Abstract
Levitating nanoparticles trapped in optical potentials at low pressure open the experimental investigation of nonlinear ballistic phenomena. With engineered non-linear potentials and fast optical detection, the observation of autonomous transient mechanical effects, such as instantaneous speed and acceleration stimulated purely by initial position uncertainty, are now achievable. By using parameters of current low pressure experiments, we simulate and analyse such uncertainty-induced particle ballistics in a cubic optical potential demonstrating their evolution, faster than their standard deviations, justifying the feasibility of the experimental verification. We predict, the maxima of instantaneous speed and acceleration distributions shift alongside the potential force, while the maximum of position distribution moves opposite to it. We report that cryogenic cooling is not necessary in order to observe the transient effects, while a low uncertainty in initial particle speed is required, via cooling or post-selection, to not mask the effects. These results stimulate the discussion for both attractive stochastic thermodynamics, and extension of recently explored quantum regime.
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Introduction
Stochastic levitating optomechanics in vacuum is a dynamically expanding experimental platform with a unique potential to test and exploit strong nonlinear motional effects without any friction, and bring them close to the quantum domain. This uniqueness arises from the possibility to combine manipulation of the optical trapping potential by a spatial light modulator, inducing new unexplored nonlinearities, and fast optical measurement to verify rapid transient effects using modern optical detectors. At low pressure, it allows direct observation of stochastic underdamped mechanical phenomena1,2,3,4,5,6,7, which allow access to the instantaneous particle speed not measurable in the overdamped motion8,9. In the transient ballistic regime, the surrounding environment does not modify the statistics of the instantaneous velocity8,10,11. Moreover, the initial uncertainty of the levitating particle can be controlled, by postselection12, feedback cooling13,14,15,16 and ultimately, by coherent scattering to the mechanical ground states17,18,19. All these key ingredients encourage broader investigation of the fundamental aspects of statistical mechanics20,21 and accelerate development of applications in mechanical sensing5,22,23,24 and thermodynamical engines25,26. Recently, the highly unstable motion of a levitating particle in the cubic potential has been analysed27,28 and experimentally verified29,30 in the overdamped regime. It was demonstrated that the mean particle position, induced by the initial position uncertainty, increases faster than that uncertainty. Atypically, the position distribution maximum shifts in the opposite direction to the mean. These investigations have already been stimulating experimentally verifiable thermodynamical consequences27.
In the low pressure limit the particle is deep in the underdamped regime so that the instantaneous particle speed and acceleration become new transient quantities to be first explored and later exploited for applications. In this paper we simulate and analyse nonlinear ballistic effects for instantaneous velocity and acceleration induced by the initial position uncertainty, and predict the experimental regime where such phenomena are visible using parameters for current setups in laboratories12,31,32,33. We observe that the only requirement for a reliable experimental observation is a reduction of initial velocity uncertainty. Importantly, we indicate that both the velocity and acceleration distributions’ maxima, stimulated by initial position uncertainty, shifts normally in the same direction as the velocity and acceleration mean. It is a crucial step to further accumulate such uncertainty-induced phenomena, and later use them in the aforementioned applications.
