Abstract
Steady improvements in ambient air quality in the USA over the past several decades, in part a result of public policy1,2, have led to public health benefits1,2,3,4. However, recent trends in ambient concentrations of particulate matter with diameters less than 2.5 μm (PM2.5), a pollutant regulated under the Clean Air Act1, have stagnated or begun to reverse throughout much of the USA5. Here we use a combination of ground- and satellite-based air pollution data from 2000 to 2022 to quantify the contribution of wildfire smoke to these PM2.5 trends. We find that since at least 2016, wildfire smoke has influenced trends in average annual PM2.5 concentrations in nearly three-quarters of states in the contiguous USA, eroding about 25% of previous multi-decadal progress in reducing PM2.5 concentrations on average in those states, equivalent to 4 years of air quality progress, and more than 50% in many western states. Smoke influence on trends in the number of days with extreme PM2.5 concentrations is detectable by 2011, but the influence can be detected primarily in western and mid-western states. Wildfire-driven increases in ambient PM2.5 concentrations are unregulated under current air pollution law6 and, in the absence of further interventions, we show that the contribution of wildfire to regional and national air quality trends is likely to grow as the climate continues to warm.
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Data availability
Data to reproduce all results in the paper are available at https://github.com/echolab-stanford/wildfire-influence.
Code availability
Code to reproduce all results in the paper are available at https://github.com/echolab-stanford/wildfire-influence.
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Acknowledgements
We thank members of Stanford ECHOLab and seminar participants at University of California Berkeley, Columbia, Duke, Montana State, Minnesota and University of California Santa Barbara for helpful comments. Some of the computing for this project was performed on the Sherlock cluster, and we thank Stanford University and the Stanford Research Computing Center for providing computational resources and support that contributed to these research results. M.L.C. was supported by an Environmental Fellowship at the Harvard University Center for the Environment. M.Q. was supported by a fellowship at Stanford’s Center for Innovation in Global Health. M.B. thanks the Keck Foundation for research support.
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M.B. and M.L.C. conceived the project. M.B., M.L.C., B.d.l.C., M.Q. and J.L. analysed data. All authors interpreted results and wrote the paper.
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Extended data figures and tables
Extended Data Fig. 1 Pollution stations and method used to construct non-smoke PM2.5 estimates.
a. Example of total and non-smoke partitioning for a single station in CA in 2020. On days without a smoke plume overhead (no grey points), all PM2.5 is assumed to be from non-smoke sources. On days with a plume overhead (grey points), PM2.5 anomalies from the non-smoke month- and station-specific 3-year median are attributed to smoke, and total PM2.5 minus anomalies are attributed to non-smoke (blue). b. Annual average total and non-smoke PM2.5 for the same station are produced by aggregating daily total observed PM2.5 (black) and the daily estimates of non-smoke PM2.5 (blue). c. Locations of PM2.5 stations throughout the contiguous US. Stations are coloured by the number of years with at least 50 observations.
Extended Data Fig. 2 Distribution in estimated breakpoints for different sample restrictions and/or statistical specifications.
a. Annual average PM2.5. b. Extreme (> 35 µg/m3) daily PM2.5. Histograms show distribution of estimated breakpoints for different sample restrictions, pooling data from all CONUS monitors. Panels labeled with number of observations and years are various sample restriction choices, while those labeled “Drop” retain our primary inclusion criteria – more than 50 observations per year for at least 15 years – but remove one of the last three years of the sample to understand their influence on estimates. Discontinuous models allow for separate intercepts on either side of the break year. Strong bunching in the discontinuous models for average PM2.5 occur because only integer years are permitted as candidate breakpoints. “Positive smoke PM2.5 anomalies” tests the sensitivity of results to bottom-coding daily smoke PM2.5 estimates to zero, i.e., not allowing negative smoke PM2.5 anomalies.
Extended Data Fig. 3 Influence of wildfire smoke on daily PM2.5 extremes is mainly concentrated in states in the West, Northwest, and Great Plains.
Black lines in each plot show percent of days in each state-year where PM2.5 values exceed 35 µg/m3, calculated using the sample of stations with over 50 observations in at least 15 years, as in Fig. 3. Blue lines show estimated percent of days that exceed 35 µg/m3 after smoke PM2.5 has been removed. Vertical dotted line indicates median CONUS-wide estimated breakpoint (2012).
Extended Data Fig. 4 Sensitivity of estimated differences in slope coefficients used to classify states.
Left column shows differences in early (β1) and recent period (β2) estimates of changes in total PM2.5, and the confidence interval on estimated differences, that are used to classify states into stagnating/reversing categories. Middle column shows differences in recent period total PM2.5 (β2) and non-smoke PM2.5 (\({\beta }_{2}^{{\prime} }\)) slopes that are used to classify states as smoke-influenced. Right column shows same, but for recent period changes in extreme days. Colors match sample as denoted in the legend at right.
Extended Data Fig. 5 Sensitivity of total PM2.5-trend classification to different sample restrictions and/or statistical specifications.
a. State-specific total PM2.5-trend classification under alternate estimates. b. Counts of states in each classification. Model specifications and samples match those in Extended Data Fig. 2.
Extended Data Fig. 6 Sensitivity of smoke-influence classification to different sample restrictions and/or statistical specifications.
a. State-specific smoke-influence classification under alternate estimates. b. Counts of states in each classification. Model specifications and samples match those in Extended Data Fig. 2. c. Regional trends in total and non-smoke PM2.5, and regional smoke-influence classifications with region-specific breakpoint estimates (vertical dashed lines).
Extended Data Fig. 7 Sensitivity of smoke-influence classification on portion of extreme days (> 35 µg/m3) to different sample restrictions.
a. State-specific smoke-influence classification under alternate estimates. b. Counts of states in each classification. Model specifications and samples match those in Extended Data Fig. 2.
Extended Data Fig. 8 Distribution of proportion of extreme days due to wildfire smoke by state.
a. Density plots show, for each year, the distribution across CONUS states of the proportion of days above 35 µg/m3 due to smoke, i.e., days that would have had concentrations < 35 µg/m3 were smoke not present. Tick marks show values for individual states. b. Cumulative distributions of the number of states where the proportion of extreme PM2.5 days due to wildfire smoke in a time period met or exceeded a given percentage threshold. For instance, the intersection of a vertical line drawn at 50% and each of the depicted lines in the plot would provide estimates of the number of states in each period where at least 50% of extreme days were due to wildfire smoke.
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Burke, M., Childs, M.L., de la Cuesta, B. et al. The contribution of wildfire to PM2.5 trends in the USA. Nature 622, 761–766 (2023). https://doi.org/10.1038/s41586-023-06522-6
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DOI: https://doi.org/10.1038/s41586-023-06522-6
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