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| Open AccessSurface plasmon induced direct detection of long wavelength photons
The detection of terahertz and millimeter waves has many applications, but there are still limitations in their technical performance. Here, Tong et al. demonstrate the direct detection of long-wavelength radiation through surface plasmon excitation and a corresponding improvement in detection performance.
- Jinchao Tong
- , Wei Zhou
- & Dao Hua Zhang
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Article
| Open AccessIntegrated Pound−Drever−Hall laser stabilization system in silicon
Frequency-stable laser systems are important for many applications, like optical communications, that require high precision and low noise. Here, Idjadi and Aflatouni demonstrate that the widely used Pound-Drever-Hall technique can be fully integrated on-chip, miniaturizing the stabilization setup.
- Mohamad Hossein Idjadi
- & Firooz Aflatouni
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Article
| Open AccessColor-selective photodetection from intermediate colloidal quantum dots buried in amorphous-oxide semiconductors
The development of highly sensitive photodetectors is important for image sensing and optical communication applications. Cho et al., report ultra-sensitive photodetectors based on monolayered quantum dots buried in between amorphous-oxide semiconductors and demonstrate color-detecting logic gates.
- Kyung-Sang Cho
- , Keun Heo
- & Sang Yeol Lee
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Article
| Open AccessInterplay of hot electrons from localized and propagating plasmons
Plasmon-induced hot electrons have potential applications spanning photodetection and photocatalysis. Here, Hoang et al. study the interplay between hot electrons generated by localized and propagating plasmons, and demonstrate wavelength-controlled polarity-switchable photoconductivity
- Chung V. Hoang
- , Koki Hayashi
- & Hiroaki Misawa
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Article
| Open AccessSilicon single-photon avalanche diodes with nano-structured light trapping
The performance of silicon single-photon avalanche detectors is currently limited by the trade-off between photon detection efficiency and timing jitter. Here, the authors demonstrate how a CMOS-compatible, nanostructured, thin junction structure can make use of tailored light trapping to break this trade-off.
- Kai Zang
- , Xiao Jiang
- & James S. Harris
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Article
| Open AccessCarbon nanotube-based three-dimensional monolithic optoelectronic integrated system
Single-material monolithic optoelectronic integrated circuits via CMOS compatible low-temperature approaches are crucial to the continued development of post-Moore electronics. Liuet al., report carbon nanotube based electrically driven 3D monolithic optoelectronic integrated circuits.
- Yang Liu
- , Sheng Wang
- & Lian-Mao Peng
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Article
| Open AccessOrganic narrowband near-infrared photodetectors based on intermolecular charge-transfer absorption
Interfaces of organic donor-acceptor blends provide intermolecular charge-transfer states with red-shifted but weak absorption. By introducing an optical micro-cavity; Siegmundet al., enhance their photoresponse to achieve narrowband NIR photodetection with broad spectral tunability.
- Bernhard Siegmund
- , Andreas Mischok
- & Koen Vandewal
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Article
| Open AccessAn integrated parity-time symmetric wavelength-tunable single-mode microring laser
The breaking of parity-time symmetric gain and loss profiles can be used to achieve single-mode lasing in coupled microring resonators. Here, Liuet al. show that this effect can be electrically controlled with a tunable lasing wavelength and strong sidemode suppression.
- Weilin Liu
- , Ming Li
- & Jianping Yao
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Article
| Open AccessTwo-step photon up-conversion solar cells
Harvesting incident photons with energy below the bandgap may lead to highly efficient solar cells. By introducing InAs quantum dots at the hetero-interface, Asahiet al. achieve efficient two step photon up-conversion resulting in additional photocurrent and very high external quantum efficiency.
- Shigeo Asahi
- , Haruyuki Teranishi
- & Takashi Kita
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Article
| Open AccessField-emission from quantum-dot-in-perovskite solids
Efficient implementation of quantum dot and well architectures are restricted to costly vacuum-epitaxially-grown semiconductors. The authors use quantum dots in perovskite to build field-emission photodiodes that are sensitive across the visible and into the short-wavelength infrared.