Results
Underdamped, overdamped and deterministic nonlinear dynamics in cubic potential
To understand the low-pressure nonlinear effects, we must distinguish them from the already measured high-pressure overdamped limit27,30, and aim to achieve them close to the zero-damping deterministic limit. First, we describe the properties of the stochastic motion of an underdamped Brownian particle in the unstable cubic potential. Second, we explore the high pressure limit in comparison to the over-damped approximation27,30, and low pressure limit with comparison to the zero-damping deterministic approximation. The dynamics of the damped Brownian particle in the cubic potential \(V(x)={Kx{^3}}/3\) is described by the following Langevin equation
where \(\kappa =K/m\) is the normalised cubic potential stiffness, \(\gamma =\Gamma /m\) is the medium damping with \(\Gamma\) the drag coefficient of the medium (e.g. air at low pressure), T is the absolute temperature, \(k_B\) is the Boltzmann constant, and \(F^{fluct}=\sqrt{2 k_B T\Gamma }\xi (t)\) is the broadband Markov Langevin force, uncorrelated in time with zero mean and variance given by the fluctuation-dissipation theorem \(\langle F^{fluct} \rangle =0\), \(\langle F^{fluct} (t) F^{fluct}(t')\rangle =\sqrt{2k_B T\gamma }\delta (t-t')\). For the short transient dynamics below the re-heating times, the uncertainty of the initial position \(\sigma _{x_0}^2\) is used, instead of the thermal noise, to induce the shift with well specified ratio to the standard deviation. We use Eq. (1) for all stochastic simulations, and also to present all the figures. The details of the simulation, comprising the re-scaling of Eq. (1) to allow usage of real experimental numbers, are described in the Methods. In the high pressure limit, the instantaneous velocity and acceleration require very fast measurement to be observed in the ballistic regime11, therefore we use the averaged velocity \({\bar{v}} = \Delta x/ \Delta t\), and averaged acceleration \({\bar{a}}=\Delta {\bar{v}}/\Delta t\) routinely measured in high pressure experiments. The time \(\Delta t\) has been adjusted to be tenfold the time-step dt to allow the computation of the averaged quantities. The details of the time scales, and convergence are presented in the Methods. Considering that \({\bar{v}}\) and \({\bar{a}}\) are still stochastic quantities, we further characterise their average motion by analysing their means, \(\langle {\bar{v}} \rangle\), and \(\langle {\bar{a}} \rangle\), and standard deviations, \(\sigma _{{\bar{v}}}\), and \(\sigma _{{\bar{a}}}\).
In the high pressure limit, Eq. (1) can be approximated by the over-damped equation of motion28,
comprising a change of mean position \(\langle x(t) \rangle \approx -(K \sigma _{x_0}^2 t + 2K k_B T t^2\Gamma ^{-1})/\Gamma\), for initial Gaussian position distribution with \(\langle x_0 \rangle =0\), evolving with standard deviation \(\sigma _x (t) \approx \sqrt{\sigma _{x_0}^2 + 8 (K/\Gamma )^2\sigma _{x_0}^4 t^2 + 2 k_BT t/\Gamma }\), and generating a \(SNR_x \approx (K^2\sigma _{x_0}^2 t^2 + K^2k_BT t^3\Gamma ^{-1})/\Gamma\)28. The direct integration of Eqs. (1), (2) unveils short transient uncertainty-induced effects experimentally measurable, beyond linearised systems. The Gaussian statistics of the initial state, however, allows to describe the non trivial effect using only first and second Gaussian moment with different powers for different nonlinearities.
At the time scale of this experiment \(t=0.1\) ms, three orders of magnitude shorter than the previous overdamped experiments \(t=1\)s29,30, the mean \(\langle x(t) \rangle \approx 0\) and standard deviation \(\sigma _{x}(t) \approx \sigma _{x_0}\) of position do not change in time, resulting in a negligible \(SNR_x\) as can be observed in Fig.1 for the high pressure regime (a). However, the average velocity \(\langle {\bar{v}} \rangle\) already feels the initial uncertainty evolving linearly with the latter as shown in Fig. 1c by the green line. The statistics of the average velocity \({\bar{v}}\), for short time \(\Delta t\) and Gaussian position and velocity distributions with \(\langle x_0 \rangle =0\) and \(\langle {\bar{v}}_0 \rangle =0\), approaches
For small environmental temperature, \(k_B T \ll K^2/\Gamma\), Eq. (3) generates a constant \(SNR_{{\bar{v}}} \approx 1/\sqrt{2}\). On the other hand, in the experiments at room temperature and \(\Gamma =10\) Hz29,30 the second term in the standard deviation of average velocity \(\sigma _{{\bar{v}}}\) reduces the \(SNR_{{\bar{v}}}\) to that of Eq. (3). The latter can be qualitatively observed in Fig.1c by the non constant azure halo as a function of initial position uncertainty. However, velocity uncertainty does not increase as quickly as in particle position, for the same short time scale. The statistics of the average acceleration \({\bar{a}}\), as shown in Fig.1e, do not change neither for the mean \(\langle {\bar{a}} \rangle\) (green), nor for the standard deviation \(\sigma _{{\bar{a}}}\) (blue–green halo) for the short time dynamics and range of parameters we are interested in, and their approximate characterisation is therefore omitted. By numerically simulating Eq. (1) for values of \(\Gamma \ge 10\) Hz, the position and average velocity statistics, obtained from Eq. (2) for the over-damped approximation, can be retrieved fully. A quantitative comparison is shown in Fig. 2(a,c, green dots).
