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| Open AccessEnhancing radiation tolerance by controlling defect mobility and migration pathways in multicomponent single-phase alloys
Radiation tolerance is a property determined both by materials structure and defect dynamics. Here authors demonstrate enhancement of radiation tolerance at elevated temperatures in equiatomic single-phase concentrated solid solution alloys and propose an underlying mechanism.
- Chenyang Lu
- , Liangliang Niu
- & Lumin Wang
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Article
| Open AccessAchieving ZT=2.2 with Bi-doped n-type SnSe single crystals
The good thermoelectric figures of merit of p-type tin selenide single crystals are actively studied. Here, the authors show that n-type SnSe can also reach a figure of merit of around 2, at high temperatures, when doped with bismuth.
- Anh Tuan Duong
- , Van Quang Nguyen
- & Sunglae Cho
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Article
| Open AccessWater striders adjust leg movement speed to optimize takeoff velocity for their morphology
How water striders escape from danger by jumping vertically from the water surface without sinking is an open question in biomechanics. Yanget al. show that water strider species with varying leg lengths and body masses tune their leg movements to maximize jump speeds without breaking the surface of the water.
- Eunjin Yang
- , Jae Hak Son
- & Ho-Young Kim
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Article
| Open AccessDynamic nuclear magnetic resonance field sensing with part-per-trillion resolution
The measurement of high magnetic fields has been limited to sensitivities in the nanotesla range. Here, the authors report advances in high-field magnetometry based on nuclear magnetic resonance, achieving resolution in the order of picoteslas or one part per trillion in relative terms.
- Simon Gross
- , Christoph Barmet
- & Klaas P. Pruessmann
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Article
| Open AccessPolarization bandgaps and fluid-like elasticity in fully solid elastic metamaterials
Controlling elastic waves in medium is essential to many applications in mechanical to earthquake engineering. Ma et al. demonstrate selective suppression of different vibrational modes in a three-dimensional rod-shape structure, which shows fluid-like elasticity with only longitudinal waves propagating.
- Guancong Ma
- , Caixing Fu
- & Ping Sheng
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Article
| Open AccessExperimental demonstration of anomalous Floquet topological insulator for sound
Topological protected acoustic wave propagation has been predicted, but yet awaits for experimental demonstration. Here, Peng et al. report one-way propagation of pseudo-spin-dependent edge states for sound, analogous to Floquet topological insulator in solid state.
- Yu-Gui Peng
- , Cheng-Zhi Qin
- & Xue-Feng Zhu
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Article
| Open AccessHigh-energy electron emission from metallic nano-tips driven by intense single-cycle terahertz pulses
High-energy electron sources are powerful tools for investigating dynamics at atomic and subatomic scales. Here, Li and Jones demonstrate the terahertz-driven emission of electrons with energies exceeding five kiloelectronvolts from nano-tips and study its dependence on the tip radius.
- Sha Li
- & R. R. Jones
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Article
| Open AccessSpontaneous assembly of chemically encoded two-dimensional coacervate droplet arrays by acoustic wave patterning
Isolated droplets can be used as micro-reactors, yet it is challenging to operate them functionally in solution and observe chemical exchanges between droplets. Here, Tian et al. use an acoustic trap to assemble water-based micro-droplets into periodic arrays, spontaneously separated from solution media.
- Liangfei Tian
- , Nicolas Martin
- & Stephen Mann
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Article
| Open AccessAcoustic omni meta-atom for decoupled access to all octants of a wave parameter space
For meta-atoms, achieving full access to the wave parameter space remains a problem. Here, Koo et al. outline the criteria for the decoupling of wave parameter from first principles, and realize an omni meta-atom that achieves independent, broad-range access to all octants of acoustic parameter space.
- Sukmo Koo
- , Choonlae Cho
- & Namkyoo Park
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Article
| Open AccessUnsupervised learning in probabilistic neural networks with multi-state metal-oxide memristive synapses
Artificial neural networks exhibit learning abilities and can perform tasks which are tricky for conventional computing systems, such as pattern recognition. Here, Serb et al. show experimentally that memristor arrays can learn reversibly from noisy data thanks to sophisticated learning rules.
