Abstract
Graphene has emerged as a promising material for active plasmonic devices in the mid-infrared (MIR) region owing to its fast tunability, strong mode confinement and long-lived collective excitation. In order to realize on-chip graphene plasmonics, several types of graphene plasmonic waveguides (GPWGs) have been investigated and most of them are with graphene ribbons suffering from the pattern-caused edge effect. Here we propose a novel nanoplasmonic waveguide with a pattern-free graphene monolayer on the top of a nano-trench. It shows that our GPWG with nanoscale light confinement, relatively low loss and slowed group velocity enables a significant modulation on the phase shift as well as the propagation loss over a broad band by simply applying a single low bias voltage, which is very attractive for realizing ultra-small optical modulators and optical switches for the future ultra-dense photonic integrated circuits. The strong light-matter interaction as well as tunable slow light is also of great interest for many applications such as optical nonlinearities.
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Introduction
Plasmonics has been regarded as one of the most promising strategies to realize light manipulation on nanoscale1. Noble metals, like silver and gold, are used popularly as the dominant materials for plasmonics because of their capability of supporting the surface plasmon polaritons (SPPs) at visible and near-infrared wavelengths. However, there is a great challenge for noble metals' application in actively tuning plasmonic devices2 due to the difficulty in modifying their permittivity. Current active plasmonic devices are usually realized with the assistance of another active optical material3,4,5.
Recently, graphene, a two-dimensional (2D) material of carbon atoms arranged in a honeycomb lattice, has been recognized as an excellent candidate for realizing inexpensive, fast and compact active plasmonic devices with reduced power consumption at ambient conditions6. This is attributed to the intriguing properties of graphene surface plasmons (GSPs)6,7,8,9,10. First, the Fermi level EF relative to the Dirac point and correspondingly the optical properties of graphene can be tuned synchronously and locally via chemical doping or electrical gating due to its two-dimensional nature11,12,13; Second, GSPs show strong mode confinement and slow group velocity with its GSP wavelength two orders smaller than that in free space14,15,16,17; Third, GSPs potentially provide smaller losses and therefore longer propagation lengths in comparison with surface plasmons in noble metals18 because of graphene's long relaxation time related to high carrier mobility μ (Ref. 19); Furthermore, GSPs mainly lie in the THz to MIR region10 where there are various significant applications for spectroscopy, chemical and biological sensing, imaging and communications, etc20.
In order to realize on-chip graphene plasmonics, the fundamental is to make an excellent waveguide. People have proposed several types of graphene plasmonic waveguides (GPWGs)9,18,21,22,23,24,25,26,27,28 and most of them are made with graphene ribbons18,21,22,25,26. However, the edge scattering effect and band gap opening in a graphene ribbon introduce extra plasmon damping to GSPs18,29. Therefore, a GPWG with a pattern-free graphene monolayer is preferred. This can be realized via creating customized conductivity patterns by employing the tunability of graphene. For example, separated gating pads can be introduced so that different bias voltages can be applied to the graphene monolayer in different positions9,27. However, the electrical operation for the gating pads is complicated due to more than one pads involved, particularly when two or more waveguides are placed close to each other (which is necessary for lots of photonic integrated devices). A patterned spacer layer can also be utilized by introducing a nano-ridge structure9,23,24 or more than one materials9 such that only one gate voltage is needed. One should note that the fabrication for the spacer with different materials is not convenient. For the design with a nano-ridge9,23,24, the transverse magnetic (TM) SPP mode is only supported in the core region. In other words, there is no TM SPP mode supported in the side-cladding region. In this case, the aspect ratio of the nano-ridge is as high as ~10 according to Ref. 9, which makes the fabrication hard.
Here we propose a novel nanoplasmonic waveguide with pattern-free graphene by introducing a spacer with a reversed nano-ridge (which is formed by etching a nano-trench on the doped silicon substrate). Unlike GPWGs reported in Ref. 9, 23, 24, the graphene surface of the proposed structure in both the core and the side-cladding regions supports the TM SPP modes with very distinct effective indices so that tight lateral confinement can be achieved. When the gate voltage varies, the Fermi levels of the graphene monolayer in the core and the side-cladding regions are modified accordingly. In this way, a significant modulation on the phase shift as well as the propagation loss over a broad band is achieved by simply applying a single low bias voltage, which is very favorable to realize some key dynamic elements including ultra-small optical modulators and optical switches, as presented in this paper. In addition, the fabrication for the proposed structure is relatively easy since the aspect ratio of the nano-trench is only 0.2 ~ 1.5.