The aim of the low-pressure regime is to (i) reach the statistics of instantaneous speed, as compared to average speed in Eq. (3), and (ii) obtain instantaneous acceleration statistics, both not achievable in the high pressure regime without very fast measurements. We consider such a short-time regime characterised by no change in initial particle position, as depicted in Fig. 1. For better and clear visualisation, the scale bar for increasing initial uncertainty \(\sigma _{x_0}^2\) changes within, while conserving the information about the profile of the probability density, up to the normalisation factor.
Such short transient regime when the particle does not move defines the time scale of such effect.
The goal in this regime is to reach the ideal classical limit of the zero-pressure regime, approaching deterministic dynamics for \(\Gamma =0\), where Eq. (1) becomes
yielding deterministic trajectories from initial position and velocity statistics. In this nonlinear ballistic regime, the Gaussian initial distribution of particle speed has \(\langle {\dot{x}}_0 \rangle = 0\) and \(\sigma _{{\dot{x}}_0}^2 =0\). The initial position and speed are statistically independent. In such regime, the initial position statistics is the only thermal energy resource that can be used in the nonlinear ballistics. For short time dynamics, from \(\langle x_0 \rangle =0\), the quantitative description of the zero-damping approximation for instantaneous acceleration gives
Notice that both mean and standard deviation are advantageously independent of initial speed statistics. This helps to distinguish the nonlinear ballistics in the experiment. The evolution of mean instantaneous acceleration \(\langle \ddot{x} \rangle\), and its standard deviation \(\sigma _{\ddot{x}}\), grow comparably with \(\sigma _{x_0}\) keeping a constant \(SNR_{\ddot{x}}\approx 1/\sqrt{2}\). In Fig.2e,f, Eq. (1) has been simulated (black dots), for damping \(\Gamma =10^{-2}\) Hz, to generate \(\langle \ddot{x} \rangle\), and \(SNR_{\ddot{x}}\). At such small pressure, the dominant dynamics observed can be already described by the zero-damping approximation introduced in Eq. (4), resulting in a linear evolution of \(\langle \ddot{x} \rangle\) with \(\sigma _{x_0}^2\) as showed in Eq. (5) (black line). Simultaneously, the \(SNR_{\ddot{x}}\) (black dots) generated with Eq. (1), converges quickly to the zero-damping approximation depicted in Eq. (4), resulting in a constant \(SNR_{\ddot{x}}\) as obtained in Eq. (5). By formally integrating Eq. (4) \({\dot{x}}(t) \approx {\dot{x}}_0 - \kappa \int _0^t x_0^2(t') dt'\) with \(\langle x_0 \rangle =0\), the short-time evolution of instantaneous velocity unfolds as
considering the initial conditions \(\langle {\dot{x}}_0 \rangle =\sigma _{{\dot{x}}_0}^2=0\). The mean \(\langle {\dot{x}}(t)\rangle\) of instantaneous velocity evolves linearly with initial position variance \(\sigma _{x_0}^2\), growing comparably with its standard deviation \(\sigma _{{\dot{x}}}(t)\), ultimately leading to the constant \(SNR_{{\dot{x}}}\approx 1/\sqrt{2}\) shown in Eq. (6). Simultaneously, by second time formally integrating Eq. (4) with \(\langle x_0 \rangle =0\), the position approaches \(x(t) \approx x_0 + \int _0^{t}{\dot{x}}_0(t') dt' -\int _0^{t}\int _0^{t'}\kappa x_0^2(t'') dt''dt'\), while its statistics for short time dynamics evolves as
For the large time scale, starting at \(t=0.9\) ms, the mean position evolves as in Eq. (7), while the standard deviation is dominated by the second term, ultimately leading to a constant \(SNR_x \approx 1/\sqrt{2}\). At this scale, the dynamics already makes the particle moving farther by initial position uncertainty. At the short time scale, \(t=0.1\) ms however, the position at average does not move, while its standard deviation remains equal to \(\sigma _{x_0}\). The resulting uncertainty-induced dynamics produces a \(SNR_x \approx 0\). At such a short time scale, the result is similar to the over-damped regime described by (2). This behavior can be observed in Fig.1b by the black arrow for the mean position, and with the azure halo for the standard deviation. The behavior of the \(SNR_x\) can be observed in Fig.2(b, black line), holding true for small pressure (black dots), as well as for high pressure (green dots).
