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| Open AccessMicrowave a.c. conductivity of domain walls in ferroelectric thin films
Conducting charged ferroelectric domain walls, as potential building blocks for future electronic devices, are unstable and uncommon in ferroelectric materials. Here, Tselev et al. show that neutral insulating domain walls in PbZrO3 and BiFeO3thin films are conductive under microwave excitation, allowing for non-destructive read-out.
- Alexander Tselev
- , Pu Yu
- & Petro Maksymovych
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Article
| Open AccessMapping the electrostatic force field of single molecules from high-resolution scanning probe images
The chemical properties of molecules are largely determined by the distribution of charge across them. Here, the authors demonstrate how the electrostatic force field, originating from the inhomogeneous charge distribution in a molecule, can be measured with sub-molecular resolution.
- Prokop Hapala
- , Martin Švec
- & Pavel Jelínek
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Article
| Open AccessGenerating giant and tunable nonlinearity in a macroscopic mechanical resonator from a single chemical bond
Macroscopic mechanical systems typically respond linearly to external force, and generating nonlinearity is challenging. Here, the authors generate nonlinearity in a macroscopic mechanical resonator by linking it to a gold contact and exploiting the anharmonicity in the chemical bonding interactions.
- Pu Huang
- , Jingwei Zhou
- & Jiangfeng Du
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Article
| Open AccessDynamic heterogeneity and non-Gaussian statistics for acetylcholine receptors on live cell membrane
Molecular motion in living cells is known to be more complicated than those determined solely by thermal equilibrium, but a quantitative analysis is still missing. Here, He et al. quantify the lateral motion of proteins on live muscle cell membranes, which doesn’t follow the normal Brownian diffusion.
- W. He
- , H. Song
- & P. Tong
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Article
| Open AccessElectrostatic control over temperature-dependent tunnelling across a single-molecule junction
The effect of temperature on charge transport mechanisms in molecular tunnel junctions is not fully understood. Here, charge transport studies of a redox-active molecule unveil multiple mechanistic regimes which may be explained by thermal broadening of the Fermi distributions of electrons in the leads.
- Alvar R. Garrigues
- , Lejia Wang
- & Christian A. Nijhuis
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Article
| Open AccessImplementation of dispersion-free slow acoustic wave propagation and phase engineering with helical-structured metamaterials
There is great interest in slow wave propagation for a variety of applications. Here, Zhu et al. present a dispersion-free helical-structured metamaterial that implements acoustic wave deceleration at broad bandwidth and demonstrates specially designed phase modulation to incident sound through helicity tuning.
- Xuefeng Zhu
- , Kun Li
- & Shengchun Liu
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Article
| Open AccessDecoupling optical function and geometrical form using conformal flexible dielectric metasurfaces
Realizing components with decoupled geometrical form and optical function are of interest for various applications. Here, Kamali et al. introduce flexible metasurfaces based on a transmitarray platform that can be conformed to a non-planar arbitrarily shaped object to modify its optical properties at will.
- Seyedeh Mahsa Kamali
- , Amir Arbabi
- & Andrei Faraon
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Article
| Open AccessSpin-texture inversion in the giant Rashba semiconductor BiTeI
In semiconductors containing heavy elements, the Rashba spin-orbit interaction can couple the momentum and spin of electrons, yielding spintronic functionality. Here, the authors image band- and orbital-dependent spin-textures in the layered polar semiconductor BiTeI, demonstrating behaviour beyond the standard Rashba model.
- Henriette Maaß
- , Hendrik Bentmann
- & Friedrich Reinert
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Article
| Open AccessDirect imaging of molecular symmetry by coherent anti-stokes Raman scattering
Coherent Raman imaging is a high fidelity technique to obtain chemical-sensitive images, however sub-diffraction molecular organization information is still missing. Here, the authors exploit molecular bond symmetries to access the microscopic organization of molecules in a single image acquisition.
