Featured
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| Open AccessTomography of memory engrams in self-organizing nanowire connectomes
Hardware architectures based on self-organized memristive networks of nano objects have attracted a growing attention. Here, nanowire connectomes are experimentally proved to translate spatially correlated short-term plasticity effects into long-lasting topological changes, thus emulating both information encoding and memory consolidation of human brain.
- Gianluca Milano
- , Alessandro Cultrera
- & Carlo Ricciardi
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Article
| Open AccessEncoding multistate charge order and chirality in endotaxial heterostructures
Phase transitions in charge density wave materials could be useful for memory and electronic device applications. Here, the authors correlate the temperature-driven transitions in the electrical and optical properties of H-TaS2/1T-TaS2 heterostructures to the number of endotaxial metallic H-TaS2 monolayers.
- Samra Husremović
- , Berit H. Goodge
- & D. Kwabena Bediako
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| Open AccessAn all 2D bio-inspired gustatory circuit for mimicking physiology and psychology of feeding behavior
Implementing emotional aspects like physiology and psychology in decision-making remains a challenge. Here, the authors propose a bio-inspired gustatory circuit based on 2D materials that mimics adaptive feeding behavior in humans, considering both physiological states (hunger) and psychological states (appetite).
- Subir Ghosh
- , Andrew Pannone
- & Saptarshi Das
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Article
| Open AccessMultimaterial fiber as a physical simulator of a capillary instability
Capillary breakup in multimaterial fibers is explored for the self-assembly of optoelectronic systems. However, its insights primarily stem from numerical simulations, qualitative at best. The authors formulate an analytical model of such breakup, obtaining a window in the governing parameters where the generally chaotic breakup becomes predictable and thus engineerable.
- Camila Faccini de Lima
- , Fan Wang
- & Alexander Gumennik
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Article
| Open AccessEngineering the formation of spin-defects from first principles
Spin defects in semiconductors are promising for quantum technologies but understanding of defect formation processes in experiment remains incomplete. Here the authors present a computational protocol to study the formation of spin defects at the atomic scale and apply it to the divacancy defect in SiC.
- Cunzhi Zhang
- , Francois Gygi
- & Giulia Galli
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Article
| Open AccessMonolithic 3D integration of 2D transistors and vertical RRAMs in 1T–4R structure for high-density memory
Designing a monolithic 3D structure with interleaved logic and high-density memory layers has been difficult to achieve due to challenges in managing the thermal budget. Here, the authors demonstrate a 3D integration of monolayer MoS2 transistors with 3D vertical RRAMs through a low-temperature fabrication process whose 1T–nR structure shows high promise for low-power and high-density memory applications.
- Maosong Xie
- , Yueyang Jia
- & Rui Yang
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Article
| Open AccessEfficient combinatorial optimization by quantum-inspired parallel annealing in analogue memristor crossbar
Combinatorial optimization problems have various important applications but are notoriously difficult to solve. Here, the authors propose a quantum inspired algorithm and apply it to classical analog memristor hardware, demonstrating an efficient solution for intricate problems.
- Mingrui Jiang
- , Keyi Shan
- & Can Li
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Article
| Open AccessLight-enhanced molecular polarity enabling multispectral color-cognitive memristor for neuromorphic visual system
Designing optoelectronic synapses having a multispectral color-discriminating ability is crucial for neuromorphic visual system. Here, the authors propose an strategy to introduce RGB color-discriminating synaptic functionality into a 2-terminals memristor regardless of switching medium and design a color image-recognizing CNN and light-programmable reservoir computing.
- Jongmin Lee
- , Bum Ho Jeong
- & Hui Joon Park
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Article
| Open AccessBroad-high operating temperature range and enhanced energy storage performances in lead-free ferroelectrics
One of the key challenges in dielectric ceramics for energy storage lies in the comprehensive optimization of their properties. Here, the authors establish an equitable system considering performance and structure evolution in a lead-free ceramic capacitor, achieving a broad-high temperature performance.
- Weichen Zhao
- , Diming Xu
- & Di Zhou
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Article
| Open AccessMultistage coupling water-enabled electric generator with customizable energy output
Liquid water or moisture discharge is a significant source of energy waste in current single-stage water-enabled electric generators. Here, authors propose a modular multistage coupling device that integrates internal liquid water flow and subsequently generated moisture to optimize energy harvesting at all stages.
