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| Open AccessDopant-additive synergism enhances perovskite solar modules
A synergistic dopant-additive combination strategy using methylammonium chloride as the dopant and a Lewis-basic ionic-liquid additive is shown to enable the fabrication of perovskite solar modules achieving record certified performance and long-term operational stability.
- Bin Ding
- , Yong Ding
- & Mohammad Khaja Nazeeruddin
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Article |
Triple-junction solar cells with cyanate in ultrawide-bandgap perovskites
Triple-junction solar cells with cyanate in ultrawide-bandgap perovskites exhibit enhanced defect formation energy and substantially decreased non-radiative recombination.
- Shunchang Liu
- , Yue Lu
- & Yi Hou
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Article |
Flexible silicon solar cells with high power-to-weight ratios
A study reports a combination of processing, optimization and low-damage deposition methods for the production of silicon heterojunction solar cells exhibiting flexibility and high performance.
- Yang Li
- , Xiaoning Ru
- & Zongping Shao
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Article
| Open AccessHomogenizing out-of-plane cation composition in perovskite solar cells
We added out-of-plane cations to homogenize the distribution of cations in perovskite films, resulting in a solar cell with improved efficiency and stability.
- Zheng Liang
- , Yong Zhang
- & Xu Pan
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Low-loss contacts on textured substrates for inverted perovskite solar cells
A co-adsorbent is used to achieve a uniform self-assembled phosphonic acid monolayer on a textured substrate, leading to more efficient inverted perovskite solar cells.
- So Min Park
- , Mingyang Wei
- & Edward H. Sargent
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Article |
Enhanced optoelectronic coupling for perovskite/silicon tandem solar cells
An independently certified power conversion efficiency of 32.5% for perovskite/silicon tandem solar cells is achieved through improved charge transfer at the amorphous indium zinc oxide interconnecting layer and reduced optical losses at the front and rear electrodes.
- Erkan Aydin
- , Esma Ugur
- & Stefaan De Wolf
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Article |
Flatband λ-Ti3O5 towards extraordinary solar steam generation
A route to greatly elevate joint densities of states by introducing a flat-band electronic structure is demonstrated, showing metallic λ-Ti3O5 powders have a high solar absorptivity and offering insights into access to cost-effective solar-to-steam generation.
- Bo Yang
- , Zhiming Zhang
- & Liang Zuo
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Article |
All-perovskite tandem solar cells with 3D/3D bilayer perovskite heterojunction
All-perovskite tandem solar cells with an immiscible 3D/3D bilayer heterojunction demonstrate a record-high PCE of 28%, as well as the ability to retain more than 90% of their initial performance after 600 h of continuous operation.
- Renxing Lin
- , Yurui Wang
- & Hairen Tan
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Perspective |
Lead immobilization for environmentally sustainable perovskite solar cells
An analysis of chemical processes to immobilize lead from perovskite solar cells is presented, highlighting the need for a standard lead-leakage test and mathematical model to reliably evaluate the potential environmental risk of perovskite optoelectronics.
- Hui Zhang
- , Jin-Wook Lee
- & Nam-Gyu Park
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Inverted perovskite solar cells using dimethylacridine-based dopants
A dimethylacridine-based molecular doping process is used to construct a well-matched p-perovskite/indium tin oxide contact, along with all-round passivation of grain boundaries, achieving a certified power conversion efficiency of 25.39%.
- Qin Tan
- , Zhaoning Li
- & Zhubing He
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Article
| Open AccessFlexible solar cells based on foldable silicon wafers with blunted edges
Modules of foldable crystalline silicon solar cells retain their power-conversion efficiency after being subjected to bending stress or exposure to air-flow simulations of a violent storm.
- Wenzhu Liu
- , Yujing Liu
- & Zhengxin Liu
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Article
| Open AccessThe electron–proton bottleneck of photosynthetic oxygen evolution
Microsecond infrared spectroscopy together with quantum chemistry reveal the rate-determining proton and electron movements and identify an oxygen-radical state of the manganese cluster as the S4 state.
