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| Open AccessThe collective photothermal effect of silver nanoparticles probed by a microbolometer
Due to their plasmonic properties, silver nanoparticles are promising across a vast range of applications, from physics instrumentation to biomedicine and environmental science. Here, the photon-to-heat conversion efficiency of individual nanoparticles is elucidated by designing and fabricating an ultra-sensitive bolometer with 26 pW power resolution.
- Hanliang Zhu
- , Evelína Gablech
- & Pavel Neuzil
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Article
| Open AccessSuperlattice assembly strategy of small noble metal nanoparticles for surface-enhanced Raman scattering
Self-assembly of small nanoparticles is difficult to control and the resultant structures have weak stability. Here, a general centimeter-scale superlattice assembly strategy for noble metal nanoparticles of less than 15 nm is used to yield stable hexagonal close-packed monolayers.
- Chang Yao
- , Wuwen Yan
- & Liangbao Yang
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Article
| Open AccessNarrow bandgap silver mercury telluride alloy semiconductor nanocrystal for self-powered midwavelength-infrared photodiode
Infrared colloidal quantum dots are interesting due to their low-cost fabrication and wavelength tunability for optoelectronic applications. Here, air-stable low-noise mid-infrared photodiode devices are fabricated using hole-doped Ag-HgTe nanocrystals.
- Haemin Song
- , So Young Eom
- & Kwang Seob Jeong
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Article
| Open AccessTransistors with ferroelectric ZrXAl1−XOY crystallized by ZnO growth for multi-level memory and neuromorphic computing
Ferroelectric field-effect transistors are interesting for their non-destructive readout characteristic and energy efficiency but are difficult to integrate on silicon platforms. Here, ferroelectricity in ZrXAl1−XOY generated by compressive strain in contact with ZnO is demonstrated, showing promising multi-level memory and synaptic weight performance for neuromorphic computing devices.
- Md Mobaidul Islam
- , Arqum Ali
- & Jin Jang
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Article
| Open AccessLocal tuning of Rydberg exciton energies in nanofabricated Cu2O pillars
Rydberg excitons in cuprous oxide feature giant optical nonlinearities that may be exploited in quantum applications if suitably confined. Here, the authors show how exciton confinement can be realised by focused-ion-beam etching of Cu2O crystals without noticeable degradation of excitonic properties.
- Anindya Sundar Paul
- , Sai Kiran Rajendran
- & Hamid Ohadi
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Article
| Open AccessVisualizing thickness-dependent magnetic textures in few-layer Cr2Ge2Te6
Magnetic ordering in 2D materials represents a promising platform for data storage, computing, and sensing. Here, nanometer scale imaging of few-layer Cr2Ge2Te6 reveals its thickness-dependent magnetic textures such as labyrinth domains and skyrmionic bubbles.
- Andriani Vervelaki
- , Kousik Bagani
- & Martino Poggio
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Article
| Open AccessTowards transparent and durable copper-containing antimicrobial surfaces
Metallic copper is a potent antimicrobial agent against microorganisms but its coating on high-touch surfaces reduces their optical transparency. Here, a transparent antimicrobial nanostructured copper surface is reported with >99.9 % antimicrobial effectiveness and high transmittance.
- Christina Graham
- , Alessia Mezzadrelli
- & Valerio Pruneri
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Article
| Open AccessLocally controlled MOF growth on functionalized carbon nanotubes
Metal-organic frameworks are versatile materials but typically suffer from poor electrical conductivity. Here, a patterning technique allows controlled metal-organic framework growth on predefined areas of functionalized carbon nanotube for increased conductivity.
- Marvin J. Dzinnik
- , Necmettin E. Akmaz
- & Rolf J. Haug
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Article
| Open AccessHistory-dependent nano-photoisomerization by optical near-field in photochromic single crystals
Memory structures are key components of any functional computing device, but achieving persistent storage of information in the form of light is extremely difficult. Here, the authors demonstrate the sequential formation of multiple memory pathways in photochromic crystals via optical near-field interactions.
- Yuji Arakawa
- , Kazuharu Uchiyama
- & Hirokazu Hori
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Article
| Open AccessThree-dimensional distribution of individual atoms in the channels of beryl
Single atom detection in nanoporous materials is challenging due to their sensitivity to electron irradiation. Here, the three-dimensional atomic occupancy of natural beryl is quantitatively analysed using high-angle annular dark-field imaging in a scanning transmission electron microscope and statistical analysis.
