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| Open AccessSwept coded aperture real-time femtophotography
The researchers showcase swept-coded aperture real-time femtophotography—an all-optical single-shot computational imaging modality at up to 156.3 trillion frames per second—video-records transient absorption in a semiconductor and ultrafast demagnetization of a metal alloy.
- Jingdan Liu
- , Miguel Marquez
- & Jinyang Liang
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Article
| Open AccessOptical Tellegen metamaterial with spontaneous magnetization
Here the authors propose an isotropic three-dimensional metamaterial with nonreciprocal magnetoelectric resonant responses at visible and mid-infrared frequencies. The proposed metamaterials do not require external magnetization.
- Shadi Safaei Jazi
- , Ihar Faniayeu
- & Viktar Asadchy
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Article
| Open AccessStrong transient magnetic fields induced by THz-driven plasmons in graphene disks
The authors provide an experimental demonstration of magnetic field generation in graphene disks via the inverse Faraday effect. When the disks are illuminated with circularly polarized radiation in resonance with the graphene plasmon frequency, the corresponding rotational motion of the charge carriers gives rise to a unipolar magnetic field.
- Jeong Woo Han
- , Pavlo Sai
- & Martin Mittendorff
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| Open AccessTopological magneto-optical effect from skyrmion lattice
In the magneto-optical Kerr effect, light incident on a magnetic material is reflected with a shifted polarization, the size of the shift characterized by the Kerr angle. Here, Kato et al introduce a topological magneto-optical Kerr effect, where the presence of skyrmions, a type of topological spin texture, leads to a significant enhancement of the Kerr signal.
- Yoshihiro D. Kato
- , Yoshihiro Okamura
- & Youtarou Takahashi
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| Open AccessRevealing broken valley symmetry of quantum emitters in WSe2 with chiral nanocavities
The microscopic origin and valley physics of quantum emitters (QEs) in 2D semiconductors are still not fully understood. Here, the authors report an anomalous magneto-optical behaviour of QEs in WSe2 monolayers coupled to chiral plasmonic nanocavities, suggesting the absence of intrinsic valley symmetry of the emitters.
- Longlong Yang
- , Yu Yuan
- & Xiulai Xu
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| Open AccessChirality selective magnon-phonon hybridization and magnon-induced chiral phonons in a layered zigzag antiferromagnet
Phonons are the collective excitations of the lattice of a material, and can, in the case of chiral phonons, carry angular momentum, allowing for strong coupling to the magnetic properties of the material. Here, Cui, Bostrom and co-authors observe chiral magnon polarons, the hybridized quasiparticles of chiral phonons and magnons, in the van der Waals antiferromagnet FePSe3.
- Jun Cui
- , Emil Viñas Boström
- & Qi Zhang
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| Open AccessTopological antichiral surface states in a magnetic Weyl photonic crystal
Here the authors report the first experimental observation of topological antichiral surface states by constructing a three-dimensional modified Haldane model in a magnetic Weyl photonic crystal.
- Xiang Xi
- , Bei Yan
- & Zhen Gao
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| Open AccessGeneration of third-harmonic spin oscillation from strong spin precession induced by terahertz magnetic near fields
The authors studied HoFeO3 crystal using multicycle THz magnetic pulses enhanced strongly by spiral-shaped microstructure. The observed Faraday ellipticity demonstrates second- and third-order harmonics of the magnetization oscillation and an asymmetric oscillation behavior.
- Zhenya Zhang
- , Fumiya Sekiguchi
- & Hideki Hirori
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Article
| Open AccessMicrowave-to-optical transduction with erbium ions coupled to planar photonic and superconducting resonators
Interfacing superconducting quantum information processors with long-distance optical networks would require coherent interfacing between microwave and optical photons. Here, the authors show a chip-integrated microwave-to-optical transducer based on rare earth ion ensembles.
- Jake Rochman
- , Tian Xie
- & Andrei Faraon
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| Open AccessTheory of optical axion electrodynamics and application to the Kerr effect in topological antiferromagnets
Electromagnetic response of topological materials is described the so called axion electrodynamics which contains additional relations between the fields. Here the authors extend the theory of axion electrodynamics to general optical frequencies and apply it to a realistic topological antiferromagnet.