Structure and Results
As shown in Figure 1(a), the proposed tunable GPWG has a doped silicon substrate with a nano-trench, an Al2O3 spacer, a pattern-free graphene monolayer on the top and an Al2O3 upper-cladding for protection. In this structure, GSPs are guided in the surface of the pattern-free graphene monolayer. The Al2O3 spacer has a flat top-surface and consequently the spacer has different thicknesses (d1 and d2) in the trenched and non-trenched regions, i.e., d1 > d2. Therefore, when a gate voltage VG is applied, the graphene in the trenched region has a lower Fermi level and higher SPP effective index neff than that in the non-trenched region according to the relationships of EF ∝ (VG/d)1/2 and neff ∝ (d/VG)1/2 (see Methods). In this way, graphene is electrostatically patterned to form a GPWG enabling strong light confinement on nanoscale, as confirmed by the calculated typical electric field profile of the fundamental SPP mode in the proposed GPWG [see Fig. 1(b)]. The operation frequency considered in the following investigations is f = 37.5 THz. In this example, the parameters are w = 100 nm, d1 = 60 nm, d2 = 40 nm and VG = 7.2 V. Correspondingly, one has EF1 = 0.3 eV and EF2 = 0.37 eV (see Methods). Here we assume that the graphene monolayer for the proposed trenched graphene nanoplasmonic waveguide has a stepped Fermi level distribution at the boundary between the trenched and non-trenched regions in a similar way shown in Ref. 9, 27. Accurate prediction for the carrier concentration and the Fermi-level distributions in graphene can be achieved with the electrostatic field distribution calculated numerically23,24.
In order to better understand the SPP mode supported in the proposed GPWG, we show the calculated effective indices Real(neff) for the fundamental mode as well as the higher-order modes as a function of the waveguide width w in Fig. 2(a). It can be seen that the guided-modes have very large effective indices varying from ~37 to ~67 and there are five modes supported even when the width is as small as w = 300 nm. In order to be single mode, the core width w should be smaller than 50 nm, which definitely helps to achieve ultra-high integration density. The propagation loss (dB/μm) for the guided-modes in the proposed GPWG is given in Fig. 2(b). It shows that the propagation loss is 2 ~ 6 dB/μm originating from the light interaction with the lossy graphene in the core region as well as in the side-cladding region. Consequently, it is not a good option for long-distance propagation, which is a common issue for almost all surface nanoplasmonic waveguides. Fortunately, the functionality elements based on the proposed GPWG could be very short because the ultra-high effective index [see Fig. 2(a)] makes it possible to achieve π phase-shift within ~100 nm. Consequently, the excess loss of such ultra-short functionality elements is still acceptable, e.g. ~1 dB or less. We also note that there is a maximum for the propagation loss of any guided-mode as the core width increases. In order to explain this, one should note that the present GPWG has three regions with different material losses (i.e., the graphene in the core region, the graphene in the side-cladding region and the lossless upper-/under-claddings) and the GP in the side-cladding region has lower propagation loss due to the higher Fermi level in comparison with the GP in the core region according to Eq. (2) (see Methods). Taking the fundamental mode as an example, the propagation loss becomes maximal around w = 90 nm. When the core width is large (w > 200 nm), the present GPWG behaves like a slab waveguide (i.e., w → ∞). In this case, light is mainly confined in the core region and interacts with the graphene in this region strongly, so that the propagation loss is not sensitive to the core width and approaches the loss for the slab waveguide. As the core width decreases from 200 nm to 90 nm, our calculation shows that the power confinement factor (the fraction of power flowing in the region of interest30) of the graphene in the core region and the side-cladding increases slightly, which indicates a stronger light-graphene interaction and thus results in a slight increase of the propagation loss. When the core width decreases further (w < 90 nm), more field extends into the side-cladding region and thus the contribution to the whole propagation loss from the light interaction with the graphene at the side-cladding becomes more and more dominant, which results in a reduction of the propagation loss. As a consequence, it is expected to have a maximum for the propagation loss of the fundamental mode, as shown in Fig. 2(b). Figure 2(c) shows the calculated effective mode width for the fundamental mode of the present GPWG. It is notable that the minimal effective mode width is as small as 53 nm to enable nanoscale light confinement and guiding. In order to synthetically evaluate the loss and the confinement ability of the present waveguide, the figure of merit (FOM) defined as Re(β)/Im(β) is also calculated and shown in Fig. 2(c). It is found that FOM ranges from 70 to 110 as the core width varies and there is a valley around w = 60 nm. One should choose the waveguide width appropriately by making a trade-off between the propagation loss and the effective mode width.