- Paul Greife
- , Matthias Schönborn
- & Holger Dau
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Article |
Improving interface quality for 1-cm2 all-perovskite tandem solar cells
A self-assembled monolayer of (4-(7H-dibenzo[c,g]carbazol-7-yl)butyl)phosphonic acid is integrated in wide-bandgap perovskite solar cells, which enables a high power conversion efficiency and low open-circuit voltage deficiency, as well as efficient centimetre-scale all-perovskite tandem solar cells.
- Rui He
- , Wanhai Wang
- & Dewei Zhao
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Article |
Controlled growth of perovskite layers with volatile alkylammonium chlorides
In situ grazing-incidence wide-angle X-ray diffraction and scanning electron microscopy were used to evaluate the crystallization process and surface morphology of perovskite thin films coated with alkylammonium chlorides, which were used to fabricate high-efficiency perovskite solar cells.
- Jaewang Park
- , Jongbeom Kim
- & Sang Il Seok
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Article |
Water splitting with silicon p–i–n superlattices suspended in solution
The simplicity of particle suspension reactors and the precise synthetic control afforded by silicon nanowire growth are used to develop a system that can produce hydrogen fuel by splitting water with sunlight.
- Taylor S. Teitsworth
- , David J. Hill
- & James F. Cahoon
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Article |
Solar-to-hydrogen efficiency of more than 9% in photocatalytic water splitting
Photocatalytic water splitting with a high solar-to-hydrogen efficiency of more than nine per cent is achieved using pure water, concentrated solar light and an indium gallium nitride photocatalyst.
- Peng Zhou
- , Ishtiaque Ahmed Navid
- & Zetian Mi
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Article |
Regulating surface potential maximizes voltage in all-perovskite tandems
Because open-circuit voltage deficit is greater in wide-bandgap perovskite solar cells, the authors introduce diammonium molecules to modify perovskite surface states and achieve a more uniform spatial distribution of surface potential, enabling record voltage all-perovskite tandem solar cells.
- Hao Chen
- , Aidan Maxwell
- & Edward H. Sargent
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Article |
Spatiotemporal imaging of charge transfer in photocatalyst particles
Photovoltage measurements on cuprous oxide photocatalyst particles are used to spatiotemporally track the charge transfer processes on the femtosecond to second timescale at the single-particle level.
- Ruotian Chen
- , Zefeng Ren
- & Can Li
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Article |
Perovskite–organic tandem solar cells with indium oxide interconnect
A thin low-loss indium oxide interconnect layer grown by atomic layer deposition enables perovskite–organic hybrid tandem solar cells with a high open-circuit voltage and a high power conversion efficiency.
- K. O. Brinkmann
- , T. Becker
- & T. Riedl
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Article |
Centimetre-scale perovskite solar cells with fill factors of more than 86 per cent
Perovskite solar cells including charge transport material fabricated using a reverse-doping process have the highest certified efficiency for cells of 1-cm2 active area and the highest fill factor reported so far.
- Jun Peng
- , Felipe Kremer
- & Kylie R. Catchpole
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Article |
All-perovskite tandem solar cells with improved grain surface passivation
A certified efficiency of 26.4% in all-perovskite tandem solar cells, exceeding that of the best-performing single-junction perovskite solar cells, is achieved by control over surface defects in the Pb–Sn subcell.
- Renxing Lin
- , Jian Xu
- & Hairen Tan
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Article |
Drop-in fuels from sunlight and air
Carbon-neutral hydrocarbon fuels can be produced using sunlight and air via a thermochemical solar fuel production chain, thus representing a pathway towards the long-term decarbonization of the aviation sector.
- Remo Schäppi
- , David Rutz
- & Aldo Steinfeld
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Article |
The role of charge recombination to triplet excitons in organic solar cells
A substantial pathway for energy loss in organic solar cells may be suppressed by engineering hybridization between non-fullerene acceptor triplet excitons and spin-triplet charge transfer excitons.
- Alexander J. Gillett
- , Alberto Privitera
- & Richard H. Friend
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Article |
Photocatalytic solar hydrogen production from water on a 100-m2 scale
Carbon-neutral hydrogen can be produced through photocatalytic water splitting, as demonstrated here with a 100-m2 array of panel reactors that reaches a maximum conversion efficiency of 0.76%.