- Junyeong Ahn
- , Su-Yang Xu
- & Ashvin Vishwanath
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| Open AccessHelicity dependent photoresistance measurement vs. beam-shift thermal gradient
Many recent studies have explored the response of magnetic systems to circularly polarised light. To achieve this, typically experiments use a birefringent crystal. Here, Yang et al show that any small error in the alignment of the crystal can result in a beam shift, and this shift can lead to spurious signals similar yet unrelated to the electron spin.
- Haozhe Yang
- , Eva Schmoranzerová
- & Ioan-Mihai Miron
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| Open AccessCoherent helicity-dependent spin-phonon oscillations in the ferromagnetic van der Waals crystal CrI3
CrI3 is a van der Waals material which exhibits magnetic ordering down to the monolayer limit. Here, using ultrafast optical spectroscopy, Padmanabhan and Buessen et al. investigate the coupling between the magnetically ordered spins and lattice distortions, finding a coherent spin-coupled phonon mode.
- P. Padmanabhan
- , F. L. Buessen
- & R. P. Prasankumar
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| Open AccessSlowdown of photoexcited spin dynamics in the non-collinear spin-ordered phases in skyrmion host GaV4S8
Skyrmions are a topological magnetic texture that have garnered considerable interest for various technological applications. Here, Sekiguchi et al. investigate the ultrafast optical response of GaV4S6, and find a significant reduction in the thermal conductivity in the skyrmion phase.
- Fumiya Sekiguchi
- , Kestutis Budzinauskas
- & Paul H. M. van Loosdrecht
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| Open AccessThe Landé factors of electrons and holes in lead halide perovskites: universal dependence on the band gap
The Landé factors govern all the spin-related basic phenomena and are the key parameters which guide spintronics applications. Here, Kirstein et al. demonstrate a universal dependence of the Landé factors on the bandgap energy of several perovskite materials.
- E. Kirstein
- , D. R. Yakovlev
- & M. Bayer
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| Open AccessObservation of optical gyromagnetic properties in a magneto-plasmonic metamaterial
Optical gyromagnetic properties are not observed in natural or metamaterials to date. Here, the authors experimentally demonstrated optical gyromagnetic properties in a magneto-plasmonic metamaterial, realizing the long-sought bi-gyrotropic medium.
- Weihao Yang
- , Qing Liu
- & Lei Bi
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| Open AccessTransient quantum beatings of trions in hybrid organic tri-iodine perovskite single crystal
Understanding photo-physics giving rise to quantum beating oscillations in hybrid organic-inorganic perovskites aids their applications in spintronics and quantum information science. Here, authors demonstrate that quantum beatings observed in single crystal perovskite at cryogenic temperatures are originating from positive and negative trions.
- Uyen N. Huynh
- , Ye Liu
- & Z. Valy Vardeny
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| Open AccessRoom-temperature optically detected magnetic resonance of single defects in hexagonal boron nitride
Optically active spins in solid-state materials hold promise for future quantum technologies. Here, the authors demonstrate optically detected magnetic resonance at room temperature for single defects in a two-dimensional material, hexagonal boron nitride.
- Hannah L. Stern
- , Qiushi Gu
- & Mete Atatüre
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| Open AccessOn-chip terahertz isolator with ultrahigh isolation ratios
Nonreciprocal devices are crucial in scientific research and practical applications at all frequencies. Here the authors demonstrate an integrated terahertz optical isolator based on the magneto-optical effect in a nonreciprocal resonator.
- Shixing Yuan
- , Liao Chen
- & Xinliang Zhang
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| Open AccessLarge ultrafast-modulated Voigt effect in noncollinear antiferromagnet Mn3Sn
Mn3Sn is an anti-ferromagnetic material which displays a large magneto-optical Kerr effect, despite lacking a ferromagnetic moment. Here, the authors show that likewise, Mn3Sn, also presents a particularly large magneto-optical Voigt signal, with a negligible change in the quench time over a wide temperature range.
- H. C. Zhao
- , H. Xia
- & H. B. Zhao
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| Open AccessObservation of strong excitonic magneto-chiral anisotropy in twisted bilayer van der Waals crystals
Systems where both time-reversal symmetry and inversion symmetry are broken can exhibit a magneto-chiral effect; however, this is usually weak. Here, Lan et al demonstrate a significantly enhanced excitonic magnetochiral effect in twisted bilayer tungsten disulphide on a ferromagnetic substrate.