- Puying Li
- , Yajie Hu
- & Liangti Qu
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Article
| Open AccessSimultaneously ultrafast and robust two-dimensional flash memory devices based on phase-engineered edge contacts
The speed-retention-endurance trade-off usually limits the performance of flash memory devices. Here, the authors report the realization of van der Waals flash memory cells based on 2H-MoS2 semiconducting channels with phase-engineered 1T-LixMoS2 edge contacts, showing program/erasing speed of ~10/100 ns, endurance of >106 cycles and expected retention lifetime of >10 years.
- Jun Yu
- , Han Wang
- & Tianyou Zhai
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Article
| Open AccessAn anisotropic van der Waals dielectric for symmetry engineering in functionalized heterointerfaces
Here, the authors demonstrate that a layered anisotropic dielectric material, SiP2, can break the rotational symmetry of 2D MoS2, leading to linearly polarized photoluminescence emission and conductance anisotropy ratios up to 1000 in gated SiP2/MoS2 heterostructures.
- Zeya Li
- , Junwei Huang
- & Hongtao Yuan
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Article
| Open AccessA single n-type semiconducting polymer-based photo-electrochemical transistor
Many phototransistors are multi-component systems with inorganic materials or involve faradaic processes that can be irreversible. Using a single photoactive polymer, Druet et al. report a reversible, water-compatible n-type photoelectrochemical transistor with potentiometric photodetection and current modulation.
- Victor Druet
- , David Ohayon
- & Sahika Inal
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Article
| Open AccessDNA nanopores as artificial membrane channels for bioprotonics
Synthetic membrane channels have many potential applications, but interfacing membrane channels with electronic devices for efficient information transfer is challenging. Here the authors integrate membrane spanning DNA nanopores with bioprotonic contacts to create programmable, modular, and efficient artificial ion-channel interfaces.
- Le Luo
- , Swathi Manda
- & Marco Rolandi
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Article
| Open AccessIntegration of microbattery with thin-film electronics for constructing an integrated transparent microsystem based on InGaZnO
In this work, authors demonstrate the full integration of miniaturized InGaZnO-based transparent energy device (lithium-ion battery), electronic device (thin-film transistor) and sensing device (photodetector) to form a monolithic integrated transparent microsystem with synergistic functions.
- Bin Jia
- , Chao Zhang
- & Xiaodong Huang
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Article
| Open AccessLayer-dependent exciton polarizability and the brightening of dark excitons in few-layer black phosphorus
Here, the authors determine the exciton polarizabilities for 3- to 11-layer black phosphorus via frequency-resolved photocurrent measurements on dual-gate devices, and unveil the exciton response for higher-index sub-bands under the gate electrical field, as well as a carrier screening effect in thicker samples.
- Yuchen Lei
- , Junwei Ma
- & Hugen Yan
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Article
| Open AccessWide-range and area-selective threshold voltage tunability in ultrathin indium oxide transistors
The doping and threshold voltage modulation of 2D transistors remain challenging. Here, the authors report a wafer-scale optical-thermal method combining ultraviolet illumination and oxygen annealing to tune the threshold voltage of atomic-layer-deposited In2O3 transistors with 2 nm thickness.
- Robert Tseng
- , Sung-Tsun Wang
- & Der-Hsien Lien
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Article
| Open AccessA universal metasurface antenna to manipulate all fundamental characteristics of electromagnetic waves
The authors show a universal metasurface antenna capable of simultaneously and independently controlling all five fundamental properties of electromagnetic waves, including amplitude, phase, frequency, polarization, and momentum.
- Geng-Bo Wu
- , Jun Yan Dai
- & Chi Hou Chan
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Article
| Open AccessTransparent dynamic infrared emissivity regulators
In this work, authors report a transparent dynamic infrared emissivity modulation mechanism based on reversible injection/extraction of electrons in aluminium-doped zinc oxide nanocrystals and demonstrate it for smart thermal management applications.
- Yan Jia
- , Dongqing Liu
- & Tianwen Liu
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Article
| Open AccessSuppressing electron-phonon coupling in organic photovoltaics for high-efficiency power conversion
Reducing non-radiative energy loss is critical to improving power conversion efficiency in organic solar cells. Jiang et al. show that alkyl side-chain engineering in acceptors reduces the free volume ratio, lowering non-radiative decay, to achieve 18.6% efficiency in bulk-heterojunction binary cells.
