## Abstract

Wavefunction collapse models modify Schrödinger’s equation so that it describes the collapse of a superposition of macroscopically distinguishable states as a dynamical process. This provides a basis for the resolution of the quantum measurement problem. An additional generic consequence of the collapse mechanism is that it causes particles to exhibit a tiny random diffusive motion. Here it is shown that for the continuous spontaneous localization (CSL) model—one of the most well developed collapse models—the diffusions of two sufficiently nearby particles are positively correlated. An experimental test of this effect is proposed in which random displacements of pairs of free nanoparticles are measured after they have been simultaneously released from nearby traps. The experiment must be carried out at sufficiently low temperature and pressure in order for the collapse effects to dominate over the ambient environmental noise. It is argued that these constraints can be satisfied by current technologies for a large region of the viable parameter space of the CSL model. The effect disappears as the separation between particles exceeds the CSL length scale. The test therefore provides a means of bounding this length scale.

## Introduction

Dynamical wavefunction collapse models^{1,2} provide a unified description of quantum dynamics encompassing both unitary evolution and state reduction. Typically the standard Schrödinger dynamics are extended so that the state behaves stochastically and in such a way that certain superposition states are unstable. The most prominent collapse model is the continuous spontaneous localization (CSL) model^{3,4} in which a superposition of quasi-localized matter states will collapse at a rate which increases with the mass of the object. This results in the rapid collapse of macroscopically distinguishable superposition states whilst micro states are little affected.

Since the CSL model involves a modification of the Schrödinger equation, it makes predictions which are in conflict with standard quantum theory. It is therefore possible to experimentally test CSL. A direct way to do this is to try to observe quantum interference for objects of increasing mass. Detailed studies show that there should be a characteristic loss of fringe visibility as the mass increases beyond a sufficient size (see Refs 5, 6, 7). Another observable effect of CSL is a random diffusive motion of particles. An isolated object will undergo a random walk induced by the collapse mechanism. As shown in Ref. 8 this can dominate over environmental effects at sufficiently low temperature and pressure.

Here we consider a situation with two non-interacting particles. We will examine how the particles behave as a result of the CSL dynamics and show that there is a potentially measurable effect whereby the diffusions undergone by each particle are correlated. A key feature of the CSL model is that the localization mechanism acts on the total smeared mass density state rather than individually on each particle. This suggests that for two nearby particles, the diffusive behaviour caused by the localization mechanism will be correlated. This should be apparent in the joint spatial probability distribution. In what follows we shall solve the two-particle CSL master equation to determine the behaviour precisely.

Our proposed experiment is shown schematically in Fig. 1. A pair of nanoparticles are trapped side by side using laser light. The particles are simultaneously released and allowed a brief period of free fall. The positions of each of the particles is then measured by light (Rayleigh) scattering. The experiment does not involve matter wave interferometry and therefore avoids much technical complication. Indeed the scheme can be performed with existing technology.

We assume that the two particles are non-interacting and of equal mass. We also assume that the two particles are identical bosons although this is not crucial to our argument—the same conclusion holds if the particles are non-identical. We could also regard the particles as composite objects made up of many constituent particles satisfying the CSL dynamics. This case is more complicated but it can be shown^{4} that the CSL dynamics can be applied to the composite object as a whole. Furthermore, any environmental particles involved in the CSL dynamics but not part of the system of interest can be traced away without effect.

There are two fixed parameters in the CSL model which are treated as fundamental constants. These are the localization rate *λ* and the localization length scale . We consider a regime in which the localization length scale is large compared to the length scale defining the spatial extent of the system. The original estimates of these parameters by Ghirardi, Rimini and Weber (GRW)^{9} are *λ* = 10^{−16} s^{−1} and . However, these values are not definitive. A recent study of the valid regions of the *λ*-*α* parameter space consistent with experiment puts no upper bound limit on the CSL length scale^{10}.

The CSL master equation is given by

with density operator and free Hamiltonian . The smeared mass density operator is given by

where *m*_{0} is the nucleon mass (used to set the mass scale), and the field annihilation and creation operators and satisfy

The two-particle state is represented by

where 1 and 2 label the two particles and *ψ* is a symmetric wavefunction. In this representation improper position eigenstates are given by

and the two-particle density matrix is represented in coordinate space as

The coordinate space representation of Eq. (1) for the two-particle state in the limit of large localization length is found to be

where

Here, the limit of large localization length specifically means that *ρ*_{t}(x_{1}, y_{1}, x_{2}, y_{2}) is only significant whenever for *i* = 1, 2 and (see Refs 11, 12).

Equation (7) applies in three dimensional space. In what follows we are concerned only with the behaviour in one dimension. We choose this to be the horizontal dimension of Fig. 1. We can trace over the coordinates of the other spatial dimensions in *ρ*_{t} resulting in a reduced one dimensional density matrix. It is straightforward to show that this satisfies a master equation with the same form as Eq. (7).