- Shoufeng Lan
- , Xiaoze Liu
- & Xiang Zhang
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| Open AccessEfficient spin excitation via ultrafast damping-like torques in antiferromagnets
Spin damping plays a fundamental role in many areas of spintronics, however, it is typically assumed that damping is irrelevant for impulsive spin excitations due to their rapid timescale. Here, the authors demonstrate that damping leads to a large and immediate spin-canting in anti-ferromagnets.
- Christian Tzschaschel
- , Takuya Satoh
- & Manfred Fiebig
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| Open AccessExtreme anti-reflection enhanced magneto-optic Kerr effect microscopy
Magneto-optic Kerr effect microscopy is useful for dynamic magnetic studies, but is limited by the weak magneto-optical activity. Here, the authors show that extreme anti-reflection result in a Kerr amplitude as large as 20° and enables real-time detection of sub-wavelength magnetic domain reversals.
- Dongha Kim
- , Young-Wan Oh
- & Min-Kyo Seo
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Article
| Open AccessAll-dielectric magnetic metasurface for advanced light control in dual polarizations combined with high-Q resonances
The authors fabricate and investigate the metasurface made of 2D iron-garnet subwavelength nanopillar array on a thin iron-garnet film. It exhibits high quality-factor resonances, leading to a multifold increase in light intensity modulation of the transmitted light with an advantage of P and S polarizations both sensitive to the medium magnetization.
- Daria O. Ignatyeva
- , Dolendra Karki
- & Vladimir I. Belotelov
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| Open AccessObservation of magneto-electric rectification at non-relativistic intensities
The role of the optical magnetic field is generally not considered at nonrelativistic light intensities. Here the authors show magneto-electric rectification, an optical nonlinear effect due to electric and magnetic field coupling, in a thin film of the organic semiconductor pentacene at non-relativistic intensities.
- M. Tuan Trinh
- , Gregory Smail
- & Stephen C. Rand
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Article
| Open AccessGiant magneto-optical responses in magnetic Weyl semimetal Co3Sn2S2
The evidence of topological origin for the recently observed anomalous Hall effect remains elusive. Here, the authors report that the resonance of the optical Hall conductivity resulted from topological electronic structure gives rise to the large intrinsic anomalous Hall effect in the magnetic Weyl semimetal Co3Sn2S2.
- Y. Okamura
- , S. Minami
- & Y. Takahashi
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Article
| Open AccessExciton g-factors in monolayer and bilayer WSe2 from experiment and theory
Excitons in various spin and valley configurations control the optical properties of ultrathin transition metal dichalcogenides. Here, the authors develop theoretical and experimental methods to determine the exciton g-factors for all possible spin-valley configurations of excitons in monolayer and bilayer WSe2, including valley-indirect excitons.
- Jonathan Förste
- , Nikita V. Tepliakov
- & Alexander Högele
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| Open AccessSingle pulse all-optical toggle switching of magnetization without gadolinium in the ferrimagnet Mn2RuxGa
Femtosecond laser pulses allow for extremely fast switching of magnetization in ferromagnetic films, but all examples so far contained gadolinium. Here the authors demonstrate room temperature all-optical toggle switching in a ferrimagnetic manganese-based half-metal without gadolinium.
- C. Banerjee
- , N. Teichert
- & J. Besbas
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| Open AccessResonant thermal energy transfer to magnons in a ferromagnetic nanolayer
Most of the energy harvesting principles are realized in heated-continuously systems. Here, the authors present a concept of high-frequency energy harvesting where the dissipated heat in a sample excites resonant magnons in a ferromagnetic metal layer.
- Michal Kobecki
- , Alexey V. Scherbakov
- & Manfred Bayer
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| Open AccessDistinct magneto-Raman signatures of spin-flip phase transitions in CrI3
Thin samples CrI3 exhibit a phase transition under an applied magnetic field from layered antiferromagnetism to ferromagnetism. Here the authors observe an associated abrupt change in the magneto-Raman spectra, illustrating the sensitivity of Raman spectra to magnetic ordering.
