Featured
-
-
Article |
High performance piezoelectric devices based on aligned arrays of nanofibers of poly(vinylidenefluoride-co-trifluoroethylene)
Piezoelectronic materials are attractive for force sensing and as energy harvesting components in electronics that interface directly with the human body. Here, the authors synthesize large area, flexible, electrospun materials capable of ultra-high sensitivity force measurements in the low-pressure regime.
- Luana Persano
- , Canan Dagdeviren
- & John A. Rogers
-
Article
| Open AccessQuantum dot imaging platform for single-cell molecular profiling
Multiplexed labelling of individual cells allows the direct observation of intracellular molecular composition, but is difficult to achieve with existing techniques. Here, self-assembled fluorescent nanoparticle probes and multicolour multicycle staining are used for the simultaneous evaluation of multiple biomolecules at subcellular resolution.
- Pavel Zrazhevskiy
- & Xiaohu Gao
-
Article |
Phase-locked indistinguishable photons with synthesized waveforms from a solid-state source
Coherent single photons can be exploited in many quantum interference applications like quantum communication or entanglement. In this work, the authors achieve the generation of phase-locked single photons from a quantum dot, thus opening a new route to solid-state quantum networks.
- Clemens Matthiesen
- , Martin Geller
- & Mete Atatüre
-
Article |
Large spin-orbit coupling in carbon nanotubes
Large spin-orbit coupling in solids has the potential to yield materials that can display unique properties such as non-trivial topological ordering. Steele et al.report an order of magnitude higher zero-field spin splitting in carbon than has been measured previously.
- G.A. Steele
- , F. Pei
- & L.P. Kouwenhoven
-
Article
| Open AccessA two-atom electron pump
Transistors that operate by the passage of electrons through a single-dopant atom achieve the ultimate limit for the miniaturization of electronic devices, but only when multiple transistors are intimately connected can they become useful. Roche et al. demonstrate the equivalent of just this, connecting two such transistors to build a two-atom electron pump.
- B. Roche
- , R.-P. Riwar
- & X. Jehl
-
Article
| Open AccessNanoscale light–matter interactions in atomic cladding waveguides
Alkali vapours are increasingly useful in photonic research and metrology applications, and they provide a useful test bed for investigating light–matter interaction. Stern et al. integrate silicon nitride waveguides with alkali vapours to study light–matter interactions on a chip-scale platform.
- Liron Stern
- , Boris Desiatov
- & Uriel Levy
-
Article |
A low-temperature method to produce highly reduced graphene oxide
The chemical reduction of graphene oxide can provide large quantities of reduced graphene oxide for potential application in electronics and composite materials. Feng et al. report a highly efficient low-temperature one-pot reduction of graphene oxide that uses sodium-ammonia solution as the reducing agent.
- Hongbin Feng
- , Rui Cheng
- & Jinghong Li
-
Article |
Directional visible light scattering by silicon nanoparticles
The scattering of light by nanoparticles could be useful for photonic nanoantenna or other light manipulation schemes. Here Kuznetsov et al. demonstrate directional light scattering from silicon nanoparticles for visible light.
- Yuan Hsing Fu
- , Arseniy I. Kuznetsov
- & Boris Luk’yanchuk
-
Article |
Voltage tunability of single-spin states in a quantum dot
Manipulation of spins in the solid state is a promising avenue for quantum information and field sensing applications. Bennett et al. demonstrate voltage tunability of single-spin states in a quantum dot as a step towards universal control of a single spin with a single electrical gate.
- Anthony J. Bennett
- , Matthew A. Pooley
- & Andrew J. Shields
-
Article |
Surface-passivated GaAsP single-nanowire solar cells exceeding 10% efficiency grown on silicon
The use of III-V semiconductor nanowires can overcome the need for lattice matching in multi-junction solar cells, which restricts the choice of materials and their bandgaps. This work demonstrates efficient solar cells with GaAsP single nanowires with tunable bandgap and grown on low-cost Si substrates.
