Abstract
Topological insulators subject to a time-reversal-symmetry-breaking perturbation are predicted to display a magneto-electric effect that causes the electric and magnetic induction fields to mix at the material’s surface. This effect induces polarization rotations of between ≈1–10 mrad per interface in an incident plane-polarized electromagnetic wave normal to a multilayered structure. Here we show, theoretically and numerically, that by using a waveguide geometry with a topological insulator guide layer and magneto-dielectric cladding it is possible to achieve rotations of ≈100 mrad and generate an elliptical polarization with only a three-layered structure. This geometry is beneficial, not only as a way to enhance the magneto-electric effect, rendering it easier to observe, but also as a method for controlling the polarization of electromagnetic radiation.
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Introduction
Topological insulators1,2 are time-reversal-symmetric materials that display non-trivial topological order, which results in an insulating bulk and protected conducting edge states3. Such behaviour has been observed in Group V/VI alloys that have strong enough spin-orbit coupling to induce band inversion, e.g. Bi1−xSbx4,5, Bi2Se3, Bi2Te3 and Sb2Te36,7,8. Owing to it’s unusual electronic properties, topological insulators have also been predicted to display a magneto-electric effect which causes the electric, E, and magnetic induction, B, fields to mix at the material’s surface9,10. This effect will induce Kerr (reflection) and Faraday (transmission) rotations in plane polarized light, with previous studies predicting a ≈1–10 mrad rotation in an incident electromagnetic wave normal to a single topological-insulator-magneto-dielectric interface11,12,13,14,15.
The magneto-electric effect is induced by applying a time-reversal-symmetry-breaking perturbation to a topological insulator’s surface. This can be done either by introducing magnetic dopants10 or by applying an external magnetic field12. Such a perturbation opens a gap in the surface states the of size of which is proportional to the perpendicular magnetic field or the 2D surface dopant density16 - current experiments in Bi2Se3 have observed a ≈50 meV gap with 16% Fe dopants17 and a ≈100 meV gap with 22% Cr dopants18, with even larger gaps predicted. Within this gap, the resulting quantum Hall effect9,10 leads to modified constitutive relations for the material
where ε(r, ω) and μ(r, ω) are the usual permittivity and permeability and Θ(r, ω) is the axion coupling which takes odd values of π in a time-reversal-symmetry-broken topological insulator and even values of π in a conventional magneto-dielectric with, α, the fine structure constant. For convenience we work in natural units with c = ε0 = μ0 = 1. The lowest Hall plateau, which is generated by the strongest magnetic perturbation, leads to Θ(r, ω) = π. Reducing the magnet perturbation will not increase the axion coupling until the next Hall plateau is reached. Thus, axion couplings of Θ(r, ω) = π, 3π, 5π, … are only accessible with magnetic perturbation on the order of Tesla. Higher plateaus are accessible at lower fields but these plateaus are narrower and can be difficult to resolve. Thus, although this effect is achievable with an infinitesimal field, strong fields may be required to observe the discrete nature axion coupling. Maxwell’s equations are unchanged by the axion coupling, however, the modified constitutive relations result in a term proportional to ∇Θ(r, ω) × E(r, ω) appearing in the wave equation19,20. Thus, gradients in the axion coupling cause the electric field to rotate in the plane perpendicular to that gradient and, hence, plane polarized electromagnetic radiation will undergo a rotation in regions of spatially varying axion coupling.
Faraday and Kerr rotations in have been observed in THz spectroscopy studies of Bi2Te321,22,23,24 and strained HgTe25,26,27. As the mechanism by which these rotations occur is directly related to the topological surface states of these materials, the effect can be a used as a probe. Studies have sought to measure the Landau level structure21,22, surface states23 and transport properties25,26 of these materials using the Faraday and Kerr rotations, as well as the band spin splitting due to an external magnetic field24. In term of application, these materials show promise for room temperature control of the phase and polarization of THz radiation27.