Robustness of the uncertainty-induced instantaneous speed and acceleration
Role of environmental temperature T
The instantaneous speed and acceleration stimulated by the initial position uncertainty, can be affected by room temperature of external environment. Generalising the above results for non-zero damping \(\gamma\), and environmental temperature T, assuming initial Gaussian distribution both in x and \({\dot{x}}\) with \(\langle x_0 \rangle =\langle {\dot{x}}_0 \rangle =0\), and vanishing variance \(\sigma _{{\dot{x}}_0}^2=0\), the role of environmental noise can be discussed using the approximate formulae obtained from Eq. (1)
The main significant difference, noticeable from Eqs. (8) to (10), is the time scale at which the environmental temperature T becomes relevant. Notice how advantageously the \(SNR_{\ddot{x}}\) of Eq. (10) is time independent, compared to Eqs. (8), and (9). In Eq. (8) for position statistics, T plays a negligible role for short time scales (up to \(t=0.1\) ms), as the \(SNR_x \approx 0\) is independent of the chosen T, as visible from Fig.2b for the range of \(\Gamma\) from overdamped to zero-damping limit. For longer time scales (from \(t=0.3\) ms) the environmental temperature competes against the uncertainty-induced effect when \(T \ge 3 m \kappa ^2 t \sigma _{x_0}^4/(4 k_B \gamma )\) (\(T \approx 800\sigma _{x_0}^4\) K, for \(\Gamma =10^{-2}\) Hz), realising a growing \(SNR_x\) slowly converging to \(SNR_x=1/\sqrt{2}\) for the higher environmental temperature T. Given the high temperature requirement, such regime is not visible for the parameters of the experimental set-up we used12. In Eq. (9), the standard deviation of instantaneous velocity \(\sigma _{{\dot{x}}}(t)\) is not affected by ambient temperature \(T=300\) K at low pressure, as the required condition to reduce the \(SNR_{{\dot{x}}}(t)\) is \(T \ge m \kappa ^2 \sigma _{x_0}^4 t/k_B \gamma\) (\(T \approx 125\times 10^2 \sigma _{x_0}^4\) for \(\Gamma =10^{-2}\) Hz (black dots). Differently is the case at higher pressures, \(\Gamma =1\) Hz (Fig.2d, purple dots), where the condition softens to \(T \approx 140 \sigma _{x_0}^4\), reducing the \(SNR_{{\dot{x}}}(t)\) at small initial uncertainty \(\sigma _{x_0}^2\). The condition, for environmental temperature T, in the standard deviation of instantaneous acceleration in Eq. (10) \(\sigma _{\ddot{x}}\), is much harder to fulfill. As can be glimpsed from Fig.2f, for the low pressure limit (black dots) the environmental noise is negligible even at ambient temperature \(T=300\) K, leaving the \(SNR_{\ddot{x}}(t) \approx 1/\sqrt{2}\) unmodified. To be able to witness the effect of the environmental noise at such low pressures \(\Gamma =10^{-2}\) Hz, Eq. (10) provides a condition \(T \ge m \kappa ^2 \sigma _{x_0}^4/k_B \gamma\) (\(T \approx 150\times 10^2 \sigma _{x_0}^4\)K, for \(\Gamma =10^{-2}\) Hz) showing the high temperature requirement, index of high robustness against environmental noise. For higher pressures, \(\Gamma =1\) Hz (purple dots), the condition softens to \(T \approx 144\times 10^2 \sigma _{x_0}^4\) K, allowing, for small \(\sigma _{x_0}^2\) to witness a reduction of the \(SNR_{\ddot{x}}(t)\) (purple dots).
Role of initial particle velocity
Thus far we have considered the case of an initially steady particle with \(\langle x_0 \rangle =0\). Assuming we have infinitely precise control over the choice of initial speed, \(\sigma _{{\dot{x}}_0}^2=0\), one can observe the uncertainty-induced effect for moving particles, rendering the experimental test broad. Generalising Eq. (7) for non-zero \(\langle {\dot{x}}_0 \rangle\), and introducing \(\Delta x = x(t) - {\dot{x}}_0 t\), to exclude deterministic position change, one obtains
As visible from Fig.3a,b, Eq. (11) holds true for particles moving at different initial speed (blue, green and red dots), showing that even quickly moving particles at the considered short time scale \(t=0.1\) ms do not move on average.
