Skip to main content

Thank you for visiting nature.com. You are using a browser version with limited support for CSS. To obtain the best experience, we recommend you use a more up to date browser (or turn off compatibility mode in Internet Explorer). In the meantime, to ensure continued support, we are displaying the site without styles and JavaScript.

  • Article
  • Published:

Dual-sensory fusion self-powered triboelectric taste-sensing system towards effective and low-cost liquid identification

Abstract

Infusing human taste perception into smart sensing devices to mimic the processing ability of gustatory organs to perceive liquid substances remains challenging. Here we developed a self-powered droplet-tasting sensor system based on the dynamic morphological changes of droplets and liquid–solid contact electrification. The sensor system has achieved accuracies of liquid recognition higher than 90% in five different applications by combining triboelectric fingerprint signals and deep learning. Furthermore, an image sensor is integrated to extract the visual features of liquids, and the recognition capability of the liquid-sensing system is improved to up to 96.0%. The design of this dual-sensory fusion self-powered liquid-sensing system, along with the droplet-tasting sensor that can autonomously generate triboelectric signals, provides a promising technological approach for the development of effective and low-cost liquid sensing for liquid food safety identification and management.

This is a preview of subscription content, access via your institution

Access options

Buy this article

Prices may be subject to local taxes which are calculated during checkout

Fig. 1: Droplet-based triboelectric taste-sensing system mimicking the human taste receptor.
Fig. 2: The working principle of a droplet-tasting sensor with one spatially arranged electrode, the sliding process of a water droplet and the electrical output of a single-electrode droplet-tasting sensor.
Fig. 3: Mechanism and sensing characteristics of a TDTS for sensing a droplet at two electrodes.
Fig. 4: Feature extraction of different liquids from droplet-induced triboelectric signals.
Fig. 5: Deep-learning-based data processing for liquid-type identification.
Fig. 6: Synergistic effect of triboelectric signals and image features for a higher accuracy of liquid identification.

Similar content being viewed by others

Data availability

All relevant data are included in the article, Supplementary Information and the source data files provided with this paper. All the other raw data are available from the corresponding authors on request.

Code availability

The code is available from the corresponding authors upon reasonable request.

References

  1. Vlasov, Y., Legin, A., Rudnitskaya, A., Di Natale, C. & D’amico, A. Nonspecific sensor arrays (‘electronic tongue’) for chemical analysis of liquids (IUPAC Technical Report). Pure Appl. Chem. 77, 1965–1983 (2005).

    Article  CAS  Google Scholar 

  2. Gabrieli, G., Muszynski, M. & Ruch, P. W. A reconfigurable integrated electronic tongue and its use in accelerated analysis of juices and wines. In 2022 IEEE International Symposium on Olfaction and Electronic Nose (ISOEN) 1–3 (IEEE, 2022).

  3. Zhu, Y. W. et al. Exploring the relationships between perceived umami intensity, umami components and electronic tongue responses in food matrices. Food Chem. 368, 130849 (2022).

    Article  CAS  PubMed  Google Scholar 

  4. Sochacki, G., Abdulali, A. & Iida, F. Mastication-enhanced taste-based classification of multi-ingredient dishes for robotic cooking. Front. Robot. AI 9, 886074 (2022).

    Article  PubMed  PubMed Central  Google Scholar 

  5. Rodríguez-Méndez, M. L. et al. Electronic noses and tongues in wine industry. Front. Bioeng. Biotechnol. 4, 81 (2016).

    Article  PubMed  PubMed Central  Google Scholar 

  6. Woertz, K., Tissen, C., Kleinebudde, P. & Breitkreutz, J. Taste sensing systems (electronic tongues) for pharmaceutical applications. Int. J. Pharm. 417, 256–271 (2011).

    Article  CAS  PubMed  Google Scholar 

  7. Winquist, F. et al. An electronic tongue in the dairy industry. Sensor. Actuat. B 111-112, 299–304 (2005).

    Article  CAS  Google Scholar 

  8. Fan, F. R., Tang, W. & Wang, Z. L. Flexible nanogenerators for energy harvesting and self-powered electronics. Adv. Mater. 28, 4283–4305 (2016).