Another feature of the magneto-electric, unique to topological insulators, is the universal quantization of the Faraday rotation. Previous theoretical studies have predicted that, for plane-polarized light normal to a topological insulator surface in either the thin film geometry, where the wavelength of the incident radiation is much greater than the thickness of the topological insulator slab, λ ≫ d, or the resonant case in the thick film geometry, where the film thickness is equal to a half integer number of wavelengths, d = Nλ/2, the Faraday rotation is quantized in integer units of the fine structure constant, α12,13,14,15. This feature distinguishes topological insulators from materials that exhibit the magneto-optical Kerr effect, which can also be used to induce Faraday rotations in waveguides28. This effect has recently been experimentally observed29,30,31. However, this universality is only occurs for normal incident light in the stated geometries and, although the Faraday rotation is still quantized, the magnitude of the rotation deviates from α for non-resonant thick film geometries or non-normal incident angles32.
There are advantages for trying to increase the Faraday rotation. As a surface state probe, an increase in the Faraday rotation would render small features of the states easier to observe and hence provide higher sensitivity for these precision measurements. In terms of applications, enhancement of the effect could lead to a large enough rotation for signal processing, thus, providing a method for controlling the polarization of THz radiation. It is possible to increase the rotation simply by adding more layers26,32. However, with each additional layer the fabrication process becomes increasingly difficult. In addition, in order to obtain consistent results, any precision experiment wishing to study a topological insulator would require that all the surfaces in a multi-layered structure to be in the same state (i.e. to have the same gating potential and experience the same fields), which can sometimes be challenging. Here, we show that it is possible to significantly enhance the magneto-electric effect using a waveguide, thus rendering the effect easier to detect whilst only using a three layered structure. In this geometry, the radiation probes only two surfaces, which is advantageous for spectroscopic measurements. Furthermore, a waveguide is a standard photonic component and provides an easily fabricable structure for on-chip THz radiation control.
Theory
Here, we study a slab waveguide geometry, layered in the y-direction with optical modes propagating in the x-direction, consisting of a homogeneous time-reversal-symmetry-broken topological insulator guide layer and a homogeneous conventional magneto-dielectric cladding. Thus, the axion coupling only varies at the interfaces between the guide layer and the cladding. Such a waveguide supports four types of mode, transverse electric odd and even modes (TE) with the electric field, E(r, ω), polarized in the z-direction and transverse magnetic odd and even modes (TM) with the magnetic field, H(r, ω), polarized in the z-direction. As the effect of the axion coupling is to rotate the polarization of the propagating field, one would expect the TE and TM polarizations to mix. Thus, one should observe a rotation in the polarization of a plane-polarized electromagnetic wave as it propagates down the waveguide. Furthermore, as the propagation constants of the TE and TM modes differ in a waveguide, one should also observe a changing ellipticity. From a geometric optics perspective, one can view the effect as a series of successive Kerr rotations from the multiple reflections at the waveguide interfaces.
There are two possible orientations for the axion coupling. These orientations are a result of the relative direction of the time-symmetry-breaking perturbation on the two sides of the guide layer and originate from the relative sign of the hall conductivities at these interfaces9,10. The first orientation is anti-parallel orientation [Fig. 1(a)], where the time-symmetry-breaking perturbation is in the opposite direction on each side of the waveguide (and, hence, the change in the axion coupling is the same on each side of the waveguide). In this case the interaction rotates the electromagnetic wave in the same direction with respect to the direction of propagation. Hence, magnetic fields of the same sign (and electric fields of opposite sign) are generated at opposing interfaces. Thus, in a symmetric waveguide, even modes will couple to even modes and odd modes to odd modes [Fig. 1(b)]. The second orientation is the parallel orientation [Fig. 1(c)], where the direction of the time-symmetry-breaking perturbation is in the same on each side of the waveguide (and, hence, the change in the axion coupling is opposite on each side of the waveguide). In this case the interaction rotates the electromagnetic wave in opposite directions with respect to the direction of propagation. Hence, magnetic fields of opposite sign (and electric fields of the same sign) are generated at opposing interfaces. Thus, in a symmetric waveguide, even modes will couple to odd modes vice versa [Fig. 1(d)].