- Amber McCreary
- , Thuc T. Mai
- & Angela R. Hight Walker
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Article
| Open AccessGiant magneto-birefringence effect and tuneable colouration of 2D crystal suspensions
Materials with tunable transmitted colours are sought after for a range of applications. The authors here present magnetic-field-controlled color tuning in a transparent suspension of 2D crystals with unusually large magneto-birefringence.
- Baofu Ding
- , Wenjun Kuang
- & Hui-Ming Cheng
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Article
| Open AccessSub-Hertz resonance by weak measurement
Although the possibility to use weak measurements for metrological purposes has long been known, its practicality and the effective potential advantage are debated. Here, the authors demonstrate a WM-based correlation spectroscopy technique allowing low-frequency fT-level magnetometry at room temperature.
- Weizhi Qu
- , Shenchao Jin
- & Yanhong Xiao
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| Open AccessOptical spin-orbit torque in heavy metal-ferromagnet heterostructures
It is known that torques can be exerted on spins in a ferromagnet (FM) layer when an in-plane electric current is injected into a heavy metal (HM) layer in contact with the FM layer. Here, the authors demonstrate that torques can be generated without the current injection by shining instead circularly polarized light on the HM.
- Gyung-Min Choi
- , Jung Hyun Oh
- & Hyun-Woo Lee
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| Open AccessAbsence of unidirectionally propagating surface plasmon-polaritons at nonreciprocal metal-dielectric interfaces
The local Drude model predicts that, under certain conditions, surface plasmon polaritons at a metal-dielectric surface have a frequency range where only unidirectional propagation is supported. Here, the authors show that in more realistic non-local models surface plasmon polaritons exhibit bidirectional propagation for all frequencies.
- Siddharth Buddhiraju
- , Yu Shi
- & Shanhui Fan
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| Open AccessTopological magneto-optical effects and their quantization in noncoplanar antiferromagnets
Magneto-optical effects in magnets are commonly attributed to the interplay between exchange splitting and spin-orbit coupling. Here, Feng et al. report a topological magneto-optical effect in non-coplanar antiferromagnets due to finite scalar spin chirality, without any reference to exchange splitting or spin-orbit coupling.
- Wanxiang Feng
- , Jan-Philipp Hanke
- & Yugui Yao
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| Open AccessMagneto-optical painting of heat current
Spin caloritronics offers advantages for the thermal management of spintronic devices. Here, the authors demonstrate that the direction of heat currents generated by spin-caloritronic phenomena can be changed by illuminating magnetic materials with visible light.
- Jian Wang
- , Yukiko K. Takahashi
- & Ken-ichi Uchida
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| Open AccessEnhancing and controlling valley magnetic response in MoS2/WS2 heterostructures by all-optical route
Van der Waals heterostructures may offer a suitable platform for all-optical manipulation of valleytronic devices. Here, the authors observe a strong enhancement of the valley magnetic response in MoS2, and magnetic tuning of the polarization of MoS2 direct optical transition
- Jing Zhang
- , Luojun Du
- & Ting Yu
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Article
| Open AccessTracking the ultrafast motion of an antiferromagnetic order parameter
Understanding antiferromagnetic dynamics enables future information technologies, but the detection remains challenging. Here, the authors show the capability of tracking the three dimensional spin motions in YMnO3 by combining time resolved measurements of Faraday rotation and magneto-optical second harmonic generation.
- Christian Tzschaschel
- , Takuya Satoh
- & Manfred Fiebig
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Article
| Open AccessTopological magnon amplification
Malz et al. show how electromagnetic driving leads to amplification of topological magnon edge states and thus a large steady-state magnon edge current. Their approach should yield experimental signatures of topological magnon edge states and has potential applications in magnon spintronics.
- Daniel Malz
- , Johannes Knolle
- & Andreas Nunnenkamp
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Article
| Open AccessUltrafast long-range spin-funneling in solution-processed Ruddlesden–Popper halide perovskites
Spin-information transport or transfer is essential for spintronics applications and often relies on high purity and quality materials. Here, the authors report on the defect-tolerant solution-processed Ruddlesden–Popper halide perovskites, where a spin propagation length of 600 nm was achieved via spin funneling.
- David Giovanni
- , Jia Wei Melvin Lim
- & Tze Chien Sum
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| Open AccessStrongly coupled magnon–phonon dynamics in a single nanomagnet
Exploring the magnon and phonon coupling may enable high efficiency magnonic applications. Here the authors show the observation, understanding and control of the magnon–phonon interaction by studying the magneto-acoustic resonance modes of a single thin-film Ni nanomagnet.