For the present GPWG, the spacer thickness d2 also plays an important role, as shown in Fig. 3(a). As d2 varies, the ratio d1/d2 is fixed as 3 here and the Fermi levels can be kept unchanged by tuning the applied gate voltage appropriately according to the relationship EF ∝ (VG/d)1/2 so that the equivalent dielectric constant of graphene does not change. For the present example, we choose w = 100 nm, EF1 = 0.3 eV and EF2 = 0.52 eV. When the spacer is very thin (d2 < 5 nm), the silicon substrate which has a larger dielectric constant than the Al2O3 spacer can “see” the modal field more and consequently, Real(neff) becomes sensitive to the spacer thickness d2. This is why Real(neff) of the fundamental mode decreases very quickly from ~480 to ~65 when d2 increases from zero to 5 nm, as show in Fig. 3(a). When d2 > 5 nm, Real(neff) becomes insensitive to the variation of d2 because little field penetrates into the silicon substrate. We also note that when d2 increases from zero, the propagation loss quickly decreases from ~18 dB/μm to the minimum ~4 dB/μm (located at d2 = ~5 nm) and then increases slightly to 5 dB/μm. One should note that the spatial dispersion (tensor conductivity) and the quantum capacitance should be taken into account31,32 for achieving accurate estimation of the value Real(neff) and the propagation loss when d2 is ultrathin (e.g., ~3 nm).
In order to further understand the dependence of Real(neff) and the propagation loss on d2, we make an equivalent slab waveguide [see Fig. 3(b)] for the present GPWG by using the effective index method (EIM, see Methods), which has been used very often to make the calculation efficient and to help understand the mode properties. Figure 3(c) shows the real part and imaginary part of the calculated indices (neff_co, neff_cl) for the core and the cladding layers of the equivalent three-layer slab waveguide for the present GPWG, both of which decrease quickly and eventually approach the values for d2 → ∞ as d2 increases. This is expected from Eq. (2) (see Methods) when the silicon substrate (which has a larger dielectric constant than the Al2O3 spacer) is separated farther. The index contrast defined as Real(neff_co) – Real(neff_cl) is also shown in the inset of Fig. 3(a), which reaches the minimum when d2 ≈ 3 nm and the effective mode width of the GPWG is expected to have a maximum correspondingly. As the mode field profile is significantly dependent on the index contrast, the power confinement factor in the core layer also becomes minimal around d2 ≈ 3 nm. Because the core layer of the equivalent three-layer slab waveguide dominates the total propagation loss [see the imaginary parts of neff_co and neff_cl shown in Fig. 3(b)], the equivalent three-layer slab waveguide also has a minimal propagation loss around d2 ≈ 3 nm, as shown by the dashed line in Fig. 3(a). The results for the equivalent three-layer slab waveguide (from EIM) agree very well with those for the GPWG (from FEM), which indicates that EIM can give reasonably accurate calculation for the present GPWG. This is very helpful for simplifying the simulation of the present GPWG, particularly for the simulation of light propagation along the GPWG circuits.
