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Stretchable silicon nanoribbon electronics for skin prosthesis
An integrated electronic platform with site-specific sensitivity is highly needed for medical applications. Here, Kim et al.report a stretchable prosthetic skin composed of ultrathin single crystalline silicon nanoribbon array, which can sense strain, pressure and temperature spontaneously.
- Jaemin Kim
- , Mincheol Lee
- & Dae-Hyeong Kim
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Nanoscale infrared spectroscopy as a non-destructive probe of extraterrestrial samples
Infrared spectral mapping offers the non-destructive analyses of samples; however, the spatial resolution is restricted to >10 microns. Here, the authors present a new infrared technique capable of sub-micron scale mineral identification, demonstrated using a chondrule and a cometary dust grain.
- Gerardo Dominguez
- , A. S. Mcleod
- & D. N. Basov
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Carbon nanotube network-silicon oxide non-volatile switches
The integration of carbon nanotubes with silicon is important for their incorporation into next-generation nano-electronics. Here, the authors demonstrate a non-volatile switch that utilizes carbon nanotube networks to electrically contact a conductive nano-crystal silicon filament in silica.
- Albert D. Liao
- , Paulo T. Araujo
- & Mildred S. Dresselhaus
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| Open AccessLattice-free prediction of three-dimensional structure of programmed DNA assemblies
DNA may be used to fabricate functional nanostructures with various possible geometries, but first being able to predict these structures is a challenging task. Here, the authors use coarse-grained modelling to predict the shape of artificial DNA nanostructures in solution.
- Keyao Pan
- , Do-Nyun Kim
- & Mark Bathe
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Programmed folding of DNA origami structures through single-molecule force control
The typical method for DNA origami fabrication uses thermal annealing of staples to a longer DNA scaffold. Here, the authors present a mechanical method to control the folding pathway, which instead relies on stretching the DNA scaffold in magnetic tweezers, prior to staple incorporation.
- Wooli Bae
- , Kipom Kim
- & Tae-Young Yoon
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Photocatalytic colour switching of redox dyes for ink-free light-printable rewritable paper
Printing text and images is a significant cause of paper and ink waste, leading to an increased focus on reusable alternatives. Here, the authors show that films of commercial dyes can be photoactivated with UV light and catalysts and, with an appropriate stabilizer, can be used as a rewritable display system.
- Wenshou Wang
- , Ning Xie
- & Yadong Yin
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Soft epitaxy of nanocrystal superlattices
Epitaxial crystal growth is widely used in electronics for the rational design of efficient devices. Here, Rupich et al. find a universal law for island size scaling, which outlines similarities and differences between self-assembly of nanocrystals and atomic epitaxial growth.
- Sara M. Rupich
- , Fernando C. Castro
- & Dmitri V. Talapin
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Optical transmission enhacement through chemically tuned two-dimensional bismuth chalcogenide nanoplates
Recent studies have shown that the electronic properties of two-dimensional bismuth chalcogenides can be modified by chemical intercalation. Here, Yao et al. demonstrate that the optical transmission in bismuth chacogenide nanoplates can be tuned by intercalation of copper atoms.
- Jie Yao
- , Kristie J. Koski
- & Yi Cui
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Sponge-like molecular cage for purification of fullerenes
Mixtures of various size fullerenes are available as a component of fullerene soot, but isolating pure fullerenes is a challenging task. Here, the authors use a porphyrin-based supramolecular cage that encapsulates fullerenes with high selectivity and releases C60by a simple washing technique.
- Cristina García-Simón
- , Marc Garcia-Borràs
- & Xavi Ribas
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| Open AccessUltralow mode-volume photonic crystal nanobeam cavities for high-efficiency coupling to individual carbon nanotube emitters
Efficient coupling to photonic structures is essential to exploit the emission properties of carbon nanotubes (CNTs). Here, Miura et al.demonstrate spontaneous emission coupling efficiency exceeding 85% from a single CNT to a silicon photonic crystal nanobeam cavity with an ultralow mode-volume.
