Article
|
Open Access
Featured
-
-
Article
| Open AccessEmbedded metallic nanoparticles facilitate metastability of switchable metallic domains in Mott threshold switches
Control of percolative dynamics of metal and insulator domains during electrically triggered insulator-metal transition underlies applications in energy-efficient switches. Jo et al. show that embedded metallic nanoparticles enhance the metastability and memory effects of metallic domains in VO2 switches.
- Minguk Jo
- , Ye-Won Seo
- & Junwoo Son
-
Article
| Open AccessSuperfluid stiffness of a KTaO3-based two-dimensional electron gas
Heterostructures based on (111)-oriented KTaO3crystals are a new platform for studying oxide interfaces. Gate-tunable superconductivity in 2D electron gases at the surface of (111)-oriented KTaO3is now reported, with the superconducting transition being of the Berezinskii-Kosterlitz-Thouless type.
- S. Mallik
- , G. C. Ménard
- & N. Bergeal
-
Article
| Open AccessAnomalous Ferromagnetism of quasiparticle doped holes in cuprate heterostructures revealed using resonant soft X-ray magnetic scattering
Long-range magnetic order of quasiparticle doped holes is important for understanding the physics of cuprate superconductors, albeit difficult to probe in experiments. Ong et al. observe ferromagnetism of quasiparticle doped holes in a cuprate heterostructure and discuss implications for cuprates in the ground state.
- B. L. Ong
- , K. Jayaraman
- & A. Rusydi
-
Article
| Open AccessTuning lower dimensional superconductivity with hybridization at a superconducting-semiconducting interface
Lower-dimensional superconductors are typically synthesized on insulating substrates. Here, the authors find that the hybrid electronic structure formed at the interface between a lead film and a semiconducting black phosphorus substrate significantly renormalizes the superconductivity in the lead film.
- Anand Kamlapure
- , Manuel Simonato
- & Alexander Ako Khajetoorians
-
Article
| Open AccessPressure-induced monotonic enhancement of Tc to over 30 K in superconducting Pr0.82Sr0.18NiO2 thin films
Despite much recent effort, the highest reported Tc of the infinite-layer nickelates remains lower than 15 K. Here, the authors apply pressure to Pr0.82Sr0.18NiO2 thin films and observe a monotonic increase of Tc to 31 K at 12.1 GPa, an increase that does not level off with increasing pressure.
- N. N. Wang
- , M. W. Yang
- & J.-G. Cheng
-
Article
| Open AccessCompeting electronic states emerging on polar surfaces
Defect-free surfaces with excess charge are typically described as a homogeneous 2D electron gas. Here, in contrast, the authors find that the KTaO3(001) surface hosts a charge density wave coexisting with a pattern of electron polarons, highly localized states of excess electrons bound to a lattice distortion.
- Michele Reticcioli
- , Zhichang Wang
- & Cesare Franchini
-
Article
| Open AccessFabrication of triboelectric polymer films via repeated rheological forging for ultrahigh surface charge density
High charge density is the foundation to promote a wide range of applications of triboelectric nanogenerators. Here, authors propose a processing method based on the repeated rheological forging of triboelectric polymers achieving an enhanced triboelectricity and further study its mechanism.
- Zhaoqi Liu
- , Yunzhi Huang
- & Jin-Ping Qu
-
Article
| Open AccessBIGDML—Towards accurate quantum machine learning force fields for materials
Most machine-learning force fields dismiss long-range interactions. Here the authors demonstrate the BIGDML approach for building materials’ potential energy surfaces that enables a broad range of materials simulations within accuracies better than 1 meV/atom using just 10–200 structures for training.
- Huziel E. Sauceda
- , Luis E. Gálvez-González
- & Alexandre Tkatchenko
-
Article
| Open AccessInvestigating water/oil interfaces with opto-thermophoresis
Charging of interfaces between water and hydrophobic media is a mysterious feature whose nature and origin remain under debate. Here, the authors use opto-thermophoretic tweezers to investigate the interfacial behavior at water/oil interfaces in terms of thermal perturbation of dipole arrangement.
