News & Views |
Featured
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Letter |
Groundwater quality and depletion in the Indo-Gangetic Basin mapped from in situ observations
Increasing groundwater abstraction in the Indo-Gangetic Basin poses a threat to groundwater supplies. In situ observations reveal that sustainable groundwater in much of the region is limited more by contamination than depletion.
- A. M. MacDonald
- , H. C. Bonsor
- & S. K. Yadav
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Article |
Redox-induced lower mantle density contrast and effect on mantle structure and primitive oxygen
The origin of large-scale mantle heterogeneities remains enigmatic. Experiments show that different oxygen fugacities lead to density differences in lower-mantle materials, which lead to a heterogeneously oxidized mantle in simulations.
- Tingting Gu
- , Mingming Li
- & Kanani K. M. Lee
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Editorial |
Not just carbon widgets
Forests are important for the global carbon cycle, and for mitigating greenhouse gas emissions. However, the role forests play in carbon sequestration should not eclipse everything else we value them for.
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News & Views |
The return of ethane
Ethane emissions can lead to ozone pollution. Measurements at 49 sites show that long-declining atmospheric ethane concentrations started rising in 2010 in the Northern Hemisphere, largely due to greater oil and gas production in the USA.
- Hannele Hakola
- & Heidi Hellén
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Letter |
Reversal of global atmospheric ethane and propane trends largely due to US oil and natural gas production
Atmospheric non-methane hydrocarbon concentrations began declining in the 1970s. Surface and column measurements show that Northern Hemisphere ethane concentrations are now rising, probably due to North American oil and natural gas emissions.
- Detlev Helmig
- , Samuel Rossabi
- & Andrea Pozzer
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Editorial |
Earth's changeable atmosphere
Billions of years ago, high atmospheric greenhouse gas concentrations were vital to life's tenuous foothold on Earth. Despite new constraints, the composition and evolution of Earth's early atmosphere remains hazy.
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Letter |
Space-based detection of missing sulfur dioxide sources of global air pollution
Sulfur dioxide is a key air contaminant. A satellite-based emissions inventory reveals a number of hitherto unknown sources, with a cluster around the Persian Gulf, and identifies large discrepancies with conventional inventories in some regions.
- Chris A. McLinden
- , Vitali Fioletov
- & Joanna Joiner
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News & Views |
A hump in ocean–air exchange
Semivolatile organic compounds from fossil fuels or incomplete combustion are ubiquitous. A suite of circumglobal measurements of their oceanic and atmospheric concentrations reveals large carbon fluxes through the deposition of these compounds.
- Christopher M. Reddy
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Letter |
High atmosphere–ocean exchange of semivolatile aromatic hydrocarbons
The global transport and fate of semivolatile aromatic hydrocarbons and their relevance for the carbon cycle are poorly quantified. Global measurements in paired atmospheric and ocean samples suggest that their contribution is substantial.
- Belén González-Gaya
- , María-Carmen Fernández-Pinos
- & Jordi Dachs
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Letter |
Airborne soil organic particles generated by precipitation
Airborne organic particles affect Earth’s climate. Imaging of particles after rain events and experimental irrigation shows that water drop impaction of soils generates solid organic particles, with impacts on clouds and radiation absorption.
- Bingbing Wang
- , Tristan H. Harder
- & Alexander Laskin
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News & Views |
The fate of phosphorus
Phosphorus is essential for food production, but it is also a key cause of eutrophication. Estimates of phosphorus flux for the past 40–70 years reveal that large river basins can experience phases of phosphorus accumulation and depletion.
- Julien Némery
- & Josette Garnier
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Letter |
Long-term accumulation and transport of anthropogenic phosphorus in three river basins
Phosphorus fertilizer use has roughly quadrupled in the past century. Budgets constructed from historical data show that phosphorus rapidly accumulates in river basins during periods of high inputs and continues to mobilize after inputs decline.