For moving particles, the equation for instantaneous velocity reads \({\dot{x}}(t) = {\dot{x}}_0 - k x_0^2t\). From the latter, the velocity difference \(\Delta {\dot{x}} = {\dot{x}}(t) - {\dot{x}}_0\) is introduced, and its statistical evaluation comes as follows
As noticeable from Fig.3c,d, the mean instantaneous velocity of Eq. (12) holds true only for values of initial velocities \(\langle {\dot{x}}_0 \rangle = \pm 0.5\) (blue dots). However, for particles initially moving at higher speed (green and red dots), the approximation in Eq. (12) fails to describe the motion now modified by higher order nonlinear terms, as the particle obtains more negative mean instantaneous velocity for smaller \(\sigma _{x_0}^2\). This high order nonlinear effects can only be investigated by numerical stochastic simulations. The \(SNR_{{\dot{x}}}\) (middle panel, right column), although affected by the change in initial velocity (green and red dots), for larger \(\sigma _{x_0}^2\) converges to its constant value \(SNR_{{\dot{x}}}=1/\sqrt{2}\) of Eq. (12).
To visualise the effect of initial velocity \({\dot{x}}_0\) on instantaneous acceleration \(\ddot{x}\), one needs to explore the second order approximation to Eq. (4). We rewrite Eq. (4) to a set of dynamical equations for the position x and speed \({\dot{x}}\). Substituting a short-time solution \(x \approx x_0 +{\dot{x}}_0 t\) of the equation for the position x, to the right side of the equation for the speed \({\dot{x}}\) , we obtain a solution for the acceleration \(\ddot{x}(t) \approx -\kappa (x_0^2 +2 x_0 {\dot{x}}_0 t +{\dot{x}}_0^2 t^2)\). Introducing the quantity \(\Delta \ddot{x} = \ddot{x}(t) + \kappa {\dot{x}}_0^2t^2\), a pure effect of \(\sigma _{x_0}^2\) on acceleration can be described, for \(\langle x_0 \rangle =0\), non vanishing \(\langle {\dot{x}}_0 \rangle\), and \(\sigma _{{\dot{x}}_0}^2=0\) as follows
Evidently, in Fig.3e,f, for a particle with small non-zero initial speed \({\dot{x}}_0\), the acceleration does not deviate from the approximation introduced in Eq. (13), but when \({\dot{x}}_0\) increases, the mean acceleration gets closer to zero and \(SNR_{\Delta \ddot{x}}\) approaches \(1/\sqrt{2}\) much slower for larger \(\sigma _{x_0}^2\), as visible in Fig.3(e,f, green). For even larger initial speed (red dots), the particle obtains less negative average acceleration for smaller \(\sigma _{x_0}^2\), producing an initially decreasing \(SNR_{\Delta \ddot{x}}\). Decreasing the time scale tenfold \(t=0.01\) ms brings the red dots closer to the zero-damping approximation (black line), indicating that the shift is generated by higher order nonlinear terms beyond the approximate result introduced in Eq. (13). The larger \(\sigma _{x_0}^2\), the more the particle accelerates, resulting in an increase of the \(SNR_{\Delta \ddot{x}}\), slowly approaching \(1/\sqrt{2}\).
Fig.3 demonstrates that the uncertainty-induced shift of particle position (a,b), instantaneous velocity (c,d) and instantaneous acceleration (e,f) can be observed also for slowly and deterministically moving particles (black, and blue, and green dots). Moreover, for \(\langle {\dot{x}}_0 \rangle >0\) stochastic breaking induced by initial uncertainty can be witnessed where the particle breaks at average \(\langle {\dot{x}} \rangle =0\) for sufficiently large initial position uncertainty \(\sigma _{x_0}^2\). Similarly for \(\langle {\dot{x}}_0 \rangle <0\) stochastic speeding is observed, where the particle gains velocity for sufficiently large initial position uncertainty \(\sigma _{x_0}^2\). The latter can be observed even during the short time period, and it is noticeable by the sign flip of mean instantaneous velocity \(\langle \Delta {\dot{x}}_0 \rangle = - |{\dot{x}}_0|\) (Fig.3c,d, dashed blue line).