- Daniel Knez
- , Christian Gspan
- & Ferdinand Hofer
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Article
| Open AccessThe impact of local pinning sites in magnetic tunnel junctions with non-homogeneous free layers
Pinning sites are extremely detrimental to the frequency tunability of nano-rectifiers based on magnetic tunnel junctions. Here, the effect of pinning defects in vortex-based magnetic tunnel junctions is thoroughly explored, revealing that an amorphous magnetic material utilized as free layer can significantly reduce the impact of pinning.
- Alex. S. Jenkins
- , Leandro Martins
- & Ricardo Ferreira
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Article
| Open AccessNano-assembled open quantum dot nanotube devices
Suspended carbon nanotubes are ideal for hosting long-lived quantum states but mechanically integrating nanotubes into circuits is challenging. Here, by engineering a transparent metal-nanotube interface, the authors can reach the open quantum dot regime and integrate the nanotube within the circuit with a 200 nm precision.
- Tim Althuon
- , Tino Cubaynes
- & Wolfgang Wernsdorfer
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Article
| Open AccessUnidirectional alignment and orientation pinning mechanism of h-BN nucleation on Ir(111) via reactive probe atomic force microscopy
The epitaxial growth of large-scale single-crystalline 2D materials requires precise control over crystallographic orientation and morphology during the initial stages of nucleation. Here, noncontact atomic force microscopy and density functional theory provide atomic-scale mechanistic insights into the nucleation of hexagonal boron nitride on Ir(111).
- Jinliang Pan
- , Tongwei Wu
- & Xiaohui Qiu
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Article
| Open AccessInterfacial interaction promoted titanium oxide-based organic-inorganic nanoheterojunctions by chiral host-guest binding
Achieving close contact between organic and inorganic components in nanostructures is critical for performance. Here, the interfacial interaction in titanium oxide-based organic-inorganic nanoheterojunctions is promoted by host-guest interactions, which are obtained through chiral recognition.
- Juexin Huang
- , Jingyi Xia
- & Chuanliang Feng
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Article
| Open AccessEnhanced thermoelectric performance via quantum confinement in a metal oxide semiconductor field effect transistor for thermal management
Cooling computer chips remains a key requirement for improving their performance. Here, a CMOS-compatible MOSFET is used to electrically, rather than physically, induce quantum confinement in a thermoelectric device, improving its thermoelectric performance and making it a viable microchip thermal management solution.
- Samuel W. Oxandale
- , Charles Reinke
- & Ihab El-Kady
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Article
| Open AccessMXene-reduced graphene oxide sponge-based solar evaporators with integrated water-thermal management by anisotropic design
Water-thermal management is difficult to coordinate in solar evaporators, limiting their performance. Here, hierarchical MXene-reduced graphene oxide sponges with anisotropic thermal conductivity and axial-directional channels integrate water-thermal management for rapid and continuous evaporation.
- Zonglin Liu
- , Renjie Ding
- & Xiaodong He
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Article
| Open AccessPtychographic X-ray computed tomography of porous membranes with nanoscale resolution
The maximum 3D morphology resolution of porous materials without vacuum has been limited to hundreds nanometer range. Here, ptychographic x-ray computed tomography has been demonstrated to study in situ polymeric membranes at nanoscale resolution with large visualization volumes.
- Radosław Górecki
- , Carla Cristina Polo
- & Suzana P. Nunes
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Article
| Open AccessImaging Fermi-level hysteresis in nanoscale bubbles of few-layer MoS2
Nanobubbles are sources of charge trapping that influence the performance and stability of devices based on 2D materials. Here, Kelvin probe force microscopy is used to study the origin and mechanism of charge trapping in nanobubbles of MoS2 on a SiO2 substrate.
- Dohyeon Jeon
- , Haesol Kim
- & Taekyeong Kim
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Article
| Open AccessImpact of exposing lithium metal to monocrystalline vertical silicon nanowires for lithium-ion microbatteries
Lithiation and de-lithiation of lithium-ion microbatteries pose a challenge for adoption due to their extreme volume change and active lithium loss. Here, the surface morphologies of a monocrystalline vertical silicon nanowire-based lithium microbattery were investigated against performance.