- Youngsun Kim
- , Hongru Ding
- & Yuebing Zheng
-
Article
| Open AccessCompositional dependence of the fragility in metallic glass forming liquids
In metallic liquids, the fragility is difficult to predict and measure. Here, the authors present the film inflation method, which reveals large fragility variations across Mg–Cu–Y, and introduce the crystallization complexity as additional contribution to glass forming ability.
- Sebastian A. Kube
- , Sungwoo Sohn
- & Jan Schroers
-
Article
| Open AccessOrthogonal interlayer coupling in an all-antiferromagnetic junction
Ferromagnet/spacer/ferromagnet sandwiches have been studied extensively, and used in a variety of spintronic devices. Here, Zhou et al. create an all anti-ferromagnetic sandwich of Fe2O3/Cr2O3/Fe2O3, and demonstrate strong orthogonal coupling between the top and bottom Fe2O3 layers.
- Yongjian Zhou
- , Liyang Liao
- & Cheng Song
-
Article
| Open AccessThird harmonic characterization of antiferromagnetic heterostructures
Harmonic measurements have been used extensively in ferromagnetic/heavy metal heterostructures to characterize the magnetization dynamic; however, it has remained unclear about whether such techniques could be applied to antiferromagnetic devices. Here, Cheng et al demonstrate such a harmonic measurement approach in an antiferromagnet.
- Yang Cheng
- , Egecan Cogulu
- & Fengyuan Yang
-
Article
| Open AccessHigh critical current density and high-tolerance superconductivity in high-entropy alloy thin films
Thin-film high-entropy alloy (HEA) superconductors have recently attracted a lot of attention, but their critical current density and potential usefulness in engineering applications has remained unclear. Here, the authors fabricate HEA films with remarkably high critical current density and resistance to radiation damage.
- Soon-Gil Jung
- , Yoonseok Han
- & Tuson Park
-
Article
| Open AccessDirect investigation of the atomic structure and decreased magnetism of antiphase boundaries in garnet
Iron garnets are widely used in magneto-optical devices, but knowledge of the effects of common defects on performance is limited. Here, using high-resolution microscopy and spectroscopy, the authors find that magnetism is weakened near these defects causing reduced performance, but can be avoided by tuning the growth rate.
- Kun Xu
- , Ting Lin
- & Jing Zhu
-
Article
| Open AccessDual phase patterning during a congruent grain boundary phase transition in elemental copper
The phase behavior of grain boundaries can influence the interfacial properties. Here the authors demonstrate nanoscale patterning of a grain boundary by two alternating phases in Cu that exhibit a congruent, diffusionless transition between the two phases.
- Lena Langenohl
- , Tobias Brink
- & Christian H. Liebscher
-
Article
| Open AccessSkyrmion pinning energetics in thin film systems
Skyrmions, topological spin textures, can be pinned by defects present in the material that hosts them, influencing their motion. Here, Gruber et al show that the skyrmions are pinned at their boundary where the finite size of the skyrmions governs their pinning, and they demonstrate that certain pinning sites can switched on and off in-situ.
- Raphael Gruber
- , Jakub Zázvorka
- & Mathias Kläui
-
Article
| Open AccessA confined-etching strategy for intrinsic anisotropic surface wetting patterning
Anisotropic functional patterned surfaces have shown significant applications in microfluidics, biomedicine, and optoelectronics. Here, authors demonstrate a fast and mask-free etching method for accurate surface patterning by confined decomposition, enabling the efficient fabrication of complex patterns.
- Rui Feng
- , Fei Song
- & Yu-Zhong Wang
-
Article
| Open AccessSelf-assembly of highly ordered micro- and nanoparticle deposits
A uniform particle deposition is crucial for sensitive applications, such as sensors and electronics. Here, authors introduce a passive protocol to suppress the coffee-ring effect and form uniform films at micro- and nanoscales combining superhydrophilic substrate with a neutral-wetting low-roughness mold.
- Hossein Zargartalebi
- , S. Hossein Hejazi
- & Amir Sanati-Nezhad
-
Article
| Open AccessBand conductivity oscillations in a gate-tunable graphene superlattice
Experiments in a tunable graphene superlattice show that the unusual 1/B periodic resistance oscillations at high temperatures in the energy spectrum of electrons in a 2D periodic potential, known as the Hofstadter butterfly, coexist with oscillations due to commensurability between the electron cyclotron radius and the superlattice’s period.
