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Article
| Open AccessTracing and constraining anthropogenic aerosol iron fluxes to the North Atlantic Ocean using iron isotopes
The relative importance of crustal vs. anthropogenic dust deposition for iron cycling in the surface ocean is unclear. Based on analysis of iron isotope data from North Atlantic aerosol samples, the authors can reveal the relative importance of anthropogenic iron emissions and its impact on marine biogeochemistry.
- Tim M. Conway
- , Douglas S. Hamilton
- & Seth G. John
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Article
| Open AccessQuantifying gravity wave forcing using scale invariance
Parametrizations of unresolved small-scale atmospheric waves are an important source of uncertainty in climate models. Scale invariance is used to estimate the forcing of these small-scale waves and it is shown to have a leading order effect on the mean flow.
- Han-Li Liu
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Article
| Open AccessRapid unimolecular reaction of stabilized Criegee intermediates and implications for atmospheric chemistry
Criegee intermediates have received much attention in atmospheric chemistry because of their importance in ozonolysis mechanisms. Here, using quantum mechanical kinetics, the authors reveal an unexpectedly fast mechanistic pathway for unimolecular reactions of large stabilized Criegee intermediates.
- Bo Long
- , Junwei Lucas Bao
- & Donald G. Truhlar
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Article
| Open AccessUncertainty in near-term global surface warming linked to tropical Pacific climate variability
Large uncertainty exists in projecting future 20-year global warming trends due to intrinsic tropical Pacific climate variability. Here the authors show that knowledge of the state of the Pacific Ocean can significantly reduce this uncertainty via the use of initialized decadal climate forecasts.
- Mohammad Hadi Bordbar
- , Matthew H. England
- & Mojib Latif
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Article
| Open AccessThe role of enhanced velocity shears in rapid ocean cooling during Super Typhoon Nepartak 2016
A better understanding of typhoon–ocean interactions is critical for improving typhoon forecasts. Here the authors use data from two buoys that captured Super Typhoon Nepartak and combine it with numerical simulations to reveal the role of enhanced velocity shear in rapid upper-ocean cooling.
- Yiing Jang Yang
- , Ming-Huei Chang
- & Ching-Ling Wei
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Article
| Open AccessIn-situ aerosol nanoparticle characterization by small angle X-ray scattering at ultra-low volume fraction
State‐of‐the‐art aerosol nanoparticle techniques are limited by the shortcomings of removing the nanoparticles from their original environment. Here, the authors apply small angle X‐ray scattering as an in‐situ measurement technique, enabling the measurement of the primary particles and the aggregates.
- P. S. Bauer
- , H. Amenitsch
- & P. M. Winkler
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Article
| Open AccessUrban pollution greatly enhances formation of natural aerosols over the Amazon rainforest
It remains unclear how urban emissions influence the formation of secondary organic aerosols (SOA), including in the Amazon forest. Here, the authors simulate the formation of SOAs in the Amazon using a high-resolution regional chemical transport model. They find that urban emissions of NOx from Manaus enhance the production of biogenic SOA by 60–200%.
- Manish Shrivastava
- , Meinrat O. Andreae
- & Chun Zhao
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Article
| Open AccessChina’s coal mine methane regulations have not curbed growing emissions
Chinese government has implemented regulations to reduce mining-related methane emission since 2010. Here the authors estimated methane emissions in China using GOSAT satellite observation and results reveal a business-as-usual increase in methane emissions since 2010 despite those ambitious targets.
- Scot M. Miller
- , Anna M. Michalak
- & Stefan Schwietzke
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Article
| Open AccessDecrease in radiative forcing by organic aerosol nucleation, climate, and land use change
Organic nucleation is an important source of atmospheric aerosol number concentration, especially in pristine continental regions and during the preindustrial period. Here the authors find a 16% reduced radiative forcing associated with anthropogenic aerosols when including organic nucleation together with climate and land use change.
- Jialei Zhu
- , Joyce E. Penner
- & Hugh Coe
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Article
| Open AccessOcean temperature impact on ice shelf extent in the eastern Antarctic Peninsula
Ocean warming contributes to the thinning of the Antarctic ice shelves, however, lack of observations has prevented a quantification of this contribution. Here the authors use geological records to show that 0.3–1.5 °C ocean warming has played a central role on regional ice shelf instability over the last 9000 years.
