Abstract
Optical solitons emerging from fiber resonators generally possess similar properties that hinge on the system parameters. However, the generation of wavepackets composed of dissimilar solitons within the same laser cavity is still challenging in ultrafast lasers. Here, we report on heteronuclear multicolor soliton compounds composed of chirp-free conventional solitons and chirped dissipative solitons, by introducing convex-concave frequency phases in mode-locked fiber lasers. In spite of different lasing wavelengths, the dissipative solitons always overlap with the conventional solitons, giving birth to trains of modulated wavepackets. The resonant sidebands of two types of solitons follow from the same phase-matching principle dominated by the absolute value of cavity dispersion. Simulations fully substantiate the experimental results, confirming that the overlapping of two solitons is dominated by the co-action of saturable absorption and group-delay compensation. It is demonstrated that the phase-managed dissipative system is capable of supporting multicolor soliton compounds with distinct properties, offering an effective platform to reveal the interaction of dissimilar nonlinear wavepackets.
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Introduction
Soliton is a self-organized wavepacket that preserves its shape during propagation in the dispersive-nonlinear medium, which is a ubiquitous phenomenon in nature and has been widely studied in various fields, ranging from hydrodynamics1, Bose–Einstein condensates2, event astronomy3 to biomedicines4. In the category of nonlinear optics, a chirp-free soliton that propagates in a particle-like fashion can be formed ascribing to the delicate balance between nonlinearity and anomalous dispersion of fibers or fiber lasers5. Via engineering the dispersion to near-zero and normal regime, stretched pulses6, similaritons7 and dissipative solitons (DSs)8,9 have been realized in fiber lasers under the complex interaction among dispersion, nonlinearity, gain and loss. Broadly speaking, the aforementioned pulses in fiber laser can be categorized as DSs since they are formed in non-conservative dissipative systems balanced by energy exchange with the external environment in the presence of fiber dispersion and nonlinearity. In a narrow sense, DSs here refer to confined wavepackets of light formed in normal dispersion regimes, in which the pulse experiences strong nonlinear gain and loss during propagation and usually features a giant frequency chirp8. Due to the gain competition effect, fiber lasers usually operate at the single-wavelength emission state, delivering a fixed type of robust pulse that depends on cavity parameters. By introducing spectral filters into the cavity, multicolor operations were realized at 1.06 μm, 1.55 μm, and 2 μm in mode-locked fiber lasers10,11,12,13,14. Attributing to the chromatic dispersion, the group velocities of these multicolor pulses differ from each other, resulting in independently evolved multiple pulse trains12.
Meanwhile, synchronization and overlap of pulses at different wavelengths give birth to multicolor wavepackets with fine temporal structures due to the beat effect, which is especially attractive for coherent combining, terahertz-wave generation, and Raman scattering spectroscopy15,16,17. Several active and passive methods have been proposed for synchronizing two-branch pulses at different wavelengths, such as phase-locked loop18, balanced optical cross-correlator19, and slave–master cavity configuration20. With the help of the filtering effect, fiber laser could directly deliver synchronized dual-color solitons via tailoring the cavity dispersion to near-zero regime21,22, or compensating the group-velocity mismatch by intermodal dispersion23. Apart from these approaches, the stimulated Raman scattering is proven to be able to generate multicolor bound chirped DS in fiber lasers24.
Recently, active manipulation of cavity parameters has advanced the development of solitons to an unprecedented state25,26,27. Runge et al. achieved high-energy pure-quartic solitons in fiber laser via introducing fourth-order dispersion and eliminating the second- and third-order dispersion of cavity28. After that, synchronized multicolor solitons29 and spectrally periodic pulses30, as the newly emerged nonlinear wavepackets, were achieved by engineering the dispersion of fiber laser with a programmable pulse shaper. These synchronized multicolor pulses are generated at the same dispersion regime, whose constituent pulses exhibit similar properties. Lately, dark-bright dual-color soliton pairs and broadband microcombs operating in opposite dispersion regimes were achieved in a micro-resonator under the effect of cross-phase modulation31,32. However, the dispersion characteristic of such a resonator cannot be actively manipulated. It is still unclear whether fiber lasers could support special wavepackets composed of dissimilar solitons, i.e., heteronuclear multicolor soliton compounds (HMSCs). Moreover, the interaction between distinct types of solitons remains less addressed in nonlinear dissipative systems.