- Robin Huber
- , Max-Niklas Steffen
- & Jonathan Eroms
-
Article
| Open AccessDefect-gradient-induced Rashba effect in van der Waals PtSe2 layers
Materials with strong Rashba-type spin-orbit coupling hold promise for spintronic applications and the investigation of topological phases of matter. Here, the authors report a method to generate layer-by-layer defect gradients in a van der Waals material, inducing broken spatial inversion symmetry and Rashba effect in the engineered layers.
- Junhyeon Jo
- , Jung Hwa Kim
- & Jung-Woo Yoo
-
Article
| Open AccessReversible morphology-resolved chemotactic actuation and motion of Janus emulsion droplets
Artificial microswimmers can emulate the autonomous regulation of chemotactic motility of living organisms. Frank et al. realize a chemotactic locomotion of emulsion droplets, composed of two phase-separated fluids, that can be reversibly directed up or down a chemical concentration gradient.
- Bradley D. Frank
- , Saveh Djalali
- & Lukas Zeininger
-
Article
| Open AccessTwisted oxide lateral homostructures with conjunction tunability
It is challenging to construct lateral homostructures with controllable geometry and repeated alternating configurations. Here the authors develop a generic approach for fabricating twisted lateral homostructures with tunable crystal orientation, epitaxial constrain, and phase stability.
- Ping-Chun Wu
- , Chia-Chun Wei
- & Jan-Chi Yang
-
Article
| Open AccessFermi surface chirality induced in a TaSe2 monosheet formed by a Ta/Bi2Se3 interface reaction
Current limitations of spintronics devices based on bulk topological materials stimulate the search for new materials and structures with interesting spin properties. Here the authors report a chiral spin texture around the Fermi level related to structural symmetry breaking in a TaSe2 layer grown on a Bi2Se3 surface.
- Andrey Polyakov
- , Katayoon Mohseni
- & Stuart S. P. Parkin
-
Article
| Open AccessObservation of Bloch oscillations dominated by effective anyonic particle statistics
Electric circuits represent a versatile platform for simulations of exotic phenomena that are difficult to realize is condensed matter systems. Here the authors simulate particle statistics-dependent Bloch oscillations with electric circuits and observe features predicted for a model of anyons on a 1D lattice.
- Weixuan Zhang
- , Hao Yuan
- & Xiangdong Zhang
-
Comment
| Open AccessTowards actinide heterostructure synthesis and science
Controlling dimensionality and strain in actinide heterostructures will provide unrivaled opportunities for exploring novel quantum phenomena. We discuss the promises, challenges, and synthesis routes for these actinide-bearing heterostructures with complex electron correlations for functional and energy materials.
- Cody A. Dennett
- , Narayan Poudel
- & Krzysztof Gofryk
-
Article
| Open AccessInducing and tuning Kondo screening in a narrow-electronic-band system
Non f-electron systems containing narrow electronic band and localized moments are a useful platform to study the Kondo lattice problem. Here, by using scanning tunneling microscopy, the authors show a transition from the insulating gap to a tuneable Kondo resonance in 1T-TaS2 by Pb intercalation.
- Shiwei Shen
- , Chenhaoping Wen
- & Shichao Yan
-
Article
| Open AccessQuantum spins and hybridization in artificially-constructed chains of magnetic adatoms on a superconductor
Previous studies of magnetic adatom chains on superconducting substrates have mostly focused on the regime of dense chains and classical spins. Here, using scanning tunnelling microscopy, the authors study the excitation spectra of Fe chains on a NbSe2 surface, adatom by adatom, in the regime of quantum spins.
- Eva Liebhaber
- , Lisa M. Rütten
- & Katharina J. Franke
-
Article
| Open AccessAtomic-scale visualization of chiral charge density wave superlattices and their reversible switching
Single-layer NbSe2 has a charge density wave with two degenerate domains, related by mirror reflection. Here, using scanning tunneling microscopy, the authors observe the time-dependent movement of domain walls, and demonstrate reversible switching between the two domain types using a voltage pulse from the microscope tip.
- Xuan Song
- , Liwei Liu
- & Yeliang Wang
-
Article
| Open AccessSpin-orbit enabled all-electrical readout of chiral spin-textures
One challenge for encoding information in chiral spin textures is how to read the information electrically. Here, Lima Fernandes et al. show that chiral spin textures exhibit a magnetoresistance signature which could allow for efficient electric readout of the chirality and helicity.