According to Fig. 3(a), we choose d2 = 40 nm for the design given below in order to have a large tolerance for the thickness d2. Figure 4(a) shows how the Fermi levels (EF2 and EF1) influences the fundamental mode of the GPWG with w = 100 nm and d2 = 40 nm. For this calculation, EF1 for the core is fixed to be 0.2 eV, 0.3 eV and 0.4 eV by adjusting the applied gate voltage accordingly while EF2 for the cladding is modified by choosing the thickness d1 appropriately to make the ratio EF2/EF1 vary in the range from 1.0 to 2.0. It can be seen that one has a smaller the effective mode width when choosing lower EF1. Figure 4(a) also shows that the effective mode width decreases steeply when EF2/EF1 increases from 1.0. The reason is that the index contrast is larger when choosing lower EF1 or higher EF2 according to Eq. (2) (see Methods). More importantly, when EF2/EF1 increases from 1.0, the index contrast increases quickly to be so large that the effective mode width is determined mainly by the core width. As a result, the effective mode width becomes insensitive to this ratio when EF2/EF1 becomes slightly larger than 1.0 (e.g. EF2/EF1 > 1.2). For example, for the case of EF1 = 0.3 eV, the effective mode width decreases from 345 nm to 105 nm when EF2/EF1 increases from 1.0 to 1.1. When the ratio increases further, the effective mode width decreases very slightly. This indicates that a deep trench is not necessary to a GPWG with strong lateral confinement and consequently, the fabrication is easy.
Figure 4(b) illustrates Real(neff) and the propagation loss of the fundamental mode as the Fermi level EF1 for the graphene in the core region varies by modifying the gate voltage. For this calculation, we choose w = 100 nm, d1 = 60 nm, d2 = 40 nm to make EF2/EF1 = 1.51/2 as an example. It shows that Real(neff) (or phase shift) as well as the propagation loss can be modulated significantly by introducing a small variation of the gate voltage. As a result, it is potential to build an optical modulator of phase or amplitude with an ultra-small footprint, which is helpful to achieve ultra-high speed. In this paper, we consider the design for an optical modulator of amplitude given the structural simplicity. As the insertion loss and the extinction ratio are the two key parameters to evaluate an optical modulator, one should make a trade-off when determining the operation point of the optical modulator. As shown in Fig. 4(b), when choosing a small Fermi level (i.e. with a low gate voltage), the optical modulator can be ultra-short to achieve an acceptable extinction ratio because of the very high slope of the curve of propagation loss. For example, when choosing VG0 = 2.0 V, the propagation loss is ~72.2 dB/μm and an extinction ratio of ~157 dB/μm can be achieved with ΔVG = −0.5 V. Note that an optical modulator should be long enough (e.g. ~100 nm) for the fabrication in the practical case. Consequently, the insertion loss of the 100-nm-long optical modulator is too high (up to 7.2 dB) to be acceptable. Alternatively, here we choose the operation point as VG0 = 7.2 V and ΔVG = −5.2 V. In this case, one has Real(neff) = 63.3 and the propagation loss of 4.6 dB/μm when the gate voltage is tuned to VG = VG0 = 7.2 V (on-state, EF1 = 0.3 eV). In contrast, one has Real(neff) = 168.3 and the propagation loss of 72.2 dB/μm when VG = VG0 + ΔVG = 2.0 V (off-state, EF1 = 0.16 eV). With this design, the optical modulator can be as short as 150 nm to achieve an extinction ratio of ~10 dB and the insertion loss is acceptable (~0.7 dB only). Figure 4(c) displays the simulated light propagation in the designed optical modulator when VG = 7.2 V and 2.0 V, respectively. It shows that there is no significant power attenuation when VG = 7.2 V while light attenuates significantly when VG = 2.0 V, as expected.
The frequency dependence of the mode properties is also analyzed in the frequency ranging from 30 THz to 45 THz, as shown in Fig. 5. In this calculation, the parameters are chosen as w = 100 nm, d1 = 60 nm and d2 = 40 nm while the Fermi level EF1 is assumed to be 0.16 eV, 0.2 eV, 0.3 eV and 0.4 eV (correspondingly the Fermi level EF2 is 0.20 eV, 0.24 eV, 0.37 eV and 0.49 eV), respectively. As shown in Fig. 5(a) and Fig. 5(b), the fundamental mode has higher propagation loss and larger Real(neff) at a higher operation frequency for any given Fermi level, which is in agreement with Eq. (2) (see Methods). More importantly, the propagation loss and Real(neff) of the present GPWG can be modulated in a broad band, so that the present GPWG is available for different operation frequencies. The inset of Figure 5(b) shows that the group velocity of the GPWG remains three orders of magnitude slower than the light speed for vacuum in the whole frequency range and can be modified significantly by tuning the Fermi level of graphene. This enables tunable slow light33, which is useful for many applications34.