In this paper, we demonstrate HMSCs in a mode-locked fiber laser, by introducing convex–concave phase and spectral filtering with a programmable pulse shaper. The convex–concave phase grants the periodic anomalous-normal dispersion distribution in the frequency domain, enabling the formation of the chirp-free conventional soliton (CS) and chirped DS in the same fiber laser. Different from the previous reports demonstrating the coexistence of two types of pulses with different group velocities13,33, the CS and DS with distinct wavelengths always co-propagate as a unit with fine temporal structure, forming a robust multicolor soliton compound composed of dissimilar solitons. Moreover, the DS here displays unique sidebands that can be controlled by the frequency phase, whose formation is not attributed to the nonlinear phase shift, but follows from the similar phase-matching principle as that of CS. Simulations validate the crucial experimental phenomena and reveal the interaction behavior between two distinct types of solitons.
Results
Experimental setup and results
Figure 1a shows the cavity configuration of the HMSC fiber laser. The 980-nm laser diode pumps a 6-m erbium-doped fiber (Nufern: EDFL-980-HP, β2 = 21.3 ps2 km−1) via a wavelength-division multiplexer, and the optical coupler extracts 10% energy for measurement. A polarization-insensitive isolator ensures the unidirectional propagation of pulses, and a programmable pulse shaper introduces the convex–concave phase and spectral filtering. The carbon nanotube saturable absorber initializes the mode-locking operation of the laser. The pigtails of fiber components are standard single-mode fibers (Corning: SMF-28e+, β2 = −21.7 ps2 km−1) with a total length of 9.2 m, and the programmable pulse shaper has an optical path of 3.7 m with an intrinsic dispersion of −0.45 ps2. Based on the above parameters, the total length and cavity dispersion are 18.9 m and −0.52 ps2, respectively.
The programmable pulse shaper (Santec, WSS-1000), composed of a diffraction grating and spatial light modulator, can arbitrarily adjust the amplitude and phase of each spectral component through a computer, and its principle is depicted in the left panel of Fig. 1b. Based on the Taylor series expansion of spectral phase34, the parabolic convex–concave frequency phase corresponds to a linear group delay with opposite slopes and an anomalous-normal dispersion regime (right panel of Fig. 1b). Therefore, the opposite dispersion regimes can be achieved within the same laser resonator by introducing the convex–concave phase, enabling the formation of HMSC composed of dissimilar solitons.
For each waveband, the dispersion depends not only on the cavity parameters, but also on the frequency phase induced by the programmable pulse shaper. As shown in Fig. 2a, after introducing the convex–concave phase, the group-delay dispersions at shorter and longer wavebands are about −15.38 ps2 and 14.33 ps2, respectively. Hence, the convex phase (i.e., shorter waveband) corresponds to the anomalous-dispersion regime, enabling the formation of CS characterized by Kelly sidebands35 and Sech2 spectral profile that is somewhat similar to the convex phase. The longer waveband locates at the normal dispersion regime, where the spectrum mimics the concave phase with a low-intensity center and strong sidebands, referred to as the DS. Note that the amplitudes of the convex–concave phase are the relative values, the phase jump (red curve in Fig. 2a) does not influence the values of group-delay dispersion at two wavebands.
Decreasing the amplitude of concave phase while keeping the convex phase unchanged, the spectrum of mode-locked pulse at longer waveband is gradually close to the typical DS observed in normal dispersion lasers. For example, the DS in Fig. 2b exhibits a “cat-ear” structure that is similar to the spectral profiles of the previously reported DSs36. In contrast to the spectral peaks arising from the nonlinear phase shift37, the “cat-ear” structure here belongs to the first-order dispersive sideband of DS, which will be elaborated in the next part. The DS exhibits the characteristic quasi-rectangular spectrum and possesses comparable intensity with CS when further decreasing the amplitude of concave phase (Fig. 2c). Note that the pulse profiles retrieved from the frequency-resolved optical gating spectrograms show beat fringes with the same period of 1.62 ps (Fig. 2d–f), coinciding with the central wavelength separation of 4.76 nm between CS and DS according to the Fourier transform principle. The beat fringe validates the overlapping of two solitons, which is further corroborated by the radio-frequency spectrum and oscilloscope trace (see details in Supplementary Note 1).