- F. Pelayo García de Arquer
- , Xiwen Gong
- & Edward Sargent
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Article
| Open AccessGraphene-based mid-infrared room-temperature pyroelectric bolometers with ultrahigh temperature coefficient of resistance
There is emerging interest in photodetectors in the mid-infrared driven by increasing need to monitor the environment for security and healthcare purposes. Sassiet al. show a thermal photodetector, based on the coupling between graphene and a pyroelectric crystal, which shows high temperature sensitivity.
- U. Sassi
- , R. Parret
- & A. Colli
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Article
| Open AccessElectrically tunable organic–inorganic hybrid polaritons with monolayer WS2
Hybrid polariton states originating from the strong coupling of photonic and excitonic states hold promise for control of nonlinear light behaviour. Here, the authors fabricate a microcavity containing organic dye and WS2, featuring hybrid polaritons arising from both Frenkel and Wannier-Mott excitons.
- Lucas C. Flatten
- , David M. Coles
- & Jason M. Smith
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Article
| Open AccessAn antireflection transparent conductor with ultralow optical loss (<2 %) and electrical resistance (<6 Ω sq−1)
Transparent conductors are fundamental for optoelectronics. Using the transfer matrix method to optimise a multistructure of anti-reflection coatings containing an ultrathin metal film, Maniyaraet al. achieve the highest transmittance of an antireflection transparent conductor combined with low resistance.
- Rinu Abraham Maniyara
- , Vahagn K. Mkhitaryan
- & Valerio Pruneri
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Article
| Open AccessMiniature optical planar camera based on a wide-angle metasurface doublet corrected for monochromatic aberrations
Metasurfaces have the potential to be used in imaging systems since they can modify optical wavefronts at subwavelength spatial resolution. Here, Arbabi et al. demonstrate a metasurface lens doublet corrected for monochromatic aberrations, and integrate it with an image sensor to realize a miniature planar camera.
- Amir Arbabi
- , Ehsan Arbabi
- & Andrei Faraon
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Article
| Open AccessSelf-assembled fibre optoelectronics with discrete translational symmetry
The thermal-draw technique offers fibre devices with a multiplicity of geometries, but these are constrainted to being translationally symmetric. Here, the authors disrupt this symmetry by applying selective capillary instability, resulting in electrically connected spherical photodetecting elements.
- Michael Rein
- , Etgar Levy
- & Yoel Fink
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Article
| Open AccessPhoto-thermionic effect in vertical graphene heterostructures
The detection of low-energy photons may be enabled by devices that make use of the excess thermal energy from photoexcited carriers as a result of light absorption. Here the authors demonstrate a vertical graphene-WSe2-graphene heterostructure that takes advantage of the photo-thermionic effect.
- M. Massicotte
- , P. Schmidt
- & F. H. L. Koppens
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Article
| Open AccessProbing the electrical switching of a memristive optical antenna by STEM EELS
Scaling of photonic devices requires materials with sufficiently strong elecro-optic effects. Here, Schoen et al.demonstrate and analyze single electrically induced switching events that can operate in the visible with a small active volume using electron energy loss in a scanning transmission electron microscope.
- David T. Schoen
- , Aaron L. Holsteen
- & Mark L. Brongersma
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Article
| Open AccessElectrically driven optical metamaterials
Active metamaterials are largely controlled by light, preventing integration in electronic systems. Here, the authors introduce electroluminescent metamaterials based on metal nano-inclusions hybridized with colloidal quantum dots and use this approach to weave intricate light-emitting surfaces.
- Quynh Le-Van
- , Xavier Le Roux
- & Aloyse Degiron
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Article
| Open AccessPhoto-induced halide redistribution in organic–inorganic perovskite films
Visual evidence for photo-induced ionic migration in perovskite films without contacts is lacking. Here, the authors use a unique combination of confocal photoluminescence microscopy and chemical imaging to correlate the local changes in photophysics with composition in CH3NH3PbI3films under illumination.
- Dane W. deQuilettes
- , Wei Zhang
- & Samuel D. Stranks
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Article
| Open AccessControlling the volatility of the written optical state in electrochromic DNA liquid crystals
Electrochromism, the dependence of light absorption upon electronic control, finds a wide range of applications in smart materials. Here, Liu et al. show an electrochromic DNA–surfactant liquid crystal system that exhibits electrically tunable optical absorption and thermally tunable memory.