Sensitivity to velocity uncertainty
Complementary to the previous section, here we investigate how sensitive the uncertainty induced effect is to an increase of initial velocity uncertainty \(\sigma _{{\dot{x}}_0}^2\), for strictly zero initial velocity \(\langle {\dot{x}}_0 \rangle =0\), and \(\langle x_0 \rangle =0\). Assuming negligible \(\gamma\), as witnessed already in Fig.2 for the short time dynamics, Eq. (1) can be studied to describe the effect of initial statistics of velocity. Due to non-zero initial velocity uncertainty, Eqs. (5)–(7) modify to
At short time scale, the mean position \(\langle x(t) \rangle\) does not move, resulting in a vanishing \(SNR_x\) independent of the value of the initial velocity uncertainty, as visible in Fig.4a,b. For time larger than \(t=0.3\) ms, when the nonlinear terms in Eq. (14) are prominent and \(SNR_x\) approaches \(1/\sqrt{2}\), the initial velocity uncertainty can modify the statistics of position if \(\sigma _{{\dot{x}}_0}^2 \gg \kappa \sigma _{x_0}^2t^2/\sqrt{2}\) (\(\sigma _{{\dot{x}}}^2 \approx 10^{-2} \sigma _{x_0}^2\), at \(t=0.3\) ms, \(\Gamma =10^{-2}\) Hz). The statistics of instantaneous velocity, as described in Eq. (15) are more affected by increasing initial velocity uncertainty at short time scales. For values of \(\sigma _{{\dot{x}}_0}^2 \gg 2\kappa ^2 t^2\sigma _{x_0}^2 \approx 4\times 10^{-2}\sigma _{x_0}^2\) (at \(t=0.1\) ms, \(\Gamma =10^{-2}\) Hz), the statistics of \(SNR_{{\dot{x}}}\) slowly approaches the constant \(1/\sqrt{2}\) value, and rather approaches that of Eq. (15) as shown in Fig.4(d, purple dashed line). As can be seen directly from Eq. (16), instantaneous acceleration bears the ability to be driven both by initial, velocity uncertainty \(\sigma _{{\dot{x}}_0^2}\), dominating in the long time scale, and initial position uncertainty \(\sigma _{x_0^2}\), dominating in the short time scale. As can be seen in Fig.4e at timescales of \(t=0.1\) ms the term \(\sigma _{x_0^2}\) dominates over the dynamics (black and purple dots), retrieving the zero-damping approximation results (black dashed line). At larger values of \(\sigma _{{\dot{x}}_0^2}\) (orange dots) the enhancing effects of initial velocity uncertainty becomes visible as the mean instantaneous acceleration becomes more negative than the zero-damping approximation (black dashed line). Simultaneously the \(SNR_{\ddot{x}}\) (e) quickly converges to \(1/\sqrt{2}\) independent of the choice of initial velocity uncertainty.
Coherent motion of maximum of distribution
To complete the analysis, the dynamics of a levitated particle in cubic potential needs to be characterised also by means of the most-likely position, speed and acceleration. The maxima of the respective distribution are not only a directly measurable characteristic of unstable motion, but they also open a new local use of Maxwell’s deamon in stochastic thermodynamics27. Both mean and maximum of instantaneous quantities, stimulated by initial uncertainty, should ideally increase coherently (typical motion in the same direction) with a constant signal-to-noise ratio. Fig.5 shows the dynamics of maximum of position distribution(a,b, red dots), in both high friction regime (a), as well as in low friction regime (b). The latter shifts more pronouncedly, while maintaining its atypical feature observed in27,30 for over-damped dynamics. A new feature arises for the-most-likely speed, where both in high and low friction regime, the maximum of average and instantaneous velocity distribution shifts alongside the potential force as seen by the red arrow in Fig. 1 (c,d). A more quantitative dynamics of the latter is shown in Fig.5c showing that the deterministic limit (red line) is reached at damping of \(\Gamma =10^{-2}\) Hz. Contrarily to the mean instantaneous velocity, shown in Fig.4, the maximum of velocity distribution does not succumb to increasing initial velocity uncertainty. The curvature on the other hand is responsible for the reduction of the \(SNR_{{\dot{x}}_{max}}\), as it becomes larger with increasing initial velocity uncertainty \(\sigma _{{\dot{x}}_0}^2\), slowing down the convergence of the \(SNR_{{\dot{x}}_{max}}\) as shown in Fig.6d.