- Cassidy Berk
- , Mike Jaris
- & Holger Schmidt
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Article
| Open AccessThe valley Zeeman effect in inter- and intra-valley trions in monolayer WSe2
The unique valley and spin texture of atomically thin transition metal dichalcogenides (TMDs) allows the observation of the valley Zeeman effect for neutral and charged excitons. Here, the authors unveil the underlying physics of the magneto-optical response and valley Zeeman splitting of trions in tungsten-based TMDs.
- T. P. Lyons
- , S. Dufferwiel
- & A. I. Tartakovskii
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Article
| Open AccessSelection rules for all-optical magnetic recording in iron garnet
The authors computationally and experimentally derive the selection rules on polarization, wavelengths, and magnetic damping for non-dissipative аll-optical magnetic recording with femtosecond laser pulses in Co-doped garnet film. The suggested approach is based on a multiple resonant pumping of localized d-electron transitions.
- A. Stupakiewicz
- , K. Szerenos
- & A. V. Kimel
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| Open AccessIntegrating all-optical switching with spintronics
The high speed switching and energy efficiency nature grant all-optical switching (AOS) great potential for future photonic integrated spintronic devices. Here the authors demonstrate the combination of AOS and domain wall propagation in Pt/Co/Gd synthetic ferrimagnetic racetrack for applications in photonic memory technologies.
- M. L. M. Lalieu
- , R. Lavrijsen
- & B. Koopmans
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Article
| Open AccessHybrid nanodiamond quantum sensors enabled by volume phase transitions of hydrogels
Nitrogen-vacancy (NV) centers in diamonds are used for quantum sensing but NV centers are not sensitive to parameters such as temperature, pressure and biomolecules. Here the authors propose a scheme based on a magnetic nanoparticle docked responsive hydrogel which acts as a transducer between the particles and the diamond.
- Ting Zhang
- , Gang-Qin Liu
- & Quan Li
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Article
| Open AccessGiant magnetic splitting inducing near-unity valley polarization in van der Waals heterostructures
In transition metal dichalcogenide monolayers, the spin and valley degrees of freedom are strongly coupled. Here, the authors engineer a WSe2/MoSe2 heterostructure in which inter-valley transitions of interlayer excitons exhibit a giant splitting and near-unity polarization in a magnetic field.
- Philipp Nagler
- , Mariana V. Ballottin
- & Tobias Korn
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Article
| Open AccessTopologically protected Dirac plasmons in a graphene superlattice
Current proposals suitable for experimental realization of topologically protected optical states rely on complicated structures or only operate in the microwave regime. Here, Pan et al. propose topological Dirac plasmons to be realized at infrared frequencies in a periodically patterned graphene monolayer, subject to a magnetic field of only 2 Tesla.
- Deng Pan
- , Rui Yu
- & F. Javier García de Abajo
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| Open AccessExcitation of coupled spin–orbit dynamics in cobalt oxide by femtosecond laser pulses
Light pulses can control magnetism in a material, and the effective creation of magnetic oscillations leads to spintronic devices with higher efficiency. Here, the authors increase the efficiency of magnon excitation by using a material in which orbital angular momenta are not quenched.
- Takuya Satoh
- , Ryugo Iida
- & B. A. Ivanov
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| Open AccessOptical-helicity-driven magnetization dynamics in metallic ferromagnets
Optical switching of ferromagnets has attracted interest for use in ultrafast spintronics but the physical origin of the effect remains unclear. Here the authors determine the contributions of two proposed mechanisms, the inverse Faraday effect and optical spin-transfer torque.
- Gyung-Min Choi
- , André Schleife
- & David G. Cahill
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| Open AccessNanoscale interface confinement of ultrafast spin transfer torque driving non-uniform spin dynamics
Fundamental understanding of ultrafast spin dynamics is crucial for spintronics applications. Here the authors demonstrate an ultrafast technique to explore the inhomogeneous THz spin dynamics in Fe/Au/Fe multilayers triggered by spin transfer torque.
- Ilya Razdolski
- , Alexandr Alekhin
- & Alexey Melnikov