- Yuanyuan Jiang
- , Yixin Li
- & Xiaozhang Zhu
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Perspective
| Open AccessToward a formal theory for computing machines made out of whatever physics offers
Learning from human brains to build powerful computers is attractive, yet extremely challenging due to the lack of a guiding computing theory. Jaeger et al. give a perspective on a bottom-up approach to engineer unconventional computing systems, which is fundamentally different to the classical theory based on Turing machines.
- Herbert Jaeger
- , Beatriz Noheda
- & Wilfred G. van der Wiel
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| Open AccessHybridization of short-range and long-range charge transfer excited states in multiple resonance emitter
Multi resonance thermally activated delayed fluorescence emitters are the next-generation blue dopants for organic light-emitting diodes. Here, the authors develop two isomeric emitters with hybridized long-range and short-range charge transfer excited states and realize device efficiency of 30.8%.
- Ha Lim Lee
- , Jihoon Kang
- & Jun Yeob Lee
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Article
| Open AccessFabrication of p-type 2D single-crystalline transistor arrays with Fermi-level-tuned van der Waals semimetal electrodes
The fabrication of high-performance p-type 2D transistors is still challenging. Here, the authors report the realization of wafer-scale p-type 2H-MoTe2 transistor arrays contacted by Fermi-level tuned semimetallic 1T’-MoTe2 electrodes, leading to improved contact resistance and device performance.
- Seunguk Song
- , Aram Yoon
- & Soon-Yong Kwon
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Article
| Open AccessHexanary blends: a strategy towards thermally stable organic photovoltaics
Non-fullerene-based organic solar cells generally suffer from poor thermal stability and especially in case of devices with thick active layers. Here, the authors report hexanary blends based on multi-component acceptor mixtures with a device efficiency of 17.6% and thermally stability for 23 days at 130 °C.
- Sri Harish Kumar Paleti
- , Sandra Hultmark
- & Derya Baran
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Article
| Open AccessAchieving tissue-level softness on stretchable electronics through a generalizable soft interlayer design
Stretchable electronics are attractive for a range of biomedical applications, but are challenging to prepare with suitable mechanical properties. Here, the authors report the use of a soft interlayer that allows the development of stretchable electronics with tissue-like material properties.
- Yang Li
- , Nan Li
- & Sihong Wang
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Article
| Open AccessAn avalanche-and-surge robust ultrawide-bandgap heterojunction for power electronics
Avalanche and surge robustness are fundamental for power devices to survive overvoltage and overcurrent stresses in typical applications. Here, authors report NiO/Ga2O3 heterojunctions with smaller reverse recovery, higher switching speed, and a robustness competitive to that of conventional homojunctions.
- Feng Zhou
- , Hehe Gong
- & Jiandong Ye
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Article
| Open AccessVertically grown ultrathin Bi2SiO5 as high-κ single-crystalline gate dielectric
Crystalline high-κ dielectric materials are desired for the development of future 2D electronic devices. Here, the authors report the in-plane and out-of-plane chemical vapor deposition growth of ultrathin Bi2SiO5 crystals with dielectric constant >30 and a band gap of ~3.8 eV, showing their effective application as gate dielectric layers of MoS2 transistors.
- Jiabiao Chen
- , Zhaochao Liu
- & Jinxiong Wu
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Article
| Open AccessImplant-to-implant wireless networking with metamaterial textiles
Implanted bioelectronic devices have proven useful for health sensing and therapy, while the interconnection of distributed implants remains challenging. Here, the authors demonstrate direct implant-to-implant wireless networking at the scale of the human body using metamaterial textiles.
- Xi Tian
- , Qihang Zeng
- & John S. Ho
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Article
| Open AccessContact-engineered reconfigurable two-dimensional Schottky junction field-effect transistor with low leakage currents
Here, the authors report the realization of WSe2 Schottky junction field-effect transistors with asymmetric multi-layer graphene and WTe2 van der Waals contacts, enabling reconfigurable polarity, low off-state currents, near-ideal rectifying behaviour and bipolar photovoltaic response.
