Featured
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All-optical seeding of a light-induced phase transition with correlated disorder
Controlling phase transitions in solids is crucial for many applications. Ultrafast laser pulses have now been shown to enable the energy-efficient generation of structural fluctuations in VO2 by harnessing the correlated disorder in the material.
- Allan S. Johnson
- , Ernest Pastor
- & Simon E. Wall
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News & Views |
At the breaking point
The shape and trajectory of a crack plays a crucial role in material fracture. High-precision experiments now directly capture this phenomenon, unveiling the intricate 3D nature of cracks.
- Michael D. Bartlett
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Article |
Flexoelectricity-driven toroidal polar topology in liquid-matter helielectrics
Exploring and exploiting electric dipole arrangements analogously to what is possible with magnetic spin textures is an emerging prospect. Now a spontaneous toroidal polar topology is observed in ferroelectric liquid crystals.
- Jidan Yang
- , Yu Zou
- & Satoshi Aya
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News & Views |
Time in a glass
Ageing is a non-linear, irreversible process that defines many properties of glassy materials. Now, it is shown that the so-called material-time formalism can describe ageing in terms of equilibrium-like properties.
- Beatrice Ruta
- & Daniele Cangialosi
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Article |
Origin of the critical state in sheared granular materials
When applying sufficient strain, the flow of dense granular matter becomes critical. It is now shown that this state corresponds to random loose packing for spheres with different friction coefficients and that these packings can be mapped onto the frictionless hard-sphere system.
- Yi Xing
- , Ye Yuan
- & Yujie Wang
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Editorial |
Twenty years of 2D materials
Two-dimensional crystals have revolutionized fundamental research across a staggering range of disciplines. We take stock of the progress gained after twenty years of work.
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Article |
Non-affine atomic rearrangement of glasses through stress-induced structural anisotropy
Resolving the structural changes of a deformed glass on the atomic scale is challenging due to its disordered nature. Now, high-energy diffraction measurements show that non-line-preserving atomic displacements in glasses correlate with structural anisotropy.
- Jie Dong
- , Hailong Peng
- & Haiyang Bai
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Article |
Ultrafast lattice disordering can be accelerated by electronic collisional forces
The Born–Oppenheimer approximation is the prevailing assumption for interpreting ultrafast electron dynamics in solids. Evidence now suggests that collisions between electrons and lattice not captured by this approximation play an important role.
- Gilberto A. de la Peña Muñoz
- , Alfredo A. Correa
- & Mariano Trigo
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News & Views |
Rejuvenated but remembering
The structure of disordered materials typically ages, but sometimes also rejuvenates, resulting in intriguing memory properties. Progress in numerical simulations of spin glasses has now enabled replication of such phenomena from simple models.
- Eric Vincent
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Article |
Visualizing slow internal relaxations in a two-dimensional glassy system
Glasses relax internally even when their structure is frozen. Observations of a two-dimensional glass former now show that although structure relaxation freezes with the glass transition, non-constrained bonds survive; this accounts for persisting internal relaxation.
- Yanshuang Chen
- , Zefang Ye
- & Peng Tan
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Article |
Quantum phase diagram of high-pressure hydrogen
It is very challenging to model hydrogen at high pressures and low temperatures because quantum effects become significant. A state-of-the-art numerical study shows that these effects cause important changes to the predicted phase diagram.
- Lorenzo Monacelli
- , Michele Casula
- & Francesco Mauri
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Article
| Open AccessUnidirectional scattering with spatial homogeneity using correlated photonic time disorder
Photonic systems can exploit time as a degree of freedom analogous to space, eliminating the need for spatial patterning to achieve functionality. A Green’s function approach allows the design of disordered time scatterers with desired properties.
- Jungmin Kim
- , Dayeong Lee
- & Namkyoo Park
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Article |
Ultrafast relaxation of lattice distortion in two-dimensional perovskites
The ultrafast structural dynamics in 2D perovskites are an important part of their non-equilibrium properties. Now, their visualization reveals a light-induced reduction in the antiferro-distortion initiated by the electron–hole plasma.
- Hao Zhang
- , Wenbin Li
- & Aditya D. Mohite
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Article |
Spin–orbital liquid state and liquid–gas metamagnetic transition on a pyrochlore lattice
At low temperatures, the orbital degrees of freedom in insulating magnets normally do not fluctuate, leaving only magnetic behaviour. Measurements now suggest that in Pr2Zr2O7, it is possible to reach a quantum regime of coupled spin–orbital dynamics.
- Nan Tang
- , Yulia Gritsenko
- & Satoru Nakatsuji
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Letter
| Open AccessTruly chiral phonons in α-HgS
The notion of chirality in dynamical systems with broken spatial symmetry but preserved time inversion symmetry has led to the concept of truly chiral phonons. These have now been observed in bulk HgS using circularly polarized Raman spectroscopy.
