Featured
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Origin of structural degradation in Li-rich layered oxide cathode
Diffractive imaging of an important class of battery electrodes during cycling shows that lattice strain is a crucial yet overlooked factor that contributes to voltage fade over time.
- Tongchao Liu
- , Jiajie Liu
- & Khalil Amine
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Article |
Programmable heating and quenching for efficient thermochemical synthesis
By using a programmable electric current to allow rapid pulsed heating and quenching, a non-equilibrium, continuous synthesis technique shows improved performance in thermochemical reactions, as well as lower energy costs.
- Qi Dong
- , Yonggang Yao
- & Liangbing Hu
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Revitalizing interface in protonic ceramic cells by acid etch
A simple acid treatment can improve high-temperature annealed electrolyte surfaces, resulting in improved performance and stability at lower temperatures for protonic ceramic fuel/electrolysis cells, offering new understanding for sustainable energy infrastructures.
- Wenjuan Bian
- , Wei Wu
- & Dong Ding
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Article
| Open AccessThermophotovoltaic efficiency of 40%
Two-junction TPV cells with efficiencies of more than 40% are reported, using an emitter with a temperature between 1,900 and 2,400 °C, for integration into a TPV system for thermal energy grid storage.
- Alina LaPotin
- , Kevin L. Schulte
- & Asegun Henry
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Article |
Perovskite–organic tandem solar cells with indium oxide interconnect
A thin low-loss indium oxide interconnect layer grown by atomic layer deposition enables perovskite–organic hybrid tandem solar cells with a high open-circuit voltage and a high power conversion efficiency.
- K. O. Brinkmann
- , T. Becker
- & T. Riedl
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Article |
Metastable hexagonal close-packed palladium hydride in liquid cell TEM
A metastable palladium hydride is synthesized where the unique environment in the liquid cell, namely the limited quantity of Pd precursors and the continuous supply of H, resulted in the formation of the hcp phase.
- Jaeyoung Hong
- , Jee-Hwan Bae
- & Dong Won Chun
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Perspective |
Towards enduring autonomous robots via embodied energy
The concept of 'Embodied Energy'—in which the components of a robot or device both store energy and provide a mechanical or structural function—is put forward, along with specific robot-design principles.
- Cameron A. Aubin
- , Benjamin Gorissen
- & Robert F. Shepherd
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Article
| Open AccessMagnetic control of tokamak plasmas through deep reinforcement learning
A newly designed control architecture uses deep reinforcement learning to learn to command the coils of a tokamak, and successfully stabilizes a wide variety of fusion plasma configurations.
- Jonas Degrave
- , Federico Felici
- & Martin Riedmiller
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Perspective |
The challenges and opportunities of battery-powered flight
The economic, technical, environmental and safety requirements of battery-powered aircraft are considered, and promising technologies and future prospects for battery innovation are discussed.
- Venkatasubramanian Viswanathan
- , Alan H. Epstein
- & Michael Winter
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Article
| Open AccessBurning plasma achieved in inertial fusion
A burning plasma, a critical step towards self-sustaining fusion, is achieved at the US National Ignition Facility, with a subset of experiments demonstrating fusion self-heating beyond radiation and conduction losses.
- A. B. Zylstra
- , O. A. Hurricane
- & G. B. Zimmerman
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Centimetre-scale perovskite solar cells with fill factors of more than 86 per cent
Perovskite solar cells including charge transport material fabricated using a reverse-doping process have the highest certified efficiency for cells of 1-cm2 active area and the highest fill factor reported so far.
- Jun Peng
- , Felipe Kremer
- & Kylie R. Catchpole
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Article |
All-perovskite tandem solar cells with improved grain surface passivation
A certified efficiency of 26.4% in all-perovskite tandem solar cells, exceeding that of the best-performing single-junction perovskite solar cells, is achieved by control over surface defects in the Pb–Sn subcell.