- Jeppe V. Holm
- , Henrik I. Jørgensen
- & Martin Aagesen
-
Article |
A synthetic nanomaterial for virus recognition produced by surface imprinting
The recognition of viruses by synthetic materials is historically difficult. Here, a templating procedure using silica nanoparticles coated with organosilanes is used to form virus-imprinted particles, possessing both shape and chemical imprints, capable of virus recognition at picomolar concentrations.
- Alessandro Cumbo
- , Bernard Lorber
- & Patrick Shahgaldian
-
Article
| Open AccessGaAs nanopillar-array solar cells employing in situ surface passivation
Arrays of III–V semiconductor nanopillars are promising photovoltaic materials due to their favourable optical properties, however, they show low power conversion efficiencies. Mariani et al. fabricate a GaAs nanopillar solar cell achieving an efficiency of 6.63% owing to surface passivation.
- Giacomo Mariani
- , Adam C. Scofield
- & Diana L. Huffaker
-
Article
| Open AccessFemtosecond nonlinear ultrasonics in gold probed with ultrashort surface plasmons
Measuring acoustic phonons across the Brillouin zone reveals important information on electrical and thermal transport in materials. Temnov et al.generate giant acoustic strain pulses in gold/cobalt bilayers and monitor their nonlinear reshaping in the gold layer with plasmonic interferometry.
- Vasily V. Temnov
- , Christoph Klieber
- & Rudolf Bratschitsch
-
Article |
Bright solid-state sources of indistinguishable single photons
For quantum technologies to become widespread and scalable, bright sources of indistinguishable single photons are essential. Through deterministic positioning of quantum dots in pillar cavities, Gazzano et al.present a solid-state single-photon source with brightness as large as 0.65 photons per pulse.
- O. Gazzano
- , S. Michaelis de Vasconcellos
- & P. Senellart
-
Article
| Open AccessNanoscale imaging and spontaneous emission control with a single nano-positioned quantum dot
The emission properties of quantum dots make them ideal for probing plasmonic nanostructures, but their small size makes them difficult to manipulate. Ropp et al.use a microfluidic system to accurately place single quantum dots around silver nanowires to probe the local density of optical states.
- Chad Ropp
- , Zachary Cummins
- & Edo Waks
-
Article
| Open AccessUltrafast universal quantum control of a quantum-dot charge qubit using Landau–Zener–Stückelberg interference
Universal control of the state of qubits on timescales much shorter than the coherence time is necessary for quantum computation. The authors demonstrate electrical control of a charge qubit in quantum dots on the picosecond scale, which is orders of magnitude faster than previously reported.
- Gang Cao
- , Hai-Ou Li
- & Guo-Ping Guo
-
Article |
Photon-mediated interaction between distant quantum dot circuits
Controlling the interaction between distant quantum dots is important if they are to be used in quantum information devices. Delbecq et al. place two quantum dot circuits in a microwave cavity and show that they interact via cavity photons, even though they are separated by 200 times their own size.
- M.R. Delbecq
- , L.E. Bruhat
- & T. Kontos
-
Article |
Composite-pulse magnetometry with a solid-state quantum sensor
Quantum magnetometry in the solid state is usually affected by short coherence times and control errors that limit the sensitivity. This work demonstrates a continuous-driving scheme based on composite pulses that improves both these shortcomings and can be used in variable sensing environments.
- Clarice D. Aiello
- , Masashi Hirose
- & Paola Cappellaro
-
Article |
Catalytic subsurface etching of nanoscale channels in graphite
Metallic particles are known to etch the surface layers of graphite by catalytic hydrogenation. Here, the authors report the sub-surface etching of graphite by Ni nanoparticles, revealing the formation of networks of tunnels, which are observed microscopically and could be modified for various applications.
- Maya Lukas
- , Velimir Meded
- & Ralph Krupke
-
Article |
Controllable unzipping for intramolecular junctions of graphene nanoribbons and single-walled carbon nanotubes
The formation of junctions between graphene and other materials could aid the development of nanoelectronics. We et al. partially unzip single-walled carbon nanotubes to produce graphene/nanotube junctions that show gate-dependent rectifying behaviour.
