Abstract
Initiated as a cable-replacement solution, short-range wireless power transfer has rapidly become ubiquitous in the development of modern high-data throughput networking in centimeter to meter accessibility range. Wireless technology is now penetrating a higher level of system integration for chip-to-chip and on-chip radiofrequency interconnects. However, standard CMOS integrated millimeter-wave antennas have typical size commensurable with the operating wavelength, and are thus an unrealistic solution for downsizing transmitters and receivers to the micrometer and nanometer scale. Herein, we demonstrate a light-in and electrical signal-out, on-chip wireless near-infrared link between a 220 nm optical antenna and a sub-nanometer rectifying antenna converting the transmitted optical energy into direct electrical current. The co-integration of subwavelength optical functional devices with electronic transduction offers a disruptive solution to interface photons and electrons at the nanoscale for on-chip wireless optical interconnects.
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Introduction
Conventional radiowave and microwave antennas operate a bilateral energy conversion between electrical signals and electromagnetic radiation. Integration of these antennas to modern consumer electronics is thus widely adopted for long-range and short-range data transfer. Vivid examples are communication between mobile devices and remote biosensors for healthcare providers1,2. Similar sub-wavelength interfacing of optics and electronics is envisioned as an archetype to reduce the size of communication devices while maintaining their necessary speed and bandwidth3,4. This is a daunting task as state-of-the-art electronics is unable to respond to the fast alternating fields associated with optical frequencies and the size of photonic components remains orders of magnitude larger than their electronic counterparts. Nanoscale antennas operating in the optical domain are technologically available, but have been mainly limited to interfacing near-field and far-field radiation by tailoring the momentum of light5.
In 2010, A. Alù and N. Engheta theoretically proposed an optical wireless channel between two nanoscale antennas6. The idea was partially demonstrated by beaming either an optical signal towards a distant luminescent receiver7 or by the mediation of surface plasmons8. Despite an optimization with highly directive antennas9,10, the link operates on the basis of a light-in and light-out configuration without transduction of the transferred optical energy to an electronic signal. Recent progress shows that tunneling nonlinearity in the conduction of an atomic scale tunnel junction can rectify the plasmonic response at optical frequencies to direct current (d.c.)11,12,13,14,15. Immediately, these rectifying antennas, or rectennas, appear to be essential ultrafast devices for merging optics and electronics at the nanoscale.
Here, we exploit these functionalities on a single platform to realize an optical wireless power transmission between laser-illuminated nanoscale dipolar antennas and a distant rectenna. We demonstrate a proof-of-principle wireless link where gold nano-antennas act as transmitters by directing an out-of-plane laser signal towards an optical rectenna where the transmitted radiation is rectified as d.c. current. We show that the rectified current is governed by the polarization of laser illuminating the distant transmitter antenna. The amount of transmitted power through the wireless link is correctly described by the Friis transmission equation and follows an inverse square relation with the distance between the transmitting antenna and the rectenna. The findings experimentally confirm that an optical signal can be transmitted and transduced between two nanoscale units without relying on a physical optical waveguide.
Results
Device principle
Figure 1a illustrates the optical line-of-sight channel presented here. The transmitter is a laser-illuminated gold nanodisc acting as an optical dipole antenna. The radiation scattered by the antenna is remotely detected and converted to a d.c. current by a distant electrically biased rectenna. A transmission optical image of the units is shown in Fig. 1b. The Au electrodes powering the rectenna feed-gap and a series of optical antennas (black dashed box) are readily seen with a dark contrast. The tunneling feed-gap of the rectenna is formed by electromigration of initially touching electrodes16. Figure 1c is a false colored scanning electron microscopy (SEM) image of the white dotted box in Fig. 1b showing the in-plane tunneling junction together with an adjacent optical antenna. The electrical characterization confirms that tunneling is driving electron transport (see Methods section). The optical antennas have a fixed diameter of 220 ± 10 nm to simultaneously induce a dipolar response and maximize the scattering efficiency (see Supplementary Figure 8). The devices are immersed in a refractive index (RI) matching oil to operate the link in a homogenous environment.