- Renxing Lin
- , Jian Xu
- & Hairen Tan
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Article |
Elastomeric electrolytes for high-energy solid-state lithium batteries
An elastomeric solid-state electrolyte shows desirable mechanical properties and high electrochemical stability, and is used to demonstrate a high-energy solid-state lithium battery at ambient temperature.
- Michael J. Lee
- , Junghun Han
- & Seung Woo Lee
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Article |
High-entropy polymer produces a giant electrocaloric effect at low fields
A study reports and characterizes a high-entropy electrocaloric polymer that switches under low fields, and discusses its potential suitability for use in caloric heat pumps.
- Xiaoshi Qian
- , Donglin Han
- & Q. M. Zhang
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Dynamic spatial progression of isolated lithium during battery operations
An electrochemical process stimulates the progression toward the electrode of isolated or ‘dead’ lithium in a battery, recovering its electrical connection, and the effect is demonstrated by increased cycle life.
- Fang Liu
- , Rong Xu
- & Yi Cui
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Article |
Drop-in fuels from sunlight and air
Carbon-neutral hydrocarbon fuels can be produced using sunlight and air via a thermochemical solar fuel production chain, thus representing a pathway towards the long-term decarbonization of the aviation sector.
- Remo Schäppi
- , David Rutz
- & Aldo Steinfeld
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Article |
Perovskite solar cells with atomically coherent interlayers on SnO2 electrodes
An atomically coherent interlayer between the electron-transporting and perovskite layers in perovskite solar cells enhances charge extraction and transport from the perovskite, enabling high power conversion efficiency.
- Hanul Min
- , Do Yoon Lee
- & Sang Il Seok
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Article |
The role of charge recombination to triplet excitons in organic solar cells
A substantial pathway for energy loss in organic solar cells may be suppressed by engineering hybridization between non-fullerene acceptor triplet excitons and spin-triplet charge transfer excitons.
- Alexander J. Gillett
- , Alberto Privitera
- & Richard H. Friend
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Article |
Unextractable fossil fuels in a 1.5 °C world
A global energy system model finds that planned fossil fuel extraction is inconsistent with limiting global warming to 1.5 °C, because the majority of fossil fuel reserves must stay in the ground.
- Dan Welsby
- , James Price
- & Paul Ekins
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Article |
Scalable production of high-performing woven lithium-ion fibre batteries
Rechargeable lithium-ion batteries produced in the form of metre-long fibres can be woven into sturdy, washable textiles on an industrial loom and used to power other fabric-based electronic components.
- Jiqing He
- , Chenhao Lu
- & Huisheng Peng
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Article |
Photocatalytic solar hydrogen production from water on a 100-m2 scale
Carbon-neutral hydrogen can be produced through photocatalytic water splitting, as demonstrated here with a 100-m2 array of panel reactors that reaches a maximum conversion efficiency of 0.76%.
- Hiroshi Nishiyama
- , Taro Yamada
- & Kazunari Domen
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Article |
Rechargeable Na/Cl2 and Li/Cl2 batteries
Rechargeable Na/Cl2 and Li/Cl2 batteries are produced with a microporous carbon positive electrode, aluminium chloride in thionyl chloride as the electrolyte, and either sodium or lithium as the negative electrode.
- Guanzhou Zhu
- , Xin Tian
- & Hongjie Dai
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Article |
A process-based approach to understanding and managing triggered seismicity
A multidisciplinary method for managing triggered seismicity is developed using detailed subsurface information to calibrate geomechanical and earthquake source physics models, and is applied to the Val d’Agri oil field in seismically active southern Italy.
- Bradford H. Hager
- , James Dieterich
- & Andreas Plesch
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Perspective |
Designing the next generation of proton-exchange membrane fuel cells
This Perspective reviews the recent technical developments in the components of the fuel cell stack in proton-exchange membrane fuel cell vehicles and outlines the road towards large-scale commercialization of such vehicles.