- Carsten Cleff
- , Alicja Gasecka
- & Julien Duboisset
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Article
| Open AccessEfficient and mechanically robust stretchable organic light-emitting devices by a laser-programmable buckling process
Highly stretchable organic light-emitting diodes tend to suffer from a lack of mechanical robustness. Here, Yin et al. fabricate ordered buckled films by laying flexible light-emitting diodes on laser-ablated, prestretched substrates. The devices exhibit good emission stability over 15,000 stretching cycles.
- Da Yin
- , Jing Feng
- & Hong-Bo Sun
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Article
| Open AccessLight-activated photocurrent degradation and self-healing in perovskite solar cells
Organometallic perovskite solar cells exhibit good efficiency but their photostability is still relatively poorly understood and controlled. Here the authors show that photo-degradation arises from the formation of light-activated meta-stable trap states, is reversible, and can be frozen at 0 °C.
- Wanyi Nie
- , Jean-Christophe Blancon
- & Aditya D. Mohite
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Article
| Open AccessAtomic-scale disproportionation in amorphous silicon monoxide
Amorphous silicon monoxide is known to undergo disproportionation to silicon- and silicon dioxide-like regions, however direct observation of the atomic-scale heterogeneity is still missing. Here, the authors use angstrom-beam electron diffraction to reveal precise structural details of this unusual material.
- Akihiko Hirata
- , Shinji Kohara
- & Mingwei Chen
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Article
| Open AccessVan der Waals interactions and the limits of isolated atom models at interfaces
Van der Waals forces are individually weak, but on scale can drive many nano- and macroscopic processes. Here, Kawai et al. directly measure the van der Waals interactions between noble gas atom pairs and show how this changes with atom size and surface adsorption.
- Shigeki Kawai
- , Adam S. Foster
- & Ernst Meyer
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Article
| Open AccessDirect electronic measurement of Peltier cooling and heating in graphene
The interaction of electric and thermal transport phenomena at the nanoscale leads to Seebeck and Peltier thermoelectric effects. Here, the authors directly detect the Peltier effect in graphene, and show that it can be reversed by controlling the type and density of the majority carriers using a back gate.
- I. J. Vera-Marun
- , J. J. van den Berg
- & B. J. van Wees
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Article
| Open AccessTunable graphene micro-emitters with fast temporal response and controllable electron emission
Controlling the electron emission of microfabricated field emitters can be challenging. Here the authors report controllable and tunable graphene thermionic micro-emitters with well-defined turn-on voltages and switching times in the microsecond range and fabricate uniform micro-emitter arrays.
- Gongtao Wu
- , Xianlong Wei
- & Lianmao Peng
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Article
| Open AccessSingle-shot read-out of a superconducting qubit using a Josephson parametric oscillator
Efficient qubit readout is essential for quantum information technology, which requires sufficient recognition of signal from noise. Here, Krantz et al. propose a simplified technique using a Josephson parametric oscillator, demonstrating single-shot readout performance of a superconducting qubit.
- Philip Krantz
- , Andreas Bengtsson
- & Jonas Bylander
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Article
| Open AccessControlling the volatility of the written optical state in electrochromic DNA liquid crystals
Electrochromism, the dependence of light absorption upon electronic control, finds a wide range of applications in smart materials. Here, Liu et al. show an electrochromic DNA–surfactant liquid crystal system that exhibits electrically tunable optical absorption and thermally tunable memory.
- Kai Liu
- , Justin Varghese
- & Andreas Herrmann
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| Open AccessRepeated quantum error correction on a continuously encoded qubit by real-time feedback
Large-scale quantum information processing requires the continuous protection of quantum states against errors. Here, the authors demonstrate active quantum error correction that improves the dephasing time of quantum states using a diamond quantum processor.
- J. Cramer
- , N. Kalb
- & T. H. Taminiau
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Article
| Open AccessTunnel electroresistance through organic ferroelectrics
Ferroelectric organic materials can be used for tunnel barriers in memory devices as a cheaper and eco-friendly replacement of their inorganic counterparts. Here, Tian et al. use poly(vinylidene fluoride) with 1–2 layer thickness to achieve giant tunnel electroresistance of 1,000% at room temperature.