- R. Miura
- , S. Imamura
- & Y. K. Kato
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Repurposing Blu-ray movie discs as quasi-random nanoimprinting templates for photon management
Quasi-random nanostructures are being considered for many photon management applications but their use has been limited by their costly fabrication. Here, Smith et al. show that the quasi-random patterns on Blu-ray movie discs are already near-optimized for light-trapping applications in solar cells.
- Alexander J. Smith
- , Chen Wang
- & Jiaxing Huang
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Ferroelectric tunnel junctions with graphene electrodes
Ferroelectric tunnel junctions, where electrical transport occurs across two electrodes separated by a ferroelectric layer, could be used for future non-volatile computer memories. Here, the authors employ graphene as an electrode in tunnel junctions for interface-facilitated enhancement of device performance.
- H. Lu
- , A. Lipatov
- & A. Gruverman
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A walk along DNA using bipedal migration of a dynamic and covalent crosslinker
The predictable assembly of DNA makes it a useful scaffold for creating pathways to guide nanotransport systems. Here the authors use reversible covalent capture of DNA by quinone methide generation, as well as diffusion along the nucleophilic surface of DNA to guide migration.
- Fazel Fakhari
- & Steven E. Rokita
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Giant enhancement in vertical conductivity of stacked CVD graphene sheets by self-assembled molecular layers
Poor electronic coupling between planes significantly reduces stacked graphene conductivity. Here, the authors measure plane-to-plane conductivity using the eutectic GaIn technique to show that insertion of self-assembled monolayers between graphene layers improves vertical conductivity by six orders of magnitude.
- Yanpeng Liu
- , Li Yuan
- & Kian Ping Loh
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Sub-optical wavelength acoustic wave modulation of integrated photonic resonators at microwave frequencies
Acousto-optic modulators use acoustic waves to control light on a chip. Here, the authors achieve modulation in nanophotonic resonators using microwave frequency surface acoustic waves with wavelength smaller than the optical wavelength towards highly integrated devices on silicon.
- Semere Ayalew Tadesse
- & Mo Li
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Spatial mapping of multimode Brownian motions in high-frequency silicon carbide microdisk resonators
Identifying and manipulating high-order modes in mechanical resonators remains a challenge. Here, the authors provide an experimental demonstration of the mapping of such modes in a silicon carbide microdisk resonator, identifying intrinsic Brownian vibrations up to the ninth flexural mode.
- Zenghui Wang
- , Jaesung Lee
- & Philip X. -L. Feng
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Giant electrode effect on tunnelling electroresistance in ferroelectric tunnel junctions
The electroresistance displayed by ferroelectric tunnel junctions could be used for non-volatile computer memories and other computing applications. Here, the authors show that effects from ferroelectric–electrode interfaces can have a strong positive impact on the electroresistance in such junctions.
- Rohit Soni
- , Adrian Petraru
- & Hermann Kohlstedt
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Nanoscale visualization of redox activity at lithium-ion battery cathodes
It is important as well as challenging to map out redox activity at battery electrodes. Here, the authors present a scanning electrochemical cell microscope approach, which allows redox activity and ion flux processes at battery electrodes to be visualized with high space and time resolution.
- Yasufumi Takahashi
- , Akichika Kumatani
- & Tomokazu Matsue
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Interlaced crystals having a perfect Bravais lattice and complex chemical order revealed by real-space crystallography
Ternary nanoparticles have shown uses in areas such as thermoelectric devices. Here, the authors synthesise such nanoparticles and observe a crystalline ordering consisting of a global Bravais lattice, wherein the cation sublattice displays a range of interlaced chemical ordering.
- Xiao Shen
- , Emil A. Hernández-Pagan
- & Sokrates T. Pantelides
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Spin–orbit coupling in surface plasmon scattering by nanostructures
The polarization state of light is analogous to the spin state of electrons, enabling equivalent phenomena to be explored in optics as in the solid state. Here, the authors study directional scattering of light from nanostructured surfaces, arising from a spin-orbit coupling effect for surface plasmon waves.