- Kui Jiao
- , Jin Xuan
- & Michael D. Guiver
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Article |
Tomographic reconstruction of oxygen orbitals in lithium-rich battery materials
High-energy X-ray Compton measurements and first-principles modelling reveal how the electronic orbital responsible for the reversible anionic redox activity can be imaged and visualized, and its character and symmetry determined.
- Hasnain Hafiz
- , Kosuke Suzuki
- & Venkatasubramanian Viswanathan
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Perspective |
The data-driven future of high-energy-density physics
This Perspective discusses how high-energy-density physics could tap the potential of AI-inspired algorithms for extracting relevant information and how data-driven automatic control routines may be used for optimizing high-repetition-rate experiments.
- Peter W. Hatfield
- , Jim A. Gaffney
- & Ben Williams
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Article |
A dynamic stability design strategy for lithium metal solid state batteries
A multi-layered electrolyte, in which a less stable electrolyte is sandwiched between two electrolyte layers that are more stable, can inhibit the growth of lithium dendrites in highly pressurized solid-state lithium metal batteries.
- Luhan Ye
- & Xin Li
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Article |
Polypeptide organic radical batteries
An environmentally friendly, all-organic radical battery is demonstrated, in which redox-active polypeptides perform as both cathode and anode materials, with a metal-free organic electrolyte.
- Tan P. Nguyen
- , Alexandra D. Easley
- & Karen L. Wooley
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Article |
A highly stable and flexible zeolite electrolyte solid-state Li–air battery
Flexible, stable and energy-dense solid-state Li–air batteries are realised using ultrathin, chemically inert ion-conductive zeolite membranes as a solid electrolyte.
- Xiwen Chi
- , Malin Li
- & Jihong Yu
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Article |
Diversity-oriented synthesis of polymer membranes with ion solvation cages
A diversity-oriented synthesis approach that yields a library of architecturally broad microporous polymers is used to develop structurally diverse polymer membranes with ion specificity and to screen their properties.
- Miranda J. Baran
- , Mark E. Carrington
- & Brett A. Helms
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Article |
Pseudo-halide anion engineering for α-FAPbI3 perovskite solar cells
Incorporation of the pseudo-halide anion formate during the fabrication of α-FAPbI3 perovskite films eliminates deleterious iodide vacancies, yielding solar cell devices with a certified power conversion efficiency of 25.21 per cent and long-term operational stability.
- Jaeki Jeong
- , Minjin Kim
- & Jin Young Kim
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Article |
Thermal-expansion offset for high-performance fuel cell cathodes
Highly active but durable perovskite-based solid oxide fuel cell cathodes are realized using a thermal-expansion offset, achieving full thermo-mechanical compatibility between the cathode and other cell components.
- Yuan Zhang
- , Bin Chen
- & Zongping Shao
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Article |
Efficient perovskite solar cells via improved carrier management
An improved device design for perovskite-based photovoltaic cells enables a certified power conversion efficiency of 25.2 per cent, translating to 80.5 per cent of the thermodynamic limit for its bandgap, which approaches those achieved by silicon solar cells.
- Jason J. Yoo
- , Gabkyung Seo
- & Jangwon Seo
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Article |
Angular momentum generation in nuclear fission
γ-ray spectroscopy experiments on the origin of spin in the products of nuclear fission of spin-zero nuclei suggest that the fission fragments acquire their spin after scission, rather than before.
- J. N. Wilson
- , D. Thisse
- & S. Ziliani
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Near-perfect photon utilization in an air-bridge thermophotovoltaic cell
An air gap embedded within the structure of a thermophotovoltaic device acts as a near-perfect reflector of low-energy photons, resulting in their recovery and recycling by the thermal source, enabling excellent power-conversion efficiency.