To quantify this effect we use the modified wave equation to develop a coupled mode theory for the system (see Supplementary Material). Owing to the relative sizes of α and ε, we assume that the axion coupling term only marginally changes the modes of the waveguide and, hence, we can treat it as a small perturbation to the usual magneto-dielectric waveguide modes. Using these modes as a basis, one finds that the mode amplitudes, , evolve as
with the coupling constants, κνμ, give by
where and are the usual electric and magnetic field profiles for a magneto-dielectric waveguide and βν are the corresponding propagation constants. Here, the indices μ and ν indicate the TE, TM, odd and even modes. Considering only the lowest four modes in a symmetric waveguide, the interaction only couples pairs of modes, hence, Eq. (3) breaks down into two independent 2 × 2 matrix equations that can be solved analytically.
Results
Faraday rotation and ellipticity
As an example, we consider a symmetric waveguide in the anti-parallel configuration with the input electromagnetic wave exciting the TE even mode only. Evaluation of the coupling constants shows that, in this situation, the interaction only couples the input electromagnetic wave to the TM even mode. Solving the resulting system of equations shows that the Ey(x) and Ez(x) components of the field evolve as the sum of two waves of different frequencies. The coupled-mode analysis described above leads to two the characteristic parameters for the waveguide, the maximum transferred power, Pc, which is the maximum power that the waveguide can transfer from the initial mode (in this case the TE even mode) to the target mode (in this case the TM even mode) and the coupling length, lc, which is the distance that the radiation must travel down the waveguide to achieve this maximum power transfer. In weak coupling limit, , which is always valid for the parameters considered here, one finds
and
with . From the field components one can also find the maximum polarization rotation, which occurs at the coupling length, lc, and the maximum ellipticity, which occurs at lc/2. In the weak coupling limit, these read
One can quantify the enhancement of the Faraday rotation by comparing Eq. (7) to the result for plane-polarized light at normal incident on a single slab with two interfaces. In this geometry the maximum rotation is achieved in the topological regime32 hence the enhancement factor reads Fψ = ψmax/α. For small enhancements this expression simplifies to .
In order to validate the theoretical model we compared the results to finite-difference-time-domain electromagnetic simulation data33. We consider a Bi2Se3 guide layer, with εg = 1634, μ = 1 and Θ = π, and a silicon cladding12,35, with εc = 12, μ = 1 and Θ = 0. Bi2Se3 has a bulk band gap of ≈300 meV36,37, and an achievable surface gap of ≈100 meV18. The strong resonance peak at ≈10 meV34 stems from the excitation of surface plasmons38, which will be absent in the presence of a surface band gap. Hence, for wavelengths >12 μm material absorption will be minimal. Therefore, we focus on the process in the absence of material loss. We insert electromagnetic radiation of wavelength ≈3.3 times the waveguide width. At this frequency there are four guided modes - the lowest order TE and TM, odd and even modes.
Figure 2(a) shows simulated data of the elliptical polarization of the electromagnetic wave at different points along the waveguide. One observes the expected changes in polarization and ellipticity as the wave propagates. Figure 2(b) shows the elliptical polarization of the wave at ≈33 wavelengths along the waveguide for both the theoretical calculation and simulated data. One observes good agreement between the two. Figure 2(c) shows the variation in the polarization angle and ellipticity along the length of the waveguide. The polarization and ellipticity oscillate, with the maximum rotation occurring at lc and maximum ellipticity occurring at lc/2. The phenomenological shift of 4 mrad that occurs in the simulated data is a result of the source partially exciting the TM even mode hence the initial polarization is 4 mrad away from the z-axis. Good agreement is seen between the numerical calculation and simulated data.
