of structure can both perform wavelength-to-time mapping of multimode states of light and couple such light to an array of single-photon avalanche detectors.
- Harikumar K Chandrasekharan
- , Frauke Izdebski
- & Robert R. Thomson
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| Open AccessMeasurement of transverse emittance and coherence of double-gate field emitter array cathodes
Field emitter arrays are key components for X-ray sources, microwave generators, RF communication and advanced light sources. Tsujinoet al., report double-gate field emitter arrays with competitive beam qualities to the state of the art UV photoexcited cathodes.
- Soichiro Tsujino
- , Prat Das Kanungo
- & R.J. Dwayne Miller
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Article
| Open AccessImprovement of system capacitance via weavable superelastic biscrolled yarn supercapacitors
Carbon nanotube yarns with high loadings of pseudocapacitive material are desirable, e.g., for emerging wearable technologies. Here authors make biscrolled yarns with high loadings of MnO2nanoparticles confined in carbon nanotube galleries, demonstrating very high linear and areal capacitances.
- Changsoon Choi
- , Kang Min Kim
- & Seon Jeong Kim
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Article
| Open AccessSpray printing of organic semiconducting single crystals
The development of organic electronics calls for low-cost printing techniques that can prepare high quality, large-area organic single crystals. Here, Rigaset al. achieve this goal by combining spray printing and antisolvent crystallization and test the method on various materials and substrates.
- Grigorios-Panagiotis Rigas
- , Marcia M. Payne
- & Maxim Shkunov