- Stephen M. Powers
- , Thomas W. Bruulsema
- & Fusuo Zhang
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Letter |
Large increases in Arctic biogenic volatile emissions are a direct effect of warming
Volatile organic compounds can affect air quality and climate. Experimental warming of vegetated tundra plots in Greenland increased biogenic volatile organic compound emissions from vegetation and soils by 260%, as a direct effect.
- Magnus Kramshøj
- , Ida Vedel-Petersen
- & Riikka Rinnan
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Letter |
Biological role in the transformation of platinum-group mineral grains
Microbes can mineralize metals such as gold. Observations of platinum-group mineral grains and incubation experiments reveal that bacteria can also transform these metals, which could affect their mobility in surface environments.
- Frank Reith
- , Carla M. Zammit
- & Joël Brugger
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Letter |
High aerosol acidity despite declining atmospheric sulfate concentrations over the past 15 years
Atmospheric sulfate levels are thought to determine the pH of small aerosol particles. Thermodynamic analysis of field aerosol data reveals that fine particles remain acidic in the southeastern United States despite large sulfate reductions.
- Rodney J. Weber
- , Hongyu Guo
- & Athanasios Nenes
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News & Views |
Clues to hidden copper deposits
Economic-grade deposits of copper are hard to find. The aluminium content of magmatic rocks at the surface may provide an indicator of ore deposits buried deep below.
- Jeremy Richards
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News & Views |
Phytoplankton in a witch's brew
Natural seafloor hydrocarbon seeps are responsible for roughly half of the oil released into the ocean. As these oils and gases rise to the surface, they transport nutrients upwards, benefiting phytoplankton in the upper sunlit layer.
- Michael Behrenfeld
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News & Views |
Your feet's too big
Humanity's nitrogen pollution footprint has increased by a factor of six since the 1930s. A global analysis reveals that a quarter of this nitrogen pollution is associated with the production of internationally traded products.
- James N. Galloway
- & Allison M. Leach
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Letter |
High solar cycle spectral variations inconsistent with stratospheric ozone observations
Variability in solar UV radiation is uncertain, but it affects Earth’s climate. Simulations of the ozone response to various data sets of spectral solar irradiance show that high-amplitude solar variability is inconsistent with ozone observations.
- W. T. Ball
- , J. D. Haigh
- & W. Schmutz
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Letter |
Elevated surface chlorophyll associated with natural oil seeps in the Gulf of Mexico
Natural hydrocarbon seeps account for up to 47% of the oil released into the oceans. In situ and remote measurements of chlorophyll concentrations suggest that natural hydrocarbons enhance productivity in surface waters in the Gulf of Mexico.
- N. A. D’souza
- , A. Subramaniam
- & J. P. Montoya
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News & Views |
Better living through mercury
Mercury is a toxic element with no known biological function. Laboratory studies demonstrate that mercury can be beneficial to microbial growth by acting as an electron acceptor during photosynthesis.
- Jeffra K. Schaefer
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Letter |
Substantial proportion of global streamflow less than three months old
Streamflow is a mixture of precipitation of various ages. Oxygen isotope data suggests that a third of global river discharge is sourced from rainfall within the past few months, which accounts for less than 0.1% of global groundwater.
- Scott Jasechko
- , James W. Kirchner
- & Jeffrey J. McDonnell
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Letter |
A physiological role for HgII during phototrophic growth
Bacteria have been shown to be involved in the reduction of HgII to elemental mercury. Laboratory experiments with HgII and different carbon sources reveal that purple bacteria can use HgII as an electron acceptor, promoting bacterial growth.
- D. S. Grégoire
- & A. J. Poulain
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Letter |
Enhanced Southern Ocean marine productivity due to fertilization by giant icebergs
Nutrient input from icebergs can fertilize productivity in the ocean. Ten years of satellite measurements reveal that giant icebergs could be responsible for up to 20% of carbon export to depth in the Southern Ocean.