Optical rectification
Let us assume an optical rectenna formed by a tunnel junction where the conduction mechanism remains the same over a pulsation range 2ωac. A d.c. current I(Vdc) is tunneling through the feed-gap when a bias of V = Vdc is applied between the two metal leads. If a small a.c. bias Vac of frequency ωac is superposed to Vdc, the total current through the junction can be expressed by a Taylor’s expansion17,
The time-independent term in Eq. 1 indicates the presence of an additional rectified current I″, which is proportional to the nonlinearity of the conductance ∂2I/ ∂V2 and \(V_{{\mathrm{ac}}}^2\): I″ = 1/4\(V_{{\mathrm{ac}}}^2\) (∂2I/ ∂V2).
To describe optical rectification, a quantum mechanical treatment is generally used18. When the rectenna is illuminated with light of energy, the response builds up an a.c. voltage Vopt of pulsation ω across the junction. This optical potential triggers a photon-assisted tunneling of electrons to produce a d.c. photocurrent in addition to the I(Vdc). If eVopt≪ ℏω, the rectified d.c. photocurrent is given by19,20
For gold and for an excitation energy ħω < 2 eV, the tunneling transmission remains smooth within the range EF ± ħω, where EF is the Fermi energy11. Therefore, Eq. 2 reduces to its classical form Iphot = 1/4\(V_{{\mathrm{opt}}}^2\)(∂2I/ ∂V2) with Vopt playing the role of Vac and Iphot of I″11,21.
We use a low frequency a.c. voltage and lock-in detection to record the conductance G = ∂I/∂V, the current proportional to the nonlinearity ∂2I/∂V2 and the laser-induced current Iphot11,12,17. The description of the complete measurement system is included in the Methods section (see Supplementary Fig. 1 for the schematic of the experimental set-up). The plot of conductance of the junction G (Vdc) in Fig. 1d features a zero bias conductance of about 10 µS (≈0.13 G0 where G0 = 77.5 μS is the quantum of conductance). Using Simmons’ model of tunneling transport22,23, we qualitatively estimate the feed-gap width to be <0.5 nm (Supplementary Fig. 2, Supplementary Fig. 3 and Supplementary Note 1). In Fig. 1e, we plot the bias dependence of I” (line) and Iphot (points) for three laser intensities when the illumination is directly focused on the rectenna feed-gap. For each excitation intensity, Vac is adjusted to obtain Iphot = I”. Under this condition, the optical voltage generated across the feed-gap equals the low frequency voltage applied between the electrodes11. From the shared voltage dependence of Iphot and I”, we conclude that the photocurrent generated at the rectenna results from optical rectification. Additional experiments to rule out any thermal contributions are presented in Supplementary Note 2 and Supplementary Fig. 4.
Optical wireless link
In the following section, we assess the operation of a wireless link when a remote optical antenna is broadcasting a signal towards this transducing rectenna. The laser is no longer directly incident on the rectenna, but is focused alternatively on the series of optical antennas displayed in Fig. 1b. Figure 2a shows a pixel-by-pixel reconstructed photocurrent map generated by the rectenna. The laser excitation is polarized along y-axis (0°) and the sample is scanned through the focal area (step size 70 nm). Vdc across the rectenna is fixed at 50 mV and the laser intensity at 353 kW cm−2. The important conclusion drawn from the current map is the presence of a rectenna response whenever the laser excites a remote optical antenna. The response is observed even for separation distances exceeding several micrometers. When the polarization is turned by 90° (x-axis), the photocurrent generated at the rectenna vanishes nearly completely (Fig. 2b). To confirm the transduction of the signal radiated by the optical antennas, we station the laser on the optical antenna located 4 µm away from the rectenna (2nd antenna from the right in Fig. 1b) and simultaneously monitor Iphot and I″ as a function of Vdc while rotating the polarization. The intensity of the laser is 540 kW cm−2 for this experiment and we verified that for all the polarizations angles, Iphot follows I″ proving thus the Iphot signal is optically rectified (Supplementary Fig. 6 and Supplementary Note 3). The value of Vac for conditioning Iphot = I″ is recorded as a measure of the optically induced a.c. voltage Vopt at the feed-gap. The evolution of Iphot and Vopt as a function of the incident laser polarization is plotted in Fig. 2c for a bias Vdc = 50 mV. It is clear that the rectification process is suppressed as the polarization is rotated by 90°. This polarization dependence of the current produced by the rectenna removes any concern about a heat-mediated transduction mechanism since the temperature of the illuminated disc antenna is driven by the absorption coefficient and not by the polarization of the incident laser beam. As an additional control experiment we map dI/dV at the frequency of the optical chopper (Supplementary Fig. 5). No measurable contrast can be related to the photocurrent map presented in Fig. 2a (more discussion in Supplementary Note 2) indicating that the gap size is not deformed by the heat produced at the distant antenna24. We reproduce the wireless link and the transduction of the optical signal with a second tested device (Supplementary Fig. 7) and assess the main parameter affecting the device-to-device variability in Supplementary Table 1 and Supplementary Note 4.