- Dacheng Wei
- , Lanfei Xie
- & Andrew Thye Shen Wee
-
Article
| Open AccessStrain-controlled magnetic domain wall propagation in hybrid piezoelectric/ferromagnetic structures
The use of electric fields to control the magnetization of ferromagnetic materials could enable more efficient electronics. Lei et al.show that by applying lateral strain to a magnetostrictive nanowire with a piezoelectric, voltage-controlled gating of magnetic domain wall motion in the wire can be achieved.
- Na Lei
- , Thibaut Devolder
- & Philippe Lecoeur
-
Article |
Quantum-coupled radial-breathing oscillations in double-walled carbon nanotubes
Double-walled carbon nanotubes are a convenient system for studying quantum mechanical interactions in distinct but coupled nanostructures. Liu et al.characterize the coupling between radial-breathing mode oscillations of inner and outer walls of many double-walled nanotubes of different diameter and chirality.
- Kaihui Liu
- , Xiaoping Hong
- & Feng Wang
-
Article
| Open AccessGlobally homochiral assembly of two-dimensional molecular networks triggered by co-absorbers
The construction of homochiral surfaces may play a significant role in applications including heterogeneous catalysis and bio-sensors. Here, globally homochiral two-dimensional assemblies of achiral molecules are formed via co-assembly with chiral co-adsorbers, demonstrating a ‘majority rules’ effect.
- Ting Chen
- , Wen-Hong Yang
- & Li-Jun Wan
-
Article |
Probing the electronic structure at semiconductor surfaces using charge transport in nanomembranes
As the electrical properties of nanostructures are strongly influenced by their surface, a thorough understanding of the surface properties is desirable. The authors demonstrate the use of charge transport in silicon nanomembranes to perform spectroscopy of the electronic structure of the surface states.
- Weina Peng
- , Zlatan Aksamija
- & Max G. Lagally
-
Article |
From chaos to selective ordering of vortex cores in interacting mesomagnets
The collective gyrotropic excitation of an array of spin vortices has frequencies that depend on the polarities and chirality of individual vortices. This work demonstrates control of the spectral response of the system by tuning the excitation frequency or the external magnetic field.
- S. Jain
- , V. Novosad
- & S.D. Bader
-
Article
| Open AccessAtomic-scale engineering of magnetic anisotropy of nanostructures through interfaces and interlines
The design and assembly of nanostructures exhibiting ferromagnetic hysteresis at room temperature are recognized goals for high-density data storage. Here, the authors engineer nanostructures with atomically sharp bimetallic interfaces and interlines, which exhibit large magnetic anisotropy and high temperature hysteresis.
- S. Ouazi
- , S. Vlaic
- & H. Brune
-
Article |
The surface plasmon modes of self-assembled gold nanocrystals
The 3D self-assembly of nanocrystals could generate materials with unique optical and electronic properties. Barrowet al. report the DNA-mediated assembly of symmetrical 3D gold tetrahedra, pentamers and hexamers, and elucidate their plasmon modes.
- Steven J. Barrow
- , Xingzhan Wei
- & Paul Mulvaney
-
Article
| Open AccessGiant Raman gain in silicon nanocrystals
In a nonlinear medium, a pump laser beam generates and amplifies a second beam at a different frequency through stimulated Raman scattering. Sirleto et al.show this effect in silicon nanocrystals in a silicon matrix, with gain greater than four orders of magnitude compared with crystalline silicon.
- Luigi Sirleto
- , Maria Antonietta Ferrara
- & Leonid Khriachtchev
-
Article
| Open AccessCarbon nanotube–liposome supramolecular nanotrains for intelligent molecular-transport systems
There is growing interest in the development of artificial molecular-transport systems. Miyakoet al. develop a supramolecular system consisting of carbon nanotubes and liposomes that allows the directional transport and controlled release of cargo molecules.
- Eijiro Miyako
- , Kenji Kono
- & Yoshihisa Hagihara
-
Article |
Flexible and low-voltage integrated circuits constructed from high-performance nanocrystal transistors
Field-effect transistors based on semiconductor nanocrystals are promising candidates for low-cost, flexible electronics. This work demonstrates fabrication on flexible substrates and low-voltage operations of integrated circuits based on nanocrystal transistors, including amplifiers and ring oscillators.