- Kai Liu
- , Justin Varghese
- & Andreas Herrmann
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Article
| Open AccessGiant photoluminescence enhancement in tungsten-diselenide–gold plasmonic hybrid structures
Two-dimensional materials have excellent electrical properties, but poor luminescence limits their application in optoelectronics. Here, the authors demonstrate a plasmon-induced 20,000-fold enhancement in photoluminescence from tungsten diselenide suspended across a nanometre-scale gap.
- Zhuo Wang
- , Zhaogang Dong
- & Andrew T. S. Wee
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Article
| Open AccessExciton localization in solution-processed organolead trihalide perovskites
The recombination dynamics of photogenerated carriers in organolead trihalide perovskites are not well understood. Here, He et al.report that the recombination of photogenerated carriers in solution-processed methylammonium-lead-halide films is dominated by excitons weakly localized in band tail states.
- Haiping He
- , Qianqian Yu
- & Zhizhen Ye
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Article
| Open AccessBroadband chirality-coded meta-aperture for photon-spin resolving
Nano-apertures cannot distinguish between distinct spin-states of photons because of information loss upon light-aperture interaction. Here, Du et al.report a subwavelength aperture integrated with metasurfaces which breaks spin degeneracy and produces opposite transmission spectra over a broad spectral range.
- Luping Du
- , Shan Shan Kou
- & Jiao Lin
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Article
| Open AccessHigh mobility emissive organic semiconductor
Organic semiconductors with high mobility and strong fluorescence are necessary for optoelectronic devices. Here, Liu et al. show an organic semiconductor, 2,6-diphenylanthracene, satisfying both requirements with mobility of 34 cm2 V−1 s−1 and emission of 6,627 cd m−2at a turn-on voltage of 2.8 V.
- Jie Liu
- , Hantang Zhang
- & Alan J. Heeger
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Article
| Open AccessEnhanced optoelectronic quality of perovskite thin films with hypophosphorous acid for planar heterojunction solar cells
An imbalance in I/Pb stoichiometry is thought to lead to defects in metal halide films. Here, Zhang et al. show that the addition of hypophosphorous acid in the precursor solution can significantly improve the film quality and enhance the photoluminescence intensity, leading to improved photovoltaic devices.
- Wei Zhang
- , Sandeep Pathak
- & Henry J. Snaith
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Article
| Open AccessPlanar-integrated single-crystalline perovskite photodetectors
Single crystals of organolead halide perovskites exhibit large carrier mobilities and long diffusion lengths. Here, the authors succeed in growing the single crystals on planar substrates and integrate them as the active layer of visible photodetectors with a large gain-bandwidth product.
- Makhsud I. Saidaminov
- , Valerio Adinolfi
- & Osman M. Bakr
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Article
| Open AccessStable ultrathin partially oxidized copper film electrode for highly efficient flexible solar cells
Light enters and exits optoelectronic devices through transparent conductive electrodes, which are one of their most expensive components. Here, the authors develop stable transparent conductive electrodes based on copper and oxide layers that lead to efficient flexible organic solar cells.
- Guoqing Zhao
- , Wei Wang
- & Jungheum Yun
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Article
| Open AccessPlanar carbon nanotube–graphene hybrid films for high-performance broadband photodetectors
Graphene has excellent electronic properties but its photoresponsivity is limited by low absorption and the ultrafast recombination of photoexcited carriers. Here, the authors demonstrate fast, high responsivity and broadband photodetectors by combining graphene with single-wall carbon nanotubes.
- Yuanda Liu
- , Fengqiu Wang
- & Rong Zhang
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Article
| Open AccessHot-carrier cooling and photoinduced refractive index changes in organic–inorganic lead halide perovskites
The use of organic–inorganic metal-halide perovskites in hot-carrier devices depends on deepening the understanding of photoexcitations in these materials. Here, Price et al. use transient absorption spectroscopy to study hot-carrier distributions in CH3NH3PbI3and quantify key semiconductors parameters.
- Michael B. Price
- , Justinas Butkus
- & Felix Deschler
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Article
| Open AccessCreating semiconductor metafilms with designer absorption spectra
Ultrathin semiconductor metafilms can be designed to achieve near-unity absorption in specific spectral regions. Here, Kim et al. engineer nanoscale optical resonances in sub-50-nm-thick germanium nanobeams metafilms to demonstrate near-unity absorption in one or more desired wavelength regions.