The shift of the most-likely acceleration is alongside the potential force, as shown in Fig.1(f, red arrow). It becomes evident only at low pressures, and disappears towards the high friction limit. The sharp shape of the acceleration distribution, displayed in the inset of Fig.5d shows a large shift of mean of instantaneous acceleration, but a small shift of its maximum, although larger compared to the shift of the maximum of velocity distribution. Despite the negligible role that the uncertainty of the initial velocity state displays in the evolution of the maximum of acceleration distribution, as shown in Fig.6e,f, it is of notice the convergence of the \(SNR_{\ddot{x}}\) to the \(1/\sqrt{2}\), denoted by the dashed black line in Fig.6f.
The minimal requirement to observe a shift of the maximum in the acceleration distribution, is a non-zero uncertainty in the initial velocity state, which mediates from the sharp tail on the right of the distribution, making its maximum hard to identify. Moreover we report that the most-likely acceleration, when the dynamics starts at different initial position \(\langle x_0 \rangle \ne 0\), shifts atypically for small values of initial position uncertainty. This is due by a pure deterministic drift in a regime dominated by inertia when the trajectory explore region away from the plateau. Moreover, their distribution shows no visible light tails, contrary to the position distribution in the over-damped regime27, where the fast and unstable dynamics of x drags all the trajectories quickly to the divergence.
Conclusion for experimental tests
We have demonstrated the uncertainty-induced instantaneous speed and acceleration of a levitated particle in the highly unstable cubic potential. Moreover, all the simulations have been performed using parameters of current underdamped experiments12, together with the parameters of cubic optical potential29,30 directly motivating our predictions to be experimentally tested to witness these new nonlinear mechanical phenomena. However, the analysis of the presented regime is also applicable to other underdamped experiments31,32,33. The first point worth experimentally verifying, shown in Figs. 1 and 2, is how the uncertainty-induced effect turns to instantaneous velocity and acceleration, reaching the zero-damping approximation described in Eqs. (5) to (7) at pressures of \(p=10^{-5}\) mbar, and room temperature. Then, the experiment can proceed to investigate how robust the previous result was when the particle, instead of being initially steady at the plateau, possessed nonzero initial velocity \(\langle {\dot{x}}_0 \rangle\) as showed in Fig. 3. The latter unveiled an interesting feature, observable in the cubic potential, consisting of stochastic breaking and speeding induced by initial position uncertainty \(\sigma _{x_0}^2\). Moreover, remarkably the uncertainty-induced effect can be observed even for slowly moving particles (see blue and green dots in Fig. 3). A parameter that needs to be kept under control is the initial velocity uncertainty, which although can drive the shift of instantaneous acceleration (Fig. 4 orange dots), is disruptive for the measurement of instantaneous velocity (purple and orange dots Fig. 4). Last, but not least, we showed that the maxima of the instantaneous speed, and acceleration distributions shift normally, alongside their respective mean in contrast to the position maximum which maintains its atypical shift as previously observed in the over-damped regime27,30 (Fig. 5). The sensitivity of maxima towards increasing initial velocity uncertainty, as shown in Fig. 6, displays a worsening of the accuracy which in turns demands increasing ensemble size. We report that imperfections to the cubic potential, i.e., \(V(x) = k_2 x^2 + k_3 x^3\), do not mask the uncertainty-induced effect for small initial uncertainty, provided that \(k_2\) is small enough to not dominate the dynamics at transient times around the origin. For single well Gaussian potential in experiment12 however, the uncertainty-induced effect is not visible, contrarily to a tilted double well potential (as in34) where the uncertainty-induced effect with increasing \(\mathrm {SNR}\) can be observed. It enlarges the possibility of upcoming experimental tests with diverse nonlinear potential landscapes.
All these experimental tests will verify new underdamped transient effects of a particle living at the edge of instability, paving the way to explore highly nonlinear stochastic phenomena. Future targets comprise of quantum mechanical analysis of deeply underdamped and highly cooled particles in the unstable cubic potential, initially close to the mechanical ground state.