- Imara Lima Fernandes
- , Stefan Blügel
- & Samir Lounis
-
Article
| Open AccessSuperheating of grain boundaries within bulk colloidal crystals
Understanding the dynamics of grain boundaries and their melting behaviour is important for controlling the mechanical properties of materials. Now, experiments show that grain boundaries can be superheated, and that they melt via a nucleation mechanism.
- Xiuming Xiao
- , Lilin Wang
- & Ziren Wang
-
Article
| Open AccessDirect imaging of the disconnection climb mediated point defects absorption by a grain boundary
Grain boundaries can improve the radiation resistance of a material by annihilating point defects formed under irradiation, however the atomistic mechanism is still unclear. Here the authors demonstrate grain boundaries absorb point defects through the climb motion of disconnections.
- Jiake Wei
- , Bin Feng
- & Yuichi Ikuhara
-
Article
| Open AccessResonant neutron reflectometry for hydrogen detection
The detection and quantification of hydrogen is becoming increasingly important in research on electronic materials and devices. Here the authors show that waveguide resonances enhance the sensitivity of neutron reflectometry, enabling fast, direct, and nondestructive measurements of hydrogen incorporation in thin-film structures.
- L. Guasco
- , Yu. N. Khaydukov
- & B. Keimer
-
Article
| Open AccessReversible writing/deleting of magnetic skyrmions through hydrogen adsorption/desorption
To use skyrmions to store information, an effective method for writing and deleting them is required. Here, Chen et al demonstrate the writing and deleting of skyrmions at room temperature by using hydrogen adsorption to change the magnetic anisotropy of the metallic multilayer hosting the skyrmions.
- Gong Chen
- , Colin Ophus
- & Kai Liu
-
Article
| Open AccessThe role of lattice dynamics in ferroelectric switching
Reducing the switching energy of ferroelectric films remains an important goal. Here, the authors elucidate the fundamental role of lattice dynamics in ferroelectric switching on both freestanding BiFeO3 membranes and films clamped to a substrate.
- Qiwu Shi
- , Eric Parsonnet
- & Ramamoorthy Ramesh
-
Article
| Open AccessAnionic character of the conduction band of sodium chloride
The current work finds that ordinary table salt behaves unexpectedly. The chloride ions alone dominate the electronic states at both edges of its band gap although sodium ions are also present. This is important when NaCl is used as an insulator.
- Christopher C. Leon
- , Abhishek Grewal
- & Olle Gunnarsson
-
Article
| Open AccessLarge-gap insulating dimer ground state in monolayer IrTe2
The interplay between reduced dimensionality and interactions in monolayer transition metal dichalcogenides has been of great research interest. Here the authors report an insulating dimer ground state in 1T-IrTe2, driven by the combined effect of the charge density wave instability and local atomic bond formation.
- Jinwoong Hwang
- , Kyoo Kim
- & Sung-Kwan Mo
-
Article
| Open AccessObservation of perfect diamagnetism and interfacial effect on the electronic structures in infinite layer Nd0.8Sr0.2NiO2 superconductors
Nickelate superconductors attract enormous attention in the field of high-temperature superconductivity. Here the authors report observation of perfect diamagnetism and interfacial effect on the electronic structures in infinite layer Nd0.8Sr0.2NiO2 superconductors.
- S. W. Zeng
- , X. M. Yin
- & A. Ariando
-
Article
| Open AccessDefect-driven antiferromagnetic domain walls in CuMnAs films
Antiferromagnets offer the potential for higher speed and density than ferromagnetic materials for spintronic devices. Here, Reimers et al study the domain structure of CuMnAs, demonstrating the role of defects in stabilizing the location and orientation of antiferromagnetic domain walls.
- Sonka Reimers
- , Dominik Kriegner
- & Kevin W. Edmonds
-
Article
| Open AccessReal-space observation of incommensurate spin density wave and coexisting charge density wave on Cr (001) surface
Spin density waves are a spatial modulation of the spin, and can be either commensurate or incommensurate with the crystal lattice. Here, Hu et al. use spin-polarised scanning tunnelling microscopy to observe the incommensurate spin density wave on cleaned Chromium surface.