- Soo Jin Kim
- , Pengyu Fan
- & Mark L. Brongersma
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Article
| Open AccessElectric-field-induced strong enhancement of electroluminescence in multilayer molybdenum disulfide
The layer-number-dependent optical and electronic properties of transition metal dichalcogenides are promising in optoelectronics. Here, Li et al. demonstrate greatly enhanced electroluminescence emission in multi-layer MoS2attributed to the electric-field-induced carrier redistribution.
- Dehui Li
- , Rui Cheng
- & Xiangfeng Duan
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Article
| Open AccessLead iodide perovskite light-emitting field-effect transistor
Hybrid organic–inorganic perovskites have shown great potential for use in optoelectronic applications. Here, the authors create solution-processed lead iodide perovskite light-emitting field-effect transistors and demonstrate both ambipolar behaviour and gate-assisted electroluminescence.
- Xin Yu Chin
- , Daniele Cortecchia
- & Cesare Soci
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Article
| Open AccessHigh-quality sandwiched black phosphorus heterostructure and its quantum oscillations
Black phosphorus is an atomically thin material that exhibits excellent properties for electronics applications, but these degrade in atmospheric conditions. Here, the authors demonstrate the fabrication of stable, ultra-clean and high-mobility black phosphorus sandwiched between the layers of boron nitride.
- Xiaolong Chen
- , Yingying Wu
- & Ning Wang
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| Open AccessHigh-performance flexible perovskite solar cells exploiting Zn2SnO4 prepared in solution below 100 °C
There has been impressive progress in the development of perovskite solar cells in recent years, but the best performing systems tend to be fabricated on glass surfaces. Here, the authors present a cell built on a polymer substrate, allowing flexibility whilst maintaining high efficiency.
- Seong Sik Shin
- , Woon Seok Yang
- & Sang Il Seok
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Article
| Open AccessOptoelectronic crystal of artificial atoms in strain-textured molybdenum disulphide
Periodically strained monolayer molybdenum disulphide funnels photogenerated electron-hole pairs across an electric field induced by a spatially graded band gap, mimicking a crystal of artificial atoms. Here, the authors experimentally demonstrate the artificial crystal in strain-textured molybdenum disulphide.
- Hong Li
- , Alex W. Contryman
- & Xiaolin Zheng
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| Open AccessThe optoelectronic role of chlorine in CH3NH3PbI3(Cl)-based perovskite solar cells
Chlorine incorporation into CH3NH3PbI3improves solar cell performance, but its optoelectronic role is still unclear. Here the authors present a strategy that decouples the morphological impact, to reveal that chlorine incorporation affects carrier transport across the heterojunction interface rather than within the perovskite crystal.
- Qi Chen
- , Huanping Zhou
- & Yang Yang
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Article
| Open AccessPerovskite–fullerene hybrid materials suppress hysteresis in planar diodes
Metal halide perovskites are promising for solar energy harvesting, but currently prone to a large hysteresis and current instability. Here, Xu et al. show improvements in a hybrid material in which the fullerene is distributed at perovskite grain boundaries and thus passivates defects effectively.
- Jixian Xu
- , Andrei Buin
- & Edward H. Sargent
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Article |
Subwavelength-thick lenses with high numerical apertures and large efficiency based on high-contrast transmitarrays
Replacing conventional components with flat optic devices such as flat lenses is desirable for imaging and on-chip integration, but performance has hindered their use. Here, Arbabi et al. report a wavelength-thin, high-contrast transmitarray micro-lens with a 0.57 λfocal spot and 82% focusing efficiency.
- Amir Arbabi
- , Yu Horie
- & Andrei Faraon
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Article
| Open AccessActive control of all-fibre graphene devices with electrical gating
Active control of light in optical fibres is of great interest, to this end, electric control of all-fibre graphene devices is desirable but highly challenging. Here, Lee et al. demonstrate electric control of the optical properties of a graphene sheet deposited on a side-polished fibre mediated by an ion liquid.