- Johan Etourneau
- , Giovanni Sgubin
- & Jung-Hyun Kim
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Article
| Open AccessCoupled ocean-atmosphere dynamics of the 2017 extreme coastal El Niño
The extreme coastal El Niño of March 2017 caused devastating flooding in coastal Peru but its mechanism remains unclear. Here the authors investigate the physical processes using observations and model simulations and suggest that such extreme coastal flooding is predictable and will become more frequent as climate warms.
- Qihua Peng
- , Shang-Ping Xie
- & Hong Zhang
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Article
| Open AccessArctic amplification is caused by sea-ice loss under increasing CO2
The cause of Arctic amplification is still heavily debated. Here the authors present climate change simulations to show that sea-ice loss is essential for the existence of Arctic amplification.
- Aiguo Dai
- , Dehai Luo
- & Jiping Liu
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Article
| Open AccessCompounding tropical and stratospheric forcing of the record low Antarctic sea-ice in 2016
Antarctic sea ice extent declined dramatically in austral spring 2016. This study shows the decline was initially driven by tropical convection resulting in a wave-3 circulation pattern, followed by weakened circumpolar surface westerlies initialised in the polar stratospheric vortex.
- Guomin Wang
- , Harry H. Hendon
- & Peter van Rensch
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Article
| Open AccessPhotoreduction of gaseous oxidized mercury changes global atmospheric mercury speciation, transport and deposition
Reduction of gaseous Hg(II) compounds drives atmospheric mercury wet and dry deposition to Earth surface ecosystems. Global Hg models assume this reduction takes place in clouds. Here the authors report a new gas-phase Hg photochemical mechanism that changes atmospheric mercury lifetime and its deposition to the surface.
- Alfonso Saiz-Lopez
- , Sebastian P. Sitkiewicz
- & Jeroen E. Sonke
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Article
| Open AccessInfluence of Tibetan Plateau snow cover on East Asian atmospheric circulation at medium-range time scales
The atmospheric response to subseasonal variability of Tibetan Plateau snow cover has been largely ignored. Here the authors show that the fast subseasonal variability of Tibetan Plateau snow cover is closely related to the subsequent East Asian atmospheric circulation at medium-range time scales.
- Wenkai Li
- , Weidong Guo
- & Jiangfeng Wei
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Article
| Open AccessResolving the mechanisms of hygroscopic growth and cloud condensation nuclei activity for organic particulate matter
The interactions between organic particulate matter and water vapour affect climate predictions, yet the mechanisms of these interactions remain unresolved. Here, the authors propose a phase separation mechanism that reconciles the observed hygroscopicity and cloud condensation nuclei activity.
- Pengfei Liu
- , Mijung Song
- & Scot T. Martin
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Article
| Open AccessContrasting effects on deep convective clouds by different types of aerosols
Aerosol effects on convection have been debated for decades when all types of aerosols are lumped together in the analyses. Using NASA satellite measurements, the authors find strong evidence that smoke inhibits convection but polluted continental aerosols invigorate convection.
- Jonathan H. Jiang
- , Hui Su
- & Zhien Wang
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Article
| Open AccessAerosol-induced intensification of cooling effect of clouds during Indian summer monsoon
The invigoration of deep convective clouds in the Indian summer monsoon region is associated with high aerosol loading. Here the authors show that convective clouds from high aerosol loads in the Indian Summer Monsoon region have a cooling effect.
- Chandan Sarangi
- , Vijay P. Kanawade
- & Dilip Ganguly
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Review Article
| Open AccessEvaluating climate geoengineering proposals in the context of the Paris Agreement temperature goals
Research and debate are intensifying on complementing CO2 emissions reductions with hypothetical climate geoengineering techniques. Here, the authors assess their potentials, uncertainties and risks, and show that they cannot yet be relied on to significantly contribute to meeting the Paris Agreement temperature goals.