- Dejiu Fan
- , Tobias Burger
- & Stephen R. Forrest
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Article |
Rare-earth–platinum alloy nanoparticles in mesoporous zeolite for catalysis
Alloy nanoparticles of platinum and rare-earth elements are formed using zeolites with pore-wall defects, producing stable, highly active and selective catalysts for the propane dehydrogenation reaction.
- Ryong Ryoo
- , Jaeheon Kim
- & Jae Won Shin
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Article |
A disordered rock salt anode for fast-charging lithium-ion batteries
A vanadium-based lithium-rich disordered rock salt oxide is shown to work as a low-potential anode with rapid intercalation kinetics for lithium-ion batteries.
- Haodong Liu
- , Zhuoying Zhu
- & Ping Liu
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Article |
A mobile robotic chemist
A mobile robot autonomously operates analytical instruments in a wet chemistry laboratory, performing a photocatalyst optimization task much faster than a human would be able to.
- Benjamin Burger
- , Phillip M. Maffettone
- & Andrew I. Cooper
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On-device lead sequestration for perovskite solar cells
Using lead-absorbing materials to coat the front and back of perovskite solar cells can prevent lead leaching from damaged devices, without affecting the device performance or long-term operation stability.
- Xun Li
- , Fei Zhang
- & Tao Xu
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Article |
Power generation from ambient humidity using protein nanowires
A new type of energy-harvesting device, based on protein nanowires from the microbe Geobacter sulforreducens, can generate a sustained power output by producing a moisture gradient across the nanowire film using natural humidity.
- Xiaomeng Liu
- , Hongyan Gao
- & Jun Yao
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Matters Arising |
Reply to: Why fossil fuel producer subsidies matter
- Jessica Jewell
- , Johannes Emmerling
- & Detlef van Vuuren
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Matters Arising |
Why fossil fuel producer subsidies matter
- Peter Erickson
- , Harro van Asselt
- & Geoffrey Supran
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Article |
A droplet-based electricity generator with high instantaneous power density
A device involving a polytetrafluoroethylene film, an indium tin oxide substrate and an aluminium electrode allows improved electricity generation from water droplets, which bridge the previously disconnected circuit components.
- Wanghuai Xu
- , Huanxi Zheng
- & Zuankai Wang
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Article |
Superstructure control of first-cycle voltage hysteresis in oxygen-redox cathodes
In oxygen-redox intercalation cathodes, voltage hysteresis can be avoided by forming cathode materials with a ‘ribbon’ superstructure in the transition metal layers that suppresses transition metal migration.
- Robert A. House
- , Urmimala Maitra
- & Peter G. Bruce
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Molecular tuning of CO2-to-ethylene conversion
Electrocatalytic reduction of CO2 over copper can be made highly selective by ‘tuning’ the copper surface with adsorbed organic molecules to stabilize intermediates for carbon-based fuels such as ethylene
- Fengwang Li
- , Arnaud Thevenon
- & Edward H. Sargent
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Article |
Thermoelectric performance of a metastable thin-film Heusler alloy
A high intrinsic thermoelectric figure of merit is found for a metastable thin-film Fe2V0.8W0.2Al Heusler alloy.
- B. Hinterleitner
- , I. Knapp
- & E. Bauer
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Review Article |
Recycling lithium-ion batteries from electric vehicles
Processes for dismantling and recycling lithium-ion battery packs from scrap electric vehicles are outlined.
- Gavin Harper
- , Roberto Sommerville
- & Paul Anderson
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Article |
Carrier-resolved photo-Hall effect
A carrier-resolved photo-Hall technique is developed to extract properties of both majority and minority carriers simultaneously and determine the critical parameters of semiconductor materials under light illumination.
- Oki Gunawan
- , Seong Ryul Pae
- & Byungha Shin
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Letter |
Intrinsically stable organic solar cells under high-intensity illumination
Organic photovoltaic cells containing an intrinsically stable organic absorber layer that are likely to be stable for many decades under illumination are demonstrated.
- Quinn Burlingame
- , Xiaheng Huang
- & Stephen R. Forrest