Permittivity contrast
The coupling constants are proportional the waveguide mode profiles, hence, by careful choice of the magneto-dielectric properties of the waveguide guide layer and cladding, the polarization rotation and ellipticity can be maximized. Figure 3(a) shows the maximum polarization rotation and ellipticity for different permittivity contrasts, εg − εc. As the contrast is reduced the maximum polarization rotation and ellipticity increases and, for contrasts of ≈0.5, one sees a rotation of ≈100 mrads (≈6o), which is two orders of magnitude larger than the rotation on transmission or reflection at a single interface. This increase in rotation is due to the reduced the phase mismatch, βTE − βTM, between the TE even and TM even modes and, hence, better transfer of energy. However, reducing the permittivity contrast also reduces the coupling constant and, hence, increases the coupling length [see Fig. 3(b)]. Thus, in order to observe the maximal rotation, very long waveguides need to be fabricated (≈1000 wavelengths). For wavelengths below the surface band gap, waveguides on the order of 1–2 cm are required to observe the ≈100 mrads rotation.
Discussion
Here we have developed a coupled mode theory to describe the propagation of electromagnetic waves in a time-reversal-symmetry-broken topological insulator waveguide. For an axion coupling of Θ = π in the anti-parallel configuration and radiation of wavelength λ > 12 μm (i.e. below the surface band gap) a Faraday rotation of ≈100 mrads (≈6o) can be achieved for waveguides of length ≈1.2 cm when the permittivity contrast is low. Fabrication of such a device is not infeasible. Current technology for on-chip optical signal processing in silicon is able to produce waveguides in the range of 1–5 cm39,40. In comparison, fabrication of structures with topological insulators, such as Bi2Se3, is still in its infancy. The widely used technique of mechanical exfoliation is the current standard and produces micron-sized flakes, which have been successfully used to create simple electronic devices. However, recent advances in epitaxial growth have resulted in Bi2Se3 thin films with areas of 3 × 3 cm that can be transferred to arbitrary substrates41. Whilst the technology to produce cm-long waveguides in Bi2Se3 is not yet fully developed, the advances in this field show that the fabrication of such a structure is possible and it is envisaged that methods to generate complex heterostructures with topological insulators will be available in the very near future.
When considering the application of a time-reversal-symmetry-broken topological insulator waveguide for control of THz frequency radiation dispersion effects need to be considered. In the previous analysis it was assumed that the electromagnetic radiation was a plane-wave. In more realistic scenarios pulsed light is more commonly used, especially in the field of signal processing. Thus, dispersion becomes an issue. Figure 4(a) shows simulated data of the polarization rotation and ellipticity at the peak of an Gaussian pulse, with temporal envelope function E(t) = exp[−t2/σ2], for various pulse widths, σ. The simulations show that the maximum polarization rotation and ellipticity are unchanged by the spectral width and, hence, are almost identical to the theoretically derived result for the continuous wave case.
As the axion coupling, Θ, is 2 orders of magnitude smaller than the permittivity, ε, dispersion effects within the waveguide are dominated by magneto-electric properties of the constituent materials. Figure 4(b) shows the allowed propagating waveguide modes as a function of frequency. The mode dispersion curves are almost identical to the equivalent magneto-dielectic waveguide mode dispersion curves vanishing axion coupling, Θ. Hence, the axion coupling only negligibly affects the dispersion properties of the waveguide. Thus a reasonable estimate of the dispersion properties of the waveguide can be found whilst neglecting the effects of the axion coupling.