- Mark G. Lawrence
- , Stefan Schäfer
- & Jürgen Scheffran
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Article
| Open AccessCritical Southern Ocean climate model biases traced to atmospheric model cloud errors
The Southern Ocean is critically important for global climate yet poorly represented by climate models. Here the authors trace sea surface temperature biases in this region to cloud-related errors in atmospheric-model simulated surface heat fluxes and provide a pathway to improve the models.
- Patrick Hyder
- , John M. Edwards
- & Stephen E. Belcher
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Article
| Open AccessTree rings reveal globally coherent signature of cosmogenic radiocarbon events in 774 and 993 CE
Despite their extensive use, the absolute dating of tree-ring chronologies has not hitherto been independently validated at the global scale. Here, the identification of distinct 14C excursions in 484 individual tree rings, enable the authors to confirm the dating of 44 dendrochronologies from five continents.
- Ulf Büntgen
- , Lukas Wacker
- & Giles H. F. Young
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Article
| Open AccessBlack carbon radiative effects highly sensitive to emitted particle size when resolving mixing-state diversity
Black carbon has a large but uncertain warming contribution to Earth’s climate. Here Matsui et al. show that black carbon mixing state and its interaction with aerosol size distribution are required for accurately estimating the radiative effect of black carbon.
- Hitoshi Matsui
- , Douglas S. Hamilton
- & Natalie M. Mahowald
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Article
| Open AccessBiogenic volatile release from permafrost thaw is determined by the soil microbial sink
Permafrost thaw allows biological activity in previously frozen ground, leading to a potential release of climate-relevant gases. Here the authors show that thawing permafrost emits volatile organic compounds but that their release to the atmosphere is limited by microbial consumption in the overlaying soil.
- Magnus Kramshøj
- , Christian N. Albers
- & Riikka Rinnan
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Article
| Open AccessDivergent global-scale temperature effects from identical aerosols emitted in different regions
The climate effects of anthropogenic aerosols depend on their spatial distribution, but emission location is often ignored in evaluating their climate impact. Here the authors show drastic divergence in the simulated global temperature response to identical aerosols emitted from eight key geopolitical regions.
- Geeta G. Persad
- & Ken Caldeira
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Article
| Open AccessSpatially similar surface energy flux perturbations due to greenhouse gases and aerosols
Anthropogenic aerosol and greenhouse gas concentrations are spatially uncorrelated, but the climate response to each shows a similar spatial pattern. Here the authors show that two-thirds of the spatial similarity in the full response manifests through fast-acting atmosphere and land surface processes alone.
- Geeta G. Persad
- , Yi Ming
- & V. Ramaswamy
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Article
| Open AccessReassessment of pre-industrial fire emissions strongly affects anthropogenic aerosol forcing
Several lines of evidence suggest that fire activity was much greater in the preindustrial era than currently assumed in climate models. Here the authors show that greater emission of aerosols from fires leads to a substantial reduction in the magnitude of aerosol radiative forcing over the Industrial Era.
- D. S. Hamilton
- , S. Hantson
- & K. S. Carslaw
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Article
| Open AccessGlobal and Arctic climate sensitivity enhanced by changes in North Pacific heat flux
The relative impacts of changes in North Pacific and North Atlantic sea surface temperature on Arctic climate are not well defined. Here the authors find that Arctic surface temperatures are more sensitive to changes in North Pacific heat flux as a result of stronger modulations in poleward moisture and latent heat transport.
- Summer Praetorius
- , Maria Rugenstein
- & Ken Caldeira
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Article
| Open AccessObservational constraint on cloud susceptibility weakened by aerosol retrieval limitations
Cloud susceptibility to aerosols in models frequently exceeds satellite estimates. Here the authors show that the discrepancy can be explained by retrieval limitations especially in clean environments, suggesting that conventional comparison strategies may lead to misunderstanding.
- Po-Lun Ma
- , Philip J. Rasch
- & Steven J. Ghan
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Article
| Open AccessA model for super El Niños
Despite advances in ENSO modeling, super El Niño events remain largely unpredictable. Hameed et al. postulate that ENSO-IOD interaction is crucial for super El Niño development and identify a self-limiting factor that constrains ENSO dynamics from generating these extreme events on their own.