The properties of CS and DS are further revealed by spectrally filtering the HMSC external to the cavity (see Supplementary Note 2). The time-bandwidth products of the CS and DS are given as 0.32 and 0.95, respectively, which confirms that the CS is chirp-free while the DS is chirped. The separations of beat fringe for three cases are identical (1.62 ps) due to the constant wavelength spacing between two solitons. Note that the group-delay differences between two spectral centers induced by convex–concave phases are 1.87 ps, 1.98 ps, and 2.06 ps, respectively, which nearly compensate for the intrinsic group-delay difference of fiber laser (−1.94 ps). In despite of the small residual group-delay differences, the saturable absorber automatically forces two solitons into a trapped state as the overlapped pulse has a higher intensity and thus results in a lower non-saturable loss. It is demonstrated that the HMSC fiber laser also follows from the same minimum-loss principle reported on the spatiotemporal mode-locked laser38.
By exploiting time-stretch dispersive Fourier transform technique39,40,41,42, we record the build-up process of the HMSC in Fig. 2a. The details of the measurement system are given in the “Methods” section. As depicted in Fig. 3a, the lasing wave undergoes a pulse-picking process from 0 to ~2100 roundtrips, wherein the weak noisy pulses are eliminated by the saturable absorber and the dominant pulses survive. Then, the laser enters the relaxation oscillation stage, lasting ~1000 roundtrips (from 2100 to 3100 roundtrips). After the beating stage, the metastable CS and DS appear at ~3200 roundtrips and experience a transient stage with damped breathing behavior. The fiber laser finally evolves into the steady state at ~4000 roundtrips, forming the stable dual-color HMSC. The build-up process is somewhat similar to previously reported fiber laser43, while the lasting time is much longer than that of CS44 or CS compounds29, which is attributed to the harsher formation condition of HMSCs. At the steady state, only CS and first-order sidebands of DS are captured as their other spectral components are relatively weak. One can find that the CS and DS reach the steady state at the same time, and they always synchronously circulate inside the cavity.
In addition to dual-color HMSCs, three- to five-color HMSCs can also be achieved in the same fiber laser by increasing the filter bandwidth from 14.4 nm to 19.1 nm and introducing more concave and convex phases into the cavity (see details in Supplementary Note 3). Figure 3b shows the typical case of four-color HMSC comprising two CSs and two DSs. The retrieved pulse exhibits a clear beat fringe (Fig. 3c), which is attributed to the overlap of these solitons. Note that the beat fringe separation (0.88 ps) corresponds to the wavelength separation between two CSs (9.38 nm). This is because, the intensity of DS is much lower than CS, and the beat fringe is dominated by two CSs. The synchronization of these solitons can be further corroborated by the oscilloscope trace and radio-frequency spectrum (see Supplementary Note 1).
Formation mechanism of sideband on DS
When pulses encounter periodic perturbations such as gain, filtering effect and loss in a fiber laser, they shed parts of energy in the form of dispersive waves45. The dispersive waves generated at the adjacent roundtrip interfere, and only the frequencies satisfying the phase-matching principle survive in the cavity. Figure 4a, b shows the phase-matching conditions of the dispersive wave for CS and DS, respectively. The blue horizontal line and curve denote the phases of CS (φCS) and DS (φDS) accumulated per roundtrip, respectively. The parabolic lines are phases of dispersive waves (φDW) accumulated in one roundtrip:
where β2 is the group-velocity dispersion of the fiber laser, δf is the frequency offset from the spectral center, and L is the cavity length. As the introduced convex (concave) phase spans from −9π to 0 (0–9π) in the studied waveband, the phase-matching between dispersive wave and pulse is achieved at several frequencies when the phase difference is the integer multiple of 2π. Note that no particular periodic perturbation is required for the first-order phase-matched frequency of DS (red dot in Fig. 4b), as the accumulated phase shift always matches that of the dispersive waves at any cavity position46. This condition is unpractical for CS unless the laser cavity has strong third-order dispersion47.
Based on the phase-matching principle between the dispersive waves and solitons48, the relationship between two adjacent sidebands on one side can be expressed as:
where δfm and δfm − 1 are frequency offsets between the spectral center and sidebands with the order of m and m − 1 (m ≥ 2), respectively.
