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The conversion efficiency of organic solar cells suffers from their low open-circuit voltages. Here, the authors expose a link between electron-vibrations coupling and non-radiative recombinations, derive a new limit for the efficiency of organic solar cells, and redefine their optimal optical gap.
High shares of variable energy sources will require different operational modes for dispatchable generation. Schill et al. explore the impact of increased wind and solar power on the German electricity system and find that the number of start-ups grows by 81% while its cost increases by 119% by 2030.
Multiple exciton generation has been shown to improve the performance of quantum-dot-based solar cells. Yan et al. now apply it to photoinduced hydrogen production and present a system using PbS quantum-dot photoelectrodes that yields an external quantum efficiency of over 100%.
Fast ionic conductivity of solid electrolytes is a must in the development of next-generation solid-electrolyte-based lithium-ion batteries. Here the authors report that composite polymer electrolytes with well-aligned inorganic nanowires can achieve much larger conductivities than those without.
Nuclear accidents generate vast echoes in public opinion, and often determine policy decisions to suspend nuclear programs. This study shows the unintended implications of nuclear plant shutdown in Tennessee Valley between 1983 and 1986, demonstrating deleterious consequences for public health.
Thin-film photovoltaic devices are often based on toxic or rare materials. Here, Wang et al. grow oriented Sb2Se3 thin film on a ZnO buffer layer, and fabricate solar cells with a certified 5.9% conversion efficiency and which pass harsh stability tests under humidity, heat and illumination.
To tackle the high energy consumption of buildings, information programs to promote investment in energy efficiency measures have been introduced. This study compares the effectiveness of three US programs and finds that despite large energy savings, progress is lacking for small and medium sized buildings.
Photoelectrochemical devices based on III–V semiconductors have high performance potential but their cost and stability inhibit their wide application. Kang et al. make printed assemblies of GaAs-based photoelectrodes with separate optical and reactive interfaces, demonstrating water-splitting efficiency up to 13.1%.
Nanostructured black silicon can be used as a photoelectrode for solar-driven water splitting, but its high surface area can increase charge recombination and accelerate corrosion. Here the authors show that a thin, conformal film of TiO2 can increase both the photocurrent and the stability of black silicon.
The application of Li–O2 batteries is hindered by severe parasitic reactions in battery cycling. Here the authors show that the highly reactive singlet oxygen is the main cause for the electrolyte and carbon electrode degradation on discharge and charge.
Perovskite-based solar cells are often fabricated by methods that are not industrially scalable. Here, Yang et al. develop an ink formulation which gives similar devices by spin coating, the lab-scale standard, and blade coating, which is a more scalable, industry-relevant deposition method.
Despite its role in electrocatalysis and hydrogen generation, a complete understanding of the hydrogen evolution reaction on platinum remains elusive. Here, a detailed kinetic study of hydrogen adsorption and evolution on Pt(111) highlights the role of interfacial water reorganization in the hydrogen adsorption step.
The efficiency of silicon solar cells has a large influence on the cost of most photovoltaics panels. Here, researchers from Kaneka present a silicon heterojunction with interdigitated back contacts reaching an efficiency of 26.3% and provide a detailed loss analysis to guide further developments.
Photoreforming can produce H2 through the simultaneous reduction of water and the oxidation of organic molecules, such as those derived from biomass, but cheaper and more active photocatalysts are required. This study shows that CdS/CdOx produces H2 from unprocessed lignocellulose suspensions at high rates under solar illumination.
Energy future scenarios are used in policy decision-making but little is known about how they influence public preferences. This study shows that engaging with an interactive scenario-building tool strengthens existing preferences, but exemplar scenarios provide reference points that anchor choices.
Solar water-splitting efficiency can be enhanced by careful bandgap selection in multi-junction semiconductor structures. Young et al. demonstrate a route that allows independent bandgap tuning of each junction in an immersed water-splitting device, enabling a solar-to-hydrogen efficiency of over 16%.
Achieving the global goals of the Paris Agreement requires ambition beyond what is currently contemplated by most governments. This study, based on long-term analysis for the UK, illustrates the challenge of achieving net-zero emissions and the need for a radical re-framing of national climate targets.
Deployment of rechargeable Li metal batteries requires fast charging capability and long-term cycling stability. Here the authors demonstrate the battery application potential of using a small amount of LiPF6 in a dual-salt electrolyte.
All-perovskite tandem solar cells hold the promise of high efficiencies whilst safeguarding the ease of fabrication intrinsic to perovskites. Here, Zhao et al. present a certified 17% efficient tin and lead perovskite solar cell, which is integrated as the low-bandgap component of a tandem device with 21% efficiency.
The large amount of uranium in the oceans could be exploited for nuclear fuel, but existing physicochemical extraction methods are limited in terms of capacity and rates of removal. Here the authors use an electrochemical extraction technique, demonstrating improved uptake capacity and kinetics.