Skip to main content

Thank you for visiting nature.com. You are using a browser version with limited support for CSS. To obtain the best experience, we recommend you use a more up to date browser (or turn off compatibility mode in Internet Explorer). In the meantime, to ensure continued support, we are displaying the site without styles and JavaScript.

  • Letter
  • Published:

Current switching of resistive states in magnetoresistive manganites

Abstract

Magnetoresistive devices (based on, for example, magnetic multilayers1) exhibit large changes in electrical resistance in response to a magnetic field, which has led to dramatic improvements in the data density and reading speed of magnetic recording systems. Manganese oxides having a perovskite structure (the so-called manganites) can exhibit a magnetoresistive response that is many orders of magnitude larger than that found for other materials, and there is therefore hope that these compounds might similarly be exploited for recording applications2,3,4,5,6,7,8,9,10,11. Here we show that the switching of resistive states in the manganites can be achieved not only by a magnetic field, but also by an electric field. For manganites of the form Pr1−xCaxMnO3, we find that an electrical current (and by implication a static electric field) triggers the collapse of the low-temperature, electrically insulating charge-ordered state to a metallic ferromagnetic state. We suggest that such a phenomenon could be exploited to pattern conducting ferromagnetic domains within an insulating antiferromagnetic matrix, and so provide a route for fabricating micrometre- or nanometre-scale electromagnets.

This is a preview of subscription content, access via your institution

Access options

Buy this article

Prices may be subject to local taxes which are calculated during checkout

Figure 1: Temperature dependence of resistance of a Pr1−xCaxMnO3 (x = 0.3) crystal measured at various applied voltages.
Figure 2: Change of resistance of Pr1−xCaxMnO3 (x = 0.3) at 20 K as a function of applied voltage, measured using the circuit shown in Fig. 1 inset.
Figure 3: Current–voltage (IV) characteristics at 20 K in magnetic fields of 0 T (a), 2 T (b) and 3 T (c).
Figure 4: Top panel, threshold voltage at 20 K, Vthreshold, from a high-resistivity (HR) to a low-resistivity (L.R) state, plotted as a function of magnetic field (see Fig. 3).

Similar content being viewed by others

References

  1. Baibich, M. N. et al. Giant magnetoresistance of (001)Fe/(001)Cr magnetic superlattices. Phys. Rev. Lett. 61, 2472–2475 (1988).

    Article  ADS  CAS  Google Scholar 

  2. Kusters, R. M., Singleton, D. A., Mcgreevy, R. & Hayes, W. Magnetoresistance measurements on the magnetic semiconductor Nd0.5Pb0.5MnO3. Physica B 155, 362–365 (1989).

    Article  ADS  CAS  Google Scholar 

  3. von Helmont, R., Wecker, J., Holzapfel, B., Schultz, M. & Samwer, K. Giant negative magnetoresistance in perovskite La2/3Ba1/3MnOxferrmomagnetic films. Phys. Rev. Lett. 71, 2331–2333 (1993).

    Article  ADS  Google Scholar 

  4. Jin, S. et al. Thousandfold change in resistivity in magnetoresistive La-Ca-Mn-O films. Science 264, 413–415 (1994).

    Article  ADS  CAS  Google Scholar 

  5. Tokura, Y. et al. Giant magnetotransport phenomena in filling-controlled Kondo lattice system: La1−xSrxMnO3. J. Phys. Soc. Jpn 63, 3931–3935 (1994).

    Article  ADS  CAS  Google Scholar 

  6. Urushibara, A. et al. Insulator-metal transition and giant magnetoresistance in La1−xSrxMnO3. Phys. Rev. B 51, 11103–14109 (1995).

    Article  Google Scholar 

  7. Tomioka, Y., Asamitsu, A., Moritomo, Y., Kuwahara, H. & Tokura, Y. Collapse of a charge-ordered state under a magnetic field in Pr1/2Sr1/2MnO3. Phys. Rev. Lett. 74, 5108–5111 (1995).

    Article  ADS  CAS  Google Scholar 

  8. Tomioka, Y., Asamitsu, A., Moritomo, Y. & Tokura, Y. Anomalous magnetotransport properties of Pr1−xCaxMnO3. J. Phys. Soc. Jpn 64, 3626–3630 (1995).

    Article  ADS  CAS  Google Scholar 

  9. Tomioka, Y., Asamitsu, A., Kuwahara, H., Moritomo, Y. & Tokura, Y. Magnetic-field-induced metal-insulator phenomena in Pr1−xCaxMnO3with controlled charge-ordering instability. Phys. Rev. B 53, R1689–R1692 (1995).

    Article  ADS  Google Scholar 

  10. Kuwahara, H., Tomioka, Y., Asamitsu, A., Moritomo, Y. & Tokura, Y. Afirst-order phase transition induced by a magnetic field. Science 270, 961–963 (1995).

    Article  ADS  CAS  Google Scholar 

  11. Kuwahara, H. et al. Striction-coupled magnetoresistance in perovskite-type manganese oxides. Science 272, 80–82 (1996).

    Article  ADS  CAS  Google Scholar 

  12. Jonker, G. H. & Van Santen, J. H. Ferromagnetic compounds of manganese with perovskite structure. Physica 16, 337–349 (1950).

    Article  ADS  CAS  Google Scholar 

  13. Zener, C. Interaction between the d-shells in the transition metals. II. Ferromagnetic compounds of manganese with perovskite structure. Phys. Rev. 82, 403–405 (1951).

    Article  ADS  CAS  Google Scholar 

  14. Anderson, P. W. & Hasegawa, H. Considerations on double exchange. Phys. Rev. 100, 675–681 (1955).

    Article  ADS  CAS  Google Scholar 

  15. de Gennes, P.-G. Effects of double exchange in magnetic crystals. Phys. Rev. 118, 141–154 (1960).

    Article  ADS  CAS  Google Scholar 

  16. Jirak, Z., Krupicka, S., Simsa, Z., Dlouha, M. & Vratislav, Z. Neutron diffraction study of Pr1−xCaxMnO3perovskite. J. Magn. Magn. Mater. 53, 153–166 (1985).

    Article  ADS  CAS  Google Scholar 

  17. Yoshizawa, H., Kawano, H., Tomioka, Y. & Tokura, Y. Neutron-diffraction study of the magnetic-field-induced metal-insulator transition in Pr0.7Ca0.3MnO3. Phys. Rev. B 52, R13145–R13148 (1995).

    Article  ADS  Google Scholar 

Download references

Acknowledgements

This work was performed at JRCAT under the joint research agreement between the NAIR and the ATP, and was supported by NEDO and by a Grant-In-Aid for Scientific Research from the Ministry of Education, Science, and Culture, Japan.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to A. Asamitsu.

Rights and permissions

Reprints and permissions

About this article

Cite this article

Asamitsu, A., Tomioka, Y., Kuwahara, H. et al. Current switching of resistive states in magnetoresistive manganites. Nature 388, 50–52 (1997). https://doi.org/10.1038/40363

Download citation

  • Received:

  • Accepted:

  • Issue Date:

  • DOI: https://doi.org/10.1038/40363

This article is cited by

Comments

By submitting a comment you agree to abide by our Terms and Community Guidelines. If you find something abusive or that does not comply with our terms or guidelines please flag it as inappropriate.

Search

Quick links

Nature Briefing

Sign up for the Nature Briefing newsletter — what matters in science, free to your inbox daily.

Get the most important science stories of the day, free in your inbox. Sign up for Nature Briefing