- Kyosuke Ishito
- , Huiling Mao
- & Takuya Satoh
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Letter
| Open AccessExperimental observation of open structures in elemental magnesium at terapascal pressures
Numerical studies have predicted that solids at extremely high pressures should exhibit changes in structure driven by quantum mechanical effects. These predictions have now been verified in magnesium.
- M. G. Gorman
- , S. Elatresh
- & M. I. McMahon
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Perspective |
From atomically resolved imaging to generative and causal models
High-resolution imaging methods have been instrumental in advancing our understanding of the structure of materials. To move microscopy and tomography methods forwards, approaches to reassess macroscopic concepts such as symmetry are needed.
- Sergei V. Kalinin
- , Ayana Ghosh
- & Maxim Ziatdinov
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News & Views |
Water untangled
Computer simulations have revealed the topological nature of the liquid–liquid phase transition in colloidal water. This finding might lead to an experimental observation of this topological transition with colloids as building blocks.
- Camille Scalliet
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Article
| Open AccessTopological nature of the liquid–liquid phase transition in tetrahedral liquids
Supercooled water undergoes a liquid–liquid phase transition. The authors show that the two phases have distinct hydrogen-bond networks, differing in their degree of entanglement, and thus the transition can be described by the topological changes of the network.
- Andreas Neophytou
- , Dwaipayan Chakrabarti
- & Francesco Sciortino
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Article |
Self-organized lasers from reconfigurable colloidal assemblies
Experiments inspired by the behaviour of active matter show that an external optical stimulus can spatially reconfigure colloidal random lasers and continuously tune their lasing threshold.
- Manish Trivedi
- , Dhruv Saxena
- & Giorgio Volpe
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Article |
Origin of the boson peak in amorphous solids
The relation between physical properties and structure in amorphous materials is poorly understood. Simulations now show that vibrations of string-like dynamical defects likely govern the low-temperature dynamics in these systems.
- Yuan-Chao Hu
- & Hajime Tanaka
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News & Views |
A wing explained
The origin of a well-known feature in relaxation data seen in many glass-forming materials has now — possibly — been resolved by means of computer simulations.
- Reiner Zorn
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News & Views |
Controlling ferroelectricity below the surface
Optical control of material properties is usually limited to the region that absorbs the light. Coupling to lattice vibrations that travel close to the speed of light allows ultrafast modulation of polarization deep inside a ferroelectric material.
- Elsa Abreu
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News & Views |
Crystals break up with a twist
When crystal defects are present in an ensemble of spinning colloids that induce transverse forces on each other, the defects assemble into grain boundaries that can break the system apart into a set of crystal whorls.
- Cynthia J. O. Reichhardt
- & Charles Reichhardt
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Article |
Motile dislocations knead odd crystals into whorls
The addition of transverse forces to an ensemble of colloidal spinners induces the appearance of odd elastic crystals, featuring self-propelled defects that organize the system into a ‘self-kneading’ crystal whorl state.
- Ephraim S. Bililign
- , Florencio Balboa Usabiaga
- & William T. M. Irvine
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News & Views |
Hot black ices
At high pressure and temperature, water forms two crystalline phases, known as hot ‘black’ ices due to their partial opaqueness. A detailed characterization of these phases may explain magnetic field formation in giant icy planets like Neptune.
- Simone Anzellini
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Structure and properties of two superionic ice phases
Measurements of the phase diagram of water reveal first-order phase transitions to face- and body-centred cubic superionic ice phases. The former is suggested to be present in the interior of ice giant planets.
- Vitali B. Prakapenka
- , Nicholas Holtgrewe
- & Alexander F. Goncharov
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Perspective |
Engineering crystal structures with light
The interaction between light and the crystal lattice of a quantum material can modify its properties. Utilizing nonlinear interactions allows this to be done in a controlled way to design specific non-equilibrium functionalities.
- Ankit S. Disa
- , Tobia F. Nova
- & Andrea Cavalleri
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Phase behaviours of superionic water at planetary conditions
Superionic water is believed to exist in the interior of ice giant planets. By combining machine learning and free-energy methods, the phase behaviours of water at the extreme pressures and temperatures prevalent in such planets are predicted.
- Bingqing Cheng
- , Mandy Bethkenhagen
- & Sebastien Hamel
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Article |
Free electron to electride transition in dense liquid potassium
Alkali metals at high pressures have a liquid–liquid transition that is difficult to study in detail. Numerical calculations now suggest that the higher-pressure state is an electride liquid, in which electrons behave like localized anions.