- D. O’Connor
- , P. Ginzburg
- & A. V. Zayats
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Crown ethers in graphene
Crown ethers have been used as strong and selective binders for alkali metals and other cations since their discovery. Here the authors observe crown ether type structures in partially oxidized graphene and through simulations predict that they have similar abilities to selectively bind cations.
- Junjie Guo
- , Jaekwang Lee
- & Matthew F. Chisholm
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Enhanced second-harmonic generation from metal-integrated semiconductor nanowires via highly confined whispering gallery modes
Nanoscale light sources using nonlinearities are needed in many applications but their small size leads to very low efficiencies. Here, Ren et al.exploit the highly confined whispering gallery modes in metal-coated nanowires to achieve enhanced second-harmonic generation with minimal Ohmic losses.
- Ming-Liang Ren
- , Wenjing Liu
- & Ritesh Agarwal
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High-resolution nanotransfer printing applicable to diverse surfaces via interface-targeted adhesion switching
There is an ongoing need for high resolution, versatile and simplistic nanoscale lithography and transfer. Here the authors report a solvent-assisted nanotransfer printing route, which allows for the easy release of 8–20 nm scale features on to a range of substrates.
- Jae Won Jeong
- , Se Ryeun Yang
- & Yeon Sik Jung
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Quantum yield and excitation rate of single molecules close to metallic nanostructures
Metal nanostructures strongly influence fluorescence of nearby molecules, ranging from significant enhancement to total quenching. To decode the precise interactions taking place, Holzmeister et al. present a method that distinguishes the contributions to excitation, radiative and non-radiative rates.
- Phil Holzmeister
- , Enrico Pibiri
- & Philip Tinnefeld
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Three-dimensional plasmonic stereoscopic prints in full colour
Plasmonic nanostructures enable control over the spatial and spectral dependence of scattered light. Here, the authors use pixels formed of nanoellipse or nanosquare dimers to show polarization-dependent full-colour scattering in reflection, and build 3D stereoscopic colour microprints from them.
- Xiao Ming Goh
- , Yihan Zheng
- & Joel K. W. Yang
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| Open AccessObservation of strongly entangled photon pairs from a nanowire quantum dot
Semiconductor quantum dots embedded in nanowires are good candidates for the realization of a nearly ideal entangled photons source. Here, Versteegh et al.demonstrate emission of single-photon pairs from a position-controlled nanowire quantum dot without the need for temporal post-selection.
- Marijn A. M. Versteegh
- , Michael E. Reimer
- & Val Zwiller
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Three-dimensional analysis of Nafion layers in fuel cell electrodes
In proton exchange membrane fuel cells, little is known about distribution of ionomers inside electrodes. Here, the authors present an electron tomography technique that allows a three dimensional visualization and quantitative analysis of ionomer layers in the electrodes.
- M. Lopez-Haro
- , L. Guétaz
- & G. Gebel
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Gram-scale synthesis of single-crystalline graphene quantum dots with superior optical properties
Graphene quantum dots (GQDs) have a wide range of potential applications, yet current cutting methods produce GQDs in low amounts and with poor optical properties. Here, the authors demonstrate, via a facile molecular fusion route, the synthesis of GQDs at the gram-scale and report excellent optical properties.
- Liang Wang
- , Yanli Wang
- & Minghong Wu
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Ordered three-dimensional interconnected nanoarchitectures in anodic porous alumina
Three-dimensional nanostructures have numerous applications and are normally fabricated via templating strategies. Here, the authors present a current-limited hard anodization approach for tunable, homogeneous anodic aluminium oxide, which can be used to template a range of periodic nanowire networks.
- Jaime Martín
- , Marisol Martín-González
- & Olga Caballero-Calero
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Reduced-dimensionality-induced helimagnetism in iron nanoislands
Spin textures, such as skyrmions, could be useful in future low-power-consumption memory devices, but they are usually only seen in materials with a strong spin-orbit interaction. Phark et al.now, however, observe such non-collinear magnetic order in nanometre-scale bilayer iron islands.