Considering that the evanescent coupling between two parallel optical waveguides is very important for the design of many devices, the evanescent coupling in a system consisting of two identical parallel waveguides is analyzed here. As an example, we choose d1 = 60 nm, d2 = 40 nm and the Fermi level is assumed as EF1 = 0.22 eV, 0.25 eV and 0.3 eV. Figure 6(a) shows the coupling length (defined as the beat length of the two super modes) for the case of w = 50 nm as the separation D between the two coupled waveguides varies while Figure 6(b) shows the coupling length for the case of D = 150 nm as the core width w varies. As can be seen, the coupling length increases significantly as the separation or the width increases. For example, when w = 50 nm, D = 150 nm and EF1 = 0.22 eV, the coupling length is as long as 50 μm. In this case, the coupling crosstalk is less than −30 dB considering that the device length is usually less than 1 μm. It indicates that an ultra-dense photonic integrated circuit can be achieved. One can also find that the coupling length is very sensitive to the Fermi level of the graphene monolayer, so that it is possible to realize electrically-switched directional coupler.
Here we propose an ultra-compact optical switch based on an asymmetrical directional coupler (ADC) which consists of two optical waveguides with different core widths w1 and w2, as shown in Fig. 6(c). In this design, the graphene monolayer on top of the coupling region is split into two parts, between which there is a narrow slot so that the two waveguides can be tuned by applying a gate voltage individually. When the gate voltages applied to the two parts are the same, the Fermi levels for the two parts of graphene are the same and the two waveguides with large width difference will have a big phase mismatch [see Fig. 2(a)]. Consequently, light launched from the input port cannot be cross-coupled from the wide waveguide to the narrow waveguide. On the other hand, when the gate voltage applied to the wider waveguide is optimally higher than that for the narrower one, the phase match condition can be satisfied, so that an efficient cross-coupling from the wide waveguide to the narrow waveguide can be realized by choosing the length of the coupling region appropriately. As an example, we choose w1 = 40 nm, w2 = 150 nm, d1 = 90 nm, d2 = 30 nm, D = 17.4 nm, L2 = 0.615 μm and L3 = 0.638 μm for the ADC optical switch [see Fig. 6(c)]. Here we choose a relatively large ratio d1/d2 in order to reduce the unwanted on-state cross-coupling. Fig. 6(d) shows the simulated light propagation in the designed ADC from FEM with the assistance of EIM. It can be seen there is little cross-coupling when the gate voltages for both waveguides are chosen as VG1 = VG2 = 10.8 V (correspondingly the Fermi levels for the two parts of graphene are EF1 = 0.3 eV). In contrast, an efficient cross-coupling is observed when choosing VG1 = 10.8 V and VG2 = 14.9 V (i.e., one has EF1 = 0.3 eV for the narrow waveguide and EF1 = 0.35 eV for the wide waveguide). With this design, the extinction ratio of the optical switch is as high as 24 dB while the length of the device is less than 1.25 μm.
Summary
In summary, we have proposed a novel nanoplasmonic waveguide with pattern-free graphene by introducing a spacer with a reversed nano-ridge. The calculations have shown that the easy-to-fabrication GPWG with nanoscale light confinement, relatively low loss and slowed group velocity enables a significant modulation on the phase shift as well as the propagation loss over a broad band by simply applying a single low bias voltage, which is very helpful for future ultra-dense photonic integrated circuits. The strong light-matter interaction as well as tunable slow light is also of great interest for many applications such as optical nonlinearities. With the proposed GPWG, an ultra-small optical modulator and optical switch have been presented. For the designed optical modulator, the extinction ratio and the insertion loss are 10 dB and 0.7 dB, respectively, while the length is as short as 150 nm (which is attractive for high-speed applications). For the designed optical switch based on an ADC, the device length is 1.25 μm and the extinction ratio is as high as 24 dB. Besides, the GPWG is also useful for other nano devices like spasers owing to the strong localization of photons and electrons deriving from the nonuniform Fermi level distribution of the graphene monolayer.