- Luis P. A. M. Duprat
- , Grant R. Bigg
- & David J. Wilton
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Letter |
Nitrous oxide sinks and emissions in boreal aquatic networks in Québec
Aquatic ecosystems are important sources of the greenhouse gas nitrous oxide. Measurements of nitrous oxide concentrations from 321 rivers, lakes and ponds in Canada reveal that some boreal aquatic systems can act as net nitrous oxide sinks.
- C. Soued
- , P. A. del Giorgio
- & R. Maranger
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Letter |
Sub-micrometre particulate matter is primarily in liquid form over Amazon rainforest
The physical state of atmospheric particulate matter affects its growth and reactivity, which can affect climate. Measurements of particle rebound reveal that particulate matter over the Amazon forest is usually liquid during wet and dry seasons.
- Adam P. Bateman
- , Zhaoheng Gong
- & Scot T. Martin
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Letter |
Chemical weathering in active mountain belts controlled by stochastic bedrock landsliding
In active mountain belts, erosion is driven by bedrock landsliding. River water chemistry in New Zealand’s Southern Alps suggests that stochastic mass wasting processes also enhance chemical weathering in such environments.
- Robert Emberson
- , Niels Hovius
- & Odin Marc
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Article |
Arsenic release metabolically limited to permanently water-saturated soil in Mekong Delta
Microbial reduction of arsenic-bearing iron oxides releases arsenic into groundwater in Asia. Laboratory and field studies in the Mekong Delta reveal that arsenic release is limited to near-surface sediments of permanently saturated wetlands.
- Jason W. Stuckey
- , Michael V. Schaefer
- & Scott Fendorf
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Editorial |
Preserve soil's riches
The International Year of Soils draws attention to our vital dependence on the fertile crumb beneath our feet. Soil is renewable, but it takes careful stewardship to keep it healthy and plentiful.
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Letter |
Significant fraction of CO2 emissions from boreal lakes derived from hydrologic inorganic carbon inputs
Lakes are a large source of CO2. An analysis of chemical and physical data from 5,118 boreal lakes reveals that a majority emit CO2 originating primarily from terrestrial sources rather than CO2 produced within the lakes.
- Gesa A. Weyhenmeyer
- , Sarian Kosten
- & Fabio Roland
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News & Views |
The ocean's pressure cooker
Little is known about the mechanisms that destroy the oldest organic molecules found in seawater. Field and laboratory observations suggest that these molecules are destroyed by the heat and pressure of deep-sea hydrothermal systems.
- Steven R. Beaupré
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Letter |
Efficient removal of recalcitrant deep-ocean dissolved organic matter during hydrothermal circulation
The fate of old, recalcitrant dissolved organic carbon in oceans is unclear. Field samples show that loss during circulation in hydrothermal vents can account for the 40-million-year lifetime of recalcitrant dissolved organic carbon in oceans.
- Jeffrey A. Hawkes
- , Pamela E. Rossel
- & Thorsten Dittmar
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Article |
Substantial iron sequestration during green-clay authigenesis in modern deep-sea sediments
Pyrite formation has been considered a key iron sink in organic-rich marine sediments. Analyses of sediments from the Ivory Coast–Ghana Marginal Ridge demonstrate that iron can be buried at greater rates during green-clay formation.
- A. Baldermann
- , L. N. Warr
- & V. Mavromatis
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News & Views |
Breathing easier in the Amazon
Fires related to Amazonian deforestation are a large source of particulate matter emissions. Satellite measurements and models reveal that reductions in deforestation and fire emissions since 2001 have prevented hundreds of premature deaths each year.
- Christine Wiedinmyer
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Letter |
Air quality and human health improvements from reductions in deforestation-related fire in Brazil
Fires are used to clear tropical forests. Satellite measurements and simulations show that reductions in deforestation and associated fires in Brazil have reduced emissions of particulate matter, preventing between 400 and 1,700 deaths annually.
- C. L. Reddington
- , E. W. Butt
- & D. V. Spracklen
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Letter |
Formation of soil organic matter via biochemical and physical pathways of litter mass loss
Soil organic matter is a large global carbon pool. Isotopic labelling of litter in the lab and the field reveals that soil organic matter forms from labile organic compounds and litter fragments early and late in decomposition, respectively.