- Yaoqiang Zhou
- , Lei Tong
- & Jian-Bin Xu
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Article
| Open AccessArtificially controlled nanoscale chemical reduction in VO2 through electron beam illumination
The authors demonstrate a nanoscale chemical reduction for VO2 into V2O3 through electron-beam illumination, showcasing potential for nanoscale manipulation of oxygen ionic evolution for advanced harvesting functionalities.
- Yang Zhang
- , Yupu Wang
- & Pu Yu
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Article
| Open AccessOn-site growth of perovskite nanocrystal arrays for integrated nanodevices
Integration of halide perovskites into nanoscale devices has been impeded by the limits of controlled perovskite patterning. Here, the authors demonstrate on-site growth of perovskite nanocrystals with sub-50 nm size and placement control, realizing nanoscale light emitting diodes.
- Patricia Jastrzebska-Perfect
- , Weikun Zhu
- & Farnaz Niroui
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Article
| Open AccessElectronic transport driven by collective light-matter coupled states in a quantum device
Here the authors investigate the electronic transport in microcavity-coupled quantum detector with strong collective electronic resonances. Their findings present a way to optimize photodetectors operating in the ultra-strong light-matter coupling regime.
- Francesco Pisani
- , Djamal Gacemi
- & Yanko Todorov
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Article
| Open AccessDetermining spin-orbit coupling in graphene by quasiparticle interference imaging
Graphene has many intriguing electronic properties. One of note is the absence of backscattering of electrons confined to a single valley. Spin-orbit interactions can allow backscattering, and here, Sun et al. use this spin-orbit coupling dependence of backscattering to measure the strength of the spin-orbit interaction in a graphene/tungsten selenide heterostructure.
- Lihuan Sun
- , Louk Rademaker
- & Christoph Renner
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Article
| Open AccessA reconfigurable binary/ternary logic conversion-in-memory based on drain-aligned floating-gate heterojunction transistors
Reconfigurable logic is desirable for high-density information processing. Here, the authors demonstrate a binary/ternary logic conversion-in-memory, which can operate in both binary and ternary logic systems to implement various types of logic gates.
- Chungryeol Lee
- , Changhyeon Lee
- & Sung Gap Im
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Comment
| Open AccessThe experimental demonstration of a topological current divider
Topological electronics is an emerging field aiming at exploiting the topological properties of matter in devices with extended functionalities. Recent experiments demonstrate a topological current divider, a key circuit element for this emerging technology.
- Francesco Romeo
- & Antonio Di Bartolomeo
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| Open AccessDirect observation of hot-electron-enhanced thermoelectric effects in silicon nanodevices
Thermoelectric property of silicon itself is important for the thermal management of post-Moore nanoelectronics. Here, Xue et al directly observe unconventional thermoelectric cooling/heating effects enhanced by hot electrons in silicon nanodevices.
- Huanyi Xue
- , Ruijie Qian
- & Wei Lu
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Article
| Open AccessA neuromorphic physiological signal processing system based on VO2 memristor for next-generation human-machine interface
Next-generation human-machine interfaces require efficient physiological signal processing systems. Here, the authors propose a hardware system that uses VO2 memristors to perform brain-like encoding and analysis of physiological signals, and is capable of identifying arrhythmia and epileptic seizures.
- Rui Yuan
- , Pek Jun Tiw
- & Yuchao Yang
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Article
| Open AccessLow power flexible monolayer MoS2 integrated circuits
The application of 2D MoS2 flexible integrated circuits (ICs) is currently limited by the material quality over large areas and the device fabrication technology. Here the authors report a gate-first fabrication technique to realize wafer-scale monolayer MoS2 ICs on rigid and flexible substrates with high performance and low power consumption.
- Jian Tang
- , Qinqin Wang
- & Guangyu Zhang
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Article
| Open AccessSnowflake-inspired and blink-driven flexible piezoelectric contact lenses for effective corneal injury repair
The cornea is susceptible to various injuries with a complicated repair process. Here, the authors propose a snowflake-inspired, blink-driven flexible piezoelectric contact lens for corneal injury repair.
- Guang Yao
- , Xiaoyi Mo
- & Yuan Lin
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Article
| Open AccessHierarchical entanglement shells of multichannel Kondo clouds
Understanding the structure of the Kondo cloud formed by conduction electrons screening the impurity spin is a long-standing problem in many-body physics. Shim et al. propose the spatial and energy structure of the multichannel Kondo cloud, by studying quantum entanglement between the impurity and the channels.