    Article  CAS  PubMed  Google Scholar 

  9. Lee, M. et al. Self-powered environmental sensor system driven by nanogenerators. Energy Environ. Sci. 4, 3359–3363 (2011).

    Article  CAS  Google Scholar 

  10. Wang, X. D. et al. Self-powered high-resolution and pressure-sensitive triboelectric sensor matrix for real-time tactile mapping. Adv. Mater. 28, 2896–2903 (2016).

    Article  CAS  PubMed  ADS  Google Scholar 

  11. Zhong, T. Y. et al. An artificial triboelectricity-brain-behavior closed loop for intelligent olfactory substitution. Nano Energy 63, 103884 (2019).

    Article  CAS  Google Scholar 

  12. Guo, H. Y. et al. A highly sensitive, self-powered triboelectric auditory sensor for social robotics and hearing aids. Sci. Robot. 3, eaat2516 (2018).

    Article  PubMed  Google Scholar 

  13. Yoon, H. J. et al. Mechanoreceptor-inspired dynamic mechanical stimuli perception based on switchable ionic polarization. Adv. Funct. Mater. 31, 2100649 (2021).

    Article  CAS  Google Scholar 

  14. Qu, X. C. et al. Artificial tactile perception smart finger for material identification based on triboelectric sensing. Sci. Adv. 8, eabq2521 (2022).

    Article  CAS  PubMed  PubMed Central  ADS  Google Scholar 

  15. Wei, X. L., Wang, B. C., Wu, Z. Y. & Wang, Z. L. An open-environment tactile sensing system: toward simple and efficient material identification. Adv. Mater. 34, 2203073 (2022).

    Article  CAS  Google Scholar 

  16. Bachmanov, A. A. & Beauchamp, G. K. Taste receptor genes. Annu. Rev. Nutr. 27, 389–414 (2007).

    Article  CAS  PubMed  PubMed Central  Google Scholar 

  17. Barretto, R. P. J. et al. The neural representation of taste quality at the periphery. Nature 517, 373–376 (2015).

    Article  CAS  PubMed  ADS  Google Scholar 

  18. Kwak, S. S. et al. Triboelectrification-induced large electric power generation from a single moving droplet on graphene/polytetrafluoroethylene. ACS Nano 10, 7297–7302 (2016).

    Article  CAS  PubMed  Google Scholar 

  19. Choi, M., Lee, W. M. & Yun, S. H. Intravital microscopic interrogation of peripheral taste sensation. Sci. Rep. 5, 8661 (2015).

    Article  CAS  PubMed  PubMed Central  ADS  Google Scholar 

  20. Wei, X. L. et al. All-weather droplet-based triboelectric nanogenerator for wave energy harvesting. ACS Nano 15, 13200–13208 (2021).

    Article  CAS  PubMed  Google Scholar 

  21. Zhao, X. J., Zhu, G., Fan, Y. J., Li, H. Y. & Wang, Z. L. Triboelectric charging at the nanostructured solid/liquid interface for area-scalable wave energy conversion and its use in corrosion protection. ACS Nano 9, 7671–7677 (2015).

    Article  CAS  PubMed  Google Scholar 

  22. Pan, L. et al. Liquid-FEP-based U-tube triboelectric nanogenerator for harvesting water-wave energy. Nano Res. 11, 4062–4073 (2018).

    Article  CAS  Google Scholar 

  23. Nie, J. H. et al. Probing contact-electrification-induced electron and ion transfers at a liquid-solid interface. Adv. Mater. 32, 1905696 (2020).

    Article  CAS  Google Scholar 

  24. Lin, S. Q., Xu, L., Chi Wang, A. & Wang, Z. L. Quantifying electron-transfer in liquid-solid contact electrification and the formation of electric double-layer. Nat. Commun. 11, 399 (2020).