- Hiroshi Nishiyama
- , Taro Yamada
- & Kazunari Domen
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Article |
Pseudo-halide anion engineering for α-FAPbI3 perovskite solar cells
Incorporation of the pseudo-halide anion formate during the fabrication of α-FAPbI3 perovskite films eliminates deleterious iodide vacancies, yielding solar cell devices with a certified power conversion efficiency of 25.21 per cent and long-term operational stability.
- Jaeki Jeong
- , Minjin Kim
- & Jin Young Kim
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Article |
On-device lead sequestration for perovskite solar cells
Using lead-absorbing materials to coat the front and back of perovskite solar cells can prevent lead leaching from damaged devices, without affecting the device performance or long-term operation stability.
- Xun Li
- , Fei Zhang
- & Tao Xu
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Article |
Carrier-resolved photo-Hall effect
A carrier-resolved photo-Hall technique is developed to extract properties of both majority and minority carriers simultaneously and determine the critical parameters of semiconductor materials under light illumination.
- Oki Gunawan
- , Seong Ryul Pae
- & Byungha Shin
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Letter |
Intrinsically stable organic solar cells under high-intensity illumination
Organic photovoltaic cells containing an intrinsically stable organic absorber layer that are likely to be stable for many decades under illumination are demonstrated.
- Quinn Burlingame
- , Xiaheng Huang
- & Stephen R. Forrest
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Letter |
Planar perovskite solar cells with long-term stability using ionic liquid additives
Addition of an ionic liquid, BMIMBF4, to metal halide perovskite solar cells improves their efficiency and long-term operation under accelerated aging conditions of high temperature and full-spectrum sunlight.
- Sai Bai
- , Peimei Da
- & Henry J. Snaith
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Letter |
Sensitization of silicon by singlet exciton fission in tetracene
A silicon and tetracene solar cell employing singlet fission uses an eight-angstrom-thick hafnium oxynitride interlayer to promote efficient triplet transfer, increasing the efficiency of the cell.
- Markus Einzinger
- , Tony Wu
- & Marc A. Baldo
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Letter |
Efficient, stable and scalable perovskite solar cells using poly(3-hexylthiophene)
A double-layered halide architecture for perovskite solar cells enables the use of dopant-free poly(3-hexylthiophene) as a hole-transport material, forming stable and scalable devices with a certified power conversion efficiency of 22.7 per cent.
- Eui Hyuk Jung
- , Nam Joong Jeon
- & Jangwon Seo
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Letter |
Ceramic–metal composites for heat exchangers in concentrated solar power plants
A robust ceramic/refractory metal (ZrC/W)-based composite for use in heat exchangers in concentrated solar power plants above 1,023 kelvin is described, having attractive high-temperature thermal, mechanical and chemical properties combined with cost-effective processing.
- M. Caccia
- , M. Tabandeh-Khorshid
- & K. H. Sandhage
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Letter |
Self-powered ultra-flexible electronics via nano-grating-patterned organic photovoltaics
Detection of biometric signals by self-powered electronic devices that are highly flexible and can be applied to skin.
- Sungjun Park
- , Soo Won Heo
- & Takao Someya
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Article |
Pumping liquid metal at high temperatures up to 1,673 kelvin
By using ceramics for the mechanical and sealing components of a mechanical pump, liquid metal can be circulated continuously at temperatures at least as high as 1,673 kelvin.
- C. Amy
- , D. Budenstein
- & A. Henry
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Letter |
A solvent- and vacuum-free route to large-area perovskite films for efficient solar modules
A new deposition method for solar-panel polycrystalline perovskite thin films enables the production of large-area uniform films and avoids the need for common solvents or vacuum.
- Han Chen
- , Fei Ye
- & Liyuan Han
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Letter |
The effect of illumination on the formation of metal halide perovskite films
Films of metal halide perovskite are used as the absorber material in solar cells, and light irradiation during their formation is shown to affect their crystallization, morphology and photovoltaic performance.
- Amita Ummadisingu
- , Ludmilla Steier
- & Michael Grätzel