Via changing the amplitude of concave and convex phases (i.e., changing group-velocity dispersions at two wavebands), we calculate the squared difference of frequency offsets between first- and second-order sidebands for CS and DS based on Eq. (2), respectively. As illustrated in Fig. 4c, d, the theoretical prediction agrees with experimental observation, verifying that the strong sidebands of DS arise from the resonant amplification of dispersive waves rather than the nonlinear phase shift accumulated in the cavity. It turns out that the sidebands of CS and DS follow the same phase-matching principle that mainly depends on the absolute value of cavity dispersion.
Simulation results
To uncover the formation mechanism of HMSCs, we perform numerical simulation based on the generalized nonlinear Schrödinger equation that incorporates nonlinearity, dispersion, gain and loss of fiber resonator29,41. The simulation starts from a weak noisy pulse, and the pulse enters the loop and passes through each fiber component sequentially. After one circulation, the resultant pulse works as the input of the next roundtrip until the fiber laser achieves a self-consistent state (see details in “Methods”).
Figure 5 shows the simulation results of three typical HMSCs, which agree well with the experimental counterparts, from spectral profiles to evolution behaviors. The separation between two spectral centers is 5.02 nm, also comparable with the experimental result of 4.76 nm (Fig. 5a–c). In the simulation, the group-delay differences induced by the convex–concave phase almost compensate for the intrinsic group-delay difference of the cavity. Although two solitons have different wavelengths, they always overlap and evolve as a unit in the cavity (Fig. 5d–f), verified by the temporal beat fringes (Fig. 5g–i). The insets of Fig. 5g–i show that the DS accumulates a linear frequency chirp, which is the typical characteristic of mode-locked pulse in normal dispersion lasers. In addition, the spectrograms show that the sidebands of CS on the blue (red) side locate at the pulse leading (trailing) edge, while it is opposite for DS, confirming that two constituents of HMSCs operate at opposite dispersion regimes.
Reducing the amplitude of the concave phase, the energy of DS transfers from the sideband to the central region of the spectrum, which also can be interpreted by the phase-matching principle. As depicted in Fig. 4b, the central frequency of DS deviates from the phase-matching condition. Such deviation becomes less apparent for the smaller amplitude of the concave phase, and the central frequency is capable of receiving more energy, leading to the energy transformation within the DS. Correspondingly, the pulse intensity increases while the duration decreases during this evolution. For previously reported DS fiber lasers49, the cavity dispersions are usually less than 2ps2, which is much smaller than the cases of Figs. 2a and 5a. Thus, the phase-matching effect is less important, and the sidebands disappear on the spectrum.
Note that the CS can always be formed in the fiber laser with or without the convex phase. However, the DS is unable to exist alone and always accompanies the CS, i.e., the CS and DS with distinct properties appear as a unit. Such a phenomenon is understandable by noting that DS requires a harsher formation condition than CS. For example, considering the self-phase modulation effect, the DS will be quickly broadened by normal dispersion while the CS may survive in the presence of anomalous dispersion. Notably, the DS has a much lower intensity than that of CS. As the transmittance of the saturable absorber relies on the pulse intensity, the DS will be eliminated due to the saturable absorption effect while the CS could survive due to the higher pulse intensity.
We further simulate the build-up process of HMSC in Fig. 5a to reveal the underlying mechanism, as shown in Fig. 6. The initial noisy pulses quickly broaden, and the spectral widths of CS and DS gradually decrease from 0 to 100 roundtrips, wherein the dispersion dominates this process. Then, the pulse envelope starts to narrow and new spectral components emerge under the effect of self-phase modulation and saturable absorption effects. In this stage, the spectrum of DS splits into two parts while that of CS maintains the Sech2 profile, which is attributed to the opposite dispersion settings at two wavebands. After that, the dispersive sidebands gradually formed on the spectra of CS and DS under the phase-matching effect, reaching a metastable state at ~150 roundtrips. Finally, the pulse evolves to a steady state after a complex pulse-shaping process. Since the CS contains most of the energy of the HMSC and the reference wavelength is 1548 nm, the pulse shifts toward the forepart of the time window. Note that two solitons reach the steady state at the same time, coinciding with the experimental observation in Fig. 3a.