- S. -H. Phark
- , J. A. Fischer
- & J. Kirschner
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Sub-diffractional volume-confined polaritons in the natural hyperbolic material hexagonal boron nitride
Hyperbolic metamaterials exhibit interesting optical phenomena that could provide useful functionalities, if the losses can be reduced. Here Caldwell et al.show that hexagonal boron nitride supports hyperbolic polaritons, presenting a natural alternative to metamaterial systems.
- Joshua D. Caldwell
- , Andrey V. Kretinin
- & Kostya S. Novoselov
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Diffusion driven layer-by-layer assembly of graphene oxide nanosheets into porous three-dimensional macrostructures
There has been significant research into the preparation of nanosheets, but less on their assembly into functional macroscale architectures. Here, the authors present a diffusion-driven layer-by-layer assembly of graphene oxide into various three-dimensional structures.
- Jianli Zou
- & Franklin Kim
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Surfactant-assisted chemical vapour deposition of high-performance small-diameter GaSb nanowires
Antimonide nanowires may have useful applications as semiconductors in optoelectronics. Here, the authors use a sulfur surfactant to produce high-performance GaSb nanowires via chemical vapour deposition, achieving very thin and uniform nanowires with diameters as small as 20 nm.
- Zai-xing Yang
- , Ning Han
- & Johnny C. Ho
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Emulating weak localization using a solid-state quantum circuit
Quantum simulators offer a test bed to emulate physical phenomena that are difficult to reproduce numerically. Using a multi-element superconducting quantum circuit, Chen et al.emulate weak localization for a mesoscopic system using a control sequence that lets them continuously tune the level of disorder.
- Yu Chen
- , P. Roushan
- & John M. Martinis
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Trinucleotide duplex formation inside a confined nanospace under supercooled conditions
The hybridization of DNA in solution is more difficult the shorter the strands become, making trimer duplexes difficult to isolate and study. Here, the authors use a silica pore in supercooled conditions to isolate and study complementary and mismatched trimer DNA duplexes.
- Hiroyuki Arafune
- , Akira Yamaguchi
- & Norio Teramae
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Vanadium dioxide nanowire-based microthermometer for quantitative evaluation of electron beam heating
Understanding localized heating of a material by a beam of electrons is important in electron microscopy, but measuring temperature at the nanoscale is difficult. Here, the authors show that a vanadium dioxide nanowire can act as a microthermometer and measure electron beam heating in silicon nanowires.
- H. Guo
- , M. I. Khan
- & A. M. Minor
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Engineering polar discontinuities in honeycomb lattices
It has been predicted that when a polar discontinuity occurs in honeycomb lattices, wires of electrons or holes would appear. Here, the authors suggest different and realistic routes to engineer such wires in current two-dimensional materials, and validate these with first-principles calculations.
- Marco Gibertini
- , Giovanni Pizzi
- & Nicola Marzari
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Conformational transitions and stop-and-go nanopore transport of single-stranded DNA on charged graphene
Advancing our understanding of the interactions between DNA and synthetic nanopores will help in the design of rapid new DNA sequencing techniques. Here, the authors analyse the effect of graphene charge on DNA adhesion and pore translocation, showing controllable stop-and-go transport.
- Manish Shankla
- & Aleksei Aksimentiev
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Local determination of the amount of integration of an atom into a crystal surface
Point defects in a surface can subtly alter the bulk phonon spectra. Here, the authors show phonon spectra of point defects that are capable of differentiating between different degrees of integration—alloyed or loose in a vacancy—of an atom into a surface.
- K. Volgmann
- , H. Gawronski
- & K. Morgenstern
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Laser-targeted photofabrication of gold nanoparticles inside cells
Photonic methods can be greatly improved by metal nanoparticles, but biological targets such as cells prevent spatial control of particles, excluding key regions of interest. Here, the authors show laser light can control nanoparticle growth locations in the cell, and probe intracellular molecules.