- M. Francesca Cotrufo
- , Jennifer L. Soong
- & William J. Parton
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News & Views |
Soil carbon in a beer can
Decomposition of soil organic matter could be an important positive feedback to climate change. Geochemical properties of soils can help determine what fraction of soil carbon may be protected from climate-induced decomposition.
- Eric A. Davidson
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Letter |
Soil carbon storage controlled by interactions between geochemistry and climate
Rising temperature can increase soil organic matter decomposition and CO2 emissions. In a 4,000 km north–south transect in Chile and Antarctica, soil geochemistry, which can be modified by climate, is the dominant direct control of carbon storage.
- Sebastian Doetterl
- , Antoine Stevens
- & Pascal Boeckx
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News & Views |
Ozone pollution from near and far
Tropospheric ozone is generated from precursor pollutants, but can be blown far afield. Satellite observations show rising ozone levels over China — and almost stable levels over western North America despite stricter regulations.
- Ruth M. Doherty
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Letter |
Rapid increases in tropospheric ozone production and export from China
Tropospheric levels of ozone and its precursors have risen in Asia since 2000. Satellite observations and chemistry–transport simulations suggest that transport of these pollutants to North America partly offsets benefits from stricter regulation.
- Willem W. Verstraeten
- , Jessica L. Neu
- & K. Folkert Boersma
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Letter |
Sources of and processes controlling CO2 emissions change with the size of streams and rivers
Rivers and streams are key sources of CO2. Estimated emissions and aquatic productivity from across the US show that small streams predominantly emit CO2 produced in soils, but the contribution from aquatic metabolism increases with river size.
- E. R. Hotchkiss
- , R. O. Hall Jr
- & J. Karlsson
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Article |
Globally significant greenhouse-gas emissions from African inland waters
Inland waters are important sources of greenhouse gases. Measurements over eight years suggest that African inland waters are a substantial source of greenhouse gases, equivalent to a quarter of the global land and ocean carbon sink.
- Alberto V. Borges
- , François Darchambeau
- & Steven Bouillon
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Letter |
A marine sink for chlorine in natural organic matter
Chloride is abundant in oceans, but is relatively unreactive. Spectroscopic imaging reveals the presence of a chloride sink in organochlorine compounds that can be produced abiotically or by phytoplankton.
- Alessandra C. Leri
- , Lawrence M. Mayer
- & Austin B. Gellis
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News & Views |
A tropical hotspot
The ocean is an important source of the potent greenhouse gas N2O. Measurements in the tropical South Pacific have revealed a massive efflux of N2O from the coastal upwelling zone.
- Imke Grefe
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Letter |
Massive nitrous oxide emissions from the tropical South Pacific Ocean
Oceans emit a third of the natural emissions of nitrous oxide. High-resolution measurements suggest that the Peruvian coast is a hotspot of nitrous oxide fluxes, representing 5–22% of global ocean emissions from previous estimates.
- D. L. Arévalo-Martínez
- , A. Kock
- & H. W. Bange
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Letter |
Stable runoff and weathering fluxes into the oceans over Quaternary climate cycles
The effect of glacial–interglacial cycles on surface weathering rates has been unclear. A beryllium-based proxy for weathering shows minimal variations in the input of silicate weathering products to the oceans for the past two million years.
- Friedhelm von Blanckenburg
- , Julien Bouchez
- & Kate Maher
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News & Views |
Hoard of fjord carbon
Fjords account for less than 0.1% of the surface of Earth's oceans. A global assessment finds that organic carbon is buried in fjords five times faster than other marine systems, accounting for 11% of global marine organic carbon burial.
- Richard Keil
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Letter |
High rates of organic carbon burial in fjord sediments globally
Fjords have been hypothesized to be hotspots of organic carbon burial. A global compilation of organic carbon data and sedimentation rates shows that fjords sequester twice as much carbon as other ocean regions.
- Richard W. Smith
- , Thomas S. Bianchi
- & Valier Galy