- Eun Jung Lee
- , Sun Young Choi
- & Dong-Il Yeom
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Article
| Open AccessPatterning two-dimensional chalcogenide crystals of Bi2Se3 and In2Se3 and efficient photodetectors
Two-dimensional chalcogenides offer great potential in electronics, but accurate control of their growth is difficult. Here, the authors combine microintaglio printing and van der Waals epitaxy to pattern various large-area arrays of single-crystal chalcogenides with remarkable properties.
- Wenshan Zheng
- , Tian Xie
- & Hailin Peng
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Article
| Open AccessPositioning and joining of organic single-crystalline wires
Aligned, one-dimensional, single-crystal materials may allow on-demand photon/electron transfer. Here, the authors use a physical vapour transport technique to grow organic single-crystal wires with the guidance of pillar-structured substrates, and perform proof of concept waveguide experiments.
- Yuchen Wu
- , Jiangang Feng
- & Lei Jiang
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Article
| Open AccessUltrafast helicity control of surface currents in topological insulators with near-unity fidelity
Bulk contributions to transport measurements often inhibit the study of the surface states of topological insulators. Here, Kastl et al. demonstrate high-fidelity helicity-dependent photocurrents in the surface states of Bi2Se3, controlled via circularly polarized light with a picosecond time-resolution.
- Christoph Kastl
- , Christoph Karnetzky
- & Alexander W. Holleitner
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Article
| Open AccessUltimate thin vertical p–n junction composed of two-dimensional layered molybdenum disulfide
Molybdenum disulfide is a two-dimensional semiconducting material that has properties that make it useful for compact electronic devices. Here, the authors use molybdenum disulfide in an ultra-thin p–n junction that demonstrate ambipolar carrier transport and current rectification.
- Hua-Min Li
- , Daeyeong Lee
- & Won Jong Yoo
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Article |
Surface transfer doping induced effective modulation on ambipolar characteristics of few-layer black phosphorus
Black phosphorus is a graphene-like material that can be harnessed for two-dimensional electronic devices. Here, Xiang et al. demonstrate that adding caesium carbonate or molybdenum trioxide can significantly enhance the electron or hole conduction, respectively, of this promising material.
- Du Xiang
- , Cheng Han
- & Wei Chen
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Bandgap tunability at single-layer molybdenum disulphide grain boundaries
Molybdenum disulphide is a two-dimensional material that, unlike graphene, has a nonzero bandgap. Here, the authors demonstrate that the bandgap of single-layer molybdenum disulphide grown on graphite by chemical vapour deposition changes with distance from the grain boundary
- Yu Li Huang
- , Yifeng Chen
- & Andrew T. S. Wee
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Seeded growth of highly crystalline molybdenum disulphide monolayers at controlled locations
Although synthesis of high-quality MoS2 has been demonstrated, growth of monolayer MoS2at controlled locations is highly desirable for applications. Here, the authors introduce a method where patterned seeds of molybdenum source material are used to grow isolated flakes at predetermined locations.
- Gang Hee Han
- , Nicholas J. Kybert
- & A. T. Charlie Johnson
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Article
| Open AccessModulator-free quadrature amplitude modulation signal synthesis
Quadrature amplitude modulation signalling is currently enabling rapid data transfer capacity growth, but it still has associated drawbacks. Here, Liu et al.use optical injection locking to generate complex modulation format signals with reduced consumption, small footprint and easy integration.
- Zhixin Liu
- , Joseph Kakande
- & Radan Slavík
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Coherent two-dimensional photocurrent spectroscopy in a PbS quantum dot photocell
Two-dimensional photocurrent spectroscopy can identify coherent electronic dynamics and offers promise for studies of numerous material systems. Karki et al. now show that the method can be used to study ultrafast carrier processes in lead sulphide quantum dots, such as multiple exciton generation.
- Khadga J. Karki
- , Julia R. Widom
- & Andrew H. Marcus
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Experimental realization of photonic topological insulator in a uniaxial metacrystal waveguide
Photonic topological insulators have been theoretically predicted but their experimental demonstration has proven challenging. Here, Chen et al.experimentally realize a photonic topological insulator by embedding a non-bianisotropic and a non-resonant metacrystal into a waveguide.
- Wen-Jie Chen
- , Shao-Ji Jiang
- & C. T. Chan