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| Open AccessChiral phonons in quartz probed by X-rays
Our experimental proof of chiral phonons demonstrates a degree of freedom in condensed matter that is of fundamental importance and opens the door to exploration of emergent phenomena based on chiral bosons.
- Hiroki Ueda
- , Mirian García-Fernández
- & Urs Staub
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Article |
Geometric frustration of Jahn–Teller order in the infinite-layer lattice
A distorted infinite-layer lattice of single-crystal CaCoO2 originates from competition between an ordered Jahn–Teller effect and geometric frustration.
- Woo Jin Kim
- , Michelle A. Smeaton
- & Harold Y. Hwang
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Article |
Preservation of high-pressure volatiles in nanostructured diamond capsules
The nanostructured diamond capsule process with the inert gases solid argon and neon is demonstrated, where the trapped volatile gases could sustain their high-pressure states without confinement of conventional high-pressure vessels, opening up the possibility of in-depth investigations of high-pressure phenomena.
- Zhidan Zeng
- , Jianguo Wen
- & Qiaoshi Zeng
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Article |
High-entropy polymer produces a giant electrocaloric effect at low fields
A study reports and characterizes a high-entropy electrocaloric polymer that switches under low fields, and discusses its potential suitability for use in caloric heat pumps.
- Xiaoshi Qian
- , Donglin Han
- & Q. M. Zhang
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Article |
Ultrahard bulk amorphous carbon from collapsed fullerene
Preparing amorphous phases of carbon with mostly sp3 bonding in bulk is challenging, but macroscopic samples that are nearly pure sp3 are synthesized here by heating fullerenes at high pressure.
- Yuchen Shang
- , Zhaodong Liu
- & Bingbing Liu
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Article |
Synthesis of paracrystalline diamond
A study describes the synthesis, structural characterization and formation mechanism of a paracrystalline state of diamond, adding an unusual form of diamond to the family of carbon-based materials.
- Hu Tang
- , Xiaohong Yuan
- & Huiyang Gou
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Article |
Percolation transitions in compressed SiO2 glasses
Amorphous–amorphous phase transitions in silicon dioxide are shown to proceed through a sequence of percolation transitions, a process that has relevance to a range of important liquid and glassy systems.
- A. Hasmy
- , S. Ispas
- & B. Hehlen
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Article |
How to design an icosahedral quasicrystal through directional bonding
Model patchy colloids with directional bonding are designed that assemble into icosahedral quasicrystals through the propagation of an icosahedral network of bonds and may be realized using DNA origami particles.
- Eva G. Noya
- , Chak Kui Wong
- & Jonathan P. K. Doye
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Article |
Determining the three-dimensional atomic structure of an amorphous solid
A method that achieves atomic-resolution tomographic imaging of an amorphous solid enables detailed quantitative characterization of the short- and medium-range order of the three-dimensional atomic arrangement.
- Yao Yang
- , Jihan Zhou
- & Jianwei Miao
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Article |
Metastability of diamond ramp-compressed to 2 terapascals
X-ray diffraction measurements of solid carbon compressed to pressures of about two terapascals (approximately twenty million atmospheres) find that carbon retains a diamond structure even under these extreme conditions.
- A. Lazicki
- , D. McGonegle
- & J. S. Wark
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Article |
Origins of structural and electronic transitions in disordered silicon
Machine learning models enable atomistic simulations of phase transitions in amorphous silicon, predict electronic fingerprints, and show that the pressure-induced crystallization occurs over three distinct stages.
- Volker L. Deringer
- , Noam Bernstein
- & Stephen R. Elliott
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Article |
Anatomy of cage formation in a two-dimensional glass-forming liquid
The onset of rigidity in a two-dimensional colloidal glass-forming system is identified by the formation and merging of locally rigid domains in which particles move in a cooperative manner.
- Bo Li
- , Kai Lou
- & Steve Granick
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Matters Arising |
Slow compression of crystalline ice at low temperature
- R. Bauer
- , J. S. Tse
- & T. Hattori
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Article |
Laser picoscopy of valence electrons in solids
Laser-generated high-harmonic emission is used to image the valence potential and electron density in magnesium fluoride and calcium fluoride at the picometre scale, enabling direct probing of material properties.
- H. Lakhotia
- , H. Y. Kim
- & E. Goulielmakis
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Article |
Synthesis and properties of free-standing monolayer amorphous carbon
The synthesis of surprisingly stable, free-standing single layers of amorphous carbon and their analysis by atomic-resolution imaging could settle a debate about their atomic arrangement and offer unusual electronics applications.
- Chee-Tat Toh
- , Hongji Zhang
- & Barbaros Özyilmaz
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Letter |
Ultrahigh-pressure isostructural electronic transitions in hydrogen
X-ray diffraction measurements of solid hydrogen provide crystallographic information for high-pressure phases of hydrogen and transitions between them, suggesting a series of isostructural transitions under compression before band closure and metallization.
- Cheng Ji
- , Bing Li
- & Ho-Kwang Mao
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Letter |
The low-energy Goldstone mode in a trapped dipolar supersolid
Observation of the collective mode responding to the superfluid stiffness—the low-energy Goldstone mode—provides direct evidence for phase rigidity, which is a key signature of supersolidity in an ultracold quantum gas.
- Mingyang Guo
- , Fabian Böttcher
- & Tilman Pfau
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Letter |
Nanosecond X-ray diffraction of shock-compressed superionic water ice
The atomic structure of H2O is documented at several million atmospheres of pressure and temperatures of several thousand degrees, revealing shockwave-induced ultrafast crystallization and a novel water ice phase, ice XVIII, with exotic superionic properties.