We now present a solution of Eq. (7) (further details of the techniques used can be found in Ref. 12). The solution is represented in terms of a density matrix propagator *J* (see Refs 13, 14) as

We find that for Eq. (7) (in one dimension), *J* is given by

where *i*, *j* = 1, 2.

We consider an initial wave function of the form

This represents the particles residing in adjacent harmonic traps of width *σ* and spaced by a distance 2*μ* ≫ *σ*. The initial density matrix is

We suppose that the particles are simultaneously released from the traps and allowed to diffuse freely. However, they remain sufficiently separated that there is negligible conventional interaction between them. Using Eqs (9 and 10) we have calculated the diagonal part of the density matrix

following a time period *t* after their release. This represents the joint probability distribution for the subsequently measured positions of the two particles. The result is simplest when expressed in terms of the variables

where we find

with

The distribution consists of two peaks, one about *X* = 0, *ξ*/2 = *μ* and another about *X* = 0, *ξ*/2 = −*μ*. Note that we have ignored a possible interference term between the two peaks in Eq. (15) since we assume that they do not disperse enough to overlap. The feature that we are interested in is the shape of these peaks and in particular their rate of dispersion in the two directions *X* and *ξ*/2. The *X* and *ξ* spreads of each of the peaks are defined by *σ*_{X} and *σ*_{ξ/2} respectively. We see that the CSL parameter *D* contributes to *σ*_{X} whilst *σ*_{ξ/2} is unaffected. Note that by setting *D* = 0 (standard quantum mechanics) in Eqs (16 and 17) we find . This reflects the fact that the two particles are behaving independently and their distributions are uncorrelated.

The physical reason for the difference between *σ*_{X} and *σ*_{ξ/2} when *D* ≠ 0 is that the diffusive shifts in position of the two particles caused by the collapse mechanism will be positively correlated if the particles are closer together than the localization length scale. The system as a whole diffuses but *ξ* = *x*_{2} − *x*_{1} is only affected by standard quantum dispersion.

Our result is clearly dependent on the fact that the localization length scale , but in this limit the spreads in *X* and *ξ*/2 do not depend on the separation 2 *μ*. For the particles would behave independently under CSL. A null observation would therefore put a constraint on *α*.

To observe the effect we must distinguish and . We can estimate these variances by repeatedly measuring the displacements of two particles simultaneously dropped from nearby traps (see Fig. 1). We assume that the traps are such that *σ *= 10 nm and the particles are released for *t* = 0.25 s corresponding to a drop of 30 cm. We further assume that position measurements have an error of *σ*_{err} = 10 nm which is normally distributed and independent of *x*_{i}. If is the unbiased estimate of based on *n* sets of position measurements, then the variance in is given by

To be able to clearly observe the effect of CSL we demand that should be at least 10 times smaller than the difference

Taking the mass of the particles to be 10^{9} amu such that *ħ*^{2}*t*^{2}/4*m*^{2}*σ*^{4} ≪ 1, this results in the following constraint on *n*:

This is shown in Fig. 2(a).

Now we consider the effects of an environment. We suppose that the particles are confined within a vacuum chamber and consider the constraints placed on temperature and pressure by the condition that the collapse effects should be dominant. We consider environmental noise contributions both from radiation and molecular collisions.

It is shown in Ref. 15 that the dominant contribution to the thermal diffusion by radiation is due to recoil from emission of photons. There it is also shown that the variance in displacement of a bulk sphere of radius *R* and density due to the emission of radiation is given (in SI units) by

where *T*_{i} is the internal temperature of the bulk object. By demanding that we can constrain the internal temperature of the particles. Using = 10^{3} kgm^{−3} and *R* = 10^{−7} m, we find

The maximum internal temperature is shown in Fig. 2(b).

The mean time between molecule-sphere collisions in the impact regime is given in seconds by^{8}

where *P* is the pressure given in picoTorr, *T*_{e} is the external temperature, and *T*_{0} = 300 K is room temperature. We make the conservative assumption that *τ*_{c} should be 10 times greater than the total experiment time *n* × *t*. Taking *T*_{e}/*T*_{0} ∼ 1 this results in

The maximum ambient pressure in the vacuum chamber is shown in Fig. 2(c).

We conclude that an experiment can be performed to test for *λα* as low as 1 m^{−2}s^{−1}. This requires *n* = 24000; *T*_{i} = 73 K and *P* = 3.3 × 10 ^{− 17} Torr. We assume a separation between traps of at least 1 mm (to avoid dispersion forces/gravity effects) so that the correlation effect should be present for . The accessible region of *λ*-*α* parameter space is shown in Fig. 3. Also shown is the region of parameter space currently ruled out by diffraction experiments involving particles of mass 10^{5} amu^{16}.