- David K. Kim
- , Yuming Lai
- & Cherie R. Kagan
-
Article
| Open AccessDirect writing of electronic devices on graphene oxide by catalytic scanning probe lithography
Controlled nanoscale reduction of graphene oxide could aid the development of graphene-based electronics. Here, a relatively mild technique is reported that uses a platinum-coated atomic force microscope tip to catalyse the reduction of graphene oxide to graphene.
- Kun Zhang
- , Qiang Fu
- & Jianguo Hou
-
Article |
Chirality-controlled synthesis of single-wall carbon nanotubes using vapour-phase epitaxy
The promising electronic properties of single-wall carbon nanotubes are strongly dependent on their chirality. Here a metal catalyst free, vapour-phase epitaxy-type cloning mechanism is shown to yield high purity metallic and semiconducting nanotubes from purified single-chirality seeds.
- Jia Liu
- , Chuan Wang
- & Chongwu Zhou
-
Article |
Self-luminescing BRET-FRET near-infrared dots for in vivo lymph-node mapping and tumour imaging
Fluorescence imaging in vivo is hampered by autofluorescence and the scattering and absorption of short-wavelength light. To address these problems, Xiong et al. produce self-luminescing nanoparticles that enable in vivonear-infrared imaging without external light excitation.
- Liqin Xiong
- , Adam J. Shuhendler
- & Jianghong Rao
-
Article |
Tracking lithium transport and electrochemical reactions in nanoparticles
Developing next generation batteries requires better understanding of the dynamics of electrochemical reactions in working electrodes. Using a transmission electron microscope, Wanget al. develop a means to track the real time flow of lithium atoms in electrodes during the discharge of a functioning electrochemical cell.
- Feng Wang
- , Hui-Chia Yu
- & Jason Graetz
-
Article
| Open AccessDetermination of monolayer-protected gold nanoparticle ligand–shell morphology using NMR
Binary mixtures of molecules on the surface of nanoparticles can arrange randomly or into different domains to form Janus, patchy or striped particles. Liuet al.show that NMR can be used to determine the ligand-shell morphology of particles coated with aliphatic and aromatic ligands.
- Xiang Liu
- , Miao Yu
- & Francesco Stellacci
-
Article |
High-efficiency Cooper pair splitting demonstrated by two-particle conductance resonance and positive noise cross-correlation
The Cooper pairs that losslessly conduct current in a superconductor can be split into two spatially separated but quantum mechanically entangled electrons. In this paper, non-local cross-correlation measurements of pairs split within a superconducting wire indicate the efficiency of this process can approach 100%.
- Anindya Das
- , Yuval Ronen
- & Hadas Shtrikman
-
Article
| Open AccessCorrelative infrared–electron nanoscopy reveals the local structure–conductivity relationship in zinc oxide nanowires
High-resolution characterisation techniques enable us to better understand the properties of nanoscale materials and devices. By combining electron microscopy and infrared nanoscopy, Stiegleret al.demonstrate a general approach to simultaneously probe the structural, chemical and electronic properties of a nanostructure.
- J.M. Stiegler
- , R. Tena-Zaera
- & R. Hillenbrand
-
Article |
Bioinspired hollow semiconductor nanospheres as photosynthetic nanoparticles
Photosynthesis occurs at the thylakoid membrane, which acts as a scaffold, precisely arranging functional proteins and electron carriers. Sunet al.synthesize hollow photosynthetic nanospheres that function as light-harvesting antennae and structured scaffolds that improve photoredox catalysis.
- Jianhua Sun
- , Jinshui Zhang
- & Xinchen Wang
-
Article
| Open AccessHybrid nanoparticle–microcavity-based plasmonic nanosensors with improved detection resolution and extended remote-sensing ability
Plasmonic nanoparticles are useful as optical sensors, but their spectral resolution is hindered by the linewidth of the plasmon resonance. Schmidtet al. find that coupling this resonance to a microcavity creates hybrid modes with enhanced sensing figure-of-merit and improved frequency resolution.
- Markus A. Schmidt
- , Dang Yuan Lei
- & Stefan A. Maier
-
Article
| Open AccessGraphene-contact electrically driven microdisk lasers
Microdisk lasers are useful for compact wavelength-scale photonic devices and circuits, but their operation by electrical injection can hamper their optical properties. Kimet al. show that a graphene-contact electrode provides efficient electrical injection while minimising optical losses.