- B. B. Tian
- , J. L. Wang
- & J. H. Chu
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| Open AccessA 14 × 14 μm2 footprint polarization-encoded quantum controlled-NOT gate based on hybrid waveguide
Photonic circuits often require separate components to manipulate light with orthogonal polarization, but this increases the chip size. Here, the authors create a polarization-dependent beam-splitter that uses dielectric loaded plasmonic waveguides to handle both polarizations in the same component.
- S. M. Wang
- , Q. Q. Cheng
- & S. N. Zhu
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Article
| Open AccessFunctionalization mediates heat transport in graphene nanoflakes
The high thermal conductivity of graphene is considerably reduced when the two-dimensional material is in contact with a substrate. Here, the authors show that thermal management of a micro heater is improved using graphene-based films covalently bonded by amino-silane molecules to graphene oxide.
- Haoxue Han
- , Yong Zhang
- & Sebastian Volz
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| Open AccessAll-optical design for inherently energy-conserving reversible gates and circuits
Reversible gates, like Fredkin gates, may be useful for energy conservation efforts. Cohen et al. present a formalism that may be used to produce any reversible logic. This method is implemented over an optical design of the Fredkin gate which utilizes only optical elements that inherently conserve energy.
- Eyal Cohen
- , Shlomi Dolev
- & Michael Rosenblit
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Correspondence
| Open AccessCorrespondence: Quantitative evaluation of X-ray dark-field images for microcalcification analysis in mammography
- Kai Scherer
- , Lorenz Birnbacher
- & Franz Pfeiffer
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Correspondence
| Open AccessCorrespondence: Reply to ‘Quantitative evaluation of X-ray dark-field images for microcalcification analysis in mammography’
- Zhentian Wang
- , Nik Hauser
- & Marco Stampanoni
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Article
| Open AccessIon selectivity of graphene nanopores
Sub-nanometer graphene nanopores are usually required to create graphene-based reverse osmosis membranes. Here, Rollings et al.show that membranes with larger pores are highly ion selective and a hundred times more permeable to potassium ions than to chloride ions, making them useful for electrodialysis.
- Ryan C. Rollings
- , Aaron T. Kuan
- & Jene A. Golovchenko
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Article
| Open AccessSize-dependent phase transition in methylammonium lead iodide perovskite microplate crystals
The orthorhombic-to-tetragonal phase transition in perovskite can alter its optical and electronic properties. Here, Li et al. report an investigation of the size dependent orthorhombic-to-tetragonal phase transition and show that the phase transition temperature decreases with reducing microplate thickness.
- Dehui Li
- , Gongming Wang
- & Xiangfeng Duan
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Article
| Open AccessExperimental realization of Bloch oscillations in a parity-time synthetic silicon photonic lattice
Bloch oscillations are a fundamental electron transport phenomenon in condensed matter. Here, the authors experimentally realize spatial Bloch oscillations in a non-Hermitian integrated photonic system using CMOS compatible fabrication processes, contributing to improving the understanding of non-Hermitian transport phenomena.
- Ye-Long Xu
- , William S. Fegadolli
- & Yan-Feng Chen
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Article
| Open AccessExperimental perfect state transfer of an entangled photonic qubit
Transferring quantum information is a fundamental task, but doing so with high fidelity is a challenging task. Here, the authors implement the perfect state transfer protocol to a photonic qubit, entangled with a second one in a different location, across eleven coupled waveguides.
- Robert J. Chapman
- , Matteo Santandrea
- & Alberto Peruzzo
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Article
| Open AccessEnhancing coherent transport in a photonic network using controllable decoherence
The efficiency of coherent transport can be enhanced through interaction between the system and a noisy environment. Here, Biggerstaff et al. report an experimental simulation of environment assisted coherent transport using laser-written waveguides, showing that controllable decoherence yields an increase in transport efficiency.
- Devon N. Biggerstaff
- , René Heilmann
- & Ivan Kassal
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Article
| Open AccessMagnetic-free non-reciprocity based on staggered commutation
Components such as isolators, circulators and gyrators are non-reciprocal in that they allow electromagnetic waves to flow in one direction but not the other. Here, the authors demonstrate a radio-frequency circulator that is compatible with and integrated in a complementary metal-oxide semiconductor integrated circuit.