Methods
Numerical simulation with experimental numbers
To numerically simulate the Langevin dynamics described in Eq. (1) using real experimental values, one has to re-scale the equation of motion. Usually, for linear dynamics, the equation is re-scaled using the mechanical Q-factor. With nonlinear systems this is not valid anymore, and a different route must be followed. In the case of Eq. (1), it is useful to re-scale position and time as follows
with q being the dimensionless position, l the position re-scaler, \({\bar{t}}\) the dimensionless time, and \(\tau\) the time re-scaler. It naturally follows from Eq. (17) that \({\dot{q}}=\tau {\dot{x}}/l\), and \(\ddot{q}=\tau ^2 \ddot{x}/l\). In order to determine the values of the re-scaler, one can use, for the position \({\bar{l}}=5\times 10^{-6}\) which is the length of the potential used in experiment30, and then focus attention on the positive part of the potential, of length \({\bar{l}}/2\). Subsequently choose a point, P belonging to it, with coordinate (xp, yp). With this point one can build a straight line passing through the origin and the chosen point, and notice that it forms a triangle containing the piece of potential up to point P chosen. The angle between the origin and the hypotenuse is then given by the stiffness k of the potential. Subsequently, the position re-scaler can be calculated as \(l=2\sqrt{A/k}\), where A denotes the area of the triangle previously built, and the factor 2 comes from the fact that we extend the calculation to the whole domain of the cubic potential. The re-scaler l calculated, now has a clear dependence on the stiffness of the potential \(K\approx k_BT \mu m^{-3}\), and subsequently on the chosen temperature T, and it varies between \(10^{-3}\mu m< l < 10^{-2}\mu m\). The time re-scaler, \(\tau\) is calculated by numerically computing the first passage time for the selected parameters.
Following the re-scaling procedure explained before, the Langevin equation can be transformed into
where \({\bar{k}}=\kappa /l^3\), and the mass m has been absorbed by \(\kappa =K/m\), \(\gamma =\Gamma /m\), \(D=k_BT\gamma /m\), and \({\bar{\xi }}(t) = \sqrt{\tau ^{-1}} \xi (t)\). The term \({\bar{k}}=\kappa /l^3\) comes from the re-normalisation of the potential stiffness, done to render the dimensions of the new stiffness, \({\bar{k}}=[1/(m s^2)]\), such that the potential term, \({\bar{k}}\tau ^2 l q^2\) becomes a-dimensional in the re-scaling.
Uncertainty-induced effects for non vanishing initial position
Throughout the paper we have always assumed to have a particle initially positioned at the inflection point \(\langle x_0 \rangle =0\). It becomes natural to ask how different \(\langle x_0 \rangle\) affect the uncertainty-induced effect described. As evidenced in Fig. 7, for small nonzero \(\langle x_0 \rangle =1\) (blue dots), Eqs. (14)–(16) still describe the dynamics for position (a,b), velocity (c,d), and acceleration (e,f), where their SNR (b,d,f) show no deviation from \(1/\sqrt{2}\). A different case is the large non zero \(\langle x_0 \rangle\) (green dots) for which Eqs. (14)–(16) no longer holds. In this case, the particle already feels strong nonlinear terms, which require more terms in the time expansion from (4). While the respective SNR undergo an initial decrease (for velocity and acceleration), they all converge to \(1/\sqrt{2}\) for increasing initial position uncertainty \(\sigma _{x_0}^2\). To preserve the short time dynamics at such nonlinear positions, a decrease of the time scale seems necessary (a tenth of \(t=0.1\)ms is sufficient for the parameters used in Fig. 7 to produce the green dots).
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Acknowledgements
We acknowledge the project 19-17765S of the Czech Science Foundation and and MEYS CR together with European Union’s Horizon 2020 (2014–2020) research and innovation framework programme under Grant Agreement No. 731473 (project 8C18003 TheBlinQC). Project TheBlinQC has received funding from the QuantERA ERA-NET Cofund in Quantum Technologies implemented within the European Union’s Horizon 2020 Programme. We acknowledge Pavel Zemánek for fruitful discussions.
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L.O. and R.F. developed theory. L.O. performed numerical simulations. R.F. supervised the project. All authors analysed data and prepared the manuscript.
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Ornigotti, L., Filip, R. Uncertainty-induced instantaneous speed and acceleration of a levitated particle. Sci Rep 11, 18185 (2021). https://doi.org/10.1038/s41598-021-97663-z
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DOI: https://doi.org/10.1038/s41598-021-97663-z
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