- Nicholas I. Smith
- , Kentaro Mochizuki
- & Yutaro Kumagai
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Few-layer molybdenum disulfide transistors and circuits for high-speed flexible electronics
Molybdenum disulfide holds great potential for advanced flexible electronic devices. Here, using a transferred gate technique, the authors fabricate molybdenum disulfide-based transistors with optimized device geometry and contact, improving device speed and demonstrating gigahertz circuits with voltage gain.
- Rui Cheng
- , Shan Jiang
- & Xiangfeng Duan
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| Open AccessGigahertz single-trap electron pumps in silicon
Devices that generate single electrons are crucial for a precise definition of the ampere—the SI unit for electrical current. Yamahata et al. now demonstrate a silicon-based transistor that can accurately emit lone electrons at a rate of over 3 billion per second.
- Gento Yamahata
- , Katsuhiko Nishiguchi
- & Akira Fujiwara
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Aligned Fe2TiO5-containing nanotube arrays with low onset potential for visible-light water oxidation
Metal oxides are desirable photoanode materials due to their low cost and chemical stability, but they only work in the ultraviolet range. Here, Liu et al. design anode architecture that can absorb the visible light, while maintaining photon-to-current efficiency of 40% at an onset potential of 0.2 V.
- Qinghua Liu
- , Jingfu He
- & Shiqiang Wei
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Semiconducting single-walled carbon nanotubes sorting with a removable solubilizer based on dynamic supramolecular coordination chemistry
Semiconducting single-wall nanotubes hold promise for the next generation of electronic devices, but separating them from metallic counterparts is still challenging. Here, the authors show how to sort semiconducting nanotubes by selectively stabilizing them in solution via a removable solubilizer.
- Fumiyuki Toshimitsu
- & Naotoshi Nakashima
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Dry-air-stable lithium silicide–lithium oxide core–shell nanoparticles as high-capacity prelithiation reagents
Anode prelithiation is used to treat the initial capacity loss and low Coulombic efficiency in lithium-ion batteries, but existing methods are not effective. Here, the authors report lithium silicide–lithium oxide core–shell nanoparticles as a promising prelithiation reagent.
- Jie Zhao
- , Zhenda Lu
- & Yi Cui
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Bottom-up approach for the low-cost synthesis of graphene-alumina nanosheet interfaces using bimetallic alloys
Graphene-dielectric interfaces play a crucial role in many electronic devices, but electronic properties of graphene are inevitably degraded when the interfaces are produced. Omiciuolo et al.solve this problem using a low-cost approach based on epitaxial growth of graphene on dielectric alloys.
- Luca Omiciuolo
- , Eduardo R. Hernández
- & Alessandro Baraldi
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Fringing-field dielectrophoretic assembly of ultrahigh-density semiconducting nanotube arrays with a self-limited pitch
Carbon nanotubes offer a route to further reducing the size of electronic components. Here, the authors demonstrate a method to assemble semiconducting nanotubes into well-aligned, ultrahigh-density and uniform arrays using an alternating electric field between surface microelectrodes and the substrate.
- Qing Cao
- , Shu-jen Han
- & George S. Tulevski
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Enhancing lithium–sulphur battery performance by strongly binding the discharge products on amino-functionalized reduced graphene oxide
Lithium–sulphur batteries are a promising candidate for next-generation electrochemical energy storage. Here, the authors report a facile strategy for covalent stabilization of sulphur and its discharge products on amino-functionalized reduced graphene oxide, which enhances the cycling stability.
- Zhiyu Wang
- , Yanfeng Dong
- & Xiong Wen (David) Lou
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Nanomotor lithography
Miniaturization of devices and machines requires advanced lithographic techniques, whilst the high cost and complexity are the bottlenecks. Li et al.now show an approach for direct, arbitrary nano-patterning using self-propelled nanomotors acting as mobile nanomasks and near-field lenses.
- Jinxing Li
- , Wei Gao
- & Joseph Wang