- Alexander Serb
- , Johannes Bill
- & Themis Prodromakis
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Article
| Open AccessRadiative heat transfer exceeding the blackbody limit between macroscale planar surfaces separated by a nanosize vacuum gap
Evanescent coupling between surfaces separated by a distance smaller than the thermal wavelength can lead to radiative heat transfer greater than the blackbody limit. Here, the authors demonstrate this between two macroscopic-scale surfaces, paving the way to harnessing the effect in thermal devices.
- Michael P. Bernardi
- , Daniel Milovich
- & Mathieu Francoeur
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Article
| Open AccessControlling the motion of multiple objects on a Chladni plate
Moving particles on a vibrating plate dates back to 1780s, but it is still challenging to control individual particles in a parallel way. Here, Zhou et al. use a single acoustic actuator and an algorithm to control multiple objects simultaneously and independently for sorting and pattern formation.
- Quan Zhou
- , Veikko Sariola
- & Ville Liimatainen
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Article
| Open AccessCoherence and multimode correlations from vacuum fluctuations in a microwave superconducting cavity
Vacuum fluctuations can produce observable phenomena which can potentially be harnessed, for example using the dynamical Casimir effect. Here, the authors show that, on the basis of the same effect, it is possible to establish distinct two-mode coherence correlations in a pumped microwave cavity owing to absence of which-way information.
- Pasi Lähteenmäki
- , Gheorghe Sorin Paraoanu
- & Pertti J. Hakonen
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Article
| Open AccessIonic imbalance induced self-propulsion of liquid metals
The control over the motion and deformation of liquid droplets is essential to many microfluidic and actuation systems. Zavabeti et al. demonstrate that applying a pH or ionic gradient across a droplet of liquid metal alloy of gallium results in its motion due to a breaking of the surface charge symmetry.
- Ali Zavabeti
- , Torben Daeneke
- & Kourosh Kalantar-zadeh
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Article
| Open AccessStructural and compositional dependence of the CdTexSe1−x alloy layer photoactivity in CdTe-based solar cells
Using a CdTexSe1−x alloy in CdTe solar cells leads to better performances. Here, Poplawsky et al. show that the photoactive properties of the alloy depend on its chemical composition and structural properties, and derive a phase diagram to further optimize alloy growth for photovoltaic devices.
- Jonathan D. Poplawsky
- , Wei Guo
- & Yanfa Yan
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Article
| Open AccessMapping two-dimensional polar active fluids to two-dimensional soap and one-dimensional sandblasting
In many groups of moving organisms, such as swarms of bacteria, their constituents pack so tightly that density cannot change. Here, Chen et al.map such incompressible flocks in two dimensions onto the growth of a one-dimensional interface, and thereby compute the large-distance behaviour of such flocks.
- Leiming Chen
- , Chiu Fan Lee
- & John Toner
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Article
| Open AccessSoft micromachines with programmable motility and morphology
In nature many microorganisms are able to change their shape to adapt to the changes in the environment. Inspired by this phenomenon, here Huang et al. build artificial microswimmers with body and flagellum made of programmable hydrogel-based materials incorporated with magnetic nanoparticles.
- Hen-Wei Huang
- , Mahmut Selman Sakar
- & Bradley J. Nelson
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Article
| Open AccessSingle-pixel three-dimensional imaging with time-based depth resolution
A three-dimensional imaging system which distributes the optical illumination over the full field-of-view is sought after. Here, the authors demonstrate the capability of reconstructing 128 × 128 pixel resolution three-dimensional scenes to an accuracy of 3 mm as well as real-time video with a frame-rate up to 12 Hz.
- Ming-Jie Sun
- , Matthew P. Edgar
- & Miles J. Padgett
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Article
| Open AccessMetal-induced rapid transformation of diamond into single and multilayer graphene on wafer scale
Direct growth of large-area graphene on dielectric substrates is a promising route to wafer scale integration. Here the authors use a rapid thermal annealing process to grow graphene layers on four-inch diameter polycrystalline diamond, eliminating the need for transfer.
- Diana Berman
- , Sanket A. Deshmukh
- & Anirudha V. Sumant
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Article
| Open AccessEigenspectra optoacoustic tomography achieves quantitative blood oxygenation imaging deep in tissues
Spectral corruption impedes imaging of blood oxygen saturation. Here Tzoumas et al.describe light fluence in the spectral domain and introduce eigenspectra Multispectral Optoacoustic Tomography to account for wavelength-dependent light attenuation and estimate blood oxygen saturation within deep tissue.