- Saji N. Hameed
- , Dachao Jin
- & Vishnu Thilakan
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Article
| Open AccessA new interhemispheric teleconnection increases predictability of winter precipitation in southwestern US
ENSO is losing predictive power of west US coast precipitation. Here the authors identify a new inter-hemispheric teleconnection that promises earlier and more accurate prediction.
- Antonios Mamalakis
- , Jin-Yi Yu
- & Efi Foufoula-Georgiou
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Perspective
| Open AccessQuantifying climate feedbacks in polar regions
Estimating the magnitude of radiative and non-radiative feedbacks is key for understanding the climate dynamics of polar regions. Here the authors propose an inclusive methodology to quantify the influence of all those feedbacks, stimulating more systematic analyses in observational and model ensembles.
- Hugues Goosse
- , Jennifer E. Kay
- & Martin Vancoppenolle
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Article
| Open AccessSensible heat has significantly affected the global hydrological cycle over the historical period
Precipitation changes are strongly linked to the Earth’s energy budget. Here the authors show that changes in sensible heat are the dominant contributor to the present global-mean precipitation change since pre-industrial time.
- G. Myhre
- , B. H. Samset
- & A. Voulgarakis
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Article
| Open AccessIncreasing occurrence of cold and warm extremes during the recent global warming slowdown
During 2002–2014, global mean temperatures stayed nearly steady, but both summertime warm and wintertime cold extreme temperature occurrences over North Hemisphere continents increased. Here the authors show that the contrasting changes in these metrics were driven by distinct climate patterns.
- Nathaniel C. Johnson
- , Shang-Ping Xie
- & Xichen Li
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Article
| Open AccessRecent strengthening of the stratospheric Arctic vortex response to warming in the central North Pacific
The stratospheric Arctic vortex plays a critical role in forecasting cold winters in northern mid-latitudes. Here the authors show that the stratospheric Arctic vortex strengthened during 1998–2016, with ~25% of this strengthening contributed by warming in the central North Pacific.
- Dingzhu Hu
- , Zhaoyong Guan
- & Rongcai Ren
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Article
| Open AccessAnthropogenic combustion iron as a complex climate forcer
As a source of soluble iron, anthropogenic combustion iron is considered less important than natural sources. Here, the authors combine new measurements with a global aerosol model and show the atmospheric burden of anthropogenic combustion iron to be 8 times greater than previous estimates.
- Hitoshi Matsui
- , Natalie M. Mahowald
- & Mark G. Flanner
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Article
| Open AccessWestward migration of tropical cyclone rapid-intensification over the Northwestern Pacific during short duration El Niño
El Niño events have important impacts on tropical cyclone activity over the western North Pacific. Here, the authors show that short duration El Niño could significantly shift the tropical cyclone rapid intensification westward by transporting ocean heat energy to the western Pacific.
- Yi-Peng Guo
- & Zhe-Min Tan
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Article
| Open AccessGreenland records of aerosol source and atmospheric lifetime changes from the Eemian to the Holocene
Past climate changes in Greenland ice were accompanied by large aerosol concentration changes. Here, the authors show that by correcting for transport effects, reliable source changes for biogenic aerosol from North America, sea salt aerosol from the North Atlantic, and dust from East Asian deserts can be derived.
- S. Schüpbach
- , H. Fischer
- & E. W. Wolff
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Article
| Open AccessRapid increase in atmospheric iodine levels in the North Atlantic since the mid-20th century
Despite its chemical importance, the evolution of atmospheric iodine concentrations over time is unknown. Here, the authors show that North Atlantic atmospheric iodine levels have tripled since 1950, and propose ozone pollution and enhanced biological production Arctic sea ice thinning as a primary driver.
- Carlos A. Cuevas
- , Niccolò Maffezzoli
- & Alfonso Saiz-Lopez
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Article
| Open AccessModel evidence for a seasonal bias in Antarctic ice cores
Periodic changes in the tilt of the Earth’s axis alter the distribution of incoming solar radiation. Here, the authors show that the temperature response to this forcing seemingly differs in models and Antarctic ice cores, with a better agreement reached if ice cores are recording a seasonally weighted signal.