- Andam Deatama Refino
- , Egy Adhitama
- & Hutomo Suryo Wasisto
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Article
| Open AccessPre-ceramic polymer-assisted nucleation and growth of copper sulfide nanoplates
It is difficult to control nanoparticle dispersion and size in preceramic polymer composites which require additional processing. Here, a pre-ceramic polymer assists in stable nanoparticle formation and serves as a surface graft for controlled dispersion in a one-pot copper sulfide synthesis.
- Patricia A. Loughney
- , Kara L. Martin
- & Vicky Doan-Nguyen
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Article
| Open AccessProlonged photostability in hexagonal boron nitride quantum emitters
Hexagonal boron nitride is a promising host for single-photon quantum emitters, but irreversible loss of emission by photobleaching hinders its practical use. Here, the mechanistic investigation of hBN emitters reveals two distinct photobleaching lifetimes, suggesting a way to mitigate the shorter, environmentally sensitive, bleaching process.
- Sylvia Xin Li
- , Takeo Ichihara
- & Michael S. Strano
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Article
| Open AccessA multi-timescale synaptic weight based on ferroelectric hafnium zirconium oxide
Brain-inspired neuromorphic computing is a key technology for processing an ever-growing amount of data. Here, an artificial synapse with dual resistance modulation mechanisms is demonstrated, achieving a dynamic range of 60, an endurance exceeding 1010 cycles, and more than 10 years of retention.
- Mattia Halter
- , Laura Bégon-Lours
- & Bert Jan Offrein
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Article
| Open AccessOrigin of electrically induced defects in monolayer MoS2 grown by chemical vapor deposition
Defects are detrimental to the performance of MoS2 field-effect transistors. Here, the origin of defects from prolonged high-field operation is attributed to long-term electrical stress in the transistor ON state, which weakens the Mo-S bonds of the original crystal.
- Ansh Ansh
- , Utpreksh Patbhaje
- & Mayank Shrivastava
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Review Article
| Open AccessNext-generation applications for integrated perovskite solar cells
Integrating perovskite photovoltaics with other systems can substantially improve their performance. This Review discusses various integrated perovskite devices for applications including tandem solar cells, buildings, space applications, energy storage, and cell-driven catalysis.
- Abdulaziz S. R. Bati
- , Yu Lin Zhong
- & Munkhbayar Batmunkh
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Article
| Open AccessScalable fabrication of graphene nanoribbon quantum dot devices with stable orbital-level spacing
Graphene nanoribbons can be used as quantum dot devices, but scalable fabrication methods are needed. Here, a nanobar technique is used to synthesize graphene nanoribbon-based quantum dot devices with a 56 % yield and stable orbital level splitting up to 20 K.
- Toshiaki Kato
- , Takahito Kitada
- & Tomohiro Otsuka
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Article
| Open AccessSub-10 second fly-scan nano-tomography using machine learning
Image reconstruction algorithms used in x-ray computed tomography require that the sample not change throughout the scan, necessitating fast data collection times. Here, a machine learning approach for image processing enables sub-10 second data acquisition times and sub-50 nm pixel resolution.
- Jiayong Zhang
- , Wah-Keat Lee
- & Mingyuan Ge
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Article
| Open AccessSub-volt switching of nanoscale voltage-controlled perpendicular magnetic tunnel junctions
Voltage-controlled magnetic random-access memory is promising for high-performance computing applications. Here, a perpendicular magnetic tunnel junction structure with high voltage-controlled magnetic anisotropy coefficient is developed, allowing sub-volt and sub-nanosecond precessional switching.
- Yixin Shao
- , Victor Lopez-Dominguez
- & Pedram Khalili Amiri
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Article
| Open AccessQubits based on merons in magnetic nanodisks
Merons are spin textures with a half-unit topological charge found in chiral magnetic materials. Here, the authors show that merons with nanometer-scale size are stable and can be used to perform quantum computing gate operations by applying a magnetic field or spin-polarized current.
- Jing Xia
- , Xichao Zhang
- & Motohiko Ezawa
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Article
| Open AccessMachine-learning for designing nanoarchitectured materials by dealloying
Nanoporous metals produced by metal agent dealloying are attractive for multiple applications. Here, a machine learning-augmented framework is reported for predicting, synthesizing and characterizing ternary systems for dealloying.