- Stratis Tzoumas
- , Antonio Nunes
- & Vasilis Ntziachristos
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Article
| Open AccessMagnetic assembly of transparent and conducting graphene-based functional composites
Transparent and electrically conducting flexible films are in high demand but production can be both time-consuming and expensive. Here, the authors report a method for assembling modified graphene flakes in controlled distributions within polymeric matrices by use of magnetic fields.
- Hortense Le Ferrand
- , Sreenath Bolisetty
- & Raffaele Mezzenga
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Article
| Open AccessSub-kBT micro-electromechanical irreversible logic gate
In computers, computation is performed by assemblies of logic gates, most of which are logically irreversible. Here, the authors explore the connection between logical and physical irreversibility through an OR gate made by a micro-electromechanical cantilever that can be operated with extremely little energy.
- M. López-Suárez
- , I. Neri
- & L. Gammaitoni
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Article
| Open AccessStructural lubricity under ambient conditions
Structural lubricity—referring to ultralow levels of friction between atomically flat, incommensurate surfaces—has previously been observed under ultrahigh vacuum. Here, the authors report structural lubricity at gold-graphite interfaces under ambient conditions and on mesoscopic scales.
- Ebru Cihan
- , Semran İpek
- & Mehmet Z. Baykara
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Article
| Open AccessMapping polaronic states and lithiation gradients in individual V2O5 nanowires
Rapid insertion and extraction of lithium ions from a cathode material is imperative for lithium-ion battery function. Here, the authors present evidence of inhomogeneities in charge localization, local structural distortions and polaron formation induced upon lithiation using scanning transmission X-ray microscopy.
- Luis R. De Jesus
- , Gregory A. Horrocks
- & Sarbajit Banerjee
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Article
| Open AccessSub-micrometre accurate free-form optics by three-dimensional printing on single-mode fibres
Combining freeform optics with micro- and nano-optics can permit wavefront shaping, phase engineering, k-space and polarization control. Here, Gissibl et al. use femtosecond 3D printing to manufacture free-form optical elements, giving sub-micrometre accuracy so that direct manufacturing on single-mode fibres is possible.
- Timo Gissibl
- , Simon Thiele
- & Harald Giessen
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Article
| Open AccessPhoton-efficient imaging with a single-photon camera
Active optical imaging systems use their own light sources to recover scene information but typically operate with large number of photon detections. Here, the authors present a 3D imaging system that acquires depth and reflectivity information with a single photon camera operating in low-light conditions.
- Dongeek Shin
- , Feihu Xu
- & Jeffrey H. Shapiro
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Article
| Open AccessReconfigurable optical assembly of nanostructures
Reconfigurable materials are of interest for many photonic applications. Here, Montelongo et al. demonstrate optical elements such as Bragg diffraction gratings, volumetric photonic crystals, lenses, and holograms in a composite with dispersed nanoparticles which can be recorded and erased.
- Yunuen Montelongo
- , Ali K. Yetisen
- & Seok-Hyun Yun
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Article
| Open AccessElectrically driven optical metamaterials
Active metamaterials are largely controlled by light, preventing integration in electronic systems. Here, the authors introduce electroluminescent metamaterials based on metal nano-inclusions hybridized with colloidal quantum dots and use this approach to weave intricate light-emitting surfaces.
- Quynh Le-Van
- , Xavier Le Roux
- & Aloyse Degiron
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Article
| Open AccessOperating organic light-emitting diodes imaged by super-resolution spectroscopy
There is a need to characterize devices during operation in real-time and at nanoscopic length scales. Here, King et al. perform electroluminescence-STED imaging with a polymer based light-emitting diode, revealing nanoscopic defects that would be unresolvable with traditional optical microscopy.
- John T. King
- & Steve Granick
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Article
| Open AccessLoss-tolerant state engineering for quantum-enhanced metrology via the reverse Hong–Ou–Mandel effect
N00N states are promising for quantum communications and metrology, but are vulnerable to losses. Here the authors develop a technique for preparing high-fidelity two-photon N00N states in a loss-free fashion, and demonstrate enhanced phase sensitivity without requiring recombination.