An important feature of the magneto-electric effect in topological insulators is the universal quantization of the Faraday rotation in units of the fine structure constant, α12,13,14,15. Clearly, if the polarization rotation is enhanced it will no longer be in units of α, however, it is still quantized. The maximum polarization rotation (ellipticity) are quantized in odd multiples of the polarization rotation (ellipticity) for Θ = π. Hence, ψmax(Θ = nπ) = nψmax(Θ = π) and χmax(Θ = nπ) = nχmax(Θ = π). Thus, by varying the value of the axion coupling, Θ, which can be achieved by varying the time-symmetry breaking perturbation, one would still observe quantized steps as each successive plateau is reached. Figure 4(c) shows the change in maximum polarization rotation and ellipticity with changing axion coupling. One can clearly see the equal steps in the polarization rotation and ellipticity as the axion coupling increases. Note that the axion coupling, as it is directly related to the quantized hall plateaus in the material, can only take odd units of π and that a smoothly varying magnetic field will lead to step like transitions in the axion coupling as one access the next hall plateau9,10.
Whilst this system does not display the universality of the single slab system, the advantage here is that the quantized transitions are much larger. As the polarization rotation is related to electron surface states, the enhanced polarization rotation can be used to probe these states with a greater degree of accuracy. Precision measurements of this type may reveal additional features to these surface states or the transitions between them that will shed light on the quantum processes that occur with topological insulators. Figure 4(c) also shows the variation in the coupling length for varying axion couplings. As the coupling length is more strongly affected by the propagation constants of the modes rather than the axion coupling, one finds that the coupling length remains approximately constant with increasing axion coupling. Thus, one can observe the quantized maximum polarization rotations merely by changing the time-reversal-symmetry breaking perturbation, without the need to change the length of the waveguide.
In terms of potential applications, topological insulators have been proposed as a platform for controlling THz radiation for photodetection42, wireless communication and biological spectroscopy27. It has also been shown that the Faraday rotation in a topological insulator can be controlled by electronic gating27. Thus, it is possible to electrically control the polarization rotation and, hence, provide high-speed optical modulation. Waveguide structures offer a compact method for the guiding of radiation and the continuing development of silicon photonics as a method for optical signal processing has demonstrated the potential of such devices. The integration of topological insulators into existing silicon heterostructure technology would add extra functionality to these photonic components.
Topological insulator waveguides offer an easily fabricable structure that can increase the rotation of plane-polarized electromagnetic radiation, a key signature of the magneto-electric effect, which itself is linked to the electronic surface states of the material, by two orders of magnitude compared to other three-layered structures, thus rendering these features much easier to study. Thus, this effect can be used as a probe of these surface states in fundamental physics experiments. Furthermore, by exploiting the enhancement effects of certain geometries, topological insulator devices, such as the waveguide described here, potentially offer new methods of controlling the polarization of THz electromagnetic radiation.
Methods
Validation of the theoretical model was carried out by comparison with finite-difference-time-domain electromagnetic simulation data. Using the constitutive equations, Eqs (1) and (2), to eliminate the magnetic induction, B(r, ω), and displacement, D(r, ω), fields from the time dependent Maxwell’s equations and neglecting terms of order O(α2) leads to two coupled equations for the electric, E(r, ω), and magnetic, H(r, ω), fields
Equations (9) and (10), subject to a unit plane wave source, Ez = −Hy = exp[−iωt], were solved on a staggered Yee lattice using standard electromagnetic finite-difference-time-domain methods33.
Additional Information
How to cite this article: Crosse, J. A. Theory of topological insulator waveguides: polarization control and the enhancement of the magneto-electric effect. Sci. Rep. 7, 43115; doi: 10.1038/srep43115 (2017).
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Acknowledgements
We acknowledge supports from the Singapore National Research Foundation under NRF Grant No. NRF-NRFF2011-07. The author would like to thank S.Y. Buhmann and M. Tsang for useful discussions.
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Crosse, J. Theory of topological insulator waveguides: polarization control and the enhancement of the magneto-electric effect. Sci Rep 7, 43115 (2017). https://doi.org/10.1038/srep43115
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