Methods
Theory
The simulation results presented in this paper are obtained with the frequency-domain finite-element method (FEM) where the graphene monolayer is treated as a thin film with the thickness t = 1 nm9. The equivalent dielectric constant of graphene is calculated as9 ε = 1 + iσ/(ε0ωt), where ω is the angular frequency, ε0 is the vacuum permittivity and σ is the frequency-dependent optical conductivity of graphene. The optical conductivity σ is given by the expression derived from the Kubo formula35 and verified by experiments12 as:
where e is the elementary charge, kB is the Boltzmann constant, ħ is the reduced Planck constant, T is the temperature (T = 300 K in this paper), τ is the relaxation time characterizing the plasmon decay attributed to impurities, defects, electron-phonon scattering and electron-electron interaction8,10,29 and the Fermi-Dirac distribution f(θ) = {exp[(θ−EF)/kBT]+ 1}−1. The first term of Eq. (1) is the contribution from intraband transitions and the second term from interband transitions. The Fermi level is given by EF = −sgn(n)ħvF(π|n|)1/2, where the Fermi velocity vF≈ 106 m/s and n is the carrier density. On the basis of a parallel-plate capacitor model, the gate-induced carrier density of graphene is given by n = −ε0εdVG/ed, where εd and d are the dielectric constant (εd = 10 for Al2O3) and the thickness of the dielectric spacer, respectively. According to the expression of Fermi level, one has the following relationship EF∝(VG/d)1/2. It reveals that the optical conductivity of graphene can be adjusted by varying the carrier-density-dependent Fermi level via e.g. modifying the gate voltage.
As it has been proved theoretically6,7,8,10 and experimentally14,15,17 that SPPs is supportable in a graphene monolayer ranging from THz to MIR spectrum, in this paper we consider the frequency f = 37.5 THz (8 μm in air) with the plasmon energy below that of optical phonons36 ħωOph≈ 0.2 eV (1580 cm−1) and Pauli-blocking interband threshold for properly doped graphene, so both the plasmon damping channel through the emission of an optical phonon with an electron-hole pair and the interband transition are suppressed6,8,10,29. In this case, the plasmon lifetime can be reasonably estimated by impurity related DC relaxation time6,8,10,29 as τ = μEF/evF2(0.5 ps in this paper). Further considering the nonretarded regime ( where β is the wavenumber of GPs and k0 is the vacuum wavenumber) and , the dispersion relationship of GPs for the TM mode in a graphene monolayer is thus approximately8
where ε1 and ε2 are the dielectric constants of the dielectric mediums above and underneath graphene. Eq. (2) reveals that the complex SPP effective index neff = β/k0 is inversely proportional to the Fermi level. Since EF ∝ (VG/d)1/2, one will obtain neff = β/k0 ∝ (d/VG)1/2. It indicates that GP modes can also be modulated flexibly by tuning the Fermi level.
Effective index method
EIM is the method that deals with a 2D waveguide as an equivalent slab waveguide. As shown in Fig. 3(b), the multilayer structure of the core and the cladding of the 2D waveguide can be equivalent to one kind of material with the TM SPP effective index for the corresponding part and the effective materials compose the core and the cladding of the equivalent slab waveguide. As a result, the characteristics of the 2D waveguide can be simply described by analyzing the TE mode of the equivalent slab waveguide.
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Acknowledgements
This project was partially supported by the Nature Science Foundation of China (No. 11374263 and 61422510), the Doctoral Fund of Ministry of Education of China (No. 20120101110094).
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J.Z. proposed the waveguide structure. J.Z., L.Y. and D.D. discussed the modal analysis and calculation. J.Z., D.D. and S.H. contributed to the scientific discussions and the manuscript writing/revision. D.D. supervised the whole project funded and finalized the paper.
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Zheng, J., Yu, L., He, S. et al. Tunable pattern-free graphene nanoplasmonic waveguides on trenched silicon substrate. Sci Rep 5, 7987 (2015). https://doi.org/10.1038/srep07987
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DOI: https://doi.org/10.1038/srep07987
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