- Alexander E. Ulanov
- , Ilya A. Fedorov
- & A. I. Lvovsky
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Article
| Open AccessTwo-dimensional shape memory graphene oxide
When reducing the size of shape memory materials to the nanoscale regime, the memory effect tends to diminish. Here, the authors report a theoretical proposal of a shape memory graphene oxide with ordered epoxy groups retaining excellent programmability and actuation capabilities.
- Zhenyue Chang
- , Junkai Deng
- & Jefferson Zhe Liu
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Article
| Open AccessSlower carriers limit charge generation in organic semiconductor light-harvesting systems
In organic solar cells, the photogeneration of free charge carriers is limited by the dissociation of interfacial charge transfer states. Here, the authors study the impact of charge carrier mobilities in operational devices and show that the slowest charge carriers limit the dissociation of charge transfer states.
- Martin Stolterfoht
- , Ardalan Armin
- & Paul Meredith
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Article
| Open AccessIntegrating an electrically active colloidal quantum dot photodiode with a graphene phototransistor
The combination of fast photo-response and high gain plays a pivotal role in photodetector devices. Here the authors combine a colloidal quantum dot photodiode with a graphene phototransistor to overcome the speed, quantum efficiency and linear dynamic range limitations of available phototransistors.
- Ivan Nikitskiy
- , Stijn Goossens
- & Gerasimos Konstantatos
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Article
| Open AccessFloquet topological insulators for sound
One-way sound propagation has been recently proposed in the context of topological acoustics, but is challenged by introducing uniform media motion. Here, Fleury et al.present a practical scheme to achieve topological propagation by modulating in time the acoustic properties of a lattice of resonators, resembling Floquet topological insulators in condensed matter.
- Romain Fleury
- , Alexander B Khanikaev
- & Andrea Alù
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| Open AccessFast nanoscale addressability of nitrogen-vacancy spins via coupling to a dynamic ferromagnetic vortex
Nitrogen vacancies in diamond present single spin defects which may be used as nanoscale magnetic sensors. Here, Wolf et al.demonstrate how a ferromagnetic vortex in an adjacent micromagnet allows for fast nanoscale addressability of individual defect spins in nanodiamonds.
- M. S. Wolf
- , R. Badea
- & J. Berezovsky
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Article
| Open AccessArrays of individually controlled ions suitable for two-dimensional quantum simulations
Analogue quantum simulators could provide insights into complex dynamics, but realizing them in a scalable way remains a technological challenge. Here, the authors demonstrate how two-dimensional arrays of three ions trapped in individually controlled wells could form a scalable platform for quantum simulation.
- Manuel Mielenz
- , Henning Kalis
- & Tobias Schaetz
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Article
| Open AccessHigh-efficiency and air-stable P3HT-based polymer solar cells with a new non-fullerene acceptor
In organic photovoltaics, the best performing devices usually involve low-bandgap polymers whose limited solubility and stability constrain the scalability of organic solar cells. Here, Holliday et al. develop a new acceptor and pair it with canonical P3HT to obtain 6.4% efficient and stable devices.
- Sarah Holliday
- , Raja Shahid Ashraf
- & Iain McCulloch
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Article
| Open AccessMultiple-stable anisotropic magnetoresistance memory in antiferromagnetic MnTe
Contrary to ferromagnets, antiferromagnets possess no net magnetic moment, which has limited their applicability as magnetic memory media. Here, the authors demonstrate a heat-assisted multiple-stable memory based on epitaxial thin films of antiferromagnet MnTe with three-fold symmetric anisotropy.
- D. Kriegner
- , K. Výborný
- & T. Jungwirth
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Article
| Open AccessDirected percolation identified as equilibrium pre-transition towards non-equilibrium arrested gel states
Gels exhibit very slow dynamics, for which a structural reason remains elusive. Here, Kohl et al. show the gel formation is accompanied by a succession of continuous and directed percolation, with only the latter found to lead to the arrested dynamics.