- Negar Reiskarimian
- & Harish Krishnaswamy
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Article
| Open AccessA multiplexed light-matter interface for fibre-based quantum networks
Scalable networks for processing and distribution of quantum information using photons can be achieved by using multiplexed quantum states. Here, the authors report frequency-multimode storage and spectral-temporal photon manipulation of heralded single photons at telecom wavelength, in a fully integrated setting.
- Erhan Saglamyurek
- , Marcelli Grimau Puigibert
- & Wolfgang Tittel
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Article
| Open AccessThe formation mechanism for printed silver-contacts for silicon solar cells
The mechanism of contact formation during the firing of screen-printed contacts to Si solar cells remains elusive. Here, Fields et al. use in situ X-ray diffraction during firing to reveal the reaction sequence, thus suggesting approaches for development of inexpensive, nontoxic solar cell contacting pastes.
- Jeremy D. Fields
- , Md. Imteyaz Ahmad
- & Maikel F. A. M. van Hest
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Article
| Open AccessEfficient and stable perovskite solar cells prepared in ambient air irrespective of the humidity
Poor stability of perovskite solar cells in humid conditions has hindered device fabrication and operation. Here, Tai et al. report the use of a lead thiocyanate precursor in preparing perovskite solar cells and without encapsulation showed better stability in air than typical perovskite solar cells.
- Qidong Tai
- , Peng You
- & Feng Yan
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Article
| Open AccessAccessing the exceptional points of parity-time symmetric acoustics
Parity-time phase transition and exceptional points contribute to the design of many components, but are hard to access due to the dispersive nature of the required materials. Here, the authors introduce a method to systematically control acoustic parity-time phase transition through an active element.
- Chengzhi Shi
- , Marc Dubois
- & Xiang Zhang
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Article
| Open AccessMicroelectromechanical reprogrammable logic device
Microelectromechanical resonators behave as logic gates thanks to the tunability of their resonance frequencies. Here, the authors combine the mechanical response to electrothermal frequency modulation to demonstrate 2- and 3-bit reprogrammable logic gates at room temperature and under modest vacuum.
- M. A. A. Hafiz
- , L. Kosuru
- & M. I. Younis
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Article
| Open AccessControllable positive exchange bias via redox-driven oxygen migration
Direct observation of ionic motion in buried metal/oxide interfaces and its correlation with physical properties is a challenging task. Here, the authors observe oxygen migration in a model system with controllable positive exchange bias, due to the redox-driven formation of a ferromagnetic interfacial layer.
- Dustin A. Gilbert
- , Justin Olamit
- & Kai Liu
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Article
| Open AccessSemiconductor-inspired design principles for superconducting quantum computing
Superconducting circuits offer great promise for quantum computing, but implementations require careful shielding from control electronics. Here, the authors take inspirations from semiconductor spin-based qubits to design Josephson junctions quantum circuits whose qubits do not require microwave control.
- Yun-Pil Shim
- & Charles Tahan
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Article
| Open AccessPolarized three-photon-pumped laser in a single MOF microcrystal
Higher-order multi-photon pumped polarized lasers promise application in future optoelectronic and biomedical applications. Here, the authors demonstrate a polarized three-photon pumped (3PP) microcavity laser in a single host-guest composite MOF crystal via a controllable in situ self-assembly strategy.
- Huajun He
- , En Ma
- & Guodong Qian
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Article
| Open AccessEffective energy storage from a triboelectric nanogenerator
Self-charging systems based on the connection of a nanogenerator and an energy storage unit through a rectifier can have low energy storage efficiencies. Here, the authors design the charging cycle to maximize the energy storage efficiency of a triboelectric nanogenerator by introducing a motion-induced switch.