During the whole build-up process, two solitons always overlap in the time domain, giving rise to the HMSC with periodic structures. This can be attributed to the co-action of saturable absorption and the group-delay compensation. To verify this, we further simulate the HMSC evolution with respect to cavity roundtrips in the absence of the saturable absorber or convex–concave phase (i.e., group-delay compensation), respectively (see details in Supplementary Note 4). When the saturable absorber is removed in the simulation model, two pulses still overlap under the group-delay compensation, whereas they broaden due to the chromatic dispersion and strongly emit non-solitary radiation per roundtrip. Once the group-delay compensation is ignored, two solitons propagate at different velocities and quickly depart from each other under the effect of chromatic dispersion.
The intracavity evolution of HMSC in a single roundtrip is shown in Fig. 7. For simplicity, the HMSC in Fig. 5a is discussed, while the other cases are given in Supplementary Note 5. The intracavity energy evolutions of CS and DS are shown in the upper panel of Fig. 7a. Due to the filtering effect, the spectral width of DS is less than 3 nm, thus the corresponding energy is significantly confined, resulting in comparable energy with CS. Moreover, the CS makes the saturable absorber easier to saturate, and thus the DS can be formed at a relatively low intensity. In the cavity, two solitons are amplified in the erbium-doped fiber segment and then weakened by the single-mode fiber, output coupler, saturable absorber, and programmable pulse shaper to realize a self-consistent evolution. The intensities of spectrum and pulse are normalized at each cavity position to highlight the imperceptible changes of the wavepacket. As shown in the middle and lower panels of Fig. 7a, the spectral profiles of CS and DS nearly keep invariant along the cavity, which results from the limited pulse intensity. Ascribing to the fixed wavelength separation between two solitons, the beat fringe of HMSC almost remains unaltered along the cavity. The white dashed line denotes the position of the introduced phase. One can observe that, the phase does not influence the spectral intensity (Fig. 7b), while affecting the temporal properties, i.e., weakens the modulation depth and changes the pulse location (Fig. 7c). Note that the first-order sidebands (or cat-ear structure) of DS always appear at the same frequency inside the cavity. In contrast, such “cat-ear” structure on previously reported DS arises from the nonlinear phase shift, periodically emerging and disappearing within the cavity due to the spectral filtering effect36. Since the “cat-ear” structure induced by nonlinear phase shift changes along the cavity, we further confirm that the sidebands of DS in our experiment arise from the phase-matching effect.
Conclusion
It is apparent that the resonant radiation from the soliton is a universal phenomenon independent of the dispersion regime. The difference is that, the central frequency is phase-matched for CS while phase-mismatched for DS. The synchronization between CS and DS is mainly attributed to the group-delay compensation, then the saturable absorption effect forces them to overlap to minimize the transmission loss, following from the principle of minimum loss in mode-locked lasers38. Besides, the filtering effect is also essential in the formation of HMSCs, which is verified by the pulse evolution in the cavity without the spectral filtering (see Supplementary Note 6). One can find that the HMSC cannot be maintained and quickly collapses into multiple sub-pulses after 10 roundtrips. Thus, the formation of such wavepackets relies on three key factors. Firstly, the spectral filtering enables the multicolor operation of laser. Secondly, the convex–concave phase creates two opposite dispersion regimes for the generation of CS and DS. Finally, the group-delay compensation, together with the saturable absorption effect, synchronizes and overlaps the CS and DS, resulting in the unique HMSCs. It is demonstrated that the phase-managed fiber laser can deliver multicolor soliton compounds with distinct spectra and chirps, which provides an interesting platform to study the interaction of dissimilar solitons.
In summary, by introducing the convex–concave phase and spectral filtering, we demonstrate HMSCs comprised of CS and DS in an erbium-doped fiber laser. The CS and DS exhibit pairs of spectral sidebands obeying the same phase-matching principle. Especially, the spectral profile and pulse intensity of DS can be actively managed by tuning the amplitude of the concave phase. Simulations fully reproduce the experimental observations and indicate that the synchronization and overlap of two solitons rely on the group-delay compensation and saturable absorption effect. This work reveals a class of wavepackets, offers a simple testbed for exploring complex soliton interaction and may facilitate applications of terahertz wave generation and nonlinear spectroscopy.