- Chonghang Zhao
- , Cheng-Chu Chung
- & Yu-chen Karen Chen-Wiegart
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Article
| Open AccessDesign and integration of single-qubit rotations and two-qubit gates in silicon above one Kelvin
Spin qubits are attractive for scalable quantum information, but integrating different classes of two-qubit logic has remained elusive. Here, the SWAP, CPHASE, and CNOT-class two-qubit gates are implemented in a silicon device operating even at temperatures above 1 K.
- Luca Petit
- , Maximilian Russ
- & Menno Veldhorst
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Article
| Open AccessNon-wetting of condensation-induced droplets on smooth monolayer suspended graphene with contact angle approaching 180 degrees
Superhydrophobic behavior of liquid droplets on a surface typically results from chemical and surface topography considerations. Here, contact angles approaching 180° are observed for condensation-induced droplets on suspended monolayer graphene.
- Haidong Wang
- , Daniel Orejon
- & Khellil Sefiane
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Article
| Open AccessNanomechanical signatures of degradation-free influence of water on halide perovskite mechanics
Humidity can change the properties of halide perovskites used in functional devices. Here, indentation experiments reveal that humidity causes an increase in elastic modulus and a decrease in hardness, which is correlated to bond length, hydrogen bonding and polarizability of the ions.
- Isaac Buchine
- , Irit Rosenhek-Goldian
- & Sidney R. Cohen
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Article
| Open AccessBandgap-independent photoconductive detection in two-dimensional Sb2Te3
Achieving photodetectors with a wide spectral range and rapid response remains challenging. Here, Sb2Te3 nanosheets are used to construct a photodetector that covers visible to millimeter wavelengths, with a fast response time of 900 ns.
- Wanli Ma
- , Tuntan Wu
- & Zhiming Huang
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Article
| Open AccessElectrokinetic Janus micromotors moving on topographically flat chemical patterns
Ionic selectivity in microfluidics is challenging due to the differing length scales between ions and channels. Here, a model system emulates ionic transport at the microscale with electrokinetic spherical Janus micromotors moving over surfaces with spatially varying charge.
- Tao Huang
- , Vyacheslav Misko
- & Larysa Baraban
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Article
| Open AccessDisentangling the electronic structure of an adsorbed graphene nanoring by scanning tunneling microscopy
Scanning tunneling microscopy is a powerful tool for determining the electronic structure of surface adsorbates. Here, carbon monoxide functionalized tips enable more accurate probing of the molecular states of graphene nanorings adsorbed on a gold surface.
- Jose Martinez-Castro
- , Rustem Bolat
- & F. Stefan Tautz
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Article
| Open AccessMulti-functional multi-gate one-transistor process-in-memory electronics with foundry processing and footprint reduction
Developing scalable strategies of miniaturization and integration is key for achieving high-density integrated circuit devices. Here, the authors propose a silicon-based one-transistor device with a 40% reduction in circuit footprint, which combines the functionalities of logic gates, memory, and artificial synapses for mass production.
- Mingzhi Dai
- , Zhitang Song
- & Junhao Chu
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Article
| Open AccessNanoscale light field imaging with graphene
Nanoscale light manipulation and characterization are essential in nano-optics, but conventional microscopy or indirect imaging methods are often limited by low resolution or invasive nature. Here, a non-destructive light-field imaging with ~20 nm resolution is realized by p-n junction photodetection in graphene controlled by gate voltage.
- Tongcheng Yu
- , Francisco Rodriguez
- & Alexander N. Grigorenko
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Article
| Open AccessThree-dimensional in situ imaging of single-grain growth in polycrystalline In2O3:Zr films
Understanding grain morphology and kinetics of solid-phase crystallization is important for controlling the functional properties of polycrystalline materials. Here, in situ coherent X-ray diffraction imaging and transmission electron microscopy elucidate quantitatively the kinetics of a single-grain growth in Zr-doped In2O3 films.
- Dmitry Dzhigaev
- , Yury Smirnov
- & Michael Elias Stuckelberger
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Article
| Open AccessExperimentally measuring weak fracture toughness anisotropy in graphene
Graphene is known to display a number of attractive mechanical properties. Here, anisotropy in the fracture toughness of graphene is investigated by in-situ mechanical testing, revealing weak anisotropy between armchair and zigzag directions.