- Yunlong Zi
- , Jie Wang
- & Zhong Lin Wang
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Article
| Open AccessA three-dimensional actuated origami-inspired transformable metamaterial with multiple degrees of freedom
Typically, most structures and devices that can be reconfigured are designed with application specific requirements. Inspired by modular origami ideas, Overveldeet al. present a mechanical metamaterial enabling the design of three-dimensional structures of arbitrary architecture with tunable shape, volume and stiffness.
- Johannes T.B. Overvelde
- , Twan A. de Jong
- & Katia Bertoldi
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Article
| Open AccessScreen-printed flexible MRI receive coils
Signal-to-noise ratio is one of the key factors that currently limit the diagnostic image quality and patient conditions of magnetic resonance imaging. Here, Corea et al. use fully printed flexible receive coils, conforming to patient bodies, to improve signals and patient comfort in clinical scanners.
- Joseph R. Corea
- , Anita M. Flynn
- & Ana C. Arias
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Article
| Open AccessAcoustic trapping of active matter
Active matter, such as swimming bacteria, show unique behaviors under confinement, but it is experimentally challenging to measure them. Takatoriet al. show the use of acoustic tweezers to trap self-propelled Janus particles as an enabling tool to investigate collective motions in living systems.
- Sho C. Takatori
- , Raf De Dier
- & John F. Brady
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Article
| Open AccessMobility overestimation due to gated contacts in organic field-effect transistors
Charge mobility, extracted from current–voltage curves, is an important parameter for evaluating the performance of organic field-effect transistors. Bittle et al. show that charge mobility can be overestimated by one order of magnitude due to the gate bias dependence of the charge injection process.
- Emily G. Bittle
- , James I. Basham
- & David J. Gundlach
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Article
| Open AccessLasing in silicon–organic hybrid waveguides
On-chip light sources for silicon photonic circuits remain a challenge since the indirect bandgap of silicon prevents efficient light emission. The authors demonstrate that lasing can be achieved by combining standard silicon-on-insulator waveguides with dye-doped organic cladding materials to provide optical gain.
- Dietmar Korn
- , Matthias Lauermann
- & Christian Koos
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Article
| Open AccessHigh-performance thermoelectric nanocomposites from nanocrystal building blocks
Nanomaterials provide a route to efficient solid-state conversion between thermal and electrical energy. Here, the authors demonstrate that a combination of metal and semiconductor colloidal nanocrystals can produce thermoelectric nanocomposites with high performance.
- Maria Ibáñez
- , Zhishan Luo
- & Andreu Cabot
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Article
| Open AccessLarge elasto-optic effect and reversible electrochromism in multiferroic BiFeO3
Modern technology such as electronics and photovoltaics requires careful control of optical responses of electronic properties. Here, Sando et al. demonstrate a large variation of optical index and light absorption in multiferroic material BiFeO3thin films, tunable by in-film strain or electric field.
- D. Sando
- , Yurong Yang
- & M. Bibes
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Article
| Open AccessEfficient linear phase contrast in scanning transmission electron microscopy with matched illumination and detector interferometry
Scanning transmission electron microscopy is a powerful material probe, but constrained to large atomic number samples due to the issues of beam damage and weak scattering. Here, Ophus et al.propose a method that produces linear phase contrast in a focused electron beam to image dose-sensitive objects.
- Colin Ophus
- , Jim Ciston
- & Peter Ercius
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Article
| Open AccessIn situ stress observation in oxide films and how tensile stress influences oxygen ion conduction
Strain engineering is used to tune physiochemical material properties, but detailed insights of how the crystal growth affects the stress are yet lacking. Here, the authors analyse in situ simultaneously the induced stress and growth mode during the epitaxial growth of an oxygen ion conductor.
- Aline Fluri
- , Daniele Pergolesi
- & Thomas Lippert
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Article
| Open AccessSuper-crystals in composite ferroelectrics
Crystalline materials are formed by the periodic order of atomic unit cells. Here, Pierangeli et al. report the formation of a ferrelectric super-crystal with micrometric unit cell from modulated nanoscale disorder in potassium-lithium-tantalate-niobate, which is potentially useful for engineering ordered states out of disorder.
- D. Pierangeli
- , M. Ferraro
- & E. DelRe