In summary, we have demonstrated an effect of the CSL model in which the diffusive behaviour of two sufficiently nearby particles is correlated. If one particle is found to have randomly moved in one direction as a result of the collapse mechanism, the other particle is more likely to have moved in the same direction. We propose attempting to observe this effect as a test of CSL against standard quantum theory and as a specific test of the CSL length scale. The experiment is possible with today’s technology.

## Additional Information

**How to cite this article**: Bedingham, D.J. and Ulbricht, H. Correlated random walks caused by dynamical wavefunction collapse. *Sci. Rep.* **5**, 13380; doi: 10.1038/srep13380 (2015).

## References

- 1.
Bassi. A. & Ghirardi, G. C. Dynamical reduction models.

*Phys. Rept.***379**, 257–426 (2003). - 2.
Bassi, A., Lochan, K., Satin, S., Singh, T. P. & Ulbricht, H. Models of wave-function collapse, underlying theories, and experimental tests.

*Rev. Mod. Phys.***85**, 471–527 (2013). - 3.
Pearle, P. Combining stochastic dynamical state-vector reduction with spontaneous localisation.

*Phys. Rev. A***39**, 2277–2289 (1989). - 4.
Ghirardi, G. C., Pearle, P. & Rimini, A. Markov process in Hilbert space and continuous spontaneous localisation of systems of identical particles.

*Phys. Rev. A***42**, 78 (1990). - 5.
Nimmrichter, S., Hornberger, K., Haslinger, P. & Arndt, M. Testing spontaneous localisations theories with matter-wave interferometer.

*Phys. Rev. A***83**, 043621 (2011). - 6.
Marshall, W., Simon, C., Penrose, R. & Bouwmeester, D. Towards quantum superpositions of a mirror.

*Phys. Rev. Lett.***91**, 130401 (2003). - 7.
Kippenberg, T. & Vahala, K. Cavity optomechanics: back-action at the mesoscale.

*Science***321**, 1172 (2008). - 8.
Collett, B. & Pearle, P. Wavefunction collapse and random walk.

*Found. Phys.***33**1495 (2003). - 9.
Ghirardi, G. C., Rimini, A. & Weber, T. Unified dynamics for microscopic and macroscopic systems

*Phys. Rev. D***34**, 470 (1986). - 10.
Feldmann, W. & Tumulka, R., Parameters diagrams of the GRW and CSL theories of wavefunctions collapse.

*J. Phys. A: Math. Theor.***45**, 06504 (2012). - 11.
Bedingham, D. J. Single Particle energy diffusion from relativistic spontaneous localisation.

*Phys. Rev. D***88**, 045032 (2013). - 12.
Bedingham, D. J. Effects of the continuous spontaneous localization model in the regime of large localisation length.

*Phys. Rev. A***89**, 032713 (2014). - 13.
Caldeira, A. O. & Leggett, A. J. Path integral approach to quantum Brownian motion.

*Physica A***121**, 587 (1983). - 14.
Anastopoulos, C. & Halliwell, J. J. Generalized uncertainty relations and long-time limits for quantum Brownian motion models.

*Phys. Rev. D***51**, 6870 (1995). - 15.
Bera, S., Motwani, B., Singh, T. P. & Ulbricht, H. A proposal for the experimental detection of CSL induced random walk.

*Sci. Rep.***5**, 7664: 10.1038/srep07664 (2015). - 16.
Eibenberger, S., Gerlich, S., Arndt, M., Mayor, M. & Tüxen, J. Matter-wave interference of particles selected from a molecular library with masses exceeding 10000 amu.

*Phys. Chem. Chem. Phys.***15**, 14696 (2013).

## Acknowledgements

D.J.B. was supported by EPSRC Research Grant No. EP/J008060/1 and a grant from the Templeton World Charity Foundation. H.U. acknowledges support by the EPSRC (EP/J014664/1), the Foundational Questions Institute (FQXi) through a Large Grant, and by the John F. Templeton foundation (grant 39530). We would like to thank Jonathan Halliwell for helpful discussions and comments.

## Author information

## Affiliations

### Faculty of Philosophy, University of Oxford, OX2 6GG, United Kingdom

- D. J. Bedingham

### School of Physics and Astronomy, University of Southampton, SO17 1BJ, United Kingdom

- H. Ulbricht

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### Contributions

D.J.B. conceived the idea for this work. D.J.B. conceptualized the theoretical part of the manuscript and did the estimate of competing heating effects. H.U. conceptualized the experimental proposal in the manuscript. Both authors wrote and discussed the manuscript.

### Competing interests

The authors declare no competing financial interests.

## Corresponding authors

Correspondence to D. J. Bedingham or H. Ulbricht.

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