- Michael P. Erb
- , Charles S. Jackson
- & Pedro N. DiNezio
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Article
| Open AccessOcean convection linked to the recent ice edge retreat along east Greenland
Warm Atlantic water circulates cyclonically around the Nordic Seas while gradually cooling. Here, the authors show that the retreat of the ice edge toward Greenland has led to further transformation of this water mass, which is no longer situated underneath sea ice when transiting the western Iceland Sea in winter.
- Kjetil Våge
- , Lukas Papritz
- & G. W. K. Moore
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Article
| Open AccessRobustness of anthropogenically forced decadal precipitation changes projected for the 21st century
Decadal precipitation changes are dominated by random natural variability, posing a challenge for projecting anthropogenic impacts. Here the authors use large suites of model simulations to show that human-induced future decadal shifts in regional precipitation can be distinguished from natural variability.
- Honghai Zhang
- & Thomas L. Delworth
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Article
| Open AccessWarm Arctic episodes linked with increased frequency of extreme winter weather in the United States
Whether accelerated Arctic warming is favorable for more frequent severe winter weather remains controversial. Here the authors present an observational analysis that links Arctic warming to severe winter weather, showing that extreme weather is 2–4 times more likely in the eastern US when the Arctic is warm.
- Judah Cohen
- , Karl Pfeiffer
- & Jennifer A. Francis
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Article
| Open AccessAerosol effects on cloud water amounts were successfully simulated by a global cloud-system resolving model
Most global climate models overestimate the aerosol effect on cloud properties, but the reason for this is unclear. Here the authors show that using explicit representation of cloud microphysics, in global scale modelling, rather than parameterisations, reduces the overestimation.
- Yousuke Sato
- , Daisuke Goto
- & Teruyuki Nakajima
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Article
| Open AccessCleaner fuels for ships provide public health benefits with climate tradeoffs
Aerosol pollution from shipping contributes to cooling but also leads to premature mortality and morbidity. Here the authors combine emission inventories, atmospheric models and health risk functions to show how cleaner marine fuels will reduce premature deaths and childhood asthma but results in larger warming.
- Mikhail Sofiev
- , James J. Winebrake
- & James J. Corbett
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Article
| Open AccessAmbient PM2.5 exposure and expected premature mortality to 2100 in India under climate change scenarios
Modulation of ambient PM2.5 exposure and premature mortality burden in India under climate change scenarios is unclear. Here the authors show that the premature mortality burden is projected to decrease in 2100 relative to present day under all possible combined climate change and socioeconomic pathways scenarios.
- Sourangsu Chowdhury
- , Sagnik Dey
- & Kirk R. Smith
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Article
| Open AccessGlobal and regional importance of the direct dust-climate feedback
Feedbacks between desert dust and climate might have amplified past climate changes, yet their role in future climate change is unclear. Here the authors find that dust feedbacks could play a key role in the future climates of Northern Africa, the Sahel, the Mediterranean, the Middle East, and Central Asia.
- Jasper F. Kok
- , Daniel S. Ward
- & Amato T. Evan
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Article
| Open AccessStratospheric ozone loss over the Eurasian continent induced by the polar vortex shift
Climate change can exert a significant effect on the ozone recovery. Here, the authors show that the Arctic polar vortex shift associated with Arctic sea-ice loss could slow down ozone recovery over the Eurasian continent.
- Jiankai Zhang
- , Wenshou Tian
- & Guang Zeng
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Article
| Open AccessImpact on short-lived climate forcers increases projected warming due to deforestation
The climate impacts of deforestation due to changes in biogenic volatile organic compound emissions, which act as short-lived climate forcers (SLCFs), are poorly understood. Here the authors show that including the impact SLCFs increases the projected warming associated with idealised deforestation scenarios.
- C. E. Scott
- , S. A. Monks
- & C. Wilson
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Article
| Open AccessDiurnal cloud cycle biases in climate models
The timing of clouds is critical to the Earth’s energy balance. Here the authors show that in current climate models, clouds over the land tend to peak too early in the morning, reflecting less solar radiation than observed.
- Jun Yin
- & Amilcare Porporato