- Jeongmin Shim
- , Donghoon Kim
- & H.-S. Sim
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Article
| Open AccessVertically integrated spiking cone photoreceptor arrays for color perception
Future intelligent vision systems need efficient capacitor-free spiking photoreceptor for color perception. Here, Wang et al. report a metal oxide-based vertically integrated spiking cone photoreceptor array which transduces light into spike trains with a power consumption of less than 400 picowatts.
- Xiangjing Wang
- , Chunsheng Chen
- & Qing Wan
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Article
| Open AccessEnergy conversion and storage via photoinduced polarization change in non-ferroelectric molecular [CoGa] crystals
Energy harvesting by utilizing optical control has emerged as a promising solution to alleviate energy and environmental crisis. However, it is challenging to realise nano-scale energy storage and conversion in the same material. Here the authors report a nonferroelectric molecular [CoGa] crystal that uses light as an external stimulus to exhibit photoenergy conversion and energy storage properties.
- Pritam Sadhukhan
- , Shu-Qi Wu
- & Osamu Sato
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Article
| Open AccessThermally stable threshold selector based on CuAg alloy for energy-efficient memory and neuromorphic computing applications
Designing efficient selector devices remains a challenge. Here, the authors propose a CuAg alloy-based selector with excellent ON/OFF ratio and thermal stability. It can effectively suppress the sneak-path current in 1S1R arrays, making it suitable for storage class memory and neuromorphic computing applications.
- Xi Zhou
- , Liang Zhao
- & Dongdong Li
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Article
| Open AccessDischarge domains regulation and dynamic processes of direct-current triboelectric nanogenerator
Arising from contact electrification and electrostatic breakdown, DC triboelectric nanogenerators are a promising solution to the air breakdown bottleneck in conventional TENGs. Here, authors reveal and regulate three discharge domains enhancing the device output power by an order of magnitude.
- Jiayue Zhang
- , Yikui Gao
- & Jie Wang
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Article
| Open AccessMulti-neuron connection using multi-terminal floating–gate memristor for unsupervised learning
Designing efficient neuromorphic systems remains a challenge. Here, the authors develop a system based on multi-terminal floating-gate memristor that mimics the temporal and spatial summation of multi-neuron connections based on leaky-integrate-and-fire functionality which is capable of high learning accuracy on unlabeled MNIST handwritten dataset.
- Ui Yeon Won
- , Quoc An Vu
- & Woo Jong Yu
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Article
| Open AccessEnabling metallic behaviour in two-dimensional superlattice of semiconductor colloidal quantum dots
Charge carrier transport in colloidal quantum dot assemblies is slow due to hopping transport nature. Here, the authors report the demonstration of gate-tuned metallic state in epitaxially-connected quantum dot superlattices by minimizing disorders.
- Ricky Dwi Septianto
- , Retno Miranti
- & Satria Zulkarnaen Bisri
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Article
| Open AccessStructure-evolution-designed amorphous oxides for dielectric energy storage
Here, the authors propose a strategy to create amorphous oxides by bridging fluorite HfO2 and perovskite hafnate, which exhibit ultrahigh breakdown strength of 12 MV/cm and energy density of 155 J/cm3.
- Yahui Yu
- , Qing Zhang
- & Zheng Wen
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Article
| Open AccessBimodal ionic photomemristor based on a high-temperature oxide superconductor/semiconductor junction
Designing efficient photonic neuromorphic systems remains a challenge. Here, the authors develop a new class of memristor sensitive to the dual electro-optical history obtained by exploiting electrochemical, photovoltaic and photo-assisted oxygen ion motion effects at a high temperature superconductor / semiconductor interface.
- Ralph El Hage
- , Vincent Humbert
- & Javier E. Villegas
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Article
| Open AccessInsulator-to-metal-like transition in thin films of a biological metal-organic framework
Temperature-induced insulator-to-metal transitions are usually accompanied by structural phase transitions. Here the authors demonstrate an enhancement of the electrical conductance in a thin film of a biologically relevant metal-organic framework, without noticeable change in the structure, assigned to be of mainly electronic origin.
- Pooja Sindhu
- , K. S. Ananthram
- & Nirmalya Ballav