Numerical modeling
Numerical simulations based on a three-dimensional finite element method (3D-FEM) bring an understanding of the polarization dependence of the rectified signal. The rectenna is modeled by two truncated Au triangles separated by a distance of 10 nm except at the middle where a small protrusion on the bottom electrode reduces the gap size to 0.5 nm. A 220 nm diameter Au disc antenna is placed 4 μm away from the feed-gap. The entire geometry is placed inside a homogeneous medium of RI = 1.52. When excited by a linear polarization at 785 nm, the disc behaves as a dipolar resonant antenna radiating its characteristic two-lobe pattern perpendicularly to the incident electric field. Figure 3a, d are schematic representations picturing the dipolar radiation for two orthogonal in-plane polarizations. Figure 3b is the calculated electric field distribution plotted in logarithmic scale when the antenna is illuminated (the white circle indicates the excitation area) with a polarization along the y-axis (vertical). Clearly, the optical antenna redirects the far-field radiation towards the rectenna feed-gap. The interaction of this receiving radiation with the tunneling gap results in a high electric field at the junction25, enhanced by a factor of approximately 5.6 compared to the excitation field, which is illustrated in the zoomed-in electric field map in Fig. 3c. When the dipolar radiation is polarized perpendicularly to the receiver (Fig. 3d), the field enhancement at the junction is reduced to 0.44 (Fig. 3e, f), explaining the vanishing photo-response of Fig. 2d. More details about the modeling procedure are included in the Methods section.
Controlling the efficiency of the wireless link
When a transmitter and a receiver constituting a wireless link are separated by a distance d, the received power is given by the Friis equation26,
Pfed is the power fed to the transmitter, λex is the operational wavelength, ηr and ηt are the radiation efficiencies, Dr and Dt are the directivities, Γr and Γt are the reflection coefficients, ar and at represent the polarizabilities of the receiving and the transmitting antennas, respectively.
We first analyze the distance dependence of the optical wireless link. The evolution of the amplitude of the rectified current Iphot is plotted in Fig. 4a as a function of the distance d separating the antenna from receiving rectenna. Iphot (black data points) is fitted with a generic power law function αdb + c where α represents the coupling strength between the transmitter and the receiver and c is the dark photocurrent of the device (≈0.32 nA). The best fit gives an exponent b = −1.8, which is close to the expected inverse square law dependence (Eq. 3). The slight mismatch may be due to the inevitable deviations in the antenna geometry, and misalignment. We also record the evolution of Vopt as a function of d, which is shown as the magenta plot in Fig. 4a. This is done by focusing the laser individually on each antenna and varying Vac to equalize Iphot and I″ for a sweep of Vdc across −0.1 V to 0.1 V (see Fig. 5a). The evolution of Vopt with the distance d is also fitted with a power law with a similar expression. Here c again indicates the noise level, which is here c = 6.5 mV. The best fit gives b = −0.85 (magenta solid plot), which is close to −1. This is expected, as Iphot is proportional \(V_{{\mathrm{opt}}}^2\) (Eq. 2).
We corroborate our experimental distance dependence of the rectified current and optically induced voltage drop at the junction (Fig. 4a) with 3D-FEM based calculation of the electric field created at the rectenna’s feed-gap for varying distance d between the rectenna and the transmitting unit. The normalized electric field produced at a gap size of 0.5 nm and a 220 nm transmitter antenna is presented in Fig. 4b (black data points). The power law fit to the distance dependence (black line) converges to an exponent close to −1, which agrees with the experimental dependence of Vopt.
As indicated in Eq. 3, the amount of power transferred not only depends on the distance, but also on parameters that are influenced by the geometry of the antenna5,27. We thus numerically explore the influence of the gap size g, and the effect of an off-resonant antenna. Figure 4b indicates that sub-nm separation favors a large electric field at the feed-gap. However, our calculations do not take into account quantum-size effects28, which may limit the amplitude of the electrical field. Broadcasting the optical signal with a non-resonant antenna of diameter D = 110 nm also leads to a reduced electrical field at the transducing feed-gap (Supplementary Fig. 8 and Supplementary Note 5). We verify the minimal influence of the presence of other antennas in the transmission path in Supplementary Fig. 9 and Supplementary Note 5.