- Marius Millot
- , Federica Coppari
- & Jon H. Eggert
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Letter |
Colossal barocaloric effects in plastic crystals
Colossal barocaloric effects are observed in the plastic crystal neopentylglycol and found to originate from the extensive molecular orientational disorder, giant compressibility and highly anharmonic lattice dynamics of the material.
- Bing Li
- , Yukinobu Kawakita
- & Zhidong Zhang
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Letter |
Granular materials flow like complex fluids
The relaxation dynamics of granular materials is more like that of complex fluids than that of thermal glass-forming systems, owing to the absence of the ‘cage effect’.
- Binquan Kou
- , Yixin Cao
- & Yujie Wang
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Letter |
In situ X-ray diffraction measurement of shock-wave-driven twinning and lattice dynamics
In situ femtosecond X-ray diffraction measurements reveal that the dominant mechanism of shock-wave-driven deformation in tantalum changes from twinning to dislocation slip as pressure increases.
- C. E. Wehrenberg
- , D. McGonegle
- & J. S. Wark
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Letter |
Probing the limits of metal plasticity with molecular dynamics simulations
The limits of dislocation-mediated metal plasticity are studied by using in situ computational microscopy to reduce the enormous amount of data from fully dynamic atomistic simulations into a manageable form.
- Luis A. Zepeda-Ruiz
- , Alexander Stukowski
- & Vasily V. Bulatov
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Letter |
Self-bound droplets of a dilute magnetic quantum liquid
A self-bound quantum droplet of magnetic atoms is observed in a trap-free levitation field.
- Matthias Schmitt
- , Matthias Wenzel
- & Tilman Pfau
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Letter |
Molecular transport through capillaries made with atomic-scale precision
Nanometre-scale graphitic capillaries with atomically flat walls are engineered and studied, revealing unexpectedly fast transport of liquid water through channels that accommodate only a few layers of water.
- B. Radha
- , A. Esfandiar
- & A. K. Geim
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Letter |
Observing the Rosensweig instability of a quantum ferrofluid
WebSpontaneous translational symmetry breaking is experimentally observed in a dipolar Bose–Einstein condensate of dysprosium atoms, whereby an instability causes a spontaneous transition from an unstructured superfluid to an ordered arrangement of droplet crystals, which is surprisingly long-lived.
- Holger Kadau
- , Matthias Schmitt
- & Tilman Pfau
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Letter |
Evidence for a new phase of dense hydrogen above 325 gigapascals
Raman spectroscopy of three isotopes of hydrogen under very high compression yields evidence of a new phase of hydrogen—phase V—which could potentially be a precursor to the long-sought non-molecular phase.
- Philip Dalladay-Simpson
- , Ross T. Howie
- & Eugene Gregoryanz
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Letter |
Rejuvenation of metallic glasses by non-affine thermal strain
This study shows that metallic glasses can be rejuvenated (taken to higher energy states with more plasticity) by thermally cycling them at relatively low temperatures (well below the glass transition temperature); this is attributed to the effect of intrinsic structural inhomogeneities in the glassy state, which translate into localized internal strains as the temperature is cycled and the different regions expand and contract by different amounts.
- S. V. Ketov
- , Y. H. Sun
- & A. L. Greer
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Review Article |
The crystallography of correlated disorder
Although classical crystallography is insufficient to determine disordered structure in crystals, correlated disorder does nevertheless contain clear crystallographic signatures that map to the type of disorder, which we are learning to decipher.
- David A. Keen
- & Andrew L. Goodwin
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Letter |
Nonlinear lattice dynamics as a basis for enhanced superconductivity in YBa2Cu3O6.5
Femtosecond X-ray diffraction and ab initio density functional theory calculations are used to determine the crystal structure of YBa2Cu3O6.5 undergoing optically driven, nonlinear lattice excitation above the transition temperature of 52 kelvin, under which conditions the electronic structure of the material changes in such a way as to favour superconductivity.
- R. Mankowsky
- , A. Subedi
- & A. Cavalleri
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Letter |
Ultrafast X-ray probing of water structure below the homogeneous ice nucleation temperature
Femtosecond X-ray laser pulses are used to probe the structure of liquid water in micrometre-sized droplets that have been cooled below the homogeneous ice nucleation temperature, revealing the existence of metastable bulk liquid water down to temperatures of 227 kelvin.
- J. A. Sellberg
- , C. Huang
- & A. Nilsson
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Letter |
Mosaic two-lengthscale quasicrystals
The unusual structures of quasicrystals, such as the 18-fold symmetry observed in polymer micelles, lack the repeating cell pattern of conventional hard crystals; here their origin is shown to be an extension of Penrose tiling with a simple, generic interparticle interaction.
- T. Dotera
- , T. Oshiro
- & P. Ziherl
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Letter |
Structural change in molten basalt at deep mantle conditions
The structure of molten basalt up to 60 GPa by means of in situ X-ray diffraction is described, with the coordination of silicon increasing from four under ambient conditions to six at 35 GPa, and subsequent reduced melt compressibility, which seems to affect siderophile-element partitioning.
- Chrystèle Sanloup
- , James W. E. Drewitt
- & Wolfgang Morgenroth
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News & Views |
Electrons do the split
Interacting electrons that are confined to move in a one-dimensional structure do not simply jam together like cars in rush hour. Inelastic X-ray scattering shows that the electrons act as if they split into separate fractional entities. See Letter p.82
- Ralph Claessen