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Article |
Bond-selective fluorescence imaging with single-molecule sensitivity
Two-photon excitation with mid- and near-infrared pulses encodes bond selectivity in fluorescence imaging. Single-molecule imaging and spectroscopy is demonstrated on individual fluorophores as well as various labelled biological targets.
- Haomin Wang
- , Dongkwan Lee
- & Lu Wei
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Letter
| Open AccessCavity-enhanced field-resolved spectroscopy
An ultrabroadband femtosecond enhancement cavity is developed, using gold-coated mirrors and a wedged-diamond-plate input coupler. Simultaneous enhancement of a 22–40 THz offset-free frequency comb allows cavity-enhanced time-domain spectroscopy of gas mixtures based on electro-optic sampling in the mid-infrared range.
- Philipp Sulzer
- , Maximilian Högner
- & Ioachim Pupeza
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Article |
A wavelength-scale black phosphorus spectrometer
A single-photodetector spectrometer based on black phosphorus is demonstrated in the wavelength range from 2 to 9 μm. The footprint is 9 × 16 μm2. The spectrometer is free from bulky interferometers and gratings, and is electrically reconfigurable.
- Shaofan Yuan
- , Doron Naveh
- & Fengnian Xia
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Article |
High-resolution, high-contrast mid-infrared imaging of fresh biological samples with ultraviolet-localized photoacoustic microscopy
Photoacoustic detection highly localized with a pulsed ultraviolet laser based on the Grüneisen relaxation effect allows water-background suppressed mid-infrared (MIR) imaging of lipids and proteins at ultraviolet resolution, at least an order of magnitude finer than the MIR diffraction limits.
- Junhui Shi
- , Terence T. W. Wong
- & Lihong V. Wang
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Letter |
Coherent injection locking of quantum cascade laser frequency combs
Quantum cascade laser frequency combs are coherently locked to an external radio-frequency source even in extremely high-feedback conditions. The internal phase-locking mechanism and the possibility of all-electric stabilization are investigated.
- Johannes Hillbrand
- , Aaron Maxwell Andrews
- & Benedikt Schwarz
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Article |
Mid-infrared frequency comb via coherent dispersive wave generation in silicon nitride nanophotonic waveguides
The direct generation of mid-infrared optical frequency combs in the region 2.5–4.0 μm from a 1.55-μm conventional and compact erbium-fibre-based femtosecond laser is demonstrated via coherent dispersive wave generation in silicon nitride nanophotonic waveguides.
- Hairun Guo
- , Clemens Herkommer
- & Tobias J. Kippenberg
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Article |
High-coherence mid-infrared dual-comb spectroscopy spanning 2.6 to 5.2 μm
By employing difference-frequency generation, a mid-infrared dual-comb spectrometer covering the 2.6 to 5.2 µm range is demonstrated with comb-tooth resolution, sub-MHz frequency precision and accuracy, and a spectral signal-to-noise ratio as high as 6,500.
- Gabriel Ycas
- , Fabrizio R. Giorgetta
- & Nathan R. Newbury
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Letter |
Generation and multi-octave shaping of mid-infrared intense single-cycle pulses
The conversion of shaped near-infrared pulses to shaped, energetic, multi-octave-spanning mid-infrared pulses lasting as little as 1.2 optical cycles is made possible by adiabatic difference frequency generation.
- Peter Krogen
- , Haim Suchowski
- & Jeffrey Moses
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Article |
Optical microresonators as single-particle absorption spectrometers
Single-particle double-modulation absorption spectrometers based on whispering-gallery-mode microresonators achieve sub-100-Hz sensitivity to photothermal resonance shifts and allow for the study of arrays of Fano resonances in the context of plasmonic–photonic hybridization.
- Kevin D. Heylman
- , Niket Thakkar
- & Randall H. Goldsmith
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Article |
Ultrafast switching of tunable infrared plasmons in indium tin oxide nanorod arrays with large absolute amplitude
Ultrafast plasmon modulation has been realized in the near- to mid-infrared range by intraband pumping of indium tin oxide nanorod arrays.
- Peijun Guo
- , Richard D. Schaller
- & Robert P. H. Chang
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Letter |
Infrared spectroscopy with visible light
The refractive index and absorption coefficient of a medium in the infrared range are measured using visible spectral range components. The technique relies on nonlinear interference of infrared and visible photons, produced by down-conversion.
- Dmitry A. Kalashnikov
- , Anna V. Paterova
- & Leonid A. Krivitsky
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Letter |
High-power sub-two-cycle mid-infrared pulses at 100 MHz repetition rate
A compact source that generates sub-two-cycle-duration pulses with an average power of 0.1 W spanning 6.8–16.4 μm combines the properties of power scalability, high repetition rate and phase coherence for the first time in this spectral region.
- I. Pupeza
- , D. Sánchez
- & J. Biegert
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Article |
Quantum cascade laser frequency stabilization at the sub-Hz level
A 10 μm quantum cascade laser is phase-locked to a remote ultrastable laser referenced to primary frequency standards using an optical frequency comb. The obtained relative stability of 2 × 10−15 is record-breaking in the mid-infrared region.
- Bérengère Argence
- , Bruno Chanteau
- & Anne Amy-Klein
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News & Views |
Entering the mid-infrared
The demonstration of chalcogenide fibre-based supercontinuum sources that reach beyond a wavelength of ten micrometres is set to have a major impact on spectroscopy and molecular sensing.
- Günter Steinmeyer
- & Julia S. Skibina
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Letter |
Ultrafast multi-terahertz nano-spectroscopy with sub-cycle temporal resolution
The authors demonstrate ultrabroadband time-resolved THz spectroscopy on a single InAs nanowire with 10 nm spatial resolution and sub-100 fs time resolution.
- M. Eisele
- , T. L. Cocker
- & R. Huber
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Letter |
Tip-enhanced infrared nanospectroscopy via molecular expansion force detection
Mid-infrared spectroscopy with nanometre spatial resolution is highly desired for materials and life sciences applications. A nanoscale mid-infrared spectrometer is demonstrated that detects mechanical forces exerted by molecules on an atomic force microscope tip upon light excitation. It operates under ambient conditions with a high sensitivity and a spatial resolution of better than 25 nm.
- Feng Lu
- , Mingzhou Jin
- & Mikhail A. Belkin
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