- Yoon-Ho Kim
- , Soon-Hong Kwon
- & Hong-Gyu Park
-
Article |
Highly stable Pt monolayer on PdAu nanoparticle electrocatalysts for the oxygen reduction reaction
Platinum is used as a cathode in fuel cells but undergoes dissolution during potential changes, hindering commercial application in electric vehicles. Sasakiet al.report a new class of stable electrocatalysts that consist of platinum monolayers on palladium–gold alloy nanoparticles.
- Kotaro Sasaki
- , Hideo Naohara
- & Radoslav R. Adzic
-
Article
| Open AccessMagnesium-free self-assembly of multi-layer DNA objects
Self-assembly of DNA can provide access to a range of nanoscale structures, but assembly using magnesium has been considered essential. Martin and Dietz report conditions that allow the assembly of templated, multi-layer DNA structures in the presence of monovalent ions, rather than magnesium.
- Thomas G. Martin
- & Hendrik Dietz
-
Article |
Top-down fabricated silicon nanowires under tensile elastic strain up to 4.5%
Strain in Si nanostructures is used to achieve higher carrier mobility, making these devices candidates for the next generation of transistors. Minamisawaet al. fabricate silicon nanowires subject to elastic tensile strain up to 4.5%, exceeding the limit achievable with the use of SiGe virtual substrates.
- R.A. Minamisawa
- , M.J. Süess
- & H. Sigg
-
Article |
Multichannel cavity optomechanics for all-optical amplification of radio frequency signals
Cavity optomechanics can exploit optical forces to achieve all-optical signal processing, but most schemes are limited to a narrow wavelength range. Using a cavity optomechanical design system with two optical channels, Liet al. show broadband readout and all-optical amplification of radio-frequency signals.
- Huan Li
- , Yu Chen
- & Mo Li
-
Article |
Insights into the biomedical effects of carboxylated single-wall carbon nanotubes on telomerase and telomeres
Single-walled carbon nanotubes can selectively stabilize telomeric i-motif DNA and have been suggested as a treatment for cancer. Here, carbon nanotubes are found to inhibit telomerase activity by stabilizing i-motif DNA, leading to telomere uncapping and altered telomere function in cancer cells.
- Yong Chen
- , Konggang Qu
- & Xiaogang Qu
-
Article |
Monodisperse conjugated polymer particles by Suzuki–Miyaura dispersion polymerization
Well-defined, monodisperse colloids of semiconducting polymers are required as new photonic and optoelectronic materials. Here, a Suzuki–Miyaura dispersion polymerization is used to produce monodisperse sub-micrometer particles of a range of semiconducting polymers.
- Alexander J.C. Kuehne
- , Malte C. Gather
- & Joris Sprakel
-
Article |
Imaging enzyme-triggered self-assembly of small molecules inside live cells
Supramolecular interactions allow some small molecules to self-assemble into nanofibres and hydrogels in aqueous environments. Gaoet al.report a hydrogelator that forms fluorescent nanofibres within cells, leading to the visualization of their self-assembly at the endoplasmic reticulum.
- Yuan Gao
- , Junfeng Shi
- & Bing Xu
-
Article
| Open AccessThree-dimensional orientation-unlimited polarization encryption by a single optically configured vectorial beam
Generating arbitrary orientation of light polarization has been an elusive goal, yet it is important to light interactions with nano-objects. By combining azimuthally and radially polarized beams, Liet al. overcome this obstacle and demonstrate its use for polarization-based encryption with gold nanorods.
- Xiangping Li
- , Tzu-Hsiang Lan
- & Min Gu
-
Article |
Symmetry breaking in the formation of magnetic vortex states in a permalloy nanodisk
Vortex states in magnetic nanoislands are characterized by a curling of the magnetization in the plane of the disk. This study demonstrates experimentally that vortices tend to form with a preferred handedness that is dictated by the Dzyaloshinskii–Moriya interaction.
- Mi-Young Im
- , Peter Fischer
- & Teruo Ono