- M. Kohl
- , R. F. Capellmann
- & M. Schmiedeberg
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Article
| Open AccessNanodiamond-based nanostructures for coupling nitrogen-vacancy centres to metal nanoparticles and semiconductor quantum dots
The coupling of nitrogen-vacancy centres with plasmonic and photonic nanostructures is usually studied by top-down preparation. Here, Gong et al. use a bottom-up approach to grow metallic and semiconducting nanoparticles on nanodiamonds, controlling the nanoparticle coverage, size and composition.
- Jianxiao Gong
- , Nat Steinsultz
- & Min Ouyang
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Article
| Open AccessCritical length scale controls adhesive wear mechanisms
Adhesive wear can proceed through qualitatively different mechanisms, with conflicting results in the literature. Here the authors observe a transition between two regimes in simulations using model interatomic potentials, allowing development of a simple analytical theory to describe past results.
- Ramin Aghababaei
- , Derek H. Warner
- & Jean-Francois Molinari
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Review Article
| Open AccessQuantum mechanical effects in plasmonic structures with subnanometre gaps
Recent work has shown that quantum mechanical effects in plasmonic nanogap structures become important as the gap distances approach the subnanometre length-scale. Here, the authors review the major findings which challenge the classical picture of these structures and discuss future directions for the field.
- Wenqi Zhu
- , Ruben Esteban
- & Kenneth B. Crozier
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Article
| Open AccessLarge-scale ordering of nanoparticles using viscoelastic shear processing
Packing nanoparticles into ordered superstructures finds applications in photonic materials, but fabrication over large scales is challenging. Zhao et al. show a roll-to-roll approach to prepare flexible films of ordered polymer nanoparticles via an oscillatory shear-induced structural transition.
- Qibin Zhao
- , Chris E. Finlayson
- & Jeremy J. Baumberg
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Article
| Open AccessSynergetic electrode architecture for efficient graphene-based flexible organic light-emitting diodes
Replacing indium tin oxide with graphene in organic light-emitting diodes is a promising approach to enhance the flexibility of displays and light sources. Here, the authors combine graphene, TiO2and low-index hole-injection layers to achieve high external quantum efficiency and good bendability.
- Jaeho Lee
- , Tae-Hee Han
- & Seunghyup Yoo
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Article
| Open AccessWafer-scale fabrication and growth dynamics of suspended graphene nanoribbon arrays
Shaping atomically thin materials in suspended structures may provide a viable platform for nanoscale mechanical oscillators. Here, the authors demonstrate wafer-scale, high-yield synthesis of suspended graphene nanoribbon arrays using a bottom-up approach and shed light into their growth dynamics.
- Hiroo Suzuki
- , Toshiro Kaneko
- & Toshiaki Kato
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Article
| Open AccessRobust and stretchable indium gallium zinc oxide-based electronic textiles formed by cilia-assisted transfer printing
The fabrication of smart textiles is currently relying on the printing of ultrathin electronics on fabric, which is subject to the poor adhesion between electronics and textile. Here, Yoon et al. propose the use of cilia-like structure to improve adhesion in addition to release mechanical stress.
- Jongwon Yoon
- , Yunkyung Jeong
- & Heung Cho Ko
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Article
| Open AccessTopological protection of multiparticle dissipative transport
Transport of a collection of classical particles involves thermal ratchet effect or adiabatic motion, which brings complexity to control multiparticle transport. Here, Loehr et al. show topologically protected multiparticle transport of diamagnetic and paramagnetic colloids, driven by periodic modulation loops of an external magnetic field.
- Johannes Loehr
- , Michael Loenne
- & Thomas M. Fischer
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Article
| Open AccessGraphene ballistic nano-rectifier with very high responsivity
The high mobility of graphene has the potential to enable design of devices working in a collisionless regime of carrier transport. Here the authors fabricate a ballistic nano-rectifier based on encapsulated graphene, showing intrinsic performances comparable to those of superconducting bolometers.
- Gregory Auton
- , Jiawei Zhang
- & Aimin Song
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Article
| Open AccessQuantum teleportation from light beams to vibrational states of a macroscopic diamond
Quantum teleportation has found important applications in quantum technologies, but pushing it to macroscopic objects is challenging because of the fragility of quantum states. Here, the authors demonstrate teleportation of states from light beams to the vibrational states of a macroscopic diamond sample.
- P.-Y. Hou
- , Y.-Y. Huang
- & L.-M. Duan