Transduction yield
We estimate the overall transduction yield κ of the link discussed here. κ is a measure of what fraction of the incident laser power is converted to electrical power through rectification and is given by the following equation:
where G is the conductance of the tunnel junction.
We estimate κ = −91 and −101 dBm for the radiation transmitted by the antennas situated 2 and 10 μm away respectively for Vdc = 50 mV applied across the junction.
The transduction yield improves with increasing the applied d.c. bias to the junction. This is observed in the experimentally recorded Iphot vs Vdc plots for three distant antennas presented in Fig. 5a. An increase of κ is indeed expected as the nonlinearity of the conductance of the rectenna increases as we raise Vdc (see the evolution of G in Fig. 1d). For the 2 µm distant antenna, setting Vdc to 100 mV improves the transduction yield to −87 dBm. Note that here κ denotes the overall efficiency of the link including antenna radiation, signal propagation, and transduction. In radio-frequency wireless communication, the received signal strength indicator (RSSI) evaluates the quality of the transmitted signal measured at the reception node before transduction. A transmission channel with a RSSI comprised between −70 and −100 dBm is considered as fair for basic connectivity.
Finally, we plot in Fig. 5b the dependence of measured rectified photocurrent on the excitation laser intensity for each remote transmitting antenna for Vdc = 50 mV. Regardless of the distance, the photocurrent scales linearly with the signal intensity fed to the optical antennas in agreement with Eq. 3. The slopes of the linear fits give the coupling strengths between each transmitter and the rectenna, which is measure of the change in the transduced currents per kW cm−2 increment in the illumination intensity. The values are reported in Table 1. In Supplementary Table 2, we compare the photocurrent produced by a direct illumination of the rectenna with the photocurrent generated via the mediation of distant optical antennas for an illumination intensity 353 kW cm−2 and Vdc = 50 mV.
Discussion
In conclusion, we demonstrate an on-chip nanoscale optical wireless link between a laser-illuminated optical antenna and a transducing rectenna. In our experiments, simple gold nanodiscs act as a polarization-sensitive transmitting antenna directing the laser radiation towards the rectifying gap antenna. The amount of power transferred maintains an inverse square relation with the distance between the transmitting antenna and the rectenna. In addition to this, the geometrical properties of the participating units contribute to the yield of power transfer. Further improvement in the efficiency of transmission can be achieved by integration of highly directional optical antennas and resonant feeds.
An integrated wireless transmission enables a new communication strategy between nanoscale devices. This can be deployed when physical links (e.g., integrated photonic waveguides) cannot be implemented or when the transmitted signal should be out-coupled via the mediation of optical antennas and metasurfaces29,30. The wireless link can immediately be applied to develop ultrafast electro-optical connectors. Transmission rates in excess of 1012 bits per second are achievable as the plasmonic response of the gap is defined by the polarizability response of the metal and not by carrier lifetime as in semiconductors31. Recent progress shows that an electrically driven tunneling junction can act as ultrafast broadband self-emitting device32,33,34. Therefore, integration of a wireless link between an electron-fed optical antenna with a transducing rectenna may enable ultrafast information transfer. Such devices will represent a paradigm for on-chip interfacing of electrons and photons at the nanoscale.
Methods
Sample preparation
The samples are prepared on a glass coverslip by a double step lithography involving electron beam lithography (EBL) and photolithography. The antennas (disc of diameter 220 ± 10 nm), a nanoscale constriction of length 400 nm and width 100 nm bridging two large triangular Au structures as well as alignment marks are fabricated during a first step by EBL. For this, we spin coat and bake a 400 nm thick double-layer of poly(methyl-methacrylate) (PMMA) constituted of two different molecular weights (50 and 200 kDa). We then sputter a sacrificial gold conductive layer (5–10 nm) on the resist layers to avoid charging during electron beam exposure. Once the PMMA is exposed and developed, a 2 nm thick Ti adhesion layer followed by a 45 nm thick Au are subsequently deposited through thermal evaporation. The excess metal is then lifted off to obtain the final nanostructures. Then the macroscopic gold electrodes contacting the triangular pads are realized via standard optical lithography. During this step, the alignment marks are used to position the sample coordinates with respect to the coordinate system of the photolithography mask. Once the nanostructrures and electrical connections are fabricated, we produce the nanoscale gap-antenna by controlling the electromigration of the constriction. The electromigration is stopped once the zero-bias d.c. conductance reaches a value lower than the quantum conductance (G0 = 77 µS). The presence of a tunnelling gap is confirmed by measuring the nonlinear I–V characteristics of the device (see Supplementary Fig. 2).