- Hongxiang Zong
- , Victor Naden Robinson
- & Graeme J. Ackland
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Morphology selection kinetics of crystallization in a sphere
The authors investigate the role of spherical confinement and curvature-induced topological defects on the crystallization of charged colloids. They conclude that crystallization in spherical confinement is due to a combination of thermodynamics and kinetic pathways.
- Yanshuang Chen
- , Zhenwei Yao
- & Peng Tan
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Letter |
Black metal hydrogen above 360 GPa driven by proton quantum fluctuations
Numerical calculations that include the quantum fluctuations of protons explain the optical properties of hydrogen at high pressure.
- Lorenzo Monacelli
- , Ion Errea
- & Francesco Mauri
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Article |
Magnetically driven phonon instability enables the metal–insulator transition in h-FeS
A detailed and systematic X-ray and neutron scattering study of hexagonal iron sulfide uncovers the critical role of spin–phonon coupling in promoting the metal–insulator transition in this system.
- Dipanshu Bansal
- , Jennifer L. Niedziela
- & Olivier Delaire
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News & Views |
Machine learning glasses
Artificial neural networks now allow the dynamics of supercooled liquids to be predicted from their structure alone in an unprecedented way, thus providing a powerful new tool to study the physics of the glass transition.
- Giulio Biroli
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Article |
Unveiling the predictive power of static structure in glassy systems
The physics that underlies the glass transition is both subtle and non-trivial. A machine learning approach based on graph networks is now shown to accurately predict the dynamics of glasses over a wide range of temperatures, pressures and densities.
- V. Bapst
- , T. Keck
- & P. Kohli
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Letter |
Observation of a ferro-rotational order coupled with second-order nonlinear optical fields
The authors use optical spectroscopy to show that RbFe(MoO4)2 hosts a ferro-rotational phase. This is the final form of ferroic order to be observed.
- Wencan Jin
- , Elizabeth Drueke
- & Liuyan Zhao
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Letter |
Two-dimensional skyrmion bags in liquid crystals and ferromagnets
Structures containing multiple skyrmions inside a larger skyrmion—called skyrmion bags—are experimentally created in liquid crystals and theoretically predicted in magnetic materials. These may have applications in information storage technology.
- David Foster
- , Charles Kind
- & Ivan I. Smalyukh
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Article |
Multiple Coulomb phase in the fluoride pyrochlore CsNiCrF6
Neutron and X-ray scattering experiments show that the partly disordered material CsNiCrF6 supports multiple Coulomb phases with structural and magnetic properties dictated by underlying local gauge symmetry.
- T. Fennell
- , M. J. Harris
- & S. T. Bramwell
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Article |
Selective breakdown of phonon quasiparticles across superionic transition in CuCrSe2
Neutron and X-ray scattering studies combined with first-principles calculations suggest that the large, liquid-like ionic mobility in the canonical superionic crystal CuCrSe2 is due to anharmonic phonon dynamics.
- Jennifer L. Niedziela
- , Dipanshu Bansal
- & Olivier Delaire
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Phase transition lowering in dynamically compressed silicon
In spite of its wide technological use, the response of silicon to rapid compression remains poorly understood. By means of an X-ray diffraction method based on a free-electron laser, the process for laser-driven dynamic shock compression is now elucidated in this system.
- E. E. McBride
- , A. Krygier
- & A. Higginbotham
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News & Views |
A new twist on phonons
Many particles — both fundamental and emergent — carry angular momentum or spin. Experiments have now demonstrated that phonons can transport angular momentum, showing that they may have spin too.
- Matthias B. Jungfleisch
- & Axel Hoffmann
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Experimental evidence for superionic water ice using shock compression
Although predicted to occur in planetary interiors, superionic water ice has proved elusive to identify experimentally. Laser-driven shock-compression experiments on water ice VII now verify its existence.
- Marius Millot
- , Sebastien Hamel
- & Jon H. Eggert
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Phase ordering of charge density waves traced by ultrafast low-energy electron diffraction
A tracing of the phase-ordering kinetics of a charge density wave system demonstrates the potential of ultrafast low-energy electron diffraction for studying phase transitions and ordering phenomena at surfaces and in low-dimensional systems.
- S. Vogelgesang
- , G. Storeck
- & C. Ropers
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Letter |
4-spin plaquette singlet state in the Shastry–Sutherland compound SrCu2(BO3)2
A detailed neutron scattering study of the Shastry–Sutherland material SrCu2(BO3)2 verifies the existence of a 4-spin plaquette singlet phase in this system.
- M. E. Zayed
- , Ch. Rüegg
- & H. M. Rønnow
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Separating the configurational and vibrational entropy contributions in metallic glasses
When a glass transforms into a liquid, is the absorbed specific heat vibrational or configurational in origin? Vibrational spectroscopy experiments on strong and fragile metallic glasses now strongly suggest the latter.
- Hillary L. Smith
- , Chen W. Li
- & B. Fultz
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