- Yining Hu
- , Tianzhen Zhang
- & Tong Zhang
-
Article
| Open AccessSpontaneous dewetting transitions of droplets during icing & melting cycle
Despite promising for anti-icing applications, structured superhydrophobic surfaces usually lose their hydrophobicity after a few icing/melting cycles. Here, authors investigate specific structured surfaces and air bubbles on frozen ice droplets to propose three criteria to enable dewetting transitions.
- Lizhong Wang
- , Ze Tian
- & Minlin Zhong
-
Article
| Open AccessEngineering of atomic-scale flexoelectricity at grain boundaries
Large strain gradient is crucial for flexoelectricity. Here, the authors reveal the generality and tunability of large strain gradients at grain boundaries in oxides, explaining the possible effects on the electrical activities of ceramics.
- Mei Wu
- , Xiaowei Zhang
- & Peng Gao
-
Article
| Open AccessSignatures of enhanced out-of-plane polarization in asymmetric BaTiO3 superlattices integrated on silicon
Integrating multifunctional oxides on silicon is highly desirable. Here, the authors present asymmetric BaTiO3 superlattices on silicon exhibiting enhanced out-of-plane polarization by harnessing the interfacial strain and broken inversion symmetry.
- Binbin Chen
- , Nicolas Gauquelin
- & Gertjan Koster
-
Article
| Open AccessUnlocking surface octahedral tilt in two-dimensional Ruddlesden-Popper perovskites
The surface octahedral tilt in exfoliated 2D perovskites is directly visualized by STM and the degree of the tilt varies with the number of layers of inorganic slabs and result in different amounts of excitonic red shift in photoluminescence.
- Yan Shao
- , Wei Gao
- & Kai Leng
-
Article
| Open AccessResonant tunneling driven metal-insulator transition in double quantum-well structures of strongly correlated oxide
The metal-insulator transition is typically controlled by carrier accumulation or chemical doping. Here, the authors realize an alternative method based on resonant tunnelling in a double quantum well structure of strongly correlated oxides, which offers practical advantages over conventional methods.
- R. Yukawa
- , M. Kobayashi
- & H. Kumigashira
-
Article
| Open AccessSelf-activating anti-infection implant
Bone implants with antibacterial and osteogenic properties are important for clinical applications, but creating both properties simultaneously remains challenging. Here, the authors demonstrate a self-activating implant using a hydroxyapatite and molybdenum disulfide coating which accelerates bone regeneration and at the same time prevents bacterial infection.
- Jieni Fu
- , Weidong Zhu
- & Shuilin Wu
-
Article
| Open AccessExperimental observation of localized interfacial phonon modes
Conventional theories for interfacial thermal transport are derived from bulk phonon properties. Here, the authors report experimental observation of interfacial phonon modes localized at interfaces, changing how interfacial thermal transport should be understood.
- Zhe Cheng
- , Ruiyang Li
- & Samuel Graham
-
Article
| Open AccessEvidence for anisotropic spin-triplet Andreev reflection at the 2D van der Waals ferromagnet/superconductor interface
The interfaces between ferromagnets and superconductors receive many attentions due to emergent relativistic spin-orbit coupling. Here, the authors provide possible evidence for spin triplet Andreev reflection at the interface between a van der Waals ferromagnet Fe0.29TaS2 and a s-wave superconductor NbN.
- Ranran Cai
- , Yunyan Yao
- & Wei Han
-
Article
| Open AccessLong range and highly tunable interaction between local spins coupled to a superconducting condensate
The possibility of using superconductivity to control indirect interactions between magnetic moments remains largely unexplored. Here, the authors report tuning the interaction between local spins of Cr atoms coupled through a superconducting condensate in Nb.
- Felix Küster
- , Sascha Brinker
- & Paolo Sessi
-
Article
| Open AccessTomographic mapping of the hidden dimension in quasi-particle interference
Quasiparticle interference is a powerful tool for characterization of electronic structure which leverages scattering off defects; however, it is limited to quasi two-dimensional materials. Here, the authors demonstrate a method for reconstructing electronic structure of three-dimensional materials from quasiparticle interference data.
- C. A. Marques
- , M. S. Bahramy
- & P. Wahl