Methods
Numerical simulations
The nonlinear Schrödinger equation in Eq. (3) models the propagation of pulse inside the cavity, and is solved by the predictor-corrector split-step Fourier technique29,50:
where u is the slowly varying envelope of the pulse, z and t represent the propagation distance and time, respectively. γ is the cubic refractive nonlinearity of the fiber and β2 is the second-order dispersion coefficient. g, α, and Ωg are the saturable gain, loss of the fiber and gain bandwidth, respectively. For the single-mode fiber, g = 0; and for the erbium-doped fiber, g = g0exp(−Ep/Es), where g0, Ep, Es are the small-signal gain coefficient, pulse energy, and the gain saturation energy, respectively. The saturable absorber has a transmittance T = 0.46 − T0/[1 + P(τ)/Psat], where T0 is the modulation depth, P(τ) is the instantaneous pulse power, and Psat is the saturable power. The spectral filter is modeled by a cosine function and has a transmittance Tf(ω)=[1 + 0.5cos(dω)]/2, where d is related to the filtering period.
The convex–concave phase is modeled by multiplying the electric field with the corresponding function in the frequency domain as Uout(ω) = Uin(ω)exp[iφ(ω)], where φ(ω) is expressed as:
The first term on the right side of Eq. (4) is the convex phase, and the second term represents the concave phase. ω0 and ω1 denote the central angular frequencies of the convex and concave phases, respectively. The central angular frequency spacing between the convex and concave phases (i.e., ω0 − ω1) is the same as the period of the spectral filter.
The simulation parameter is set as follows to match the experiment: Es are 340 pJ, 250 pJ, and 220 pJ, corresponding to the cases of Fig. 2a, Fig. 2b, and Fig. 2c, respectively. T0 = 0.08, Psat = 8 W. For the single-mode fiber, g0 = 0, α = 4.6 × 10−5 m−1, β2 = −21.7 ps2 km−1, γ = 1.3 W−1 km−1. For the programmable pulse shaper, β2 = −120.3 ps2 km−1, γ = 0. For the erbium-doped fiber, g0 = 0.7 dB m−1, β2 = 21.3 ps2 km−1, γ = 3.9 W−1 km−1, Ωg = 30 nm. For the spectral filter, d = 1.53 × 10−12 s. For the convex phase, A is −7.95ps2 during the whole simulation. For the concave phase, B is 7.95 ps2, 2.65 ps2, and 1.32 ps2, corresponding to the cases of Fig. 2a, Fig. 2b, and Fig. 2c, respectively.
Measurement system
The spectrum, pulse profile, signal-to-noise ratio, and pulse duration of HMSC are recorded by an optical spectrum analyzer (YOKOGAWA, AQ6370), a frequency-resolved optical gating (Femtoeasy, FS-600), a radio frequency analyzer (Agilent, E4440A) and an autocorrelator (Pulsecheck, USB-150), respectively. The time-stretch dispersive Fourier transform system comprises a 5-km dispersion compensation fiber with the dispersion of −150 ps nm−1 km−1, a 4 GHz oscilloscope and a 5 GHz photodetector. Based on the above parameters, the overall spectral resolution of the system is calculated as 0.33 nm51.
Reporting summary
Further information on research design is available in the Nature Portfolio Reporting Summary linked to this article.
Data availability
The data supporting the results of this paper are available from the corresponding author upon reasonable request.
Code availability
The simulation code is available upon reasonable written request, which excludes any commercial interest.
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Acknowledgements
This work was supported by the National Key R&D Program of China (2017YFA0303800), the National Natural Science Foundation of China (11874300, 61805277, 62105264), the Fundamental Research Funds for the Central Universities (3102019JC008), and the Natural Science Foundation of Shaanxi Province (2021JC-09, 2019JQ-447).
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H.Z. performed the experiments, carried out the numerical simulations and wrote the manuscript. D.M. designed the experiments, carried out the theoretical analysis and revised the manuscript. Y.D. and C.Z. plotted the figures and discussed the results. Z.S. and J.Z. contributed to the interpretation of the results and revising of the manuscript.
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Zhang, H., Mao, D., Du, Y. et al. Heteronuclear multicolor soliton compounds induced by convex-concave phase in fiber lasers. Commun Phys 6, 191 (2023). https://doi.org/10.1038/s42005-023-01313-x
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DOI: https://doi.org/10.1038/s42005-023-01313-x
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