- Shizhe Feng
- , Ke Cao
- & Zhiping Xu
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Article
| Open AccessProximity-induced superconductivity in (Bi1−xSbx)2Te3 topological-insulator nanowires
Topological insulator nanowires are interesting because, in the presence of superconductivity, they may host elusive Majorana fermions. Here, superconductivity in (Bi1−xSbx)2Te3 topological-insulator nanowires is realized by using palladium diffusion, providing a tunable platform for Majorana zero modes.
- Mengmeng Bai
- , Xian-Kui Wei
- & Yoichi Ando
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Article
| Open AccessPtychography at the carbon K-edge
Ptychography is an imaging technique based on algorithmic reconstruction of diffraction patterns that improves the spatial resolution of scanning transmission X-ray microscopy. Here, the possibility of ptychography at the carbon K-edge is demonstrated on carbon nanotube bundles, using a defocused beam to reduce radiation damage.
- Nicolas Mille
- , Hao Yuan
- & Adam P. Hitchcock
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Article
| Open AccessObservation of a flat band and bandgap in millimeter-scale twisted bilayer graphene
Magic-angle twisted bilayer graphene is interesting for its correlated superconducting and insulating states, but samples are typically micrometer-scale. Here, 3 × 5 mm2 twisted bilayer graphene samples are fabricated, exhibiting a flat band and large bandgap revealed by angle-resolved photoemission spectroscopy.
- Keiju Sato
- , Naoki Hayashi
- & Wataru Norimatsu
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Article
| Open AccessIn-plane magnetic field-driven symmetry breaking in topological insulator-based three-terminal junctions
Topological surface states of three-dimensional topological insulators exhibit distinct magnetotransport properties. Here, a steering effect is demonstrated for three-terminal junctions, which is driven by an in-plane magnetic field and makes the junction act as a topoelectric current switch.
- Jonas Kölzer
- , Kristof Moors
- & Thomas Schäpers
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Review Article
| Open AccessDesign principles and biological applications of red-emissive two-photon carbon dots
Carbon dots are suitable for a range of biological applications due to their unique physicochemical properties and biological behavior. This Review summarizes research related to the emerging field of red-emissive two-photon carbon dots for bioimaging, biosensing, and phototherapeutic applications.
- Pooria Lesani
- , Aina Hazeera Mohamad Hadi
- & Hala Zreiqat
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Article
| Open AccessNano-patterning on multilayer MoS2 via block copolymer lithography for highly sensitive and responsive phototransistors
Thin-film phototransistors based on multilayer MoS2 are of great technological importance, but their photoresponsivity may be hindered by an indirect bandgap. Here, nano-patterning of multilayer MoS2 overcomes this limitation by inducing trap states within the bandgap, resulting in a high photoresponsivity of 622.2 A W−1.
- Heekyeong Park
- , Jiyoul Lee
- & Sunkook Kim
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Article
| Open AccessVirtual experimentations by deep learning on tangible materials
Artificial intelligence may significantly accelerate the discovery of new materials but is not easily applicable to non-periodic structures. Here, a deep learning framework is proposed to predict properties of tangible carbon nanotubes by generating virtual structures at different scales and compositions.
- Takashi Honda
- , Shun Muroga
- & Kenji Hata
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Article
| Open AccessMechanical origin of martensite-like structures in two-dimensional ReS2
Two-dimensional materials have well-defined atomic-scale structure, which has the potential to be tuned by processing. Here, substrate-induced straining during the growth of ReS2 causes the formation of martensite-like domain structures.
- Lingli Huang
- , Fangyuan Zheng
- & Thuc Hue Ly
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Article
| Open AccessElectron dynamics of tip-tunable oxygen species on TiO2 surface
Oxygen species on a TiO2 surface exist in different redox states, which can be switched between by electron tunneling with an atomic force tip. Here, a fast experimental setup enables statistically significant tunneling rates to be determined, revealing changes in electronic structure.
- Yuuki Adachi
- , Ján Brndiar
- & Lev Kantorovich
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Article
| Open AccessOrigin and control of ionic hydration patterns in nanopores
The redistribution of water molecules when an ion passes through a nanopore is known to create complex patterns. Here, an analytical model accurately predicts the patterns when an ion passes through a graphene nanopore, and reveals the physical origins of the patterns.
- Miraslau L. Barabash
- , William A. T. Gibby
- & Peter V. E. McClintock