    Article  CAS  PubMed  PubMed Central  ADS  Google Scholar 

  25. Ying, Z. H. et al. Self-powered liquid chemical sensors based on solid-liquid contact electrification. Analyst 146, 1656–1662 (2021).

    Article  CAS  PubMed  ADS  Google Scholar 

  26. Shi, Q. F. et al. Deep learning enabled smart mats as a scalable floor monitoring system. Nat. Commun. 11, 4609 (2020).

    Article  CAS  PubMed  PubMed Central  ADS  Google Scholar 

  27. Wen, F. et al. Machine learning glove using self-powered conductive superhydrophobic triboelectric textile for gesture recognition in VR/AR applications. Adv. Sci. 7, 2000261 (2020).

    Article  CAS  Google Scholar 

  28. Shi, Q. F. et al. Artificial intelligence of things (AIoT) enabled floor monitoring system for smart home applications. ACS Nano 15, 18312–18326 (2021).

    Article  CAS  PubMed  Google Scholar 

  29. Sundaram, S. et al. Learning the signatures of the human grasp using a scalable tactile glove. Nature 569, 698–702 (2019).

    Article  CAS  PubMed  ADS  Google Scholar 

  30. Rodriguez-Mendez, M. L. et al. Fusion of three sensory modalities for the multimodal characterization of red wines. IEEE Sens. J. 4, 348–354 (2004).

    Article  CAS  ADS  Google Scholar 

  31. Simonyan, K. & Zisserman, A. Very deep convolutional networks for large-scale image recognition. Preprint at https://arxiv.org/abs/1409.1556 (2014).

Download references

Acknowledgements

This research was supported by the National Natural Science Foundation of China (grant number 61503051; Z.W.).

Author information

Authors and Affiliations

Authors

Contributions

Z.W. and Z.L.W. planned the study and supervised the whole project. X.W., Z.W. and Z.L.W. conceived the idea, analysed the data and wrote the paper. B.W., X.C. and H.Z. helped with the experiments. All the authors discussed the results and commented on the paper.

Corresponding authors

Correspondence to Zhiyi Wu or Zhong Lin Wang.

Ethics declarations

Competing interests

The authors declare no competing interests.

Peer review

Peer review information

Nature Food thanks Zong-Hong Lin and the other, anonymous, reviewer(s) for their contribution to the peer review of this work.

Additional information

Publisher’s note Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Supplementary information

Supplementary Information

Supplementary Figs. 1–28, Table 1 and Note 1.

Reporting Summary

Supplementary Video 1

The dynamic of one water droplet captured by a high-speed camera (a front view).

Supplementary Video 2

A water droplet sliding down an inclined surface.

Supplementary Video 3

Simulation of droplet sliding along an inclined plane by volume fraction of fluid.

Supplementary Video 4

Simulation of droplet sliding along an inclined plane by velocity field.

Supplementary Video 5

The signal response triggered by a coffee droplet sliding.

Supplementary Video 6

The signal response triggered by a water droplet sliding.

Supplementary Video 7

The taste-sensing system effectively identifies different liquids in a real environment.

Supplementary Data

Source data for supplementary figures.

Source data

Source Data Fig. 2

Statistical source data.

Source Data Fig. 3

Statistical source data.

Source Data Fig. 4

Statistical source data.

Source Data Fig. 5

Statistical source data.

Source Data Fig. 6

Statistical source data.

Rights and permissions

Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Wei, X., Wang, B., Cao, X. et al. Dual-sensory fusion self-powered triboelectric taste-sensing system towards effective and low-cost liquid identification. Nat Food 4, 721–732 (2023). https://doi.org/10.1038/s43016-023-00817-7

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1038/s43016-023-00817-7

Search

Quick links

Nature Briefing

Sign up for the Nature Briefing newsletter — what matters in science, free to your inbox daily.

Get the most important science stories of the day, free in your inbox. Sign up for Nature Briefing