Electrical and optical measurements
The schematic of the experimental setup we use for the optical and electrical characterizations presented in the paper is illustrated in the Supplementary Fig. 1. With the help of an inverted optical microscope (Nikon, Eclipse), we focus the 785 nm wavelength laser on the sample through an oil immersion objective lens of numerical aperture (NA) 1.49. During the whole experiment, nanostructures are immersed in RI matching oil of RI = 1.52. For electrical measurements, the sample is biased with an applied d.c. bias Vdc added with a small modulation a.c. voltage Vaccosω1t at Vac = 20 mV where f1 = ω1/2π = 12.37 kHz is the modulation frequency. A first lock-in amplifier (Zurich Instrument, HF2LI) referenced at f1 and 2f1 is used to simultaneously record the first harmonic (∂I/∂V) and second harmonic (1/4 \(V_{{\mathrm{ac}}}^2\) ∂2I/∂V2), of the current tunneling through the gap. The first harmonic is proportional to the conductance and second harmonic signifies nonlinearity in the junction’s conductance. To extract the laser-induced current Iphot the laser beam is chopped by a chopper (Thorlabs) at frequency fchop = 831 Hz and the tunnelling current is demodulated at fchop using a second lock-in amplifier (Zurich Instrument, HF2LI). Therefore with this arrangement, I(Vdc), ∂I/∂V, ∂2 I/∂V2 and Iphot can be measured simultaneously as a function of Vdc. For mapping, the sample is scanned through the laser spot by the moving the sample with a linearized piezoelectric stage (PI, P-545) and the data are recorded by a scanning data acquisition system (RHK, R9).
Numerical modeling
We have performed the 3 dimensional-finite element method (3D-FEM) modeling of the system using a commercial FEM solver COMSOL Multiphysics. We use the RF module of the solver to perform all the simulations. For simplicity, the rectenna is modeled as a gap junction between two 40 nm thick Au triangles. The gap width is 10 nm except at the center where a small protrusion on the bottom electrode reduces the gap size to 0.5 nm. The optical antennas are modeled by 220 nm diameter 40 nm thick Au cylinders. The electrical permittivity of Au is taken from the experimental values provided by Johnson and Christy35. The entire geometry is placed inside a homogeneous medium of RI = 1.52. The excitation is a 785 nm focused Gaussian beam incident on the antenna. The focal spot of the excitation beam is 600 nm diameter. This corresponds to an intensity full-width at half-maximum comparable to the point-spread function of the objective (i.e., 320 nm). We then calculate the electric field distribution in the computation window encompassing the transmitting antennas and the rectenna. We use perfectly-matched layer at the boundary to mitigate spurious reflections.
Data availability
Data are available from the corresponding author upon reasonable request.
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Acknowledgements
This work has been supported by the European Research Council under the European Community’s Seventh Framework Program FP7/ 2007–2013 Grant Agreement No. 306772. Device fabrication was performed in the technological platform ARCEN Carnot with the support of the Région de Bourgogne. We thank I. Smetanin, O. Demichel for discussions, J. Dellinger for its initial implication in the setup, S. Pernot, and B. Sinardet for developing part of the electronic unit and L. Novotny for an initial reading of the manuscript.
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A.D. conducted the experiment, analyzed the data, and performed the simulations. M.M.M. developed the experimental and fitting procedures, N.C. and M.B. constructed the measurement apparatus to control the electromigration process, G.C.D.F. supervised the simulations. A.B. conceived the experiment and supervised the research. A. D. and A. B. wrote the manuscript, with revisions by all.
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Dasgupta, A., Mennemanteuil, MM., Buret, M. et al. Optical wireless link between a nanoscale antenna and a transducing rectenna. Nat Commun 9, 1992 (2018). https://doi.org/10.1038/s41467-018-04382-7
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DOI: https://